Inferring saline tracer transport characteristics from time-lapse GPR experiments

2021 ◽  
Author(s):  
Peter-Lasse Giertzuch ◽  
Alexis Shakas ◽  
Bernard Brixel ◽  
Joseph Doetsch ◽  
Mohammadreza Jalali ◽  
...  
Keyword(s):  
Electrical Conductivity ◽  
Velocity Field ◽  
Nuclear Waste ◽  
Time Lapse ◽  
Transport Processes ◽  
Nuclear Waste Repository ◽  
Tracer Transport ◽  
Tracer Injection ◽  
Flow And Transport ◽  
Conductivity Sensor

<p>Monitoring and characterization of flow and transport processes in the subsurface has been a key focus of hydrogeological research for several decades. Such processes can be relevant for numerous applications, such as hydrocarbon and geothermal reservoir characterization and monitoring, risk assessment of soil contaminants, or nuclear waste disposal strategies.</p><p>Monitoring of flow and transport processes in the subsurface is often challenging, as they are usually not directly observable. Here, we present an approach to monitor saline tracer migration through a weakly fractured crystalline rock mass by means of Ground Penetrating Radar (GPR), and we evaluate the data quantitatively in terms of a flow velocity field and localized difference GPR breakthrough curves (DRBTC).</p><p>Two comparable and repeated tracer injection experiments were performed within saturated rock on the decameter scale. Time-lapse single-hole reflection data were acquired from two different boreholes during these experiments using unshielded and omnidirectional borehole antennas. The individual surveys were analyzed by difference imaging techniques, which allowed ultimately for tracer breakthrough monitoring at different locations in the subsurface. By combining the two complimentary GPR data sets, the 3D tracer velocity field could be reconstructed.</p><p>Our DRBTCs agree well with measured BTCs of the saline tracer at different electrical conductivity monitoring positions. Additionally, we were able to calculate a DRBTC for a location not previously monitored with borehole sensors. The reconstructed velocity field is in good agreement with previous studies on dye tracer data at the same research locations. Furthermore, we were able to resolve separate flow paths towards different monitoring locations, which could not be inferred from the electrical conductivity sensor data alone. The GPR data thus helped to disentangle the complex flow field through the fractured rock.</p><p>Out technique can be adapted to other use cases such as 3D monitoring of fluid migration (and thus permeability enhancement) during hydraulic stimulation and tracing fluid contaminants – e.g. for nuclear waste repository monitoring.</p>

Time-lapse ground penetrating radar difference reflection imaging of saline tracer flow in fractured rock

Geophysics ◽  
2020 ◽  
Vol 85 (3) ◽  
pp. H25-H37 ◽  
Author(s):  
Peter-Lasse Giertzuch ◽  
Joseph Doetsch ◽  
Mohammadreza Jalali ◽  
Alexis Shakas ◽  
Cédric Schmelzbach ◽  
...  
Keyword(s):  
Ground Penetrating Radar ◽  
Fractured Rock ◽  
Sampling Rate ◽  
Time Lapse ◽  
Transport Processes ◽  
Local Data ◽  
Tracer Injection ◽  
Flow Through ◽  
Reflection Imaging ◽  
Ground Penetrating

The characterization of flow and transport processes in fractured rock is challenging because they cannot be observed directly and hydrologic tests can only provide sparse and local data. Time-lapse ground penetrating radar (GPR) can be a valuable tool to monitor such processes in the subsurface, but it requires highly reproducible data. As part of a tracer injection experiment at the Grimsel Test Site (GTS) in Switzerland, borehole reflection GPR data were acquired in a time-lapse survey to monitor saline tracer flow through a fracture network in crystalline rock. Because the reflections from the tracer in the sub-mm fractures appear extremely weak, a differencing approach has been necessary to identify the tracer signal. Furthermore, several processing steps and corrections had to be applied to meet the reproducibility requirements. These steps include (1) single-trace preprocessing, (2) temporal trace alignment, (3) correction of sampling rate fluctuations, (4) spatial trace alignment, (5) spike removal, and (6) postprocessing procedures applied to the difference images. This allowed successful tracer propagation monitoring with a clear signal that revealed two separate tracer flow paths. The GPR results are confirmed by conductivity meters that were placed in boreholes in the GTS. If sufficient data processing is applied, GPR is shown to be capable of resolving tracer flow through sub-mm aperture fractures by difference reflection imaging even in challenging surroundings where many reflectors are present.

