scholarly journals Vertical profile of tropospheric ozone derived from synergetic retrieval using three different wavelength ranges, UV, IR, and Microwave: sensitivity study for satellite observation

2017 ◽  
Author(s):  
Yasuko Kasai ◽  
Tomohiro O. Sato ◽  
Takao M. Sato ◽  
Hideo Sagawa ◽  
Katsuyuki Noguchi ◽  
...  

Abstract. We performed a quantitative feasibility study of constraining the vertical profile of the amount of ozone in the troposphere by using a synergetic retrieval method on multiple spectra, i.e., ultraviolet (UV), thermal infrared (TIR) and microwave (MW) ranges, measured from space. Twenty atmospheric scenarios for East Asia in summer and winter seasons were assumed in this study. Geometry of line-of-sight was nadir down-looking for UV and TIR measurements, and limb-sounding for MW measurement. The sensitivities of retrieved ozone in the upper troposphere (UT), middle troposphere (MT) and lowermost troposphere (LMT) were estimated using values of the degree of freedom for signal (DFS), partial column error, and averaging kernel matrix, derived based on the optimal estimation method. The measurement noises were assumed at the same level as the currently available instruments. The weighting functions for the UV, TIR and MW ranges were calculated using the SCIATRAN radiative transfer model, the Line-By-Line Radiative Transfer Model, and the Advanced Model for Atmospheric Terahertz Radiation Analysis and Simulation, respectively. In the UT region, the DFS value was enhanced by about 200 % by adding the MW measurements to the combination of UV and TIR measurements. We found that the DFS value of the LMT ozone was increased by approximately 40 % by adding the MW measurements to the combination of UV and TIR measurements; nevertheless, the MW measurement alone has no sensitivity for the LMT ozone. Better information of the LMT ozone can be educed by adding constraints on the UT and MT ozone from the MW measurement. The results of this study will be implemented in the Japanese air-quality monitoring missions, APOLLO, GMAP-Asia and uvSCOPE.

2018 ◽  
Vol 11 (3) ◽  
pp. 1653-1668 ◽  
Author(s):  
Tomohiro O. Sato ◽  
Takao M. Sato ◽  
Hideo Sagawa ◽  
Katsuyuki Noguchi ◽  
Naoko Saitoh ◽  
...  

Abstract. We performed a feasibility study of constraining the vertical profile of the tropospheric ozone by using a synergetic retrieval method on multiple spectra, i.e., ultraviolet (UV), thermal infrared (TIR), and microwave (MW) ranges, measured from space. This work provides, for the first time, a quantitative evaluation of the retrieval sensitivity of the tropospheric ozone by adding the MW measurement to the UV and TIR measurements. Two observation points in East Asia (one in an urban area and one in an ocean area) and two observation times (one during summer and one during winter) were assumed. Geometry of line of sight was nadir down-looking for the UV and TIR measurements, and limb sounding for the MW measurement. The retrieval sensitivities of the ozone profiles in the upper troposphere (UT), middle troposphere (MT), and lowermost troposphere (LMT) were estimated using the degree of freedom for signal (DFS), the pressure of maximum sensitivity, reduction rate of error from the a priori error, and the averaging kernel matrix, derived based on the optimal estimation method. The measurement noise levels were assumed to be the same as those for currently available instruments. The weighting functions for the UV, TIR, and MW ranges were calculated using the SCIATRAN radiative transfer model, the Line-By-Line Radiative Transfer Model (LBLRTM), and the Advanced Model for Atmospheric Terahertz Radiation Analysis and Simulation (AMATERASU), respectively. The DFS value was increased by approximately 96, 23, and 30 % by adding the MW measurements to the combination of UV and TIR measurements in the UT, MT, and LMT regions, respectively. The MW measurement increased the DFS value of the LMT ozone; nevertheless, the MW measurement alone has no sensitivity to the LMT ozone. The pressure of maximum sensitivity value for the LMT ozone was also increased by adding the MW measurement. These findings indicate that better information on LMT ozone can be obtained by adding constraints on the UT and MT ozone from the MW measurement. The results of this study are applicable to the upcoming air-quality monitoring missions, APOLLO, GMAP-Asia, and uvSCOPE.


