Potential Source Contribution Function Analysis of High Latitude Dust Sources over the Arctic: Preliminary Results and Prospects

The results of a preliminary investigation of the dust sources in the Arctic based on their geochemical properties by potential source contribution function (PSCF) analysis are presented in this paper. For this purpose, we considered one year of aerosol geochemical data from Ny-Ålesund, Svalbard, and a short list of chemical elements (i.e., Al, Fe, Mn, Ti, Cr, V, Ni, Cu, and Zn) variably related to the dust fraction. Based on PSCF analysis: (i) four different dust source areas (i.e., Eurasia, Greenland, Arctic-Alaska, and Iceland) were characterized by distinguishing geochemical ranges and seasonal occurrence; and (ii) a series of typical dust days from the distinct source areas were identified based on the corresponding back trajectory patterns. Icelandic dust samples revealed peculiar but very variable characteristics in relation to their geographical source regions marked by air mass back trajectories. The comparison between pure and mixed Icelandic dust samples (i.e., aerosols containing Icelandic dust along with natural and/or anthropogenic components) revealed the occurrence of different mixing situations. Comparison with Icelandic soils proved the existence of dilution effects related to the emission and the transport processes.

Pollution Characteristics, Transport Pathways, and Potential Source Regions of PM2.5 and PM10 in Changchun City in 2018

Air pollution has attracted increasing attention in recent years. Cluster analysis, scene analysis, and the potential source contribution function (PSCF), based on the backward trajectory model, were used to identify the transport pathways and potential source regions of PM2.5 and PM10 (particulate matter with an aerodynamic diameter of not more than 2.5 µm and 10 µm) in Changchun in 2018. In addition, the PSCF was slightly improved. The highest average monthly concentrations of PM2.5 and PM10 appeared in March and April, when they reached 53.9μg/m3 and 120.0 μg/m3, respectively. The main potential source regions of PM2.5 and PM10 were generally similar: western Jilin Province, northwestern Inner Mongolia, northeastern Liaoning Province, and the Yellow Sea region. The secondary potential source regions were southern Russia, central Mongolia, western Shandong Province, eastern Hebei Province, and eastern Jiangsu Province. The northwest and southwest directions were found to be the two pathways that mainly affect the air quality of Changchun City. Moreover, the northwestern pathway had a larger potential contribution source area than the southwestern pathway. The airflow in the southwest direction came from Liaoning Province, Shandong Province, and the Yellow Sea region. This mainly occurred in summer; its transmission distance was short; it had a relatively higher weight potential source contribution function (WPSCF) value; it can be regarded as a local source; and its representative pollutants were SO2 (sulfur dioxide), CO (carbon monoxide), and O3 (ozone). The northwestern pathway passed through Russia, Mongolia, and Inner Mongolia. The transmission distance of this pathway was longer; it had a relatively lower WPSCF value; it can be considered as a natural source to a certain extent; it mainly occurred in autumn and, especially, in winter; and the representative pollutants of this pathway were NO (nitric oxide), NOx (nitrogen oxide), PM2.5, and PM10.

Characterization and sources of black carbon in PM2.5at a site close to a roadway in Gwangju, Korea, during winter

Potential source contribution function maps for black carbon (BC) observed at a roadway site indicate that the BC observed during episode “A” was most likely attributed to local emissions, while local sources and regional transport of air masses contributed to the enhanced BC concentrations during episode “B”.