scholarly journals Stratospheric aerosol radiative forcing simulated by the chemistry climate model EMAC using aerosol CCI satellite data

2018 ◽  
Author(s):  
Christoph Brühl ◽  
Jennifer Schallock ◽  
Klaus Klingmüller ◽  
Charles Robert ◽  
Christine Bingen ◽  
...  
Keyword(s):  
Optical Depth ◽  
Radiative Forcing ◽  
General Circulation ◽  
Asian Summer Monsoon ◽  
Michelson Interferometer ◽  
Circulation Model ◽  
Volcanic Eruptions ◽  
Radiative Heating ◽  
Tropospheric Aerosol ◽  
Atmospheric Sounding

Abstract. This paper presents decadal simulations of stratospheric and tropospheric aerosol by the chemistry general circulation model EMAC constrained with satellite observations in the framework of the ESA-Aerosol-CCI project like GOMOS (Global Ozone Monitoring by Occultation of Stars) and (A)ATSR ((Advanced) Along Track Scanning Radiometer) on ENVISAT (European Environmental Satellite), and IASI (Infrared Atmospheric Sounding Interferometer) on Metop (Meteorological Operational Satellite). The EMAC simulations with modal interactive aerosol and observations by GOMOS show that sulfate particles from about 230 volcanic eruptions identified mostly from MIPAS (Michelson Interferometer for Passive Atmospheric Sounding) SO2 limb measurements dominate the interannual variability of aerosol extinction in the lower stratosphere, and of radiative forcing at the tropopause. To explain the observations, desert dust and organic and black carbon, transported to the lowermost stratosphere by the Asian summer monsoon and tropical convection, are also important. This holds also for radiative heating by aerosol in the lowermost stratosphere. Comparison with (A)ATSR total aerosol optical depth at different wavelengths and IASI dust optical depth shows that the model is able to represent stratospheric and tropospheric aerosol in a consistent way.

scholarly journals Stratospheric aerosol radiative forcing simulated by the chemistry climate model EMAC using Aerosol CCI satellite data

2018 ◽  
Vol 18 (17) ◽  
pp. 12845-12857 ◽  
Author(s):  
Christoph Brühl ◽  
Jennifer Schallock ◽  
Klaus Klingmüller ◽  
Charles Robert ◽  
Christine Bingen ◽  
...  
Keyword(s):  
Optical Depth ◽  
Radiative Forcing ◽  
Volcanic Eruptions ◽  
Stratospheric Aerosol ◽  
Radiative Heating ◽  
Aerosol Radiative Forcing ◽  
Tropospheric Aerosol ◽  
Model Aerosol ◽  
Atmospheric Sounding ◽  
Aerosol Radiative

Abstract. This paper presents decadal simulations of stratospheric and tropospheric aerosol and its radiative effects by the chemistry general circulation model EMAC constrained with satellite observations in the framework of the ESA Aerosol CCI project such as GOMOS (Global Ozone Monitoring by Occultation of Stars) and (A)ATSR ((Advanced) Along Track Scanning Radiometer) on the ENVISAT (European Environmental Satellite), IASI (Infrared Atmospheric Sounding Interferometer) on MetOp (Meteorological Operational Satellite), and, additionally, OSIRIS (Optical Spectrograph and InfraRed Imaging System). In contrast to most other studies, the extinctions and optical depths from the model are compared to the observations at the original wavelengths of the satellite instruments covering the range from the UV (ultraviolet) to terrestrial IR (infrared). This avoids conversion artifacts and provides additional constraints for model aerosol and interpretation of the observations. MIPAS (Michelson Interferometer for Passive Atmospheric Sounding) SO2 limb measurements are used to identify plumes of more than 200 volcanic eruptions. These three-dimensional SO2 plumes are added to the model SO2 at the eruption times. The interannual variability in aerosol extinction in the lower stratosphere, and of stratospheric aerosol radiative forcing at the tropopause, is dominated by the volcanoes. To explain the seasonal cycle of the GOMOS and OSIRIS observations, desert dust simulated by a new approach and transported to the lowermost stratosphere by the Asian summer monsoon and tropical convection turns out to be essential. This also applies to the radiative heating by aerosol in the lowermost stratosphere. The existence of wet dust aerosol in the lowermost stratosphere is indicated by the patterns of the wavelength dependence of extinction in observations and simulations. Additional comparison with (A)ATSR total aerosol optical depth at different wavelengths and IASI dust optical depth demonstrates that the model is able to represent stratospheric as well as tropospheric aerosol consistently.

