scholarly journals Unexpectedly high ultrafine aerosol concentrations above East Antarctic sea-ice

2015 ◽  
Vol 15 (20) ◽  
pp. 29125-29170 ◽  
Author(s):  
R. S. Humphries ◽  
A. R. Klekociuk ◽  
R. Schofield ◽  
M. Keywood ◽  
J. Ward ◽  
...  

Abstract. The effect of aerosols on clouds and their radiative properties is one of the largest uncertainties in our understanding of radiative forcing. A recent study has concluded that better characterisation of pristine, natural aerosol processes leads to the largest reduction in these uncertainties. Antarctica, being far from anthropogenic activities, is an ideal location for the study of natural aerosol processes. Aerosol measurements in Antarctica are often limited to boundary layer air-masses at spatially sparse coastal and continental research stations, with only a handful of studies in the sea ice region. In this paper, the first observational study of sub-micron aerosols in the East Antarctic sea ice region is presented. Measurements were conducted aboard the ice-breaker Aurora Australis in spring 2012 and found that boundary layer condensation nuclei (CN3) concentrations exhibited a five-fold increase moving across the Polar Front, with mean Polar Cell concentrations of 1130 cm−3 – higher than any observed elsewhere in the Antarctic and Southern Ocean region. The absence of evidence for aerosol growth suggested that nucleation was unlikely to be local. Air parcel trajectories indicated significant influence from the free troposphere above the Antarctic continent, implicating this as the likely nucleation region for surface aerosol, a similar conclusion to previous Antarctic aerosol studies. The highest aerosol concentrations were found to correlate with low pressure systems, suggesting that the passage of cyclones provided an accelerated pathway, delivering air-masses quickly from the free-troposphere to the surface. After descent from the Antarctic free troposphere, trajectories suggest that sea ice boundary layer air-masses travelled equator-ward into the low albedo Southern Ocean region, transporting with them emissions and these aerosol nuclei where, after growth, may potentially impact on the region's radiative balance. The high aerosol concentrations and their transport pathways described here, could help reduce the discrepancy currently present between simulations and observations of cloud and aerosol over the Southern Ocean.

2016 ◽  
Vol 16 (4) ◽  
pp. 2185-2206 ◽  
Author(s):  
R. S. Humphries ◽  
A. R. Klekociuk ◽  
R. Schofield ◽  
M. Keywood ◽  
J. Ward ◽  
...  

Abstract. Better characterisation of aerosol processes in pristine, natural environments, such as Antarctica, have recently been shown to lead to the largest reduction in uncertainties in our understanding of radiative forcing. Our understanding of aerosols in the Antarctic region is currently based on measurements that are often limited to boundary layer air masses at spatially sparse coastal and continental research stations, with only a handful of studies in the vast sea-ice region. In this paper, the first observational study of sub-micron aerosols in the East Antarctic sea ice region is presented. Measurements were conducted aboard the icebreaker Aurora Australis in spring 2012 and found that boundary layer condensation nuclei (CN3) concentrations exhibited a five-fold increase moving across the polar front, with mean polar cell concentrations of 1130 cm−3 – higher than any observed elsewhere in the Antarctic and Southern Ocean region. The absence of evidence for aerosol growth suggested that nucleation was unlikely to be local. Air parcel trajectories indicated significant influence from the free troposphere above the Antarctic continent, implicating this as the likely nucleation region for surface aerosol, a similar conclusion to previous Antarctic aerosol studies. The highest aerosol concentrations were found to correlate with low-pressure systems, suggesting that the passage of cyclones provided an accelerated pathway, delivering air masses quickly from the free troposphere to the surface. After descent from the Antarctic free troposphere, trajectories suggest that sea-ice boundary layer air masses travelled equatorward into the low-albedo Southern Ocean region, transporting with them emissions and these aerosol nuclei which, after growth, may potentially impact on the region's radiative balance. The high aerosol concentrations and their transport pathways described here, could help reduce the discrepancy currently present between simulations and observations of cloud and aerosol over the Southern Ocean.


2021 ◽  
Author(s):  
Tristan Vadsaria ◽  
Sam Sherriff-Tadano ◽  
Ayako Abe-Ouchi ◽  
Takashi Obase ◽  
Wing-Le Chan ◽  
...  

