scholarly journals Dust emission size distribution impact on aerosol budget and radiative forcing over the Mediterranean region: a regional climate model approach

2012 ◽  
Vol 12 (7) ◽  
pp. 17835-17886 ◽  
Author(s):  
P. Nabat ◽  
F. Solmon ◽  
M. Mallet ◽  
J. F. Kok ◽  
S. Somot

Abstract. The present study investigates the dust emission and load over the Mediterranean basin using the coupled-chemistry-aerosol regional climate model RegCM-4. The first step of this work focuses on dust particle emission size distribution modeling. We compare a parameterization in which the emission is based on the individual kinetic energy of the aggregates striking the surface to a recent parameterization based on an analogy with the fragmentation of brittle materials. The main difference between the two dust schemes concerns the mass proportion of fine aerosol which is reduced in the case of the new dust parameterization, with consequences for optical properties. At the episodic scale, comparisons between RegCM-4 simulations, satellite and ground-based data show a clear improvement using the new dust distribution in terms of Aerosol Optical Depth (AOD) values and geographic gradients. These results are confirmed at the seasonal scale for the investigated year 2008. A multi-annual simulation is finally carried out using the new dust distribution over the period 2000–2009. This change of dust distribution has sensitive impacts on the simulated regional dust budget, notably dry dust deposition and the regional direct aerosol radiative forcing over the Mediterranean basin. This could clearly modify the possible effects of dust aerosols on the biogeochemical activity and climate of the Mediterranean basin. In particular, we find that the new size distribution produces a higher dust deposition flux, and smaller top of atmosphere (TOA) dust radiative cooling.

2012 ◽  
Vol 12 (21) ◽  
pp. 10545-10567 ◽  
Author(s):  
P. Nabat ◽  
F. Solmon ◽  
M. Mallet ◽  
J. F. Kok ◽  
S. Somot

Abstract. The present study investigates the dust emission and load over the Mediterranean basin using the coupled chemistry–aerosol–regional climate model RegCM-4. The first step of this work focuses on dust particle emission size distribution modeling. We compare a parameterization in which the emission is based on the individual kinetic energy of the aggregates striking the surface to a recent parameterization based on an analogy with the fragmentation of brittle materials. The main difference between the two dust schemes concerns the mass proportion of fine aerosol that is reduced in the case of the new dust parameterization, with consequences for optical properties. At the episodic scale, comparisons between RegCM-4 simulations, satellite and ground-based data show a clear improvement using the new dust distribution in terms of aerosol optical depth (AOD) values and geographic gradients. These results are confirmed at the seasonal scale for the investigated year 2008. This change of dust distribution has sensitive impacts on the simulated regional dust budget, notably dry dust deposition and the regional direct aerosol radiative forcing over the Mediterranean basin. In particular, we find that the new size distribution produces a higher dust deposition flux, and smaller top of atmosphere (TOA) dust radiative cooling. A multi-annual simulation is finally carried out using the new dust distribution over the period 2000–2009. The average SW radiative forcing over the Mediterranean Sea reaches −13.6 W m−2 at the surface, and −5.5 W m−2 at TOA. The LW radiative forcing is positive over the basin: 1.7 W m−2 on average over the Mediterranean Sea at the surface, and 0.6 W m−2 at TOA.


2017 ◽  
Vol 13 (3) ◽  
pp. 249-265 ◽  
Author(s):  
Odile Peyron ◽  
Nathalie Combourieu-Nebout ◽  
David Brayshaw ◽  
Simon Goring ◽  
Valérie Andrieu-Ponel ◽  
...  

