scholarly journals Recent Progress of Two-Dimensional Thermoelectric Materials

2020 ◽  
Vol 12 (1) ◽  
Author(s):  
Delong Li ◽  
Youning Gong ◽  
Yuexing Chen ◽  
Jiamei Lin ◽  
Qasim Khan ◽  
...  

AbstractThermoelectric generators have attracted a wide research interest owing to their ability to directly convert heat into electrical power. Moreover, the thermoelectric properties of traditional inorganic and organic materials have been significantly improved over the past few decades. Among these compounds, layered two-dimensional (2D) materials, such as graphene, black phosphorus, transition metal dichalcogenides, IVA–VIA compounds, and MXenes, have generated a large research attention as a group of potentially high-performance thermoelectric materials. Due to their unique electronic, mechanical, thermal, and optoelectronic properties, thermoelectric devices based on such materials can be applied in a variety of applications. Herein, a comprehensive review on the development of 2D materials for thermoelectric applications, as well as theoretical simulations and experimental preparation, is presented. In addition, nanodevice and new applications of 2D thermoelectric materials are also introduced. At last, current challenges are discussed and several prospects in this field are proposed.

Nanophotonics ◽  
2020 ◽  
Vol 9 (7) ◽  
pp. 1717-1742
Author(s):  
Xiao-Guang Gao ◽  
Xiao-Kuan Li ◽  
Wei Xin ◽  
Xu-Dong Chen ◽  
Zhi-Bo Liu ◽  
...  

AbstractTwo-dimensional (2D) materials such as graphene, black phosphorus, and transition metal dichalcogenides have attracted significant research attention due to their novel properties and wide range of applications in electronic and optoelectronic devices. In particular, investigation of twist-controlled 2D materials has attracted tremendous attention due to their excellent properties such as smooth heterointerfaces, highly gate-tunable bandgaps, and ultrafast carrier transport. Twist-controlled 2D materials combined with their fascinating electronic structures have also indicated their outstanding potential in electronic and optoelectronic applications. In this review, the recent developments in twisted 2D materials are summarized, covering aspects related to their fabrication, twist angle-dependent optical properties, and optoelectronic applications. The photodetectors and orientation-dependent van der Waals junctions are introduced and discussed systematically. Finally, we deliver a summary and outlook to provide a guideline for the future development of this rapidly growing field.


Author(s):  
Sai Manoj Gali ◽  
David Beljonne

Transition Metal Dichalcogenides (TMDCs) are emerging as promising two-dimensional (2D) materials. Yet, TMDCs are prone to inherent defects such as chalcogen vacancies, which are detrimental to charge transport. Passivation of...


2019 ◽  
Vol 116 (42) ◽  
pp. 20844-20849 ◽  
Author(s):  
Cong Su ◽  
Zongyou Yin ◽  
Qing-Bo Yan ◽  
Zegao Wang ◽  
Hongtao Lin ◽  
...  

Two-dimensional van der Waals materials have rich and unique functional properties, but many are susceptible to corrosion under ambient conditions. Here we show that linear alkylamines n-CmH2m+1NH2, with m = 4 through 11, are highly effective in protecting the optoelectronic properties of these materials, such as black phosphorus (BP) and transition-metal dichalcogenides (TMDs: WS2, 1T′-MoTe2, WTe2, WSe2, TaS2, and NbSe2). As a representative example, n-hexylamine (m = 6) can be applied in the form of thin molecular monolayers on BP flakes with less than 2-nm thickness and can prolong BP’s lifetime from a few hours to several weeks and even months in ambient environments. Characterizations combined with our theoretical analysis show that the thin monolayers selectively sift out water molecules, forming a drying layer to achieve the passivation of the protected 2D materials. The monolayer coating is also stable in air, H2 annealing, and organic solvents, but can be removed by certain organic acids.


2019 ◽  
Vol 10 (1) ◽  
Author(s):  
Lei Yin ◽  
Peng He ◽  
Ruiqing Cheng ◽  
Feng Wang ◽  
Fengmei Wang ◽  
...  

Abstract Defects play a crucial role in determining electric transport properties of two-dimensional transition metal dichalcogenides. In particular, defect-induced deep traps have been demonstrated to possess the ability to capture carriers. However, due to their poor stability and controllability, most studies focus on eliminating this trap effect, and little consideration was devoted to the applications of their inherent capabilities on electronics. Here, we report the realization of robust trap effect, which can capture carriers and store them steadily, in two-dimensional MoS2xSe2(1-x) via synergistic effect of sulphur vacancies and isoelectronic selenium atoms. As a result, infrared detection with very high photoresponsivity (2.4 × 105 A W−1) and photoswitching ratio (~108), as well as nonvolatile infrared memory with high program/erase ratio (~108) and fast switching time, are achieved just based on an individual flake. This demonstration of defect engineering opens up an avenue for achieving high-performance infrared detector and memory.