scholarly journals Stratospheric SO<sub>2</sub> and sulphate aerosol, model simulations and satellite observations

2013 ◽  
Vol 13 (4) ◽  
pp. 11395-11425 ◽  
Author(s):  
C. Brühl ◽  
J. Lelieveld ◽  
M. Höpfner ◽  
H. Tost
Keyword(s):  
Atmospheric Chemistry ◽  
Radiative Forcing ◽  
General Circulation ◽  
Middle Atmosphere ◽  
Lower Boundary ◽  
Circulation Model ◽  
Volcanic Eruptions ◽  
Satellite Observations ◽  
Quasi Biennial Oscillation ◽  
Tropospheric Aerosol

Abstract. A multiyear study with the atmospheric chemistry general circulation model EMAC with the aerosol module GMXe at high altitude resolution demonstrates that the sulfur gases COS and SO2, the latter from low-latitude volcanic eruptions, predominantly control the formation of stratospheric aerosol. The model consistently uses the same parameters in the troposphere and stratosphere for 7 aerosol modes applied. Lower boundary conditions for COS and other long-lived trace gases are taken from measurement networks, while estimates of volcanic SO2 emissions are based on satellite observations. We show comparisons with satellite data for aerosol extinction (e.g. SAGE) and SO2 in the middle atmosphere (MIPAS on ENVISAT). This corroborates the interannual variability induced by the Quasi-Biennial Oscillation, which is internally generated by the model. The model also realistically simulates the radiative effects of stratospheric and tropospheric aerosol including the effects on the model dynamics. The medium strength volcanic eruptions of 2005 and 2006 exerted a nonnegligible radiative forcing of up to −0.6 W m−2 in the tropics, while the large Pinatubo eruption caused a maximum though short term tropical forcing of about −10 W m−2. The study also shows that observed upper stratospheric SO2 can be simulated accurately only when a sulphur sink on meteoritic dust is included and the photolysis of gaseous H2SO4 in the near infrared is higher than assumed previously.

scholarly journals Microphysical simulations of sulfur burdens from stratospheric sulfur geoengineering

2012 ◽  
Vol 12 (1) ◽  
pp. 2517-2558 ◽  
Author(s):  
J. M. English ◽  
O. B. Toon ◽  
M. J. Mills
Keyword(s):  
Optical Depth ◽  
Radiative Forcing ◽  
General Circulation ◽  
Climate Model ◽  
Regional Climate ◽  
Three Dimensional ◽  
Circulation Model ◽  
Injection Rate ◽  
Tropospheric Aerosol ◽  
So2 Gas

Abstract. Recent microphysical studies suggest that geoengineering by continuous stratospheric injection of SO2 gas may be limited by the growth of the aerosols. We study the efficacy of SO2, H2SO4 and aerosol injections on aerosol mass and optical depth using a three-dimensional general circulation model with sulfur chemistry and sectional aerosol microphysics (WACCM/CARMA). We find increasing injection rates of SO2 in a narrow band around the equator to have limited efficacy while broadening the injecting zone as well as injecting particles instead of SO2 gas increases the sulfate burden for a given injection rate, in agreement with previous work. We find that injecting H2SO4 gas instead of SO2 does not discernibly alter sulfate size or mass, in contrast with a previous study using a plume model with a microphysical model. However, the physics and chemistry in aircraft plumes, which are smaller than climate model grid cells, need to be more carefully considered. We find equatorial injections increase aerosol optical depth in the Northern Hemisphere more than the Southern Hemisphere, potentially inducing regional climate changes. We also find significant perturbations to tropospheric aerosol for all injections studied, particularly in the upper troposphere and near the poles, where sulfate burden increases by up to 100 times. This enhanced burden could have implications for tropospheric radiative forcing and chemistry. These results highlight the need to mitigate greenhouse gas emissions through means other than geoengineering, and to further study geoengineering before it can be seriously considered as a climate intervention option.

