Reactivity insertion accident analysis during uranium foil target irradiation in the RSG-GAS reactor core

Analysis of the steady-state and reactivity insertion accident is very important for the safety of reactor operations. In this study, steady-state and reactivity insertion accident analysis when the low enriched uranium foil target is irradiated in the reactor core has been carried out. The analysis is carried out by the best estimate method by using a coupled neutronic, kinetic, and thermal-hydraulic code, MTR-DYN. The MTR-DYN code is based on the 3-D multigroup neutron diffusion method. The cell calculations for the target are carried out by the WIMSD/5 and MTR-DYN code. After reactivity insertion, the coolant, fuel, and clad temperature are observed. The calculation results for the initial power of 1 W showed that the maximum temperature of the coolant, clad, and fuel are 49.76?C, 65.01?C, and 65.26?C, respectively. Meanwhile, when the reactivity insertion at the initial power of 1 MW, the maximum temperature of the coolant, clad, and fuel are 72.23?C, 140.79?C, and 141.97?C, respectively. Based on those calculation results during irradiation low enriched uranium foil target, the temperature in the steady-state and reactivity insertion accident does not exceed the allowable safety limit.

Preventing damage to floating foils caused by Rayleigh-Taylor instabilities

An evaporated metal foil target is often produced on a layer of water-soluble parting agent previously applied to a massive substrate. The foil is then floated onto a water surface by immersing the substrate into a water bath. and is picked up later if the foil survives. During the foil's release, a significant fraction of the dissolved parting agent may remain close to the floating foil, as a "heavy" thin layer of solution having higher density than water. This layer of parting agent solution and the lower-density water bath below it form a gravitationally unstable configuration known as a Rayleigh-Taylor instability. If the foil is sufficiently thin, its mass and elastic properties can be ignored, and the motion of the liquids is determined by only the liquids' properties. This system can spontaneously adjust itself toward stability in several ways, one of which involves rotating a cylindrical liquid cell having a horizontal axis, and its cylindrical surface tangent to the surface. This motion moves part of the heavy layer from the top surface downward. The target maker detects this occurrence by the motions of the foil floating on the top of the bath; if the foil is frail, these motions may result in the crumpling, wrinkling, or tearing of the foil. We have observed such behavior with aluminum foils having thickness of 37 nm and diameter of 920 mm on NaCl parting agent, and have successfully implemented methods to prevent such damage.

Role of magnetic field evolution on filamentary structure formation in intense laser–foil interactions

Filamentary structures can form within the beam of protons accelerated during the interaction of an intense laser pulse with an ultrathin foil target. Such behaviour is shown to be dependent upon the formation time of quasi-static magnetic field structures throughout the target volume and the extent of the rear surface proton expansion over the same period. This is observed via both numerical and experimental investigations. By controlling the intensity profile of the laser drive, via the use of two temporally separated pulses, both the initial rear surface proton expansion and magnetic field formation time can be varied, resulting in modification to the degree of filamentary structure present within the laser-driven proton beam.

Comparative Study with 89Y-foil and 89Y-pressed Targets for the Production of 89Zr †

Zirconium-89 (89Zr, t1/2 = 3.27 days) owns great potential in nuclear medicine, being extensively used in the labelling of antibodies and nanoparticules. 89Zr can be produced by cyclotron via an 89Y(p,n)89Zr reaction while using an 89Y-foil target. In this study, we investigated for the first time the use of 89Y-pressed target for the preparation of 89Zr-oxalate via a (p,n) reaction. We performed comparative studies with an 89Y-foil target mounted on custom-made target supports. A new automated cassette-based purification module was used to facilitate the purification and the fractionation of 89Zr-oxalate. The effective molar activity (EMA) was calculated for both approaches via titration with deferoxamine (DFO). The radionuclidic purity was determined by gamma-ray spectroscopy and the metal impurities were quantified by ICP-MS on the resulting 89Zr-oxalate solution. The cassette-based purification process leading to fractionation is simple, efficient, and provides very high EMA of 89Zr-oxalate. The total recovered activity was 81 ± 4% for both approaches. The highest EMA was found at 13.3 MeV and 25 μA for 0.25-mm thick 89Y-foil. Similar and optimal production yields were obtained at 15 MeV and 40 μA while using 0.50-mm thick 89Y-foil and pressed targets. Metallic impurities concentration was below the general limit of 10 ppm for heavy metals in the US and Ph.Eur for both 89Y-foil and pressed targets. Overall, these results show that the irradiation of 89Y-pressed targets is a very effective process, offering an alternative method for 89Zr production.