Impacts of Large-Scale Circulation on Urban Ambient Concentrations of Gaseous Elemental Mercury in New York, USA
Abstract. The impact of large-scale circulation on urban gaseous elemental mercury (GEM) was investigated through analysis of 2008–2015 measurement data from an urban site in New York City (NYC), New York, USA. Distinct annual cycles were observed in 2009–2010 with mixing ratios in warm seasons (i.e. spring–summer) 10–20 ppqv (~ 10 %–25 %) higher than in cool seasons (i.e. fall–winter). This annual cycle was disrupted in 2011 by an anomalously strong influence of the North American trough in that warm season and was reproduced in 2014 with annual amplitude enhanced up to ~ 70 ppqv associated with a particularly strong Bermuda High. North American trough axis index (TAI) and intensity index (TII) were used to characterize the effect of the North American trough on NYC GEM especially in winter and summer. The intensity and position of the Bermuda High had a significant impact on GEM in warm seasons supported by a strong correlation (r reaching 0.96, p