<p>Southern Ocean sea ice and oceanic fronts are known to play an important role on the climate system, carbon cycles, bottom ocean circulation, and Antarctic ice sheet. However, many models of the previous Past-climate Model Intercomparison Project (PMIP) underestimated sea-ice extent (SIE) for the Last Glacial Maximum (LGM)(Roche et al., 2012; Marzocchi and Jensen, 2017), mainly because of surface bias (Flato et al., 2013) that may have an impact on mean ocean temperature (MOT). Indeed, recent studies further suggest an important link between Southern Ocean sea ice and mean ocean temperature (Ferrari et al., 2014; Bereiter et al., 2018 among others). Misrepresent the Antarctic sea-ice extent could highly impact deep ocean circulation, the heat transport and thus the MOT. In this study, we will stress the relationship between the distribution of Antarctic sea-ice extent and the MOT through the analysis of the PMIP3 and PMIP4 exercise and by using a set of MIROC models. To date, the latest version of MIROC improve its representation of the LGM Antarctic sea-ice extent, affecting the deep circulation and the MOT distribution (Sherriff-Tadano et al., under review).</p><p>Our results show that available PMIP4 models have an overall improvement in term of LGM sea-ice extent compared to PMIP3, associated to colder deep and bottom ocean temperature. Focusing on MIROC (4m) models, we show that models accounting for Southern Ocean sea-surface temperature (SST) bias correction reproduce an Antarctic sea-ice extent, 2D-distribution, and seasonal amplitude in good agreement with proxy-based data. Finally, using PMIP-MIROC analyze, we show that it exists a relationship between the maximum SIE and the MOT, modulated by the Antarctic intermediate and bottom waters.</p>


2016 ◽  
Vol 29 (9) ◽  
pp. 3199-3218 ◽  
Author(s):  
Feng Li ◽  
Yury V. Vikhliaev ◽  
Paul A. Newman ◽  
Steven Pawson ◽  
Judith Perlwitz ◽  
...  

Abstract Stratospheric ozone depletion plays a major role in driving climate change in the Southern Hemisphere. To date, many climate models prescribe the stratospheric ozone layer’s evolution using monthly and zonally averaged ozone fields. However, the prescribed ozone underestimates Antarctic ozone depletion and lacks zonal asymmetries. This study investigates the impact of using interactive stratospheric chemistry instead of prescribed ozone on climate change simulations of the Antarctic and Southern Ocean. Two sets of 1960–2010 ensemble transient simulations are conducted with the coupled ocean version of the Goddard Earth Observing System Model, version 5: one with interactive stratospheric chemistry and the other with prescribed ozone derived from the same interactive simulations. The model’s climatology is evaluated using observations and reanalysis. Comparison of the 1979–2010 climate trends between these two simulations reveals that interactive chemistry has important effects on climate change not only in the Antarctic stratosphere, troposphere, and surface, but also in the Southern Ocean and Antarctic sea ice. Interactive chemistry causes stronger Antarctic lower stratosphere cooling and circumpolar westerly acceleration during November–January. It enhances stratosphere–troposphere coupling and leads to significantly larger tropospheric and surface westerly changes. The significantly stronger surface wind stress trends cause larger increases of the Southern Ocean meridional overturning circulation, leading to year-round stronger ocean warming near the surface and enhanced Antarctic sea ice decrease.


2014 ◽  
Vol 14 (8) ◽  
pp. 4169-4183 ◽  
Author(s):  
K. Hara ◽  
M. Hayashi ◽  
M. Yabuki ◽  
M. Shiobara ◽  
C. Nishita-Hara

