Regional transport patterns for heavy PM2.5 pollution driven by strong cold airflows in Twain-Hu Basin, Central China

2021 ◽  
pp. 118847
Author(s):  
Lijuan Shen ◽  
Tianliang Zhao ◽  
Jane Liu ◽  
Honglei Wang ◽  
Yongqing Bai ◽  
...  
2020 ◽  
Vol 230 ◽  
pp. 117508
Author(s):  
Zhisheng Xiao ◽  
Yucong Miao ◽  
Xiaohui Du ◽  
Wei Tang ◽  
Yang Yu ◽  
...  

2021 ◽  
Author(s):  
Xiaoyun Sun ◽  
Tianliang Zhao ◽  
Yongqing Bai ◽  
Shaofei Kong ◽  
Huang Zheng ◽  
...  

Abstract. As an important issue in atmospheric environment, the contributions of anthropogenic emissions and meteorological conditions to air pollution have been few assessed over the receptor region in regional transport of air pollutants. In this study on observations of environment and meteorology over 2015–2019, the Kolmogorov–Zurbenko (KZ) filter was performed to decompose the PM2.5 variations into multi-time scale components over the Twain-Hu Basin (THB), a receptor region in regional transport of air pollutants in central China, where the short-term, seasonal and long-term components accounted for respectively 47.5 %, 41.4 % and 3.7 % to daily PM2.5 changes. The short-term and seasonal components dominated the day-to-day PM2.5 variations with long-term component determining the change trend of PM2.5 concentrations over recent years. The emission- and meteorology-related long-term PM2.5 components over the THB were identified. The meteorological contribution to PM2.5 declining trend presented the distinct spatial pattern over the THB with northern positive rates up to 61.92 % and southern negative rates down to −24.93 %. The opposite effects of meteorology on PM2.5 pollution could accelerate and offset the effects of emission reductions in the northern and southern THB, which is attributed to the upwind diffusion and downward accumulation of air pollutants over the receptor region in regional PM2.5 transport. It is noteworthy that the increasing conversion efficiencies of SO2 and NO2 to sulfate and nitrate for secondary PM2.5 could offset the effects of PM2.5 emission reduction on air pollution in the THB during recent years, revealing the enhancing contribution of gaseous precursor emissions to PM2.5 concentrations with controlling anthropogenic emissions of PM2.5 and the gaseous precursors over the receptor region in regional transport of air pollutants.


2017 ◽  
Vol 231 ◽  
pp. 612-621 ◽  
Author(s):  
Miaomiao Lu ◽  
Xiao Tang ◽  
Zifa Wang ◽  
Alex Gbaguidi ◽  
Shengwen Liang ◽  
...  

2020 ◽  
Vol 222 ◽  
pp. 117104 ◽  
Author(s):  
Lingjun Xia ◽  
Gen Zhang ◽  
Lixin Liu ◽  
Bozhen Li ◽  
Mingjing Zhan ◽  
...  

Atmosphere ◽  
2020 ◽  
Vol 11 (11) ◽  
pp. 1258 ◽  
Author(s):  
Weiyang Hu ◽  
Tianliang Zhao ◽  
Yongqing Bai ◽  
Lijuan Shen ◽  
Xiaoyun Sun ◽  
...  

The Twain-Hu basin (THB), covering the lower plain of Hubei and Hunan provinces in Central China, has experienced severe air pollution in recent years. However, the terrain effects of such sub-basin on air quality over the THB have been incomprehensibly understood. A heavy PM2.5 pollution event occurred over the THB during 4–10 January 2019. By using the observations and WRF-Chem simulations, we investigated the underlying mechanisms of sub-basin effects on the air pollution with several sensitivity experiments. Observationally, air pollution in the western THB urban area with an average PM2.5 concentration of 189.8 μg m−3, which was more serious than the eastern urban area with the average PM2.5 concentration of 106.3 μg m−3, reflecting a different influence of topography on air pollution over the THB. Simulation results revealed that the terrain effect can contribute 12.0% to increasing the PM2.5 concentrations in the western THB, but slightly mitigate the pollution extent in the eastern THB with the contribution of −4.6% to PM2.5 during the heavy pollution episode. In particular, the sub-basin terrain was conducive to the accumulation of PM2.5 by regional transport with the contribution of 39.1 %, and contrarily lowered its local pollution by −57.0% via the enhanced atmospheric boundary layer height and ventilation coefficients. Given a heavy air pollution episode occurring over the THB, such inverse contribution of terrain effects reflected a unique importance of sub-basin topography in regional transport of air pollutants for air pollution in central China.


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