Abstract. Climate evolution of the Mediterranean region during the Holocene exhibits strong spatial and temporal variability, which is notoriously difficult for models to reproduce. We propose here a new proxy-based climate synthesis synthesis and its comparison – at a regional (∼ 100 km) level – with a regional climate model to examine (i) opposing northern and southern precipitation regimes and (ii) an east-to-west precipitation dipole during the Holocene across the Mediterranean basin. Using precipitation estimates inferred from marine and terrestrial pollen archives, we focus on the early to mid-Holocene (8000 to 6000 cal yr BP) and the late Holocene (4000 to 2000 cal yr BP), to test these hypotheses on a Mediterranean-wide scale. Special attention was given to the reconstruction of season-specific climate information, notably summer and winter precipitation. The reconstructed climatic trends corroborate the north–south partition of precipitation regimes during the Holocene. During the early Holocene, relatively wet conditions occurred in the south–central and eastern Mediterranean regions, while drier conditions prevailed from 45° N northwards. These patterns then reverse during the late Holocene. With regard to the existence of a west–east precipitation dipole during the Holocene, our results show that the strength of this dipole is strongly linked to the reconstructed seasonal parameter; early-Holocene summers show a clear east–west division, with summer precipitation having been highest in Greece and the eastern Mediterranean and lowest over Italy and the western Mediterranean. Summer precipitation in the east remained above modern values, even during the late-Holocene interval. In contrast, winter precipitation signals are less spatially coherent during the early Holocene but low precipitation is evidenced during the late Holocene. A general drying trend occurred from the early to late Holocene, particularly in the central and eastern Mediterranean. For the same time intervals, pollen-inferred precipitation estimates were compared with model outputs, based on a regional-scale downscaling (HadRM3) of a set of global climate-model simulations (HadAM3). The high-resolution detail achieved through the downscaling is intended to enable a better comparison between site-based paleo-reconstructions and gridded model data in the complex terrain of the Mediterranean; the model outputs and pollen-inferred precipitation estimates show some overall correspondence, though modeled changes are small and at the absolute margins of statistical significance. There are suggestions that the eastern Mediterranean experienced wetter summer conditions than present during the early and late Holocene; the drying trend in winter from the early to the late Holocene also appears to be simulated. The use of this high-resolution regional climate model highlights how the inherently patchy nature of climate signals and paleo-records in the Mediterranean basin may lead to local signals that are much stronger than the large-scale pattern would suggest. Nevertheless, the east-to-west division in summer precipitation seems more marked in the pollen reconstruction than in the model outputs. The footprint of the anomalies (like today, or dry winters and wet summers) has some similarities to modern analogue atmospheric circulation patterns associated with a strong westerly circulation in winter (positive Arctic Oscillation–North Atlantic Oscillation (AO–NAO)) and a weak westerly circulation in summer associated with anticyclonic blocking; however, there also remain important differences between the paleo-simulations and these analogues. The regional climate model, consistent with other global models, does not suggest an extension of the African summer monsoon into the Mediterranean. Therefore, the extent to which summer monsoonal precipitation may have existed in the southern and eastern Mediterranean during the mid-Holocene remains an outstanding question.


2017 ◽  
Vol 17 (2) ◽  
pp. 769-791 ◽  
Author(s):  
Athanasios Tsikerdekis ◽  
Prodromos Zanis ◽  
Allison L. Steiner ◽  
Fabien Solmon ◽  
Vassilis Amiridis ◽  
...  

Abstract. We investigate the sensitivity of aerosol representation in the regional climate model RegCM4 for two dust parameterizations for the period 2007–2014 over the Sahara and the Mediterranean. We apply two discretization methods of the dust size distribution keeping the total mass constant: (1) the default RegCM4 4-bin approach, where the size range of each bin is calculated using an equal, logarithmic separation of the total size range of dust, using the diameter of dust particles, and (2) a newly implemented 12-bin approach with each bin defined according to an isogradient method where the size ranges are dependent on the dry deposition velocity of dust particles. Increasing the number of transported dust size bins theoretically improves the representation of the physical properties of dust particles within the same size bin. Thus, more size bins improve the simulation of atmospheric processes. The radiative effects of dust over the area are discussed and evaluated with the CALIPSO dust optical depth (DOD). This study is among the first studies evaluating the vertical profile of simulated dust with a pure dust product. Reanalysis winds from ERA-Interim and the total precipitation flux from the Climate Research Unit (CRU) observational gridded database are used to evaluate and explain the discrepancies between model and observations. The new dust binning approach increases the dust column burden by 4 and 3 % for fine and coarse particles, respectively, which increases DOD by 10 % over the desert and the Mediterranean. Consequently, negative shortwave radiative forcing (RF) is enhanced by more than 10 % at the top of the atmosphere and by 1 to 5 % on the surface. Positive longwave RF locally increases by more than 0.1 W m−2 in a large portion of the Sahara, the northern part of the Arabian Peninsula and the Middle East. The four-bin isolog method is to some extent numerically efficient, nevertheless our work highlights that the simplified representation of the four-bin approach produces less dust optical depth and RF, a fact that should be taken into account by future studies of the same region.


2015 ◽  
Vol 15 (14) ◽  
pp. 8051-8064 ◽  
Author(s):  
F. Solmon ◽  
V. S. Nair ◽  
M. Mallet

Abstract. Over the past decade, aerosol optical depth (AOD) observations based on satellite and ground measurements have shown a significant increase over Arabia and the Arabian Sea, attributed to an intensification of regional dust activity. Recent studies have also suggested that west Asian dust forcing could induce a positive response of Indian monsoon precipitations on a weekly timescale. Using observations and a regional climate model including interactive slab-ocean and dust aerosol schemes, the present study investigates possible climatic links between the increasing June–July–August–September (JJAS) Arabian dust activity and precipitation trends over southern India during the 2000–2009 decade. Meteorological reanalysis and AOD observations suggest that the observed decadal increase of dust activity and a simultaneous intensification of summer precipitation trend over southern India are both linked to a deepening of JJAS surface pressure conditions over the Arabian Sea. In the first part of the study, we analyze the mean climate response to dust radiative forcing over the domain, discussing notably the relative role of Arabian vs. Indo-Pakistani dust regions. In the second part of the study, we show that the model skills in reproducing regional dynamical patterns and southern Indian precipitation trends are significantly improved only when an increasing dust emission trend is imposed on the basis of observations. We conclude that although interannual climate variability might primarily determine the observed regional pattern of increasing dust activity and precipitation during the 2000–2009 decade, the associated dust radiative forcing might in return induce a critical dynamical feedback contributing to enhancing regional moisture convergence and JJAS precipitations over southern India.


