scholarly journals On inferring isoprene emission surface flux from atmospheric boundary layer concentration measurements

2009 ◽  
Vol 9 (11) ◽  
pp. 3629-3640 ◽  
Author(s):  
J. Vilà-Guerau de Arellano ◽  
K. van den Dries ◽  
D. Pino
Keyword(s):  
Boundary Layer ◽  
Mixed Layer ◽  
Convective Boundary Layer ◽  
Surface Flux ◽  
Lapse Rate ◽  
Accurate Estimation ◽  
Emission Flux ◽  
Convective Boundary ◽  
Diurnal Variability ◽  
Layer Technique

Abstract. We examine the dependence of the inferred isoprene surface emission flux from atmospheric concentration on the diurnal variability of the convective boundary layer (CBL). A series of systematic numerical experiments carried out using the mixed-layer technique enabled us to study the sensitivity of isoprene fluxes to the entrainment process, the partition of surface fluxes, the horizontal advection of warm/cold air masses and subsidence. Our findings demonstrate the key role played by the evolution of boundary layer height in modulating the retrieved isoprene flux. More specifically, inaccurate values of the potential temperature lapse rate lead to changes in the dilution capacity of the CBL and as a result the isoprene flux may be overestimated or underestimated by as much as 20%. The inferred emission flux estimated in the early morning hours is highly dependent on the accurate estimation of the discontinuity of the thermodynamic values between the residual layer and the rapidly forming CBL. Uncertainties associated with the partition of the sensible and latent heat flux also yield large deviations in the calculation of the isoprene surface flux. Similar results are obtained if we neglect the influence of warm or cold advection in the development of the CBL. We show that all the above-mentioned processes are non-linear, for which reason the dynamic and chemical evolutions of the CBL must be solved simultaneously. Based on the discussion of our results, we suggest the measurements needed to correctly apply the mixed-layer technique in order to minimize the uncertainties associated with the diurnal variability of the convective boundary layer.

scholarly journals On inferring isoprene emission surface flux from atmospheric boundary layer concentration measurements

2009 ◽  
Vol 9 (1) ◽  
pp. 4159-4193
Author(s):  
J. Vilà-Guerau de Arellano ◽  
K. van den Dries ◽  
D. Pino
Keyword(s):  
Boundary Layer ◽  
Mixed Layer ◽  
Convective Boundary Layer ◽  
Surface Flux ◽  
Lapse Rate ◽  
Accurate Estimation ◽  
Emission Flux ◽  
Convective Boundary ◽  
Diurnal Variability ◽  
Layer Technique

Abstract. We examine the dependence of the inferred isoprene surface emission flux from atmospheric concentration on the diurnal variability of the convective boundary layer (CBL). A series of systematic numerical experiments carried out using the mixed-layer technique enabled us to study the sensitivity of isoprene fluxes to the entrainment process, the partition of surface fluxes, the horizontal advection of warm/cold air masses and subsidence. Our findings demonstrate the key role played by the evolution of boundary layer height in modulating the retrieved isoprene flux. More specifically, inaccurate values of the potential temperature lapse rate lead to changes in the dilution capacity of the CBL and as a result the isoprene flux may be overestimated or underestimated by as much as 20%. The inferred emission flux estimated in the early morning hours is highly dependent on the accurate estimation of the discontinuity of the thermodynamic values between the residual layer and the rapidly forming CBL. Uncertainties associated with the partition of the sensible and latent heat flux also yield large deviations in the calculation of the isoprene surface flux. Similar results are obtained if we neglect the influence of warm or cold advection in the development of the CBL. We show that all the above-mentioned processes are non-linear, for which reason the dynamic and chemical evolutions of the CBL must be solved simultaneously. Based on the discussion of our results, we suggest the measurements needed to correctly apply the mixed-layer technique in order to minimize the uncertainties associated with the diurnal variability of the convective boundary layer.

scholarly journals Reexamining the Gradient and Countergradient Representation of the Local and Nonlocal Heat Fluxes in the Convective Boundary Layer

2018 ◽  
Vol 75 (7) ◽  
pp. 2317-2336 ◽  
Author(s):  
Bowen Zhou ◽  
Shiwei Sun ◽  
Kai Yao ◽  
Kefeng Zhu
Keyword(s):  
Boundary Layer ◽  
Temperature Gradient ◽  
Mixed Layer ◽  
Convective Boundary Layer ◽  
Correction Term ◽  
Potential Temperature ◽  
Heat Fluxes ◽  
Gradient Term ◽  
Convective Boundary ◽  
Upper Mixed Layer

