scholarly journals Impacts of Large-Scale Circulation on Urban Ambient Concentrations of Gaseous Elemental Mercury in New York, USA

Author(s):  
Huiting Mao ◽  
Dolly Hall ◽  
Zhuyun Ye ◽  
Ying Zhou ◽  
Dirk Felton ◽  
...  

Abstract. The impact of large-scale circulation on urban gaseous elemental mercury (GEM) was investigated through analysis of 2008–2015 measurement data from an urban site in New York City (NYC), New York, USA. Distinct annual cycles were observed in 2009–2010 with mixing ratios in warm seasons (i.e. spring–summer) 10–20 ppqv (~ 10 %–25 %) higher than in cool seasons (i.e. fall–winter). This annual cycle was disrupted in 2011 by an anomalously strong influence of the North American trough in that warm season and was reproduced in 2014 with annual amplitude enhanced up to ~ 70 ppqv associated with a particularly strong Bermuda High. North American trough axis index (TAI) and intensity index (TII) were used to characterize the effect of the North American trough on NYC GEM especially in winter and summer. The intensity and position of the Bermuda High had a significant impact on GEM in warm seasons supported by a strong correlation (r reaching 0.96, p 

2017 ◽  
Vol 17 (18) ◽  
pp. 11655-11671 ◽  
Author(s):  
Huiting Mao ◽  
Dolly Hall ◽  
Zhuyun Ye ◽  
Ying Zhou ◽  
Dirk Felton ◽  
...  

Abstract. The impact of large-scale circulation on urban gaseous elemental mercury (GEM) was investigated through analysis of 2008–2015 measurement data from an urban site in New York City (NYC), New York, USA. Distinct annual cycles were observed in 2009–2010 with mixing ratios in warm seasons (i.e., spring–summer) 10–20 ppqv ( ∼  10–25 %) higher than in cool seasons (i.e., fall–winter). This annual cycle was disrupted in 2011 by an anomalously strong influence of the US East Coast trough in that warm season and was reproduced in 2014 associated with a particularly strong Bermuda High. The US East Coast trough axis index (TAI) and intensity index (TII) were used to characterize the effect of the US East Coast trough on NYC GEM, especially in winter and summer. The intensity and position of the Bermuda High appeared to have a significant impact on GEM in warm seasons. Regional influence on NYC GEM was supported by the GEM–carbon monoxide (CO) correlation with r of 0.17–0.69 (p ∼  0) in most seasons. Simulated regional and local anthropogenic contributions to wintertime NYC anthropogenically induced GEM concentrations were averaged at  ∼  75 % and 25 %, with interannual variation ranging over 67 %–83 % and 17 %–33 %, respectively. Results from this study suggest the possibility that the increasingly strong Bermuda High over the past decades could dominate over anthropogenic mercury emission control in affecting ambient concentrations of mercury via regional buildup and possibly enhancing natural and legacy emissions.


2013 ◽  
Vol 26 (22) ◽  
pp. 8787-8801 ◽  
Author(s):  
Kerrie L. Geil ◽  
Yolande L. Serra ◽  
Xubin Zeng

Abstract Precipitation, geopotential height, and wind fields from 21 models from phase 5 of the Coupled Model Intercomparison Project (CMIP5) are examined to determine how well this generation of general circulation models represents the North American monsoon system (NAMS). Results show no improvement since CMIP3 in the magnitude (root-mean-square error and bias) of the mean annual cycle of monthly precipitation over a core monsoon domain, but improvement in the phasing of the seasonal cycle in precipitation is notable. Monsoon onset is early for most models but is clearly visible in daily climatological precipitation, whereas monsoon retreat is highly variable and unclear in daily climatological precipitation. Models that best capture large-scale circulation patterns at a low level usually have realistic representations of the NAMS, but even the best models poorly represent monsoon retreat. Difficulty in reproducing monsoon retreat results from an inaccurate representation of gradients in low-level geopotential height across the larger region, which causes an unrealistic flux of low-level moisture from the tropics into the NAMS region that extends well into the postmonsoon season. Composites of the models with the best and worst representations of the NAMS indicate that adequate representation of the monsoon during the early to midseason can be achieved even with a large-scale circulation pattern bias, as long as the bias is spatially consistent over the larger region influencing monsoon development; in other words, as with monsoon retreat, it is the inaccuracy of the spatial gradients in geopotential height across the larger region that prevents some models from realistic representation of the early and midseason monsoon system.


