Influences of offshore background wind on the formation of sea-land breeze and the characteristics of pollutant diffusion

Author(s):  
Jiajia Xu ◽  
Hongwei Jia ◽  
Huayuan Zhou ◽  
Yanming Kang ◽  
Ke Zhong
2005 ◽  
Vol 5 (11) ◽  
pp. 2927-2934 ◽  
Author(s):  
L. J. Carpenter ◽  
D. J. Wevill ◽  
S. O'Doherty ◽  
G. Spain ◽  
P. G. Simmonds

Abstract. In situ atmospheric observations of bromoform (CHBr3) made over a 2.5 year period at Mace Head, Ireland from May 2001- Dec 2003, including during the NAMBLEX (North Atlantic Marine Boundary Layer Experiment) campaign, show broad maxima from spring until autumn and winter minima, with mixing ratios of 5.3+1.0 pptv (mid March - mid October) and 1.8+0.8 pptv (December-February). This indicates that, unlike CHCl3, which has a summer minimum and winter maximum at Mace Head, local biological sources of CHBr3 have a greater influence on the atmospheric data than photochemical decay during long-range transport. The emission sources are predominantly macroalgal, but we find evidence for a small terrestrial flux from peatland ecosystems, which so far has not been accounted for in the CHBr3 budget. Sharp increases in CHCl3 and CHBr3 concentrations and decreases in O3 concentrations occurred at night when the wind direction switched from an ocean- to a land-based sector (land breeze) and the wind speed dropped to below 5 ms-1. These observations infer a shallow atmospheric boundary layer with increased O3 deposition and concentration of local emissions of both CHCl3 and CHBr3. The ratio of ΔCHCl3/ΔCHBr3 varied strongly according to the prevailing wind direction; from 0.60+0.15 in south-easterly (100-170° and northerly (340-20°) air to 2.5+0.4 in north-easterly (40-70°) air. Of these land-sectors, the south-easterly air masses are likely to be strongly influenced by macroalgal beds along the coast and the emission ratios probably reflect those from seaweeds in addition to land sources. The north-easterly airmasses however had an immediate fetch inland, which locally is comprised of coastal peatland ecosystems (peat bogs and coastal conifer plantations), previously identified as being strong sources of atmospheric CHCl3 under these conditions. Although we cannot entirely rule out other local land or coastal sources, our observations also suggest peatland ecosystem emissions of CHBr3. We use correlations between CHCl3 and CHBr3 during the north-easterly land breeze events in conjunction with previous estimates of local wetland CHCl3 release to tentatively deduce a global wetland CHBr3 source of 20.4(0.4-948) Gg yr-1, which is approximately 7% of the total global source.


SOLA ◽  
2006 ◽  
Vol 2 (0) ◽  
pp. 21-24
Author(s):  
Takuya Sugiyama ◽  
Yuko Sugimura ◽  
Yoshifumi Yamashita

2021 ◽  
Vol 21 (18) ◽  
pp. 13763-13795
Author(s):  
Manfred Ern ◽  
Mohamadou Diallo ◽  
Peter Preusse ◽  
Martin G. Mlynczak ◽  
Michael J. Schwartz ◽  
...  

Abstract. Gravity waves play a significant role in driving the semiannual oscillation (SAO) of the zonal wind in the tropics. However, detailed knowledge of this forcing is missing, and direct estimates from global observations of gravity waves are sparse. For the period 2002–2018, we investigate the SAO in four different reanalyses: ERA-Interim, JRA-55, ERA-5, and MERRA-2. Comparison with the SPARC zonal wind climatology and quasi-geostrophic winds derived from Microwave Limb Sounder (MLS) and Sounding of the Atmosphere using Broadband Emission Radiometry (SABER) satellite observations show that the reanalyses reproduce some basic features of the SAO. However, there are also large differences, depending on the model setup. Particularly, MERRA-2 seems to benefit from dedicated tuning of the gravity wave drag parameterization and assimilation of MLS observations. To study the interaction of gravity waves with the background wind, absolute values of gravity wave momentum fluxes and a proxy for absolute gravity wave drag derived from SABER satellite observations are compared with different wind data sets: the SPARC wind climatology; data sets combining ERA-Interim at low altitudes and MLS or SABER quasi-geostrophic winds at high altitudes; and data sets that combine ERA-Interim, SABER quasi-geostrophic winds, and direct wind observations by the TIMED Doppler Interferometer (TIDI). In the lower and middle mesosphere the SABER absolute gravity wave drag proxy correlates well with positive vertical gradients of the background wind, indicating that gravity waves contribute mainly to the driving of the SAO eastward wind phases and their downward propagation with time. At altitudes 75–85 km, the SABER absolute gravity wave drag proxy correlates better with absolute values of the background wind, suggesting a more direct forcing of the SAO winds by gravity wave amplitude saturation. Above about 80 km SABER gravity wave drag is mainly governed by tides rather than by the SAO. The reanalyses reproduce some basic features of the SAO gravity wave driving: all reanalyses show stronger gravity wave driving of the SAO eastward phase in the stratopause region. For the higher-top models ERA-5 and MERRA-2, this is also the case in the lower mesosphere. However, all reanalyses are limited by model-inherent damping in the upper model levels, leading to unrealistic features near the model top. Our analysis of the SABER and reanalysis gravity wave drag suggests that the magnitude of SAO gravity wave forcing is often too weak in the free-running general circulation models; therefore, a more realistic representation is needed.