Abstract Turbulent mixing in the daytime convective boundary layer (CBL) is carried out by organized nonlocal updrafts and smaller local eddies. In the upper mixed layer of the CBL, heat fluxes associated with nonlocal updrafts are directed up the local potential temperature gradient. To reproduce such countergradient behavior in parameterizations, a class of planetary boundary layer schemes adopts a countergradient correction term in addition to the classic downgradient eddy-diffusion term. Such schemes are popular because of their simple formulation and effective performance. This study reexamines those schemes to investigate the physical representations of the gradient and countergradient (GCG) terms, and to rebut the often-implied association of the GCG terms with heat fluxes due to local and nonlocal (LNL) eddies. To do so, large-eddy simulations (LESs) of six idealized CBL cases are performed. The GCG fluxes are computed a priori with horizontally averaged LES data, while the LNL fluxes are diagnosed through conditional sampling and Fourier decomposition of the LES flow field. It is found that in the upper mixed layer, the gradient term predicts downward fluxes in the presence of positive mean potential temperature gradient but is compensated by the upward countergradient correction flux, which is larger than the total heat flux. However, neither downward local fluxes nor larger-than-total nonlocal fluxes are diagnosed from LES. The difference reflects reduced turbulence efficiency for GCG fluxes and, in terms of physics, conceptual deficiencies in the GCG representation of CBL heat fluxes.

scholarly journals Role of the residual layer and large-scale subsidence on the development and evolution of the convective boundary layer

2013 ◽  
Vol 13 (12) ◽  
pp. 31527-31562 ◽  
Author(s):  
E. Blay-Carreras ◽  
D. Pino ◽  
A. Van de Boer ◽  
O. De Coster ◽  
C. Darbieu ◽  
...  
Keyword(s):  
Boundary Layer ◽  
Mixed Layer ◽  
Convective Boundary Layer ◽  
Large Scale ◽  
Temporal Evolution ◽  
Residual Layer ◽  
Mixing Ratio ◽  
Convective Boundary ◽  
Previous Night ◽  
Morning Transition

Abstract. Observations, mixed-layer theory and the Dutch Large-Eddy Simulation model (DALES) are used to analyze the dynamics of the boundary layer during an intensive operational period (1 July 2011) of the Boundary Layer Late Afternoon and Sunset Turbulence campaign. Continuous measurements made by remote sensing and in situ instruments in combination with radio soundings, and measurements done by remotely piloted airplane systems and two aircrafts probed the vertical structure and the temporal evolution of the boundary layer during the campaign. The initial vertical profiles of potential temperature, specific humidity and wind, and the temporal evolution of the surface heat and moisture fluxes prescribed in the numerical simulations are inspired by some of these observations. The research focuses on the role played by the residual layer during the morning transition and by the large-scale subsidence on the evolution of the boundary layer. By using DALES, we show the importance of the dynamics of the boundary layer during the previous night in the development of the boundary layer at the morning. DALES numerical experiments including the residual layer are capable to model the observed sudden increase of the boundary-layer depth during the morning transition and the subsequent evolution of the boundary layer. The simulation shows a large increase of the entrainment buoyancy heat flux when the residual layer is incorporated into the mixed layer. We also examine how the inclusion of the residual layer above a shallow convective boundary layer modifies the turbulent kinetic energy budget. Large-scale subsidence mainly acts when the boundary layer is fully developed and, for the studied day, it is necessary to be considered to reproduce the afternoon observations. Additionally, we investigate how carbon dioxide (CO2) mixing ratio stored the previous night in the residual layer plays a fundamental role in the evolution of the CO2 mixing ratio during the following day.

scholarly journals Integrating canopy and large-scale effects in the convective boundary-layer dynamics during the CHATS experiment

2017 ◽  
Vol 17 (3) ◽  
pp. 1623-1640 ◽  
Author(s):  
Metodija M. Shapkalijevski ◽  
Huug G. Ouwersloot ◽  
Arnold F. Moene ◽  
Jordi Vilà-Guerau de Arrellano
Keyword(s):  
Boundary Layer ◽  
Latent Heat ◽  
Convective Boundary Layer ◽  
Friction Velocity ◽  
Surface Fluxes ◽  
Convective Boundary ◽  
Diurnal Variability ◽  
Drag Coefficients ◽  
Boundary Layer Dynamics ◽  
The Impact