Nanoscale ◽  
2021 ◽  
Author(s):  
Zihao He ◽  
Xingyao Gao ◽  
Di Zhang ◽  
Ping Lu ◽  
Xuejing Wang ◽  
...  

Two-dimensional (2D) materials with robust ferromagnetic behavior have attracted great interest because of their potential applications in next-generation nanoelectronic devices. Aside from graphene and transition metal dichalcogenides, Bi-based layered oxide...


2021 ◽  
Author(s):  
Mubashir A. Kharadi ◽  
Gul Faroz A. Malik ◽  
Farooq A. Khanday

2D materials like transition metal dichalcogenides, black phosphorous, silicene, graphene are at the forefront of being the most potent 2D materials for optoelectronic applications because of their exceptional properties. Several application-specific photodetectors based on 2D materials have been designed and manufactured due to a wide range and layer-dependent bandgaps. Different 2D materials stacked together give rise to many surprising electronic and optoelectronic phenomena of the junctions based on 2D materials. This has resulted in a lot of popularity of 2D heterostructures as compared to the original 2D materials. This chapter presents the progress of optoelectronic devices (photodetectors) based on 2D materials and their heterostructures.


Nanophotonics ◽  
2020 ◽  
Vol 9 (8) ◽  
pp. 2169-2189 ◽  
Author(s):  
Bo Fu ◽  
Jingxuan Sun ◽  
Gang Wang ◽  
Ce Shang ◽  
Yuxuan Ma ◽  
...  

AbstractSince graphene was first reported as a saturable absorber to achieve ultrafast pulses in fiber lasers, many other two-dimensional (2D) materials, such as topological insulators, transition metal dichalcogenides, black phosphorus, and MXenes, have been widely investigated in fiber lasers due to their broadband operation, ultrafast recovery time, and controllable modulation depth. Recently, solution-processing methods for the fabrication of 2D materials have attracted considerable interest due to their advantages of low cost, easy fabrication, and scalability. Here, we review the various solution-processed methods for the preparation of different 2D materials. Then, the applications and performance of solution-processing-based 2D materials in fiber lasers are discussed. Finally, a perspective of the solution-processed methods and 2D material-based saturable absorbers are presented.


RSC Advances ◽  
2015 ◽  
Vol 5 (23) ◽  
pp. 17572-17581 ◽  
Author(s):  
Hongsheng Liu ◽  
Nannan Han ◽  
Jijun Zhao

Monolayer transition metal dichalcogenides (TMDs) stand out in two-dimensional (2D) materials due to their potential applications in future microelectronic and optoelectronic devices.


2020 ◽  
Vol 12 (1) ◽  
Author(s):  
Yanping Liu ◽  
Cheng Zeng ◽  
Jiahong Zhong ◽  
Junnan Ding ◽  
Zhiming M. Wang ◽  
...  

AbstractSpintronics, exploiting the spin degree of electrons as the information vector, is an attractive field for implementing the beyond Complemetary metal-oxide-semiconductor (CMOS) devices. Recently, two-dimensional (2D) materials have been drawing tremendous attention in spintronics owing to their distinctive spin-dependent properties, such as the ultra-long spin relaxation time of graphene and the spin–valley locking of transition metal dichalcogenides. Moreover, the related heterostructures provide an unprecedented probability of combining the different characteristics via proximity effect, which could remedy the limitation of individual 2D materials. Hence, the proximity engineering has been growing extremely fast and has made significant achievements in the spin injection and manipulation. Nevertheless, there are still challenges toward practical application; for example, the mechanism of spin relaxation in 2D materials is unclear, and the high-efficiency spin gating is not yet achieved. In this review, we focus on 2D materials and related heterostructures to systematically summarize the progress of the spin injection, transport, manipulation, and application for information storage and processing. We also highlight the current challenges and future perspectives on the studies of spintronic devices based on 2D materials.


Nanoscale ◽  
2017 ◽  
Vol 9 (48) ◽  
pp. 19124-19130 ◽  
Author(s):  
Lili Zhang ◽  
Chenyu Wang ◽  
Xue-Lu Liu ◽  
Tao Xu ◽  
Mingsheng Long ◽  
...  

As one of the most important family members of two-dimensional (2D) materials, the growth and damage-free transfer of transition metal dichalcogenides (TMDs) play crucial roles in their future applications.


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