Abstract. Unusual aerosol enhancement is often observed at Syowa Station, Antarctica, during winter and spring. Simultaneous aerosol measurements near the surface and in the upper atmosphere were conducted twice using a ground-based optical particle counter, a balloon-borne optical particle counter, and micropulse lidar (MPL) in August and September 2012. During 13–15 August, aerosol enhancement occurred immediately after a storm condition. A high backscatter ratio and high aerosol concentrations were observed from the surface to ca. 2.5 km over Syowa Station. Clouds appeared occasionally at the top of the aerosol-enhanced layer during the episode. Aerosol enhancement was terminated on 15 August by strong winds from a cyclone's approach. In the second case, on 5–7 September, aerosol number concentrations in Dp > 0.3 μm near the surface reached > 104 L−1 at about 15:00 UT (Universal Time) on 5 September despite calm wind conditions, whereas MPL measurement exhibited aerosols were enhanced at about 04:00 UT at 1000–1500 m above Syowa Station. The aerosol enhancement occurred near the surface to ca. 4 km. In both cases, air masses with high aerosol enhancement below 2.5–3 km were transported mostly from the boundary layer over the sea-ice area. In addition, air masses at 3–4 km in the second case came from the boundary layer over the open-sea area. This air mass history strongly suggests that dispersion of sea-salt particles from the sea-ice surface contributes considerably to aerosol enhancement in the lower free troposphere (about 3 km) and that the release of sea-salt particles from the ocean surface engenders high aerosol concentrations in the free troposphere (3–4 km). Continuous MPL measurements indicate that high aerosol enhancement occurred mostly in surface–lower free troposphere (3 km) during the period July–September.


2013 ◽  
Vol 13 (10) ◽  
pp. 26269-26303
Author(s):  
K. Hara ◽  
M. Hayashi ◽  
M. Yabuki ◽  
M. Shiobara ◽  
C. Nishita-Hara

Abstract. Unusual aerosol enhancement is often observed at Syowa Station, Antarctica during winter through spring. Simultaneous aerosol measurements near the surface and in the upper atmosphere were conducted twice using a ground-based optical particle counter, a balloon-borne optical particle counter, and micro-pulse LIDAR (MPL) in August and September 2012. During 13–15 August, aerosol enhancement occurred immediately after a storm condition. A high backscatter ratio and aerosol concentrations were observed from the surface to ca. 2.5 km over Syowa Station. Clouds appeared occasionally at the top of aerosol-enhanced layer during the episode. Aerosol enhancement was terminated on 15 August by strong winds caused by a cyclone's approach. In the second case on 5–7 September, aerosol number concentrations in Dp > 0.3 μm near the surface reached > 104 L−1 at about 15:00 UT on 5 September in spite of calm wind conditions, whereas MPL measurement exhibited aerosols were enhanced at about 04:00 UT at 1000–1500 m above Syowa Station. The aerosol enhancement occurred near the surface–ca. 4 km. In both cases, air masses with high aerosol enhancement below 2.5–3 km were transported mostly from the boundary layer over the sea-ice area. In addition, air masses at 3–4 km in the second case came from the boundary layer over the open-sea area. This air mass history strongly suggests that dispersion of sea-salt particles from the sea-ice surface contributes considerably to the aerosol enhancement in the lower free troposphere (about 3 km) and that the release of sea-salt particles from the ocean surface engenders high aerosol concentrations in the free troposphere (3–4 km).


2020 ◽  
Vol 48 (2) ◽  
pp. 163-165
Author(s):  
I. A. Melnikov

During the seasonal work of the Russian Antarctic expedition (RAE-65), the monitoring of the water-ice ecological system was conducted in the Nella fjord (Prude Bay, East Antarctica). This monitoring is conducted annually since the IPY in 2007 in frames of the project “Assessment of the ecology of the Antarctic sea ice zone” (“Krial”) (Melnikov, 2020). The purpose of the monitoring is the assessment of the role of water-ice biota in global biosphere processes in the Southern Ocean.


2015 ◽  
Vol 15 (23) ◽  
pp. 13339-13364 ◽  
Author(s):  
R. S. Humphries ◽  
R. Schofield ◽  
M. D. Keywood ◽  
J. Ward ◽  
J. R. Pierce ◽  
...  