2015 ◽  
Vol 15 (4) ◽  
pp. 4879-4907 ◽  
Author(s):  
F. Solmon ◽  
V. S. Nair ◽  
M. Mallet

Abstract. Over the past decade, Aerosol Optical Depth (AOD) observations based on satellite and ground measurements have shown a significant increase over Arabia and the Arabian Sea, attributed to an intensification of regional dust activity. Recent studies have also suggested that west Asian dust forcing could induce a positive response of Indian monsoon precipitations on a weekly time scale. Using observations and a regional climate model including interactive slab ocean and dust aerosol schemes, the present study investigates possible climatic links between the increasing June-July-August-September (JJAS) Arabian dust activity and precipitation trends over southern India during the 2000–2009 decade. Meteorological reanalysis and AOD observations suggest that the observed decadal increase of dust activity and a simultaneous intensification of summer precipitation trend over southern India are both linked to a deepening of JJAS surface pressure conditions over the Arabian Sea. We show that the model skills in reproducing this trends and patterns are significantly improved only when an increasing dust emission trend is imposed on the basis of observations. We conclude that although climate variability might primarily determine the observed regional pattern of increasing dust activity and precipitation during the 2000–2009 decade, the associated dust radiative forcing might however induce a critical dynamical feedback contributing to enhanced regional moisture convergence and JJAS precipitation over Southern India.


2017 ◽  
Author(s):  
Nizar Jaidan ◽  
Laaziz El Amraoui ◽  
Jean-Luc Attié ◽  
Philippe Ricaud ◽  
François Dulac

Abstract. In the framework of the Chemistry and Aerosol Mediterranean Experiment project (ChArMEx, http://charmex.lsce.ipsl.fr), we study the evolution of surface ozone (O3) over the Mediterranean Basin (MB) with a focus on summertime over the time period 2000–2100, using the Atmospheric Chemistry and Climate Model Intercomparison Project (ACCMIP) outputs from 11 models. We consider three different periods (2000, 2030 and 2100) and the four Representative Concentration Pathways (RCP2.6, RCP4.5, RCP6.0 and RCP8.5) to study the changes in the future ozone trend and its budget. We use a statistical approach to compare and discuss the results of the models. We discuss the behavior of the models that simulate the surface O3 over the MB. The ensemble mean of ACCMIP models simulates very well the annual cycle of surface O3. Compared to measured summer surface O3 datasets, we found that most of the models overestimate surface O3 and underestimate its variability over the most recent period (1990–2010) when independent observations are available. Compared to the reference period (2000), we found a net decrease in the ensemble mean surface O3 over the MB in 2030 (2100) for 3 RCPs: −13 % (−36 %) for RCP2.6, −7 % (−22 %) for RCP4.5 and −11 % (−33 %) for RCP6.0. The surface O3 decrease over the MB for these scenarios is much more pronounced than the relative changes of the tropospheric ozone burden. This is mainly due to the reduction in O3 precursors and to the NOx-limited regime over the MB. For the RCP8.5, the ensemble mean surface O3 is almost constant over the MB from 2000 to 2100. We show how the future climate change and the increase in CH4 concentrations can offset the benefit of the reduction in emissions of O3 precursors over the MB.


2020 ◽  
Vol 13 (12) ◽  
pp. 5897-5915
Author(s):  
Laura Palacios-Peña ◽  
Jerome D. Fast ◽  
Enrique Pravia-Sarabia ◽  
Pedro Jiménez-Guerrero

Abstract. The size distribution of atmospheric aerosols plays a key role for understanding and quantifying the uncertainties related to aerosol–radiation and aerosol–cloud interactions. These interactions ultimately depend on the size distribution through optical properties (such as aerosol optical depth, AOD) or cloud microphysical properties. Hence, the main objective of this contribution is to disentangle the impact of the representation of aerosol size distribution on aerosol optical properties over central Europe, particularly over the Mediterranean Basin, during a summertime aerosol episode. To fulfill this objective, a sensitivity test has been conducted using the coupled chemistry–meteorology model WRF-Chem (Weather Research Forecast model coupled with Chemistry). The test modified the parameters defining a lognormal size distribution (geometric diameter and standard deviation) by 10 %, 20 %, and 50 %. Results reveal that the reduction in the standard deviation of the accumulation mode leads to the largest impacts on AOD due to a transfer of particles from the accumulation mode to the coarse mode. A reduction in the geometric diameter of the accumulation mode also has an influence on AOD representation since particles in this mode are assumed to be smaller. In addition, an increase in the geometric diameter of the coarse mode produces a redistribution through the total size distribution by relocating particles from the finer modes to the coarse.


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