2020 ◽  
Author(s):  
Yang Wang ◽  
Arnoud Apituley ◽  
Alkiviadis Bais ◽  
Steffen Beirle ◽  
Nuria Benavent ◽  
...  

Abstract. We present the inter-comparison of delta slant column densities (SCDs) and vertical profiles of nitrous acid (HONO) derived from measurements of different MAX-DOAS instruments and using different inversion algorithms during the Second Cabauw Inter-comparison campaign for Nitrogen Dioxide measuring Instruments (CINDI-2), in September 2016, at Cabauw, The Netherlands (51.97° N, 4.93° E). Systematic discrepancies of HONO delta SCDs are observed in the range of ±0.3 × 1015 molecules cm−2, which is half of the typical random discrepancy of 0.6 × 1015 molecules cm−2. For a typical high HONO delta SCD of 2 × 1015 molecules cm−2, the relative systematic and random discrepancies are about 15 % and 30 %, respectively. The inter-comparison of HONO profiles shows that both systematic and random discrepancies of HONO VCDs and near-surface volume mixing ratios (VMRs) are mostly in the range of ~ ±0.5 × 1015 molecules cm−2 and ~ ±0.1 ppb (typically ~ 20 %). Further we find that the discrepancies of the retrieved HONO profiles are dominated by discrepancies of the HONO delta SCDs. The profile retrievals only contribute to the discrepancies of the HONO profiles by ~ 5 %. However, some data sets with substantial larger discrepancies than the typical values indicate that inappropriate implementations of profile inversion algorithms and configurations of radiative transfer models in the profile retrievals can also be an important uncertainty source. In addition, estimations of measurement uncertainties of HONO dSCDs, which can significantly impact profile retrievals using the optimal estimation method, need to consider not only DOAS fit errors, but also atmospheric variability, especially for an instrument with a DOAS fit error lower than ~ 3 × 1015 molecules cm−2. The MAX-DOAS results during the CINDI-2 campaign indicate that the peak HONO levels (e.g. near-surface VMRs of ~ 0.4 ppb) often appeared in the early morning and below 0.2 km. The near-surface VMRs retrieved from the MAX-DOAS observations are compared with those measured using a co-located long-path DOAS instrument. The systematic differences are smaller than 0.15 ppb and 0.07 ppb during early morning and around noon, respectively. Since true HONO values at high altitudes are not known in the absence of real measurements, in order to evaluate the abilities of profile inversion algorithms to respond to different HONO profile shapes, we performed sensitivity studies using synthetic HONO delta SCDs simulated by a radiative transfer model with assumed HONO profiles. The tests indicate that the profile inversion algorithms based on the optimal estimation method with proper configurations can well reproduce the different HONO profile shapes. Therefore we conclude that the feature of HONO accumulated near the surface derived from MAX-DOAS measurements are expected to well represent the ambient HONO profiles.


2013 ◽  
Vol 52 (3) ◽  
pp. 710-726 ◽  
Author(s):  
Chenxi Wang ◽  
Ping Yang ◽  
Steven Platnick ◽  
Andrew K. Heidinger ◽  
Bryan A. Baum ◽  
...  

AbstractA computationally efficient high-spectral-resolution cloudy-sky radiative transfer model (HRTM) in the thermal infrared region (700–1300 cm−1, 0.1 cm−1 spectral resolution) is advanced for simulating the upwelling radiance at the top of atmosphere and for retrieving cloud properties. A precomputed transmittance database is generated for simulating the absorption contributed by up to seven major atmospheric absorptive gases (H2O, CO2, O3, O2, CH4, CO, and N2O) by using a rigorous line-by-line radiative transfer model (LBLRTM). Both the line absorption of individual gases and continuum absorption are included in the database. A high-spectral-resolution ice particle bulk scattering properties database is employed to simulate the radiation transfer within a vertically nonisothermal ice cloud layer. Inherent to HRTM are sensor spectral response functions that couple with high-spectral-resolution measurements in the thermal infrared regions from instruments such as the Atmospheric Infrared Sounder (AIRS) and Infrared Atmospheric Sounding Interferometer. When compared with the LBLRTM and the discrete ordinates radiative transfer model (DISORT), the root-mean-square error of HRTM-simulated single-layer cloud brightness temperatures in the thermal infrared window region is generally smaller than 0.2 K. An ice cloud optical property retrieval scheme is developed using collocated AIRS and Moderate Resolution Imaging Spectroradiometer (MODIS) data. A retrieval method is proposed to take advantage of the high-spectral-resolution instrument. On the basis of the forward model and retrieval method, a case study is presented for the simultaneous retrieval of ice cloud optical thickness τ and effective particle size Deff that includes a cloud-top-altitude self-adjustment approach to improve consistency with simulations.


