Seasonal variation and source identification of atmospheric speciated mercury in an industrial harbor area in East Asia

Author(s):  
Chung-Shin Yuan ◽  
Cheng-En Lee ◽  
Iau-Ren Ie ◽  
Kuan-Chen Chiang ◽  
Yu-Lun Tseng ◽  
...  
2018 ◽  
Vol 18 (9) ◽  
pp. 6441-6460 ◽  
Author(s):  
Hewen Niu ◽  
Shichang Kang ◽  
Hailong Wang ◽  
Rudong Zhang ◽  
Xixi Lu ◽  
...  

Abstract. Deposition and accumulation of light-absorbing carbonaceous aerosol on glacier surfaces can alter the energy balance of glaciers. In this study, 2 years (December 2014 to December 2016) of continuous observations of carbonaceous aerosols in the glacierized region of the Mt. Yulong and Ganhaizi (GHZ) basin are analyzed. The average elemental carbon (EC) and organic carbon (OC) concentrations were 1.51±0.93 and 2.57±1.32 µg m−3, respectively. Although the annual mean OC ∕ EC ratio was 2.45±1.96, monthly mean EC concentrations during the post-monsoon season were even higher than OC in the high altitudes (approximately 5000 ma.s.l.) of Mt. Yulong. Strong photochemical reactions and local tourism activities were likely the main factors inducing high OC ∕ EC ratios in the Mt. Yulong region during the monsoon season. The mean mass absorption efficiency (MAE) of EC, measured for the first time in Mt. Yulong, at 632 nm with a thermal-optical carbon analyzer using the filter-based method, was 6.82±0.73 m2 g−1, comparable with the results from other studies. Strong seasonal and spatial variations of EC MAE were largely related to the OC abundance. Source attribution analysis using a global aerosol–climate model, equipped with a black carbon (BC) source tagging technique, suggests that East Asia emissions, including local sources, have the dominant contribution (over 50 %) to annual mean near-surface BC in the Mt. Yulong area. There is also a strong seasonal variation in the regional source apportionment. South Asia has the largest contribution to near-surface BC during the pre-monsoon season, while East Asia dominates the monsoon season and post-monsoon season. Results in this study have great implications for accurately evaluating the influences of carbonaceous matter on glacial melting and water resource supply in glacierization areas.


2019 ◽  
Vol 11 (6) ◽  
pp. 701 ◽  
Author(s):  
Di Liu ◽  
Tianliang Zhao ◽  
Richard Boiyo ◽  
Siyu Chen ◽  
Zhengqi Lu ◽  
...  

The spatiotemporal and especially the vertical distributions of dust aerosols play crucial roles in the climatic effect of dust aerosol. In the present study, the spatial-temporal distribution of dust aerosols over East Asia was investigated using Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observations (CALIPSO) retrievals (01/2007–12/2011) from the perspective of the frequency of dust occurrence (FDO), dust top layer height (TH) and profile of aerosol subtypes. The results showed that a typical dust belt was generated from the dust source regions (the Taklimakan and Gobi Deserts), in the latitude range of 25°N~45°N and reaching eastern China, Japan and Korea and, eventually, the Pacific Ocean. High dust frequencies were found over the dust source regions, with a seasonal sequence from high to low as follows: spring, summer, autumn and winter. Vertically, FDOs peaked at about 2 km over the dust source regions. In contrast, FDOs decreased with altitude over the downwind regions. On the dust belt from dust source regions to downwind regions, the dust top height (TH) was getting higher and higher. The dust TH varied in the range of 1.9–3.1 km above surface elevation (a.s.e.), with high values over the dust source regions and low values in the downwind areas, and a seasonally descending sequence of summer, spring, autumn and winter in accord with the seasonal variation of the boundary layer height. The annual AOD (Aerosol Optical Depth) was generally characterized by two high and two low AOD centers over East Asia. The percent contribution of the Dust Aerosol Optical Depth to the total AOD showed a seasonal variation from high to low as follows: spring, winter, autumn and summer. The vertical profile of the extinction coefficient revealed the predominance of pure dust particles in the dust source regions and a mixture of dust particles and pollutants in the downwind regions. The dust extinction coefficients over the Taklimakan Desert had a seasonal pattern from high to low as follows: spring, winter, summer and autumn. The results of the present study offered an understanding of the horizontal and vertical structures of dust aerosols over East Asia and can be used to evaluate the performance aerosol transport models.


Chemosphere ◽  
2022 ◽  
Vol 287 ◽  
pp. 132309
Author(s):  
Anas Ahmad Jamhari ◽  
Mohd Talib Latif ◽  
Muhammad Ikram A. Wahab ◽  
Hanashriah Hassan ◽  
Murnira Othman ◽  
...  

Sign in / Sign up

Export Citation Format

Share Document