Abstract. By characterizing the dynamics of a convective boundary layer above a relatively sparse and uniform orchard canopy, we investigated the impact of the roughness-sublayer (RSL) representation on the predicted diurnal variability of surface fluxes and state variables. Our approach combined numerical experiments, using an atmospheric mixed-layer model including a land-surface-vegetation representation, and measurements from the Canopy Horizontal Array Turbulence Study (CHATS) field experiment near Dixon, California. The RSL is parameterized using an additional factor in the standard Monin–Obukhov similarity theory flux-profile relationships that takes into account the canopy influence on the atmospheric flow. We selected a representative case characterized by southerly wind conditions to ensure well-developed RSL over the orchard canopy. We then investigated the sensitivity of the diurnal variability of the boundary-layer dynamics to the changes in the RSL key scales, the canopy adjustment length scale, Lc, and the β = u*/|U| ratio at the top of the canopy due to their stability and dependence on canopy structure. We found that the inclusion of the RSL parameterization resulted in improved prediction of the diurnal evolution of the near-surface mean quantities (e.g. up to 50 % for the wind velocity) and transfer (drag) coefficients. We found relatively insignificant effects on the modelled surface fluxes (e.g. up to 5 % for the friction velocity, while 3 % for the sensible and latent heat), which is due to the compensating effect between the mean gradients and the drag coefficients, both of which are largely affected by the RSL parameterization. When varying Lc (from 10 to 20 m) and β (from 0.25 to 0.4 m), based on observational evidence, the predicted friction velocity is found to vary by up to 25 % and the modelled surface-energy fluxes (sensible heat, SH, and latent heat of evaporation, LE) vary up to 2 and 9 %. Consequently, the boundary-layer height varies up to 6 %. Furthermore, our analysis indicated that to interpret the CHATS measurements above the canopy, the contributions of non-local effects such as entrainment, subsidence and the advection of heat and moisture over the CHATS site need to be taken into account.

scholarly journals The Impact of Sensor Response and Airspeed on the Representation of the Convective Boundary Layer and Airmass Boundaries by Small Unmanned Aircraft Systems

2018 ◽  
Vol 35 (8) ◽  
pp. 1687-1699 ◽  
Author(s):  
Adam L. Houston ◽  
Jason M. Keeler
Keyword(s):  
Boundary Layer ◽  
Convective Boundary Layer ◽  
Sensor Response ◽  
Unmanned Aircraft ◽  
Unmanned Aircraft Systems ◽  
Lapse Rate ◽  
Convective Boundary ◽  
Aircraft Systems ◽  
The Impact ◽  
Rotary Wing

AbstractThe objective of the research presented is to assess the impact of sensor response and aircraft airspeed on the accuracy of in situ observations collected by small unmanned aircraft systems profiling the convective boundary layer or transecting airmass boundaries. Estimates are made using simulated aircraft flown within large-eddy simulations. Both instantaneous errors (differences between observed temperature, which include the effects of sensor response and airspeed, and actual temperature) and errors in representation (differences between serial observations and representative snapshots of the atmospheric state) are considered. Synthetic data are retrieved assuming a well-aspirated first-order sensor mounted on rotary-wing aircraft operated as profilers in a simulated CBL and fixed-wing aircraft operated through transects across a simulated airmass boundary. Instantaneous errors are found to scale directly with sensor response time and airspeed for both CBL and airmass boundary experiments. Maximum errors tend to be larger for airmass boundary transects compared to the CBL profiles. Instantaneous errors for rotary-wing aircraft profiles in the CBL simulated for this work are attributable to the background lapse rate and not to turbulent temperature perturbations. For airmass boundary flights, representation accuracy is found to degrade with decreasing airspeed. This signal is most pronounced for flights that encounter the density current wake. When representation errors also include instantaneous errors resulting from sensor response, instantaneous errors are found to be dominant for flights that remain below the turbulent wake. However, for flights that encounter the wake, sensor response times generally need to exceed ~5 s before instantaneous errors become larger than errors in representation.

scholarly journals Scalar Turbulence in Convective Boundary Layers by Changing the Entrainment Flux

2013 ◽  
Vol 70 (1) ◽  
pp. 248-265 ◽  
Author(s):  
Alessandra S. Lanotte ◽  
Irene M. Mazzitelli
Keyword(s):  
Boundary Layer ◽  
Convective Boundary Layer ◽  
Spatial Scales ◽  
Surface Flux ◽  
Scalar Fields ◽  
Temperature Inversion ◽  
Trace Gas ◽  
Free Atmosphere ◽  
Convective Boundary ◽  
Homogeneous Surface