2016 ◽  
Author(s):  
Shouguo Ding ◽  
Jun Wang ◽  
Xiaoguang Xu

Abstract. Theoretical analysis is conducted to reveal the information content of aerosol vertical profile in space-borne measurements of the backscattered radiance and degree of linear polarization (DOLP) in the O2 A and B bands. Assuming a quasi-Gaussian shape for aerosol vertical profile characterized by peak height H and half width γ (at half maximum), the Unified Linearized Vector Radiative Transfer Model (UNL-VRTM) is used to simulate the Stokes 4-vector elements of upwelling radiation at the top of atmosphere (TOA) and their Jacobians with respect to H and γ. Calculations for different aerosol types and different combinations of H and γ values show that the wide range of gas absorption optical depth in O2 A and B band enables the sensitivity of backscattered DOLP and radiance at TOA to the aerosol layer at different altitudes. Quantitatively, DOLP in O2 A and B bands is found to be more sensitive to H and γ than radiance, especially over the bright surfaces (with large visible reflectance). In many O2 wavelengths, Degree of Freedom for Signal (DFS) for retrieving H (or γ) generally increases with H (and γ) and can be close to unity in many cases, assuming that the composite uncertainty from surface and aerosol scattering properties as well as measurements is less than 5%. Further analysis demonstrates that DFS needed for simultaneous retrieval of H and γ for high-lofted aerosol profiles (H > 2 km) can be obtained from a combined use of DOLP measurements at ~10 O2 absorption A and B absorption wavelengths. However, challenges still remain for resolving aerosol profiles with H less than 2 km. Future hyperspectral measurements of DOPL in O2 A and B bands are needed to continue studying their potential and their combination with radiance and DOPL in atmospheric window channels for retrieving the vertical profiles of aerosols, especially highly scattering aerosols, over land.


2019 ◽  
Author(s):  
Bin Yao ◽  
Chao Liu ◽  
Yan Yin ◽  
Zhiquan Liu ◽  
Chunxiang Shi ◽  
...  

Abstract. Extensive observational and numerical investigations have been performed to better characterize cloud properties. However, due to the large variations of cloud spatiotemporal distributions and physical properties, quantitative depictions of clouds in different atmospheric reanalysis datasets are still highly uncertain, and cloud parameters in the models to produce those datasets remain largely unconstrained. A radiance-based evaluation approach is introduced and performed to assess the quality of cloud properties by directly comparing reanalysis-driven forward radiative transfer results with radiances from satellite observation. The newly developed China Meteorological Administration Reanalysis data (CRA), the ECMWF’s Fifth-generation Reanalysis (ERA5), and the Modern-Era Retrospective Analysis for Applications, Version 2 (MERRA-2) are considered in the present study. To avoid the unrealistic assumptions and uncertainties on satellite retrieval algorithms and products, the radiative transfer model (RTM) is used as a bridge to “translate” the reanalysis to corresponding satellite observations. The simulated reflectance and brightness temperatures (BTs) are directly compared with observations from the Advanced Himawari Imager (AHI) onboard the Himawari-8 satellite in the region from 80° E to 160° W between 60° N and 60° S, especially for results over East Asia. Comparisons of the reflectance in the solar and BTs in the infrared (IR) window channels reveal that CRA reanalysis better represents the total cloud cover than the other two reanalysis datasets. The simulated BTs for CRA and ERA5 are close to each other in many pixels, whereas the vertical distributions of cloud properties are significantly different, and ERA5 depicts a better deep convection structure than CRA reanalysis. Comparisons of the BT differences (BTDs) between the simulations and observations suggest that the water clouds are generally overestimated in ERA5 and MERRA-2, whereas the ice cloud is responsible for the overestimation over the center of cyclones in ERA5. Overall, the cloud from CRA, ERA5, and MERRA-2 show their own advantages in different aspects. The ERA5 reanalysis is found the most capability in representing the cloudy atmosphere over East Asia, and the results in CRA are close to those in ERA5.


