scholarly journals Comparison of Emissions Inventories of Anthropogenic Air Pollutants in China

2016 ◽  
Author(s):  
Eri Saikawa ◽  
Hankyul Kim ◽  
Min Zhong ◽  
Yu Zhao ◽  
Greet Janssens-Maenhout ◽  
...  

Abstract. Anthropogenic air pollutant emissions have been increasing rapidly in China. Modelers use emissions inventories to assess temporal and spatial distribution of these emissions to estimate their impacts on regional and global air quality. However, large uncertainties exist in emissions estimates and assessing discrepancies in these inventories is essential for better understanding of the trends in air pollution over China. We compare five different emissions inventories estimating emissions of carbon monoxide (CO), nitrogen oxides (NOx), sulfur dioxide (SO2), particulate matter with an aerodynamic diameter of 10 um or less (PM10) from China. The emissions inventories analyzed in this paper include Regional Emissions inventory in ASia v2.1 (REAS); Multi-resolution Emission Inventory for China (MEIC); Emission Database for Global Atmospheric Research v4.2 (EDGAR); the inventory by Yu Zhao (ZHAO); and the Greenhouse Gas and Air Pollution Interactions and Synergies (GAINS). We focus on the period between 2000 and 2008 during which the Chinese economic activities have more than doubled. In addition to the national total, we also analyzed emissions from four source sectors (industry, transportation, power, and residential) and within seven regions in China (East, North, Northeast, Central, Southwest, Northwest, and South) and found that large disagreements (~ seven fold) exist among the five inventories at disaggregated levels. These discrepancies lead to differences of 67 ug/m3, 15 ppbv, and 470 ppbv for monthly mean PM10, O3, and CO, respectively, in modelled regional concentrations in China. We also find that MEIC inventory emissions estimates create a VOC-limited environment that produces much lower O3 mixing ratio in the East and Central China compared to the simulations using REAS and EDGAR estimates. Our results illustrate that a better understanding of Chinese emissions at more disaggregated levels is essential for finding an effective mitigation measure for reducing national and regional air pollution in China.

2017 ◽  
Vol 17 (10) ◽  
pp. 6393-6421 ◽  
Author(s):  
Eri Saikawa ◽  
Hankyul Kim ◽  
Min Zhong ◽  
Alexander Avramov ◽  
Yu Zhao ◽  
...  

Abstract. Anthropogenic air pollutant emissions have been increasing rapidly in China, leading to worsening air quality. Modelers use emissions inventories to represent the temporal and spatial distribution of these emissions needed to estimate their impacts on regional and global air quality. However, large uncertainties exist in emissions estimates. Thus, assessing differences in these inventories is essential for the better understanding of air pollution over China. We compare five different emissions inventories estimating emissions of carbon dioxide (CO2), carbon monoxide (CO), nitrogen oxides (NOx), sulfur dioxide (SO2), and particulate matter with an aerodynamic diameter of 10 µm or less (PM10) from China. The emissions inventories analyzed in this paper include the Regional Emission inventory in ASia v2.1 (REAS), the Multi-resolution Emission Inventory for China (MEIC), the Emission Database for Global Atmospheric Research v4.2 (EDGAR), the inventory by Yu Zhao (ZHAO), and the Greenhouse Gas and Air Pollution Interactions and Synergies (GAINS). We focus on the period between 2000 and 2008, during which Chinese economic activities more than doubled. In addition to national totals, we also analyzed emissions from four source sectors (industry, transport, power, and residential) and within seven regions in China (East, North, Northeast, Central, Southwest, Northwest, and South) and found that large disagreements exist among the five inventories at disaggregated levels. These disagreements lead to differences of 67 µg m−3, 15 ppbv, and 470 ppbv for monthly mean PM10, O3, and CO, respectively, in modeled regional concentrations in China. We also find that all the inventory emissions estimates create a volatile organic compound (VOC)-limited environment and MEIC emissions lead to much lower O3 mixing ratio in East and Central China compared to the simulations using REAS and EDGAR estimates, due to their low VOC emissions. Our results illustrate that a better understanding of Chinese emissions at more disaggregated levels is essential for finding effective mitigation measures for reducing national and regional air pollution in China.


2020 ◽  
Vol 117 (32) ◽  
pp. 18984-18990 ◽  
Author(s):  
Zander S. Venter ◽  
Kristin Aunan ◽  
Sourangsu Chowdhury ◽  
Jos Lelieveld

The lockdown response to coronavirus disease 2019 (COVID-19) has caused an unprecedented reduction in global economic and transport activity. We test the hypothesis that this has reduced tropospheric and ground-level air pollution concentrations, using satellite data and a network of >10,000 air quality stations. After accounting for the effects of meteorological variability, we find declines in the population-weighted concentration of ground-level nitrogen dioxide (NO2: 60% with 95% CI 48 to 72%), and fine particulate matter (PM2.5: 31%; 95% CI: 17 to 45%), with marginal increases in ozone (O3: 4%; 95% CI: −2 to 10%) in 34 countries during lockdown dates up until 15 May. Except for ozone, satellite measurements of the troposphere indicate much smaller reductions, highlighting the spatial variability of pollutant anomalies attributable to complex NOxchemistry and long-distance transport of fine particulate matter with a diameter less than 2.5 µm (PM2.5). By leveraging Google and Apple mobility data, we find empirical evidence for a link between global vehicle transportation declines and the reduction of ambient NO2exposure. While the state of global lockdown is not sustainable, these findings allude to the potential for mitigating public health risk by reducing “business as usual” air pollutant emissions from economic activities. Explore trends here:https://nina.earthengine.app/view/lockdown-pollution.


2014 ◽  
Vol 14 (18) ◽  
pp. 25617-25650 ◽  
Author(s):  
H. Y. Zhao ◽  
Q. Zhang ◽  
S. J. Davis ◽  
D. Guan ◽  
Z. Liu ◽  
...  

Abstract. High anthropogenic emissions from China have resulted in serious air pollution, and it has attracted considerable academic and public concern. The physical transport of air pollutants in the atmosphere has been extensively investigated, however, understanding the mechanisms how the pollutants were transferred through economic and trade activities remains challenge. In this work, we assessed China's virtual air pollutant transport embodied in trade, by using consumption-based accounting approach. We first constructed a consumption-based emission inventory for China's four key air pollutants (primary PM2.5, sulfur dioxide (SO2), nitrogen oxides (NOx) and non-methane volatile organic compounds (NMVOC)) in 2007, based on the bottom-up sectoral emission inventory concerning their production activities – a production-based inventory. We used a multiregional input-output (MRIO) model to integrate the sectoral production-based emissions and the associated economic and trade activities, and finally obtained consumption-based inventory. Unlike the production-based inventory, the consumption-based inventory tracked emissions throughout the supply chain related to the consumption of goods and services and hereby identified the emission flows followed the supply chains. From consumption-based perspective, emissions were significantly redistributed among provinces due to interprovincial trade. Large amount of emissions were embodied in the net imports of east regions from northern and central regions; these were determined by differences in the regional economic status and environmental policies. We also calculated the emissions embodied in exported and imported goods and services. It is found that 15–23% of China's pollutant emissions were related to exports for foreign consumption; that proportion was much higher for central and export-oriented coastal regions. It is suggested that measures should be introduced to reduce air pollution by integrating cross-regional consumers and producers in national agreements to encourage efficiency improvement in the supply chain and optimizing consumption structure internationally. The consumption-based air pollutants emission inventory developed in this work can be further used to attribute pollution to different economic activities and final demand types with the aid of air quality models.


2020 ◽  
Author(s):  
Sabine Schindlbacher ◽  
Christine Brendle ◽  
Katarina Mareckova ◽  
Bradley Matthews ◽  
Marion Pinterits ◽  
...  