Modelling high-latitude explosive eruptions and their atmospheric and environmental impacts

2021 ◽  
Author(s):  
Herman Fuglestvedt ◽  
Zhihong Zhuo ◽  
Michael Sigl ◽  
Matthew Toohey ◽  
Michael Mills ◽  
...  
Keyword(s):  
Environmental Impacts ◽  
High Latitude ◽  
Radiative Forcing ◽  
General Circulation ◽  
Lower Thermosphere ◽  
Circulation Model ◽  
Ice Cores ◽  
Volcanic Eruptions ◽  
Explosive Eruptions ◽  
Sulphate Deposition

&lt;p&gt;Large explosive volcanic eruptions inject sulphur into the stratosphere where it is converted to sulphur dioxide and sulphate aerosols. Due to atmospheric circulation patterns, aerosols from high-latitude eruptions typically remain concentrated in the hemisphere in which they are injected. Eruptions in the high-latitude Northern Hemisphere could thus lead to a stronger hemispheric radiative forcing and surface climate response than tropical eruptions, a claim that is supported by a previous study based on proxy records and the coupled aerosol-general circulation model MAECHAM5-HAM. Additionally, the subsequent surface deposition of volcanic sulphate is potentially harmful to humans and ecosystems, and an improved understanding of the deposition over polar ice sheets can contribute to better reconstructions of historical volcanic forcing. On this basis, we model Icelandic explosive eruptions in a pre-industrial atmosphere, taking both volcanic sulphur and halogen loading into account. We use the fully coupled Earth system model CESM2 with the atmospheric component WACCM6, which extends to the lower thermosphere and has prognostic stratospheric aerosols and full chemistry. In order to study the volcanic impacts on the atmosphere, environment, and sulphate deposition, we vary eruption parameters such as sulphur and halogen loading, and injection altitude and season. The modelled volcanic sulphate deposition is compared to the deposition in ice cores following comparable historical eruptions. Furthermore, we evaluate the potential environmental impacts of sulphate deposition. To study inter-model differences, we also compare the CESM2-WACCM6 simulations to similar Icelandic eruption experiments simulated with MAECHAM5-HAM.&amp;#160;&lt;/p&gt;

scholarly journals Microphysical simulations of sulfur burdens from stratospheric sulfur geoengineering

2012 ◽  
Vol 12 (10) ◽  
pp. 4775-4793 ◽  
Author(s):  
J. M. English ◽  
O. B. Toon ◽  
M. J. Mills
Keyword(s):  
Radiative Forcing ◽  
General Circulation ◽  
Climate Model ◽  
Three Dimensional ◽  
Circulation Model ◽  
Injection Rate ◽  
Sulfur Chemistry ◽  
Aerosol Mass ◽  
Tropospheric Aerosol ◽  
So2 Gas

Abstract. Recent microphysical studies suggest that geoengineering by continuous stratospheric injection of SO2 gas may be limited by the growth of the aerosols. We study the efficacy of SO2, H2SO4 and aerosol injections on aerosol mass and optical depth using a three-dimensional general circulation model with sulfur chemistry and sectional aerosol microphysics (WACCM/CARMA). We find increasing injection rates of SO2 in a narrow band around the equator to have limited efficacy while broadening the injecting zone as well as injecting particles instead of SO2 gas increases the sulfate burden for a given injection rate, in agreement with previous work. We find that injecting H2SO4 gas instead of SO2 does not discernibly alter sulfate size or mass, in contrast with a previous study using a plume model with a microphysical model. However, the physics and chemistry in aircraft plumes, which are smaller than climate model grid cells, need to be more carefully considered. We also find significant perturbations to tropospheric aerosol for all injections studied, particularly in the upper troposphere and near the poles, where sulfate burden increases by up to 100 times. This enhanced burden could have implications for tropospheric radiative forcing and chemistry. These results highlight the need to mitigate greenhouse gas emissions rather than attempt to cool the planet through geoengineering, and to further study geoengineering before it can be seriously considered as a climate intervention option.

