Long Persistent Luminescence: A Road Map Toward Promising Future Developments in Energy and Environmental Science

2021 ◽  
Vol 51 (1) ◽  
Author(s):  
Chiara Chiatti ◽  
Claudia Fabiani ◽  
Anna Laura Pisello
Keyword(s):  
Environmental Science ◽  
Energy Savings ◽  
Materials Science ◽  
Annual Review ◽  
Publication Date ◽  
Luminescent Materials ◽  
Persistent Luminescence ◽  
Road Map ◽  
Lighting Energy

In recent decades, research on persistent luminescence has led to new phosphors and promising performance. Efforts to improve the quality of phosphors’ afterglow have paved the way toward innovative solutions for many disciplines. However, there are few examples of the implementation of luminescent materials. In addition to providing a general background on persistent luminescence, the techniques used for its analysis, and its multidisciplinary potential in energy and environmental science, this article aims to explain the existing gap between the physical-chemical approach and the effective implementation of luminescent materials in larger-scale applications. It investigates engineering solutions in terms of the possible benefits of luminescence in lighting energy savings and passive cooling of urban surfaces. Finally, this article aims to reduce the abovementioned gap by suggesting what is most needed for the successful application of luminescent materials in the built environment. Expected final online publication date for the Annual Review of Materials Science, Volume 51 is July 2021. Please see http://www.annualreviews.org/page/journal/pubdates for revised estimates.

Heart Failure with Preserved Ejection Fraction: Mechanisms and Treatment Strategies

2021 ◽  
Vol 73 (1) ◽  
Author(s):  
Kazunori Omote ◽  
Frederik H. Verbrugge ◽  
Barry A. Borlaug
Keyword(s):  
Heart Failure ◽  
Ejection Fraction ