Aerosol versus greenhouse gas impacts on Southern Hemisphere general circulation changes

2018 ◽  
Vol 52 (7-8) ◽  
pp. 4127-4142 ◽  
Author(s):  
Jung Choi ◽  
Seok-Woo Son ◽  
Rokjin J. Park
2020 ◽  
Author(s):  
Bo-Reum Han ◽  
Jung Choi ◽  
Seok-Woo Son

<p> The impacts of stratospheric ozone and greenhouse gas changes on the Southern Hemisphere (SH) climate are re-visited by examining the single forcing experiments from the Chemistry-Climate Model Initiative (CCMI) project. In particular, the fixed ozone-depleting substance (ODS) runs and the fixed greenhouse gas (GHG) concentration runs are directly compared with the reference runs for both the past and future. Consistent with the previous studies, the SH-summer general circulation changes, such as changes in the jet location, Hadley cell edge, and Southern Annular Mode (SAM), show the opposite trends from the past to the future in response to the Antarctic ozone depletion and recovery. The GHG-induced circulation changes largely enhance the ozone-induced circulation changes in the past, but partly cancel them in the future. The ozone recovery-related tropospheric circulation return dates are also estimated in this study. We will further discuss the inter-model diversity among the CCMI models.</p>


2011 ◽  
Vol 24 (3) ◽  
pp. 795-812 ◽  
Author(s):  
Lorenzo M. Polvani ◽  
Darryn W. Waugh ◽  
Gustavo J. P. Correa ◽  
Seok-Woo Son

Abstract The importance of stratospheric ozone depletion on the atmospheric circulation of the troposphere is studied with an atmospheric general circulation model, the Community Atmospheric Model, version 3 (CAM3), for the second half of the twentieth century. In particular, the relative importance of ozone depletion is contrasted with that of increased greenhouse gases and accompanying sea surface temperature changes. By specifying ozone and greenhouse gas forcings independently, and performing long, time-slice integrations, it is shown that the impacts of ozone depletion are roughly 2–3 times larger than those associated with increased greenhouse gases, for the Southern Hemisphere tropospheric summer circulation. The formation of the ozone hole is shown to affect not only the polar tropopause and the latitudinal position of the midlatitude jet; it extends to the entire hemisphere, resulting in a broadening of the Hadley cell and a poleward extension of the subtropical dry zones. The CAM3 results are compared to and found to be in excellent agreement with those of the multimodel means of the recent Coupled Model Intercomparison Project (CMIP3) and Chemistry–Climate Model Validation (CCMVal2) simulations. This study, therefore, strongly suggests that most Southern Hemisphere tropospheric circulation changes, in austral summer over the second half of the twentieth century, have been caused by polar stratospheric ozone depletion.


2014 ◽  
Vol 27 (5) ◽  
pp. 1863-1875 ◽  
Author(s):  
Axel Timmermann ◽  
Tobias Friedrich ◽  
Oliver Elison Timm ◽  
Megumi O. Chikamoto ◽  
Ayako Abe-Ouchi ◽  
...  

Abstract The effect of obliquity and CO2 changes on Southern Hemispheric climate is studied with a series of numerical modeling experiments. Using the Earth system model of intermediate complexity Loch–VECODE–ECBilt–CLIO–Agism Model (LOVECLIM) and a coupled general circulation model [Model for Interdisciplinary Research on Climate (MIROC)], it is shown in time-slice simulations that phases of low obliquity enhance the meridional extratropical temperature gradient, increase the atmospheric baroclinicity, and intensify the lower and middle troposphere Southern Hemisphere westerlies and storm tracks. Furthermore, a transient model simulation is conducted with LOVECLIM that covers the greenhouse gas, ice sheet, and orbital forcing history of the past 408 ka. This simulation reproduces reconstructed glacial–interglacial variations in temperature and sea ice qualitatively well and shows that the meridional heat transport associated with the orbitally paced modulation of middle troposphere westerlies and storm tracks partly offsets the effects of the direct shortwave obliquity forcing over Antarctica, thereby reinforcing the high correlation between CO2 radiative forcing and Antarctic temperature. The overall timing of temperature changes in Antarctica is hence determined by a balance of shortwave obliquity forcing, atmospheric heat transport changes, and greenhouse gas forcing. A shorter 130-ka transient model experiment with constant CO2 concentrations further demonstrates that surface Southern Hemisphere westerlies are primarily modulated by the obliquity cycle rather than by the CO2 radiative forcing.