scholarly journals Competing Atmospheric and Surface-Driven Impacts of Absorbing Aerosols on the East Asian Summertime Climate

2017 ◽  
Vol 30 (22) ◽  
pp. 8929-8949 ◽  
Author(s):  
Geeta G. Persad ◽  
David J. Paynter ◽  
Yi Ming ◽  
V. Ramaswamy
Keyword(s):  
Land Surface ◽  
Radiative Forcing ◽  
General Circulation ◽  
Asian Summer Monsoon ◽  
Regional Climate ◽  
East Asian ◽  
Circulation Model ◽  
Anthropogenic Aerosols ◽  
Atmospheric Heating ◽  
Absorbing Aerosols

East Asia has some of the largest concentrations of absorbing aerosols globally, and these, along with the region’s scattering aerosols, have both reduced the amount of solar radiation reaching Earth’s surface regionally (solar dimming) and increased shortwave absorption within the atmosphere, particularly during the peak months of the East Asian summer monsoon (EASM). This study analyzes how atmospheric absorption and surface solar dimming compete in driving the response of regional summertime climate to anthropogenic aerosols, which dominates, and why—issues of particular importance for predicting how East Asian climate will respond to projected changes in absorbing and scattering aerosol emissions in the future. These questions are probed in a state-of-the-art general circulation model using a combination of realistic and novel idealized aerosol perturbations that allow analysis of the relative influence of absorbing aerosols’ atmospheric and surface-driven impacts on regional circulation and climate. Results show that even purely absorption-driven dimming decreases EASM precipitation by cooling the land surface, counteracting climatological land–sea contrast and reducing ascending atmospheric motion and onshore winds, despite the associated positive top-of-the-atmosphere regional radiative forcing. Absorption-driven atmospheric heating does partially offset the precipitation and surface evaporation reduction from surface dimming, but the overall response to aerosol absorption more closely resembles the response to its surface dimming than to its atmospheric heating. These findings provide a novel decomposition of absorbing aerosol’s impacts on regional climate and demonstrate that the response cannot be expected to follow the sign of absorption’s top-of-the-atmosphere or even atmospheric radiative perturbation.

scholarly journals The Sectional Stratospheric Sulfate Aerosol module (S3A-v1) within the LMDZ general circulation model: description and evaluation against stratospheric aerosol observations

2017 ◽  
Vol 10 (9) ◽  
pp. 3359-3378 ◽  
Author(s):  
Christoph Kleinschmitt ◽  
Olivier Boucher ◽  
Slimane Bekki ◽  
François Lott ◽  
Ulrich Platt
Keyword(s):  
Atmospheric Chemistry ◽  
General Circulation ◽  
Circulation Model ◽  
Volcanic Eruptions ◽  
Stratospheric Aerosol ◽  
Climate Impacts ◽  
Radiative Heating ◽  
Model Description ◽  
Quasi Biennial Oscillation ◽  
Microphysical Processes

Abstract. Stratospheric aerosols play an important role in the climate system by affecting the Earth's radiative budget as well as atmospheric chemistry, and the capabilities to simulate them interactively within global models are continuously improving. It is important to represent accurately both aerosol microphysical and atmospheric dynamical processes because together they affect the size distribution and the residence time of the aerosol particles in the stratosphere. The newly developed LMDZ-S3A model presented in this article uses a sectional approach for sulfate particles in the stratosphere and includes the relevant microphysical processes. It allows full interaction between aerosol radiative effects (e.g. radiative heating) and atmospheric dynamics, including e.g. an internally generated quasi-biennial oscillation (QBO) in the stratosphere. Sulfur chemistry is semi-prescribed via climatological lifetimes. LMDZ-S3A reasonably reproduces aerosol observations in periods of low (background) and high (volcanic) stratospheric sulfate loading, but tends to overestimate the number of small particles and to underestimate the number of large particles. Thus, it may serve as a tool to study the climate impacts of volcanic eruptions, as well as the deliberate anthropogenic injection of aerosols into the stratosphere, which has been proposed as a method of geoengineering to abate global warming.