2015 ◽  
Vol 8 (11) ◽  
pp. 11817-11852 ◽  
Author(s):  
J. M. Kopeć ◽  
K. Kwiatkowski ◽  
S. de Haan ◽  
S. P. Malinowski

Abstract. Navigational information broadcast by commercial aircraft in the form of Mode-S and ADS-B messages can be considered a new and valid source of upper air turbulence measurements. A set of three processing methods is proposed and analysed using a quality record of turbulence encounters made by a research aircraft. The proposed methods are based on processing the vertical acceleration or the background wind into the eddy dissipation rate. All the necessary parameters are conveyed in the Mode-S/ADS-B messages. The comparison of the results of application of the processing against a reference eddy dissipation rate obtained using on-board accelerometer indicate a significant potential of those methods. The advantages and limitation of the presented approaches are discussed.


2021 ◽  
Vol 21 (9) ◽  
pp. 7293-7319
Author(s):  
Benjamin Chazeau ◽  
Brice Temime-Roussel ◽  
Grégory Gille ◽  
Boualem Mesbah ◽  
Barbara D'Anna ◽  
...  

Abstract. This study reports results of PM1 chemical composition determined using a Time-of-Flight Aerosol Chemical Speciation Monitor (ToF-ACSM) over a 14-month period (1 February 2017–13 April 2018) at the Marseille–Longchamp supersite (MRS-LCP) in France. Parallel measurements were performed with an aethalometer, an ultrafine particle monitor and a suite of instruments to monitor regulated pollutants (PM2.5, PM10, NOx, O3 and SO2). The average PM1 chemical composition over the period was dominated by organic aerosol (OA; 49.7 %) and black carbon (BC; 17.1 %), while sulfate accounted for 14.6 %, nitrate for 10.2 %, ammonium for 7.9 % and chloride for 0.5 % only. Wintertime was found to be the season contributing the most to the annual PM1 mass concentration (30 %), followed by autumn (26 %), summer (24 %) and spring (20 %). During this season, OA and BC concentrations were found to contribute 32 % and 31 % of their annual concentrations, respectively, as a combined result of heavy urban traffic, high emissions from residential heating and low planetary boundary layer (PBL) height. Most (75 %) of the 15 days exceeding the target daily PM2.5 concentration value recommended by the World Health Organization (WHO) occurred during this season. Local and long-range pollution episodes with contrasting chemical composition could be distinguished, accounting for 40 % and 60 % of the exceedance days, respectively. Enhanced OA and BC concentrations, mostly originating from domestic wood burning under nocturnal land breeze conditions, were observed during local pollution episodes, while high levels of oxygenated OA and inorganic nitrate were associated with medium-/long-range transported particles. In summertime, substantially higher concentrations of sulfate were found, with an average and a maximum contribution to the PM1 mass of 24 % and 66 %, respectively. Results from k-means clustering analysis of daily profiles of sulfate concentrations clearly reveal the significant influence of local harbour/industrial activities on air quality in addition to the more regional contribution of shipping traffic that originates from the Mediterranean basin.


2013 ◽  
Vol 13 (4) ◽  
pp. 10757-10807 ◽  
Author(s):  
F. Chane Ming ◽  
C. Ibrahim ◽  
S. Jolivet ◽  
P. Keckhut ◽  
Y.-A. Liou ◽  
...  

Abstract. Activity and spectral characteristics of gravity-waves (GWs) are analyzed during tropical cyclone (TC) Ivan (2008) in the troposphere and lower stratosphere using radiosonde and GPS radio occultation data, ECMWF outputs and simulations of French numerical model Meso-NH with vertical resolution varying between 150 m near the surface and 500 m in the lower stratosphere. Conventional methods for GW analysis and signal and image processing tools provide information on a wide spectrum of GWs with horizontal wavelengths of 40–1800 km and short vertical wavelengths of 0.6–10 km respectively and periods of 20 min–2 days. MesoNH model, initialized with Aladin-Réunion analyses, produces realistic and detailed description of TC dynamics, GWs, variability of the tropospheric and stratospheric background wind and TC rainband characteristics at different stages of TC Ivan. In particular a dominant eastward propagating TC-related quasi-inertia GW is present during intensification of TC Ivan with horizontal and vertical wavelengths of 400–600 km and 1.5–3.5 km respectively during intensification. A wavenumber-1 vortex Rossby wave is identified as a source of this medium-scale mode while short-scale modes located at north-east and south-east of the TC could be attributed to strong localized convection in spiral bands resulting from wavenumber-2 vortex Rossby waves. Meso-NH simulations also reveal high-frequency GWs with horizontal wavelengths of 20–80 km near the TC eye and high-frequency GWs-related clouds behind TC Ivan. In addition, GWs produced during landfall are likely to strongly contribute to background wind in the middle and upper troposphere as well as the stratospheric quasi-biennial oscillation.


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