scholarly journals Experimental consolidation and absolute measurement of the $$^\text {nat}$$C(p,x)$$^{11}$$C nuclear activation cross section at 100 MeV for particle therapy physics

2021 ◽  
Vol 57 (8) ◽  
Author(s):  
Claus Maximilian Bäcker ◽  
Felix Horst ◽  
Wihan Adi ◽  
Christian Bäumer ◽  
Marcel Gerhardt ◽  
...  
Keyword(s):  
Cross Section ◽  
Cross Sections ◽  
Proton Therapy ◽  
Gamma Ray ◽  
Absolute Measurement ◽  
Nuclear Data ◽  
Particle Therapy ◽  
Absolute Cross Section ◽  
Activation Cross Section ◽  
Gamma Ray Spectrometer

AbstractThe $$^\text {nat}$$ nat C(p,x)$$^{11}$$ 11 C reaction has been discussed in detail in the past [EXFOR database, Otuka et al. (Nuclear Data Sheets 120:272–276, 2014)]. However, measured activation cross sections by independent experiments are up to 15% apart. The aim of this study is to investigate underlying reasons for these observed discrepancies between different experiments and to determine a new consensus reference cross section at 100 MeV. Therefore, the experimental methods described in the two recent publications [Horst et al. (Phys Med Biol https://doi.org/10.1088/1361-6560/ab4511, 2019) and Bäcker et al. (Nuclear Instrum Methods Phys Res B 454:50–55, 2019)] are compared in detail and all experimental parameters are investigated for their impact on the results. For this purpose, a series of new experiments is performed. With the results of the experiments a new reference cross section of (68±3) mb is derived at (97±3) MeV proton energy. This value combined with the reliably measured excitation function could provide accurate cross section values for the energy region of proton therapy. Because of the well-known gamma-ray spectrometer used and the well-defined beam characteristics of the treatment machine at the proton therapy center, the experimental uncertainties on the absolute cross section could be reduced to 3%. Additionally, this setup is compared to the in-beam measurement setup from the second study presented in the literature (Horst et al. 2019). Another independent validation of the measurements is performed with a PET scanner.

scholarly journals 14.8 MeV Neutron Activation Cross Section Measurements for Ge Isotopes

2009 ◽  
Vol 1 (2) ◽  
pp. 173-181 ◽  
Author(s):  
M. M. Haque ◽  
M. T. Islam ◽  
M. A. Hafiz ◽  
R. U. Miah ◽  
M. S. Uddin
Keyword(s):  
Cross Section ◽  
Cross Sections ◽  
Gamma Ray ◽  
Reaction Cross ◽  
Activation Cross Section ◽  
Section Data ◽  
Gamma Ray Spectroscopy ◽  
24Na Reaction ◽  
The Cross ◽  
Good Agreement

The cross sections of Ge isotopes were measured with the activation method at 14.8 MeV neutron energy. The quasi-monoenergetic neutron beams were produced via the 3H(d,n)4He reaction at the 150 kV J-25 neutron generator of INST, AERE. The characteristics γ-lines of the product nuclei were measured with a closed end coaxial 17.5 cm2 high purity germanium (HPGe) detector gamma ray spectroscopy. The cross sections were determined with reference to the known 27Al(n,α)24Na reaction. Cross section data are presented for 72Ge(n,p)72Ga, 74Ge(n,α)71mZn and 76Ge(n,2n)75m+gGe reactions. The cross section values obtained for the above reactions were 24.78±1.75 mb, 1.69±0.11 mb and 860±50 mb, respectively. The results obtained were compared with the values reported in literature as well as theoretical calculation performed by the statistical code SINCROS-II. The experimental data were found fairly in good agreement with the calculated and literature data.  Keywords: Activation cross section; Neutron induced reaction; Gamma-ray spectroscopy; 14.8 MeV. © 2009 JSR Publications. ISSN: 2070-0237 (Print); 2070-0245 (Online). All rights reserved. DOI: 10.3329/jsr.v1i2.1532  

Absolute inner-shell cross section determination for EELS analysis

1988 ◽  
Vol 46 ◽  
pp. 534-535
Author(s):  
P.A. Crozier
Keyword(s):  
Cross Section ◽  
Cross Sections ◽  
Absolute Cross Section ◽  
Specimen Thickness ◽  
Mass Thickness ◽  
Scattering Cross ◽  
Before And After ◽  
Estimated Error ◽  
Scattering Cross Sections ◽  
Electron Microscopist

Absolute inelastic scattering cross sections or mean free paths are often used in EELS analysis for determining elemental concentrations and specimen thickness. In most instances, theoretical values must be used because there have been few attempts to determine experimental scattering cross sections from solids under the conditions of interest to electron microscopist. In addition to providing data for spectral quantitation, absolute cross section measurements yields useful information on many of the approximations which are frequently involved in EELS analysis procedures. In this paper, experimental cross sections are presented for some inner-shell edges of Al, Cu, Ag and Au.Uniform thin films of the previously mentioned materials were prepared by vacuum evaporation onto microscope cover slips. The cover slips were weighed before and after evaporation to determine the mass thickness of the films. The estimated error in this method of determining mass thickness was ±7 x 107g/cm2. The films were floated off in water and mounted on Cu grids.

scholarly journals Activation cross section of the (n,2n) reaction on Hf isotopes

2019 ◽  
Vol 23 ◽  
pp. 47
Author(s):  
A. Kalamara ◽  
M. Serris ◽  
A. Spiliotis ◽  
D. Sigalos ◽  
N. Patronis ◽  
...  
Keyword(s):  
Cross Section ◽  
Cross Sections ◽  
Reaction Cross Section ◽  
Beam Energy ◽  
Reaction Cross ◽  
Activation Technique ◽  
Incident Neutron ◽  
Activation Cross Section ◽  
Reference Reaction

Cross sections of the 174Hf(n,2n)173Hf and 176Hf(n,2n)175Hf reactions have been experimentally determined relative to the 27Al(n,α)24Na reference reaction at incident neutron energies of 15.3 and 17.1 MeV by means of the activation technique. The irradiations were carried out at the 5 MV tandem T11/25 Accelerator Laboratory of NCSR "Demokritos" with monoenergetic neutron beams provided via the 3H(d,n)4He reaction, using a new Ti-tritiated target of 373 GBq activity. In the determination of the 176Hf(n,2n)175Hf reaction cross section the contamination of the 174Hf(n,γ)175Hf and 177Hf(n,3n)175Hf reactions has been taken into account. Moreover, the neutron beam energy has been studied by means of Monte Carlo simulation codes and the neutron flux has been determined via the 27Al(n,α)24Na reference reaction.

scholarly journals Photoionisation Cross Sections of Chlorine Atoms and Molecules at 584 Å

1986 ◽  
Vol 39 (5) ◽  
pp. 779 ◽  
Author(s):  
WJ van der Meer ◽  
RJ Butselaar ◽  
CA de Lange
Keyword(s):  
Cross Section ◽  
Cross Sections ◽  
Ground State ◽  
Modulation Method ◽  
Absolute Cross Section ◽  
Molecular Chlorine ◽  
Chlorine Atoms ◽  
Atoms And Molecules ◽  
Ionic States ◽  
State Ionic

A recently developed modulation method is used to obtain cross sections for the photoionisation of ground state neutral to ground state ionic, atomic and molecular chlorine relative to that of the HCl + (X2n 1IZ,3IZ) +-- HCl(XI ~ +) transition at the He Ia wavelength. With the known absolute cross section of the latter process, determined by (e,2e) coincidence spectroscopy, the present ell,periments provide absolute photoionisation cross sections of the CI + epz,l,o) +-- Clep) and Cli (XZ n g, 1IZ,3 IZ) +-- Clz (X I ~ t) transitions. Relative cross sections, previously determined for the transitions to the additional Cl and Clz ionic states accessible with He Ia radiation, are used to obtain absolute cross sections for the Cl+(IDz, ISO) +-- Clep) and Cli(AZnu,1IZ,3IZ, BZ~t) +-- Clz(XI~t) ionisation processes.

scholarly journals Absolute cross section measurements of 238U(n,f) and 237Np(n,f) in the neutron energy range 1-2.4 MeV

2019 ◽  
Vol 211 ◽  
pp. 03009
Author(s):  
Paula Salvador-Castiñeira ◽  
Franz-Josef Hambsch ◽  
Alf Göök ◽  
Marzio Vidali ◽  
Nigel P. Hawkes ◽  
...  
Keyword(s):  
Cross Section ◽  
Neutron Energy ◽  
Cross Sections ◽  
Energy Region ◽  
Power Plants ◽  
National Physical Laboratory ◽  
Absolute Cross Section ◽  
Neutron Energy Range ◽  
Physical Laboratory ◽  
Low Energies

New standard (n,f) cross sections other than 235U are important to study the relevant cross sections for Generation-IV power plants. A specific need for such standards is for performing new experiments with quasimonoenergetic neutron beams, such as those produced by Van de Graaf accelerators. Neutrons down-scattered to low energies in the experimental environment, so called room-return, become relevant for this type of measurements. Hence, a standard (n,f) cross section with a fission threshold is of great interest, in order to suppress the contribution from room-return background. For this reason we have performed two experiments at the VDG of the National Physical Laboratory to measure absolutely the (n,f) cross sections of 235U, 238U and 237Np in the fast neutron energy region. Our preliminary results are in agreement with the most up-to-date evaluations.

scholarly journals CESAR5.3: Isotopic depletion for Research and Testing Reactor decommissioning

2018 ◽  
Vol 4 ◽  
pp. 10 ◽  
Author(s):  
Guillaume Ritter ◽  
Romain Eschbach ◽  
Richard Girieud ◽  
Maxime Soulard
Keyword(s):  
Nuclear Fuel ◽  
Cross Section ◽  
Cross Sections ◽  
Power Plants ◽  
Fuel Cycle ◽  
Nuclear Data ◽  
Computer Code ◽  
Test Case ◽  
Industrial Facilities ◽  
Transport Code

CESAR stands in French for “simplified depletion applied to reprocessing”. The current version is now number 5.3 as it started 30 years ago from a long lasting cooperation with ORANO, co-owner of the code with CEA. This computer code can characterize several types of nuclear fuel assemblies, from the most regular PWR power plants to the most unexpected gas cooled and graphite moderated old timer research facility. Each type of fuel can also include numerous ranges of compositions like UOX, MOX, LEU or HEU. Such versatility comes from a broad catalog of cross section libraries, each corresponding to a specific reactor and fuel matrix design. CESAR goes beyond fuel characterization and can also provide an evaluation of structural materials activation. The cross-sections libraries are generated using the most refined assembly or core level transport code calculation schemes (CEA APOLLO2 or ERANOS), based on the European JEFF3.1.1 nuclear data base. Each new CESAR self shielded cross section library benefits all most recent CEA recommendations as for deterministic physics options. Resulting cross sections are organized as a function of burn up and initial fuel enrichment which allows to condensate this costly process into a series of Legendre polynomials. The final outcome is a fast, accurate and compact CESAR cross section library. Each library is fully validated, against a stochastic transport code (CEA TRIPOLI 4) if needed and against a reference depletion code (CEA DARWIN). Using CESAR does not require any of the neutron physics expertise implemented into cross section libraries generation. It is based on top quality nuclear data (JEFF3.1.1 for ∼400 isotopes) and includes up to date Bateman equation solving algorithms. However, defining a CESAR computation case can be very straightforward. Most results are only 3 steps away from any beginner's ambition: Initial composition, in core depletion and pool decay scenario. On top of a simple utilization architecture, CESAR includes a portable Graphical User Interface which can be broadly deployed in R&D or industrial facilities. Aging facilities currently face decommissioning and dismantling issues. This way to the end of the nuclear fuel cycle requires a careful assessment of source terms in the fuel, core structures and all parts of a facility that must be disposed of with “industrial nuclear” constraints. In that perspective, several CESAR cross section libraries were constructed for early CEA Research and Testing Reactors (RTR’s). The aim of this paper is to describe how CESAR operates and how it can be used to help these facilities care for waste disposal, nuclear materials transport or basic safety cases. The test case will be based on the PHEBUS Facility located at CEA − Cadarache.

Bremsstrahlung linear polarization

1989 ◽  
Vol 67 (6) ◽  
pp. 545-561
Author(s):  
W. Del Bianco ◽  
M. Carignan
Keyword(s):  
Differential Cross Section ◽  
Cross Section ◽  
Cross Sections ◽  
Linear Polarization ◽  
Differential Cross ◽  
Born Approximation ◽  
Gamma Ray ◽  
High Energy ◽  
Scattered Electron ◽  
Triple Differential Cross Section

The dependence of the bremsstrahlung perpendicular and parallel triple differential cross sections and the linear polarization on the angles and energies of the incident and scattered electron and of the emitted gamma-ray has been studied in the high-energy small-angle hypothesis. The expression used for the bremsstrahlung triple differential cross section is valid in the Born approximation and for an unscreened Coulomb potential of the nucleus.

Activation cross section and isomeric cross-section ratio for the (n,2n) reaction on 132,134Ba

2017 ◽  
Vol 105 (10) ◽  
Author(s):  
Junhua Luo ◽  
Chunlei Wu ◽  
Li Jiang ◽  
Suyuan Li
Keyword(s):  
Cross Section ◽  
Cross Sections ◽  
Cross Section Ratio ◽  
Activation Cross Section ◽  
Section Ratio ◽  
Isomeric Cross Section Ratio

AbstractCross sections of the

scholarly journals Analysis of cross sections on iron and oxygen using Cf-252 neutron source

2020 ◽  
Vol 239 ◽  
pp. 18005
Author(s):  
Bohumil Jansky ◽  
Jiri Rejchrt ◽  
Evzen Novak ◽  
Anatoly Blokhin
Keyword(s):  
Cross Section ◽  
Neutron Source ◽  
Neutron Spectrum ◽  
Heavy Water ◽  
Cross Sections ◽  
Energy Region ◽  
Nuclear Data ◽  
Data Section ◽  
Neutron Spectra ◽  
Artificial Changes

The leakage neutron spectra measurements have been done on benchmark spherical assemblies with Cf-252 source in center of 1) heavy water sphere with diameter of 30 cm (with Cd cover) and of 2) iron spheres with diameter of 100 cm and 50 cm. It has been stated for years that transport calculations by iron overestimate measured spectra in energy region around 300 keV by about 20-40 % (calculation to measurement ratio C/E = 1.2-1.4). The influence of an artificial changes in cross-section XS-Fe-56 (n,elastic)designed by IAEA, Nuclear Data Section, has been studied on the iron spheres. Influence of those XS-corrections to calculated neutron spectrum is presented.

scholarly journals Developments in New Measurements of Fission Cross-Sections, Fragment Yields, and Prompt and Quasi-Prompt Gammas for Nuclear Data Needs

2020 ◽  
Vol 242 ◽  
pp. 01002
Author(s):  
Adam Hecht ◽  
Phoenix Baldez ◽  
Baldez Baldez
Keyword(s):  
Cross Sections ◽  
Ionization Chamber ◽  
Gamma Ray ◽  
Fission Products ◽  
Product Yield ◽  
Nuclear Data ◽  
University Of New Mexico ◽  
Alpha Emission ◽  
Time Projection ◽  
The University

The University of New Mexico Fission Spectrometer was developed to measure fission product yield, as part of the LANL SPIDER collaboration. The spectrometer operates as an E-v detector to extract product mass event-by-event, with a time of flight region followed by an ionization chamber for kinetic energy measurements. By using the ionization chamber as a singlecathode/single-anode time projection chamber, stopping power and thus Z information is extracted, for coupled A and Z measurements. New work is being performed to add gamma ray detectors in the data stream, placed near the target region for prompt gammas and near the ionization chamber for quasiprompt (>50 ns) and later gammas, correlated with individual fission products. A stand-alone parallel plate ionization chamber (PPIC) is also being developed for fission tagging gamma ray data. The PPIC will also allow discrimination between charged particle out events and (n,n’γ), and discriminate between alpha emission and fission. Using layers in the PPIC, other targets can be measured simultaneously with a calibration target, giving relative fission cross sections. Past measurements with the spectrometer were performed at LANSCE and we plan to continue measurements there. The current work is supported by the NNSA Stewardship Science Academic Alliance.

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