2019 ◽  
Vol 32 (18) ◽  
pp. 5799-5814 ◽  
Author(s):  
Nicholas J. Lutsko ◽  
Jane Wilson Baldwin ◽  
Timothy W. Cronin

Abstract The impact of large-scale orography on wintertime near-surface (850 hPa) temperature variability on daily and synoptic time scales (from days to weeks) in the Northern Hemisphere is investigated. Using a combination of theory, idealized modeling work, and simulations with a comprehensive climate model, it is shown that large-scale orography reduces upstream temperature gradients, in turn reducing upstream temperature variability, and enhances downstream temperature gradients, enhancing downstream temperature variability. Hence, the presence of the Rockies on the western edge of the North American continent increases temperature gradients over North America and, consequently, increases North American temperature variability. By contrast, the presence of the Tibetan Plateau and the Himalayas on the eastern edge of the Eurasian continent damps temperature variability over most of Eurasia. However, Tibet and the Himalayas also interfere with the downstream development of storms in the North Pacific storm track, and thus damp temperature variability over North America, by approximately as much as the Rockies enhance it. Large-scale orography is also shown to impact the skewness of downstream temperature distributions, as temperatures to the north of the enhanced temperature gradients are more positively skewed while temperatures to the south are more negatively skewed. This effect is most clearly seen in the northwest Pacific, off the east coast of Japan.


2009 ◽  
Vol 9 (5) ◽  
pp. 22407-22458 ◽  
Author(s):  
S. M. Gourdji ◽  
A. I. Hirsch ◽  
K. L. Mueller ◽  
A. E. Andrews ◽  
A. M. Michalak

Abstract. Using synthetic continuous CO2 measurements from the nine sampling locations operational across North America in 2004, this paper investigates the optimal setup for, and constraint on fluxes achieved by, a regional geostatistical atmospheric CO2 inversion over the continent. The geostatistical framework does not require explicit prior flux estimates, nor any other process-based information, and is therefore particularly well suited for investigating the information content of the atmospheric CO2 measurements from a limited network. The atmospheric data are first used with the Restricted Maximum Likelihood (RML) algorithm to infer the model-data mismatch and a priori spatial covariance parameters applied in the inversion. The implemented RML algorithm is found to infer robust spatial covariance parameters from the atmospheric data, as compared to the "true" solution, for cases where the flux and measurement timescales match, while model-data mismatch variances are inferred correctly across all examined cases. A series of analyses is also performed investigating the impact of the temporal scale of concentration measurements and fluxes on inversion results. Inversions using measurement data at sub-daily resolution are found to yield fluxes with a lower Root Mean Square Error (RMSE) relative to inversions using coarser-scale observations, whereas the flux resolution appears to have a lesser impact on the inversion quality. In addition, night-time data for the tall and marine boundary layer towers are found to help constrain fluxes across the continent, although they can potentially bias near-field fluxes. These general conclusions are likely to also be applicable to inversions using a synthesis Bayesian inversion approach. Overall, despite the relatively sparse and unevenly distributed network of nine towers across the North American continent, a geostatistical inversion using an optimal setup and relying solely on the atmospheric data constraint is found to estimate the North American sink for June 2004 to within approximately 10%.