2021 ◽  
Vol 14 (9) ◽  
pp. 638-644
Author(s):  
Brian Zambri ◽  
Susan Solomon ◽  
David W. J. Thompson ◽  
Qiang Fu

2017 ◽  
Author(s):  
Hannah M. Horowitz ◽  
Daniel J. Jacob ◽  
Yanxu Zhang ◽  
Theodore S. Dibble ◽  
Franz Slemr ◽  
...  

Abstract. Mercury (Hg) is emitted to the atmosphere mainly as volatile elemental Hg0. Oxidation to water-soluble HgII controls Hg deposition to ecosystems. Here we implement a new mechanism for atmospheric Hg0 / HgII redox chemistry in the GEOS-Chem global model and examine the implications for the global atmospheric Hg budget and deposition patterns. Our simulation includes a new coupling of GEOS-Chem to an ocean general circulation model (MITgcm), enabling a global 3-D representation of atmosphere-ocean Hg0 / HgII cycling. We find that atomic bromine (Br) of marine organobromine origin is the main atmospheric Hg0 oxidant, and that second-stage HgBr oxidation is mainly by the NO2 and HO2 radicals. The resulting lifetime of tropospheric Hg0 against oxidation is 2.7 months, shorter than in previous models. Fast HgII atmospheric reduction must occur in order to match the ~ 6-month lifetime of Hg against deposition implied by the observed atmospheric variability of total gaseous mercury (TGM ≡ Hg0 + HgII(g)). We implement this reduction in GEOS-Chem as photolysis of aqueous-phase HgII-organic complexes in aerosols and clouds, resulting in a TGM lifetime of 5.2 months against deposition and matching both mean observed TGM and its variability. Model sensitivity analysis shows that the interhemispheric gradient of TGM, previously used to infer a longer Hg lifetime against deposition, is misleading because southern hemisphere Hg mainly originates from oceanic emissions rather than transport from the northern hemisphere. The model reproduces the observed seasonal TGM variation at northern mid-latitudes (maximum in February, minimum in September) driven by chemistry and oceanic evasion, but does not reproduce the lack of seasonality observed at southern hemisphere marine sites. Aircraft observations in the lowermost stratosphere show a strong TGM-ozone relationship indicative of fast Hg0 oxidation, but we show that this relationship provides only a weak test of Hg chemistry because it is also influenced by mixing. The model reproduces observed Hg wet deposition fluxes over North America, Europe, and China, including the maximum over the US Gulf Coast driven by HgBr oxidation by NO2 and HO2. Low Hg wet deposition observed over rural China is attributed to fast HgII reduction in the presence of high organic aerosol concentrations. We find that 80 % of global HgII deposition takes place over the oceans, reflecting the marine origin of Br and low concentrations of marine organics for HgII reduction, and most of HO2 and NO2 for second-stage HgBr oxidation.


2021 ◽  
Author(s):  
Liang Guo ◽  
Laura J. Wilcox ◽  
Massimo Bollasina ◽  
Steven T. Turnock ◽  
Marianne T. Lund ◽  
...  