2013 ◽  
Vol 13 (1) ◽  
pp. 2415-2456 ◽  
Author(s):  
L. Zhang ◽  
Q. B. Li ◽  
Y. Gu ◽  
K. N. Liou ◽  
B. Meland

Abstract. Atmospheric mineral dust particles exert significant direct radiative forcings and are critical drivers of climate change. Here, we use the GEOS-Chem global three-dimensional chemical transport model (3-D CTM) coupled online with the Fu-Liou-Gu (FLG) radiative transfer model (RTM) to investigate the dust radiative forcing and heating rates based on different dust vertical profiles. The coupled calculations using a realistic dust vertical profile simulated by GEOS-Chem minimize the physical inconsistencies between 3-D CTM aerosol fields and the RTM. The use of GEOS-Chem simulated aerosol optical depth (AOD) vertical profiles as opposed to the FLG prescribed AOD vertical profiles leads to greater and more spatially heterogeneous changes in estimated radiative forcing and heating rate produced by dust. Both changes can be attributed to a different vertical structure between dust and non-dust source regions. Values of the dust AOD are much larger in the middle troposphere, though smaller at the surface when the GEOS-Chem simulated AOD vertical profile is used, which leads to a much stronger heating rate in the middle troposphere. Compared to FLG vertical profile, the use of GEOS-Chem vertical profile reduces the solar radiative forcing effect by about 0.2–0.25 W m−2 and the Infrared (IR) radiative forcing over the African and Asia dust source regions by about 0.1–0.2 W m−2. Differences in the solar radiative forcing at the surface between using the GEOS-Chem vertical profile and the FLG vertical profile are most significant over the Gobi desert with a value of about 1.1 W m−2. The radiative forcing effect of dust particles is more pronounced at the surface over the Sahara and Gobi deserts by using FLG vertical profile, while it is less significant over the downwind area of Eastern Asia.


2021 ◽  
Author(s):  
Huan Yu ◽  
Arve Kylling ◽  
Claudia Emde ◽  
Bernhard Mayer ◽  
Michel Van Roozendael ◽  
...  

<p>Operational retrievals of tropospheric trace gases from space-borne spectrometers are made using 1D radiative transfer models. To minimize cloud effects generally only partially cloudy pixels are analysed using simplified cloud contamination treatments based on radiometric cloud fraction estimates and photon path length corrections based on oxygen collision pair (O2-O2) or O2A-absorption band measurements. In reality, however, the impact of clouds can be much more complex, involving unresolved sub-pixel clouds, scattering of clouds in neighbouring pixels, and cloud shadow effects, such that 3D radiation scattering from unresolved boundary layer clouds may give significant biases in the trace gas retrievals. In order to quantify this impact, we use the MYSTIC 3D radiative transfer model to generate synthetic data. The realistic 3D cloud fields, needed for MYSTIC input, are generated by the ICOsahedral Non-hydrostatic (ICON) atmosphere model for a region including Germany, the Netherlands and parts of other surrounding countries. The retrieval algorithm is applied to the synthetic data and comparison to the known input trace gas concentrations yields the retrieval error due to 3D cloud effects. <br>In this study, we study NO2, which is a key tropospheric trace gas measured by TROPOMI and the future atmospheric Sentinels (S4 and S5). The work starts with a sensitivity study for the simulations with a simple 2D box cloud. The influence of cloud parameters (e.g., cloud top height, cloud optical thickness), observation geometry, and spatial resolution are studied, and the most significant dependences of retrieval biases are identified and investigated. Several approaches to correct the NO2 retrieval in the cloud shadow are explored and ultimately applied to both synthetic data with realistic 3D clouds and real observations.</p>


2018 ◽  
Vol 10 (8) ◽  
pp. 1309 ◽  
Author(s):  
Peng-Wang Zhai ◽  
Emmanuel Boss ◽  
Bryan Franz ◽  
P. Werdell ◽  
Yongxiang Hu

We report the first radiative transfer model that is able to simulate phytoplankton fluorescence with both photochemical and non-photochemical quenching included. The fluorescence source term in the inelastic radiative transfer equation is proportional to both the quantum yield and scalar irradiance at excitation wavelengths. The photochemical and nonphotochemical quenching processes change the quantum yield based on the photosynthetic active radiation. A sensitivity study was performed to demonstrate the dependence of the fluorescence signal on chlorophyll a concentration, aerosol optical depths and solar zenith angles. This work enables us to better model the phytoplankton fluorescence, which can be used in the design of new space-based sensors that can provide sufficient sensitivity to detect the phytoplankton fluorescence signal. It could also lead to more accurate remote sensing algorithms for the study of phytoplankton physiology.