<p>Under the Convention on Long-range Transboundary Air Pollution (CLRTAP), 51 northern hemisphere countries are obliged to regularly report their national emissions inventories for selected anthropogenic air pollutants to the United Nations Economic Commission for Europe (UNECE). The EMEP Centre on Emissions Inventories and Projections (CEIP) of the Convention is tasked with administering, archiving and reviewing these data and compiling the EMEP emissions dataset, a complete and gridded inventory for the area between 30 and 82 °N and 30 °W and 90°E.</p><p>The reported national emissions inventories and the EMEP emissions dataset are often used by the scientific community as input drivers of air pollution models or as priors for inverse estimation of emissions. However, interpreting model outputs, validation and uncertainties may be restricted by limited knowledge of the peculiarities of such reported data. The purpose of this conference contribution by CEIP is to provide atmospheric modellers with further insight into these reported emissions data. The presentation will introduce the Convention and discuss how complexities of this international agreement have led to diversified reporting requirements and heterogeneity in the frequency and quality of the reported inventories. Current issues with respect to emissions of particulate matter (e.g. reporting of condensable particulate matter and black carbon) will furthermore be discussed and the presentation will also provide perspectives on how the recently agreed long-term strategy for Convention may impact future emissions reporting over the next decade and beyond.</p>


2018 ◽  
Vol 1 (6) ◽  
pp. 247-257
Author(s):  
Bang Quoc Ho ◽  
Tam Thoai Nguyen ◽  
Khue Hoang Ngoc Vu

Can Tho City is one the 5th largest city in Vietnam, with hight rate of economic growth and densely populated with 1,251,809 people, butsling traffic activities with 566,593 motobikes and 15,105 cars and hundreds of factories. The air in Can Tho city is polluted by dust and ozone. However, Can Tho city currently does not have a study on the simulation air pollution spread, therefore we do not have an overview on the status of air pollution in order to do not have solutions to limit the increase of pollution status of the city. The purpose of this study is to collect air pollutant emissions from other study. After that, TAPOM model is used to simulate the effects of ozone on the surrounding areas and study the ozone regime in Cantho city. The study results showed that the highest ozone concentration for an hour everage is 196 μg/m3. Compare with national technical regulation about ambient air QCVN 5:2013/BTNMT, ozone concentration is approximately at the allowable limit. The study of ozone regime had identified that VOC sensitive areas are Ninh Kieu district and a part in the south of Binh Thuy district, and NOx sensitive areas are the rested areas of Cantho city. The main cause contributing to increased VOC emission in the central area of the city is motorcycles, NOx emissions in the remaining areas of Cantho city are from the rice production factories. Proposals to protect the air quality in Cantho city are suggested.


2017 ◽  
Vol 17 (14) ◽  
pp. 9223-9236 ◽  
Author(s):  
Wolfgang Knorr ◽  
Frank Dentener ◽  
Jean-François Lamarque ◽  
Leiwen Jiang ◽  
Almut Arneth

Abstract. Wildfires pose a significant risk to human livelihoods and are a substantial health hazard due to emissions of toxic smoke. Previous studies have shown that climate change, increasing atmospheric CO2, and human demographic dynamics can lead to substantially altered wildfire risk in the future, with fire activity increasing in some regions and decreasing in others. The present study re-examines these results from the perspective of air pollution risk, focussing on emissions of airborne particulate matter (PM2. 5), combining an existing ensemble of simulations using a coupled fire–dynamic vegetation model with current observation-based estimates of wildfire emissions and simulations with a chemical transport model. Currently, wildfire PM2. 5 emissions exceed those from anthropogenic sources in large parts of the world. We further analyse two extreme sets of future wildfire emissions in a socio-economic, demographic climate change context and compare them to anthropogenic emission scenarios reflecting current and ambitious air pollution legislation. In most regions of the world, ambitious reductions of anthropogenic air pollutant emissions have the potential to limit mean annual pollutant PM2. 5 levels to comply with World Health Organization (WHO) air quality guidelines for PM2. 5. Worst-case future wildfire emissions are not likely to interfere with these annual goals, largely due to fire seasonality, as well as a tendency of wildfire sources to be situated in areas of intermediate population density, as opposed to anthropogenic sources that tend to be highest at the highest population densities. However, during the high-fire season, we find many regions where future PM2. 5 pollution levels can reach dangerous levels even for a scenario of aggressive reduction of anthropogenic emissions.