Abstract. Despite local emission reductions, severe haze events remain a serious issue in Beijing. Previous studies have suggested that both greenhouse gas increases and aerosol decreases are likely to increase the frequency of weather patterns conducive to haze events. However, the combined effect of atmospheric circulation changes and aerosol and precursor emission changes on Beijing haze remains unclear. We use the Shared Socioeconomic Pathways (SSPs) to explore the effects of aerosol and greenhouse gas emission changes on both haze weather and Beijing haze itself. We confirm that the occurrence of haze weather patterns is likely to increase in future under all SSPs, and show that even though aerosol reductions play a small role, greenhouse gas increases are the main driver, especially during the second half of the 21st century. However, the severity of the haze events decreases on decadal timescales by as much as 70 % by 2100. The main influence on the haze itself is the reductions in local aerosol emissions, which outweigh the effects of changes in atmospheric circulation patterns. This demonstrates that aerosol reductions are beneficial, despite their influence on the circulation.


2021 ◽  
Author(s):  
Rishav Goyal ◽  
Martin Jucker ◽  
Alex Sen Gupta ◽  
Harry Hendon ◽  
Matthew England

Abstract A distinctive feature of the Southern Hemisphere (SH) extratropical atmospheric circulation is the quasi-stationary zonal wave 3 (ZW3) pattern, characterized by three high and three low-pressure centers around the SH extratropics. This feature is present in both the mean atmospheric circulation and its variability on daily, seasonal and interannual timescales. While the ZW3 pattern has significant impacts on meridional heat transport and Antarctic sea ice extent, the reason for its existence remains uncertain, although it has long been assumed to be linked to the existence of three major land masses in the SH extratropics. Here we use an atmospheric general circulation model to show that the stationery ZW3 pattern is instead driven by zonal asymmetric deep atmospheric convection in the tropics, with little to no role played by the orography or land masses in the extratropics. Localized regions of deep convection in the tropics form a local Hadley cell which in turn creates a wave source in the subtropics that excites a poleward and eastward propagating wave train which forms stationary waves in the SH high latitudes. Our findings suggest that changes in tropical deep convection, either due to natural variability or climate change, will impact the zonal wave 3 pattern, with implications for Southern Hemisphere climate, ocean circulation, and sea-ice.


2007 ◽  
Vol 7 (9) ◽  
pp. 2183-2196 ◽  
Author(s):  
D. Cariolle ◽  
H. Teyssèdre

Abstract. This article describes the validation of a linear parameterization of the ozone photochemistry for use in upper tropospheric and stratospheric studies. The present work extends a previously developed scheme by improving the 2-D model used to derive the coefficients of the parameterization. The chemical reaction rates are updated from a compilation that includes recent laboratory work. Furthermore, the polar ozone destruction due to heterogeneous reactions at the surface of the polar stratospheric clouds is taken into account as a function of the stratospheric temperature and the total chlorine content. Two versions of the parameterization are tested. The first one only requires the solution of a continuity equation for the time evolution of the ozone mixing ratio, the second one uses one additional equation for a cold tracer. The parameterization has been introduced into the chemical transport model MOCAGE. The model is integrated with wind and temperature fields from the ECMWF operational analyses over the period 2000–2004. Overall, the results from the two versions show a very good agreement between the modelled ozone distribution and the Total Ozone Mapping Spectrometer (TOMS) satellite data and the "in-situ" vertical soundings. During the course of the integration the model does not show any drift and the biases are generally small, of the order of 10%. The model also reproduces fairly well the polar ozone variability, notably the formation of "ozone holes" in the Southern Hemisphere with amplitudes and a seasonal evolution that follow the dynamics and time evolution of the polar vortex. The introduction of the cold tracer further improves the model simulation by allowing additional ozone destruction inside air masses exported from the high to the mid-latitudes, and by maintaining low ozone content inside the polar vortex of the Southern Hemisphere over longer periods in spring time. It is concluded that for the study of climate scenarios or the assimilation of ozone data, the present parameterization gives a valuable alternative to the introduction of detailed and computationally costly chemical schemes into general circulation models.


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