2016 ◽  
Vol 9 (5) ◽  
pp. 2077-2092 ◽  
Author(s):  
Shouguo Ding ◽  
Jun Wang ◽  
Xiaoguang Xu

Abstract. Theoretical analysis is conducted to reveal the information content of aerosol vertical profile in space-borne measurements of the backscattered radiance and degree of linear polarization (DOLP) in oxygen (O2) A and B bands. Assuming a quasi-Gaussian shape for aerosol vertical profile characterized by peak height H and half width γ (at half maximum), the Unified Linearized Vector Radiative Transfer Model (UNL-VRTM) is used to simulate the Stokes four-vector elements of upwelling radiation at the top of atmosphere (TOA) and their Jacobians with respect to H and γ. Calculations for different aerosol types and different combinations of H and γ values show that the wide range of gas absorption optical depth in O2 A and B band enables the sensitivity of backscattered DOLP and radiance at TOA to the aerosol layer at different altitudes. Quantitatively, DOLP in O2 A and B bands is found to be more sensitive to H and γ than radiance, especially over the bright surfaces (with large visible reflectance). In many O2 absorption wavelengths, the degree of freedom of signal (DFS) for retrieving H (or γ) generally increases with H (and γ) and can be close to unity in many cases, assuming that the composite uncertainty from surface and aerosol scattering properties as well as measurements is less than 5 %. Further analysis demonstrates that DFS needed for simultaneous retrieval of H and γ can be obtained from a combined use of DOLP measurements at  ∼ 10–100 O2 A and B absorption wavelengths (or channels), depending on the specific values of H. The higher the aerosol layer, the fewer number of channels for DOLP measurements in O2 A and B bands are needed for characterizing H and γ. Future hyperspectral measurements of DOLP in O2 A and B bands are needed to continue studying their potential and their combination with radiance and DOLP in atmospheric window channels for retrieving the vertical profiles of aerosols, especially highly scattering aerosols, over land.


2021 ◽  
Vol 13 (3) ◽  
pp. 481
Author(s):  
Pengyu Huang ◽  
Qiang Guo ◽  
Changpei Han ◽  
Chunming Zhang ◽  
Tianhang Yang ◽  
...  

In our study, a retrieval method of temperature profiles is proposed which combines an improved one-dimensional variational algorithm (1D-Var) and artificial neural network algorithm (ANN), using FY-4A/GIIRS (Geosynchronous Interferometric Infrared Sounder) infrared hyperspectral data. First, according to the characteristics of the FY-4A/GIIRS observation data using the conventional 1D-Var, we introduced channel blacklists and discarded the channels that have a large negative impact on retrieval, then used the information capacity method for channel selection and introduced a neural network to correct the satellite observation data. The improved 1D-Var effectively used the observation information of 1415 channels, reducing the impact of the error of the satellite observation and radiative transfer model, and realizing the improvement of retrieval accuracy. We subsequently used the improved 1D-Var and ANN algorithms to retrieve the temperature profiles, respectively, from the GIIRS data. The results showed that the accuracy when using ANN is better than using improved 1D-Var in situations where the pressure ranges from 800 hPa to 1000 hPa. Therefore, we combined the improved 1D-Var and ANN method to retrieve temperature profiles for different pressure levels, calculating the error by taking sounding data published by the University of Wyoming as the true values. The results show that the average error of the retrieved temperature profiles is smaller than 2 K when using our method, this method makes the accuracy of the retrieved temperature profiles superior to the accuracy of the GIIRS products from 10 hPa to 575 hPa. All in all, through the combination of the physical retrieval method and the machine learning retrieval method, this paper can certainly provide a reference for improving the accuracy of products.


Sign in / Sign up

Export Citation Format

Share Document