1988 ◽  
Vol 6 (6) ◽  
pp. 447-464
Author(s):  
Jan Vernon

Over the last decade, environmental concerns have played an increasing role in energy decision making, from siting of new energy facilities to national policy changes, such as Sweden's decision to phase out nuclear power. Concern about atmospheric pollution from fossil fuel combustion, reflected in increasingly strict emission limits, has imposed additional costs and technical demands on coal-fired plants. Estimates from the Federal Republic of Germany, the USA and the OECD indicate that air pollution control can account for a third of the capital costs for a new coal-fired power plant. This article outlines the current status of regulations on air pollutant emissions from coal-fired plants, describes action being taken to meet regulations and its potential impacts on coal utilisation. The article focuses on sulphur dioxide and nitrogen oxides, which have seen major recent developments in regulations and control methods.


2017 ◽  
Vol 10 (9) ◽  
pp. 3255-3276 ◽  
Author(s):  
Augustin Colette ◽  
Camilla Andersson ◽  
Astrid Manders ◽  
Kathleen Mar ◽  
Mihaela Mircea ◽  
...  

Abstract. The EURODELTA-Trends multi-model chemistry-transport experiment has been designed to facilitate a better understanding of the evolution of air pollution and its drivers for the period 1990–2010 in Europe. The main objective of the experiment is to assess the efficiency of air pollutant emissions mitigation measures in improving regional-scale air quality. The present paper formulates the main scientific questions and policy issues being addressed by the EURODELTA-Trends modelling experiment with an emphasis on how the design and technical features of the modelling experiment answer these questions. The experiment is designed in three tiers, with increasing degrees of computational demand in order to facilitate the participation of as many modelling teams as possible. The basic experiment consists of simulations for the years 1990, 2000, and 2010. Sensitivity analysis for the same three years using various combinations of (i) anthropogenic emissions, (ii) chemical boundary conditions, and (iii) meteorology complements it. The most demanding tier consists of two complete time series from 1990 to 2010, simulated using either time-varying emissions for corresponding years or constant emissions. Eight chemistry-transport models have contributed with calculation results to at least one experiment tier, and five models have – to date – completed the full set of simulations (and 21-year trend calculations have been performed by four models). The modelling results are publicly available for further use by the scientific community. The main expected outcomes are (i) an evaluation of the models' performances for the three reference years, (ii) an evaluation of the skill of the models in capturing observed air pollution trends for the 1990–2010 time period, (iii) attribution analyses of the respective role of driving factors (e.g. emissions, boundary conditions, meteorology), (iv) a dataset based on a multi-model approach, to provide more robust model results for use in impact studies related to human health, ecosystem, and radiative forcing.


2020 ◽  
Author(s):  
Freya A. Squires ◽  
Eiko Nemitz ◽  
Ben Langford ◽  
Oliver Wild ◽  
Will S. Drysdale ◽  
...  

Abstract. Direct measurements of NOx, CO and aromatic VOC (benzene, toluene, C2-benzenes and C3-benzenes) flux were made for a central area of Beijing using the eddy covariance technique. Measurements were made during two intensive field campaigns in central Beijing as part of the Air Pollution and Human Health (APHH) project, the first in November–December 2016 and the second during May–June 2017, to contrast winter and summertime emission rates. There was little difference in the magnitude of NOx flux between the two seasons (mean NOx flux was 4.41 mg m−2 h−1 in the winter compared to 3.55 mg m−2 h−1 in the summer). CO showed greater seasonal variation with mean CO flux in the winter campaign (34.7 mg m−2 h−1) being over twice that of the summer campaign (15.2 mg m−2 h−1). Larger emissions of aromatic VOCs in summer were attributed to increased evaporation due to higher temperatures. The largest fluxes in NOx and CO generally occurred during the morning and evening rush hour periods indicating a major traffic source with high midday emissions of CO indicating an additional influence from cooking fuel. Measured NOx and CO fluxes were then compared to the MEIC 2013 emissions inventory which was found to significantly overestimate emissions for this region, providing evidence that proxy-based emissions inventories have positive biases in urban centres. This first set of pollutant fluxes measured in Beijing provides an important benchmark of emissions from the city which can help to inform and evaluate current emissions inventories.


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