Abstract A large-eddy simulation model is adopted to investigate the evolution of scalars transported by atmospheric cloud-free convective boundary layer flows. Temperature fluctuations due to the ground release of sensible heat and concentration fluctuations of a trace gas emitted at the homogeneous surface are mixed by turbulence within the unstable boundary layer. On the top, the entrainment zone is varied to obtain two distinct situations: (i) the temperature inversion is strong and the trace gas increment across the entrainment region is small, yielding to a small top flux with respect to the surface emission; (ii) the temperature inversion at the top of the convective boundary layer is weak, and the scalar increment large enough to achieve a concentration flux toward the free atmosphere that overwhelms the surface flux. In both cases, an estimation of the entrainment flux is obtained within a simple model, and it is tested against numerical data. The evolution of the scalar profiles is discussed in terms of the different entrainment–surface flux ratios. Results show that, when entrainment at the top of the boundary layer is weak, temperature and trace gas scalar fields are strongly correlated, particularly in the lower part of the boundary layer. This means that they exhibit similar behavior from the largest down to the smallest spatial scales. However, when entrainment is strong, as moving from the surface, differences in the transport of the two scalars arise. Finally, it is shown that, independently of the scalar regime, the temperature field exhibits more intermittent fluctuations than the trace gas.

scholarly journals The Influence of Idealized Heterogeneity on Wet and Dry Planetary Boundary Layers Coupled to the Land Surface

2005 ◽  
Vol 62 (7) ◽  
pp. 2078-2097 ◽  
Author(s):  
Edward G. Patton ◽  
Peter P. Sullivan ◽  
Chin-Hoh Moeng
Keyword(s):  
Boundary Layer ◽  
Boundary Layers ◽  
Convective Boundary Layer ◽  
Land Surface ◽  
Surface Flux ◽  
Scalar Fields ◽  
Surface Fluxes ◽  
Convective Boundary ◽  
Turbulent Statistics ◽  
The Impact

Abstract This manuscript describes numerical experiments investigating the influence of 2–30-km striplike heterogeneity on wet and dry convective boundary layers coupled to the land surface. The striplike heterogeneity is shown to dramatically alter the structure of the convective boundary layer by inducing significant organized circulations that modify turbulent statistics. The impact, strength, and extent of the organized motions depend critically on the scale of the heterogeneity λ relative to the boundary layer height zi. The coupling with the land surface modifies the surface fluxes and hence the circulations resulting in some differences compared to previous studies using fixed surface forcing. Because of the coupling, surface fluxes in the middle of the patches are small compared to the patch edges. At large heterogeneity scales (λ/zi ∼18) horizontal surface-flux gradients within each patch are strong enough to counter the surface-flux gradients between wet and dry patches allowing the formation of small cells within the patch coexisting with the large-scale patch-induced circulations. The strongest patch-induced motions occur in cases with 4 < λ/zi < 9 because of strong horizontal pressure gradients across the wet and dry patches. Total boundary layer turbulence kinetic energy increases significantly for surface heterogeneity at scales between λ/zi = 4 and 9; however, entrainment rates for all cases are largely unaffected by the striplike heterogeneity. Velocity and scalar fields respond differently to variations of heterogeneity scale. The patch-induced motions have little influence on total vertical scalar flux, but the relative contribution to the flux from organized motions compared to background turbulence varies with heterogeneity scale. Patch-induced motions are shown to dramatically impact point measurements in a free-convective boundary layer. The magnitude and sign of this impact depends on the location of the measurement within the region of heterogeneity.

scholarly journals A Grid-Refinement-Based Approach for Modeling the Convective Boundary Layer in the Gray Zone: A Pilot Study

2017 ◽  
Vol 74 (11) ◽  
pp. 3497-3513 ◽  
Author(s):  
Bowen Zhou ◽  
Ming Xue ◽  
Kefeng Zhu
Keyword(s):  
Boundary Layer ◽  
Surface Layer ◽  
Mixed Layer ◽  
Convective Boundary Layer ◽  
Analytic Model ◽  
Gray Zone ◽  
Ensemble Averaging ◽  
Convective Boundary ◽  
Fine Grid ◽  
Turbulence Closures

Abstract The model gray zone refers to the range of grid spacings comparable to the dominant length scale of the flow. In the gray zone, the flow is partially resolved and partially subgrid scale (SGS). Neither ensemble-averaging-based parameterizations nor turbulence closures are appropriate for parameterizing the effects of SGS motions on the resolved flow. The gray zone of the convective boundary layer (CBL) is in the range of CBL depth, typically O(1) km. A new approach that seeks explicit resolution of the unstable surface layer through a nest layer of fine grid spacing is proposed to improve CBL parameterization in the gray zone. To provide the theoretical basis for the approach, a linear analytic model is presented, and one-way nested simulations are performed to investigate the dynamical coupling between the surface layer and the mixed layer. The analytic model shows that at the onset of thermal instability, the vertical and horizontal structures of the mixed layer are set by surface-layer forcings. The nested 3D simulations extend the findings from the analytic model and further reveal potential improvements in high-order statistics and resolved convective structures both including and extending above the nest region compared to the stand-alone gray-zone simulations. This study suggests that when the most energetic scales of CBL convection are resolved in the surface layer, the overall simulation of the CBL improves at gray-zone resolutions.

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