scholarly journals A new radiation infrastructure for the Modular Earth Submodel System (MESSy, based on version 2.51)

2016 ◽  
Author(s):  
Simone Dietmüller ◽  
Patrick Jöckel ◽  
Holger Tost ◽  
Markus Kunze ◽  
Cathrin Gellhorn ◽  
...  
Keyword(s):  
Optical Properties ◽  
Atmospheric Chemistry ◽  
Radiative Forcing ◽  
General Circulation ◽  
Circulation Model ◽  
Shortwave Radiation ◽  
Aerosol Optical Properties ◽  
On Line ◽  
User Friendly ◽  
Radiation Scheme

Abstract. The Modular Earth Submodel System (MESSy) provides an interface to couple submodels to a basemodel via a highly flexible data management facility (Jöckel et al., 2010). In the present paper we present the four new radiation related submodels RAD, AEROPT, CLOUDOPT and ORBIT. The submodel RAD (with shortwave radiation scheme RAD_FUBRAD) simulates the radiative transfer, the submodel AEROPT calculates the aerosol optical properties, the submodel CLOUDOPT calculates the cloud optical properties, and the submodel ORBIT is responsible for Earth orbit calculations. These submodels are coupled via the standard MESSy infrastructure and are largely based on the original radiation scheme of the general circulation model ECHAM5, however, expanded with additional features. These features comprise, among others, user-friendly and flexibly controllable (by namelists) on-line radiative forcing calculations by multiple diagnostic calls of the radiation routines. With this, it is now possible to calculate radiative forcing (instantaneous as well as stratosphere adjusted) of various greenhouse gases simultaneously in only one simulation, as well as the radiative forcing of cloud perturbations. Examples of on-line radiative forcing calculations in the ECHAM/MESSy Atmospheric Chemistry (EMAC) model are presented.

scholarly journals Climatic effects of 1950–2050 changes in US anthropogenic aerosols – Part 1: Aerosol trends and radiative forcing

2011 ◽  
Vol 11 (8) ◽  
pp. 24085-24125 ◽  
Author(s):  
E. M. Leibensperger ◽  
L. J. Mickley ◽  
D. J. Jacob ◽  
W.-T. Chen ◽  
J. H. Seinfeld ◽  
...  
Keyword(s):  
Radiative Forcing ◽  
General Circulation ◽  
Transport Model ◽  
Circulation Model ◽  
Anthropogenic Sources ◽  
So2 Emissions ◽  
Anthropogenic Aerosols ◽  
Climatic Effects ◽  
Anthropogenic Aerosol ◽  
Direct Forcing

Abstract. We use the GEOS-Chem chemical transport model combined with the GISS general circulation model to calculate the aerosol direct and indirect (warm cloud) radiative forcings from US anthropogenic sources over the 1950–2050 period, based on historical emission inventories and future projections from the IPCC A1B scenario. The aerosol simulation is evaluated with observed spatial distributions and 1980–2010 trends of aerosol concentrations and wet deposition in the contiguous US. The radiative forcing from US anthropogenic aerosols is strongly localized over the eastern US. We find that it peaked in 1970–1990, with values over the eastern US (east of 100° W) of −2.0 W m−2 for direct forcing including contributions from sulfate (−2.0 W m−2), nitrate (−0.2 W m−2), organic carbon (−0.2 W m−2), and black carbon (+0.4 W m−2). The aerosol indirect effect is of comparable magnitude to the direct forcing. We find that the forcing declined sharply from 1990 to 2010 (by 0.8 W m−2 direct and 1.0 W m−2 indirect), mainly reflecting decreases in SO2 emissions, and project that it will continue declining post-2010 but at a much slower rate since US SO2 emissions have already declined by almost 60 % from their peak. This suggests that much of the warming effect of reducing US anthropogenic aerosol sources may have already been realized by 2010, however some additional warming is expected through 2020. The small positive radiative forcing from US BC emissions (+0.3 W m−2 over the eastern US in 2010) suggests that an emission control strategy focused on BC would have only limited climate benefit.

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