2020 ◽  
Vol 81 ◽  
pp. 167-185
Author(s):  
M Di Bacco ◽  
AR Scorzini

The present study is an analysis of recent changes (1981-2016) in air temperature across the north-eastern region of Italy (NERI), located in a transition zone influenced by the Mediterranean and continental climatological regimes. Annual and seasonal trends in mean maximum and minimum temperatures as well as in selected extreme indices are investigated using high-quality and homogenised daily data deriving from a distributed network of 50 weather stations. The results reveal an overall widespread warming, particularly intense in spring and summer, with significant positive trends in mean and daytime (maximum-related) temperature extremes, especially at lower altitudes. No substantial elevation dependency is observed for trends in minimum-related temperature indices, which are generally characterised by lower spatial variability. Comparable positive and negative trends are identified in the frequency and duration of warm- and cold-related extremes indices. Finally, the influence on temperature extremes of dominant large-scale circulation modes in southern Europe (North Atlantic Oscillation [NAO] and East-Atlantic [EA] pattern) is examined. The results indicate that especially NAO-induced changes can explain observed temperature trends over the NERI, while the impact of the EA pattern is slightly weaker.


2019 ◽  
Vol 32 (24) ◽  
pp. 8771-8790 ◽  
Author(s):  
Tiina Nygård ◽  
Rune G. Graversen ◽  
Petteri Uotila ◽  
Tuomas Naakka ◽  
Timo Vihma

Abstract This study gives a comprehensive picture of how atmospheric large-scale circulation is related to moisture transport and to distributions of moisture, clouds, and surface downward longwave radiation in the Arctic in winter. Anomaly distributions of the abovementioned variables are compared in 30 characteristic wintertime atmospheric circulation regimes, which are allocated from 15 years (2003–17) of mean sea level pressure data of ERA-Interim reanalysis applying the self-organizing map method. The characteristic circulation regimes are further related to known climate indices—the North Atlantic Oscillation (NAO), the Arctic Oscillation (AO), and Greenland blocking index—as well as to a frequent high pressure pattern across the Arctic Ocean from Siberia to North America, herein called the Arctic bridge. Effects of large-scale circulation on moisture, cloud, and longwave radiation are to a large extent occurring through the impact of horizontal moisture transport. Evaporation is typically not efficient enough to shape those distributions, and much of the moisture evaporated in the Arctic is transported southward. The positive phase of the NAO and AO increases moisture and clouds in northern Europe and the eastern North Atlantic Ocean, and a strong Greenland blocking typically increases those in the southwest of Greenland. When the Arctic bridge is lacking, the amount of moisture, clouds, and downward longwave radiation is anomalously high near the North Pole. Our results reveal a strong dependence of moisture, clouds, and longwave radiation on atmospheric pressure fields, which also appears to be important from a climate change perspective.


Atmosphere ◽  
2021 ◽  
Vol 12 (2) ◽  
pp. 136
Author(s):  
Yahya Darmawan ◽  
Huang-Hsiung Hsu ◽  
Jia-Yuh Yu

This study aims to explore the contrasting characteristics of large-scale circulation that led to the precipitation anomalies over the northern parts of Sumatra Island. Further, the impact of varying the Asian–Australian Monsoon (AAM) was investigated for triggering the precipitation variability over the study area. The moisture budget analysis was applied to quantify the most dominant component that induces precipitation variability during the JJA (June, July, and August) period. Then, the composite analysis and statistical approach were applied to confirm the result of the moisture budget. Using the European Centre for Medium-Range Weather Forecasts (ECMWF) Re-Anaysis Interim (ERA-Interim) from 1981 to 2016, we identified 9 (nine) dry and 6 (six) wet years based on precipitation anomalies, respectively. The dry years (wet years) anomalies over the study area were mostly supported by downward (upward) vertical velocity anomaly instead of other variables such as specific humidity, horizontal velocity, and evaporation. In the dry years (wet years), there is a strengthening (weakening) of the descent motion, which triggers a reduction (increase) of convection over the study area. The overall downward (upward) motion of westerly (easterly) winds appears to suppress (support) the convection and lead to negative (positive) precipitation anomaly in the whole region but with the largest anomaly over northern parts of Sumatra. The AAM variability proven has a significant role in the precipitation variability over the study area. A teleconnection between the AAM and other global circulations implies the precipitation variability over the northern part of Sumatra Island as a regional phenomenon. The large-scale tropical circulation is possibly related to the PWC modulation (Pacific Walker Circulation).


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