Abstract. Aerosol observations above the Southern Ocean and Antarctic sea ice are scarce. Measurements of aerosols and atmospheric composition were made in East Antarctic pack ice on board the Australian icebreaker Aurora Australis during the spring of 2012. One particle formation event was observed during the 32 days of observations. This event occurred on the only day to exhibit extended periods of global irradiance in excess of 600 W m−2. Within the single air mass influencing the measurements, number concentrations of particles larger than 3 nm (CN3) reached almost 7700 cm−3 within a few hours of clouds clearing, and grew at rates of 5.6 nm h−1. Formation rates of 3 nm particles were in the range of those measured at other Antarctic locations at 0.2–1.1 ± 0.1 cm−3 s−1. Our investigations into the nucleation chemistry found that there were insufficient precursor concentrations for known halogen or organic chemistry to explain the nucleation event. Modelling studies utilising known sulfuric acid nucleation schemes could not simultaneously reproduce both particle formation or growth rates. Surprising correlations with total gaseous mercury (TGM) were found that, together with other data, suggest a mercury-driven photochemical nucleation mechanism may be responsible for aerosol nucleation. Given the very low vapour pressures of the mercury species involved, this nucleation chemistry is likely only possible where pre-existing aerosol concentrations are low and both TGM concentrations and solar radiation levels are relatively high (∼ 1.5 ng m−3 and ≥ 600 W m−2, respectively), such as those observed in the Antarctic sea ice boundary layer in this study or in the global free troposphere, particularly in the Northern Hemisphere.


2006 ◽  
Vol 44 ◽  
pp. 53-57 ◽  
Author(s):  
Thorsten Markus ◽  
Donald J. Cavalieri

AbstractSnow depth on sea ice plays a critical role in the heat exchange between ocean and atmosphere because of its thermal insulation property. Furthermore, a heavy snow load on the relatively thin Southern Ocean sea-ice cover submerges the ice floes below sea level, causing snow-to-ice conversion. Snowfall is also an important freshwater source into the weakly stratified ocean. Snow-depth on sea-ice information can be used as an indirect measure of solid precipitation. Satellite passive microwave data are used to investigate the interannual and regional variability of the snow cover on sea ice. In this study we make use of 12 years (1992–2003) of Special Sensor Microwave/Imager (SSM/I) radiances to calculate average monthly snow depth on the Antarctic sea-ice cover. For the Antarctic sea-ice region as a whole, we find that September snow depth and sea-ice area are negatively correlated, which is not the case for individual regions. An analysis of the snow depth around Antarctica was undertaken. The results show an overall increase in snow depth for each of the five Antarctic sectors and the region as a whole, but only the Indian Ocean sector and the entire Southern Ocean show a statistically significant increase. There is a partial eastward propagation of maximum snow depths, which may be related to the Antarctic Circumpolar Wave. The overall trend and the variability of regional snow-depth distributions are also in agreement with cyclone density.


Polar Record ◽  
1991 ◽  
Vol 27 (162) ◽  
pp. 249-253 ◽  
Author(s):  
Gotthilf Hempel

AbstractSeasonal ice of the Southern Ocean, occupying some 15 x 106 km2, supports a distinctive biota based on algae that live on, within and immediately beneath the ice floes. How this annually-forming habitat recruits its biota, and the fate of the biota after the ice thaws in late summer, are little-known. Studies in the Weddell Sea in 1984–88 have shown that the seasonal ice is important as the wintering substrate of krill Euphausia superba which, together with other zooplankton and fish, supports a large breeding population of seals and penguins. Clearly a key habitat in the economy of the Southern Ocean, this seasonal ice is likely to be vulnerable to small climatic changes.


2021 ◽  
Author(s):  
Charles Pelletier ◽  
Lars Zipf ◽  
Konstanze Haubner ◽  
Deborah Verfaillie ◽  
Hugues Goosse ◽  
...  

<p>From at least 1979 up until 2016, the surface of the Southern Ocean cooled down, leading to a small Antarctic sea ice extent increase, which is in stark contrast with the Arctic Ocean. The attribution of the origin of these robust observations is still very uncertain. Among other phenomena, the direct, two-way interactions between the Southern Ocean and the Antarctic ice sheet, through basal melting of its numerous and large ice-shelf cavities, have been suggested as a potentially important contributor of this cooling. In order to address this question, we perform multidecadal coupled ice sheet – ocean numerical simulations relying on f.ETISh-v1.7 and NEMO3.6-LIM3 for simulating the Antarctic ice sheet and Southern Ocean (including sea ice), respectively. This presentation is twofold. First, we present the technical aspects of the coupling infrastructure (e.g. workflow and exchanged information in between models). Second, we investigate the ice sheet – ocean feedbacks on the Southern Ocean, their interactions, and the roles of the related physical mechanisms on the ocean surface cooling.</p>


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