scholarly journals Electrical Imaging of Saline Tracer Migration for the Investigation of Unsaturated Zone Transport Mechanisms

1997 ◽  
Vol 1 (2) ◽  
pp. 291-302 ◽  
Author(s):  
L. Slater ◽  
M. D. Zaidman ◽  
A. M. Binley ◽  
L. J. West
Keyword(s):  
Unsaturated Zone ◽  
Transport Processes ◽  
Transport Mechanisms ◽  
Tracer Transport ◽  
Field Scale ◽  
Tracer Injection ◽  
Electrical Imaging ◽  
Spatial Coverage ◽  
Tracer Migration ◽  
The Uk

Abstract. Abstract: Better understanding of field-scale unsaturated zone transport mechanisms is required if the fate of contaminants released at the surface is to be predicted accurately. Interpretation of results from direct tracer sampling in terms of operative hydraulic processes is often limited by the poor spatial coverage and the invasive nature of such techniques. Cross-borehole electrical imaging during progress of saline tracer migration is proposed to assist investigation of field-scale solute transport in the unsaturated zone. Electrical imaging provides non-destructive, high density and spatially continuous sampling of saline tracer transport injected over an area of the ground surface between two boreholes. The value of electrical imaging was tested at a field site on an interfluve of the UK Chalk aquifer. Improved understanding of active transport mechanisms in the unsaturated zone of the UK Chalk is required to predict its vulnerability to surface pollutants. In a tracer experiment in May 1996, a conductive saline tracer was infiltrated over 18 m2 at an average rate of 47 mm day-1 for 56 hours. Cross-borehole images obtained during and after infiltration show a large, homogenous, resistivity reduction in the top 3 m, no change between 3 m and 6 m depth, and smaller, inhomogeneous, resistivity reductions below 6 m depth. The resistivity has reduced at down to 15 m depth less than 2 days after tracer infiltration began. Hydrological interpretation of a sequence of electrical images obtained prior to, during, and up to three months after tracer injection suggests: (1) rapid tracer entry into the soil zone and upper 2 m of weathered Chalk, (2) intergranular transport of the bulk of the tracer, (3) a significant fissure flow component transporting tracer to at least 15 m depth in 31 hours, and (4) vertical changes in transport mechanisms possibly caused by interception of fissures by marl layers. The results of this experiment suggest that electrical imaging can assist the description of unsaturated zone hydraulic mechanisms through visual identification of spatial and temporal variations in transport processes.

scholarly journals Computing Localized Breakthrough Curves and Velocities of Saline Tracer from Ground Penetrating Radar Monitoring Experiments in Fractured Rock

Energies ◽  
2021 ◽  
Vol 14 (10) ◽  
pp. 2949
Author(s):  
Peter-Lasse Giertzuch ◽  
Alexis Shakas ◽  
Joseph Doetsch ◽  
Bernard Brixel ◽  
Mohammadreza Jalali ◽  
...  
Keyword(s):  
Electrical Conductivity ◽  
Ground Penetrating Radar ◽  
Fractured Rock ◽  
Time Lapse ◽  
Test Site ◽  
Breakthrough Curves ◽  
Flow Path ◽  
Transport Processes ◽  
Grimsel Test Site ◽  
Ground Penetrating

Solute tracer tests are an established method for the characterization of flow and transport processes in fractured rock. Such tests are often monitored with borehole sensors which offer high temporal sampling and signal to noise ratio, but only limited spatial deployment possibilities. Ground penetrating radar (GPR) is sensitive to electromagnetic properties, and can thus be used to monitor the transport behavior of electrically conductive tracers. Since GPR waves can sample large volumes that are practically inaccessible by traditional borehole sensors, they are expected to increase the spatial resolution of tracer experiments. In this manuscript, we describe two approaches to infer quantitative hydrological data from time-lapse borehole reflection GPR experiments with saline tracers in fractured rock. An important prerequisite of our method includes the generation of GPR data difference images. We show how the calculation of difference radar breakthrough curves (DRBTC) allows to retrieve relative electrical conductivity breakthrough curves for theoretically arbitrary locations in the subsurface. For sufficiently small fracture apertures we found the relation between the DRBTC values and the electrical conductivity in the fracture to be quasi-linear. Additionally, we describe a flow path reconstruction procedure that allows computing approximate flow path distances using reflection GPR data from at least two boreholes. From the temporal information during the time-lapse GPR surveys, we are finally able to calculate flow-path averaged tracer velocities. Our new methods were applied to a field data set that was acquired at the Grimsel Test Site in Switzerland. DRBTCs were successfully calculated for previously inaccessible locations in the experimental rock volume and the flow path averaged velocity field was found to be in good accordance with previous studies at the Grimsel Test Site.

Investigating the Temperature Limits of Bentonite Backfilled Repositories: Coupled THMC Modeling, Lab Mockup Testing and Field Experiments

2020 ◽  
Author(s):  
Jens Birkholzer ◽  
Liange Zheng ◽  
Jonny Rutqvist ◽  
Sharon Borglin ◽  
Chun Chang ◽  
...  
Keyword(s):  
Nuclear Waste ◽  
Field Experiments ◽  
Elevated Temperatures ◽  
Spent Nuclear Fuel ◽  
The United States ◽  
Transport Processes ◽  
Maximum Temperature ◽  
Nuclear Waste Repository ◽  
Swelling Properties ◽  
Clay Formation

<p>Compacted bentonite is commonly considered for use as backfill material in emplacement tunnels of nuclear waste repositories because of its low permeability, high swelling pressure, and retardation capacity of radionuclide. To assess whether this material can maintain its favorable features when undergoing heating from the waste package and hydration from the host rock, we need a thorough understanding of the thermal, hydrological, mechanical, and chemical evolution under disposal conditions. Laboratory and field tests integrated with THMC modeling have provided an effective way to deepen such understanding; however, most of this work has been conducted for maximum temperatures around 100°C. In contrast, some international disposal programs have recently started investigations to understand whether local temperatures in the bentonite of up to 200°C could be tolerated with no significant changes in safety relevant properties. For example, the United States disposal program is evaluating the feasibility of geological disposal of large spent nuclear fuel canisters that are currently in dry storage. Direct disposal of these canisters is attractive for economical and safety reasons, but faces the challenge of exposing the bentonite to significant temperatures increases. As a result, strong thermal gradients may induce complex moisture transport processes and bentonite-rock interactions while cementation and perhaps also illitization effects may occur, all of which could  strongly affect the bentonite properties.</p><p>Here, we present initial investigations of bentonite behavior exposed to strongly elevated temperatures. We first show results from coupled thermal, hydrological, mechanical and chemical (THMC) simulations of a generic nuclear waste repository in a clay formation with a bentonite-based buffer exposed to a maximum temperature of 200°C. Modeling results illustrate possible performance impacts, such as the time frame and condition of the early unsaturated phase during bentonite hydration, the porosity and permeability after the bentonite becomes fully saturated, and changing in swelling properties. We then discuss preliminary data from a bench-scale laboratory mockup experiment which was designed to represents the strong THMC gradients occurring in a “hot” repository, and we briefly touch on a full-scale field experiment to be conducted soon in the Grimsel Test Site underground research laboratory in Switzerland (referred to as HotBENT, with bentonite exposure from up to 200<sup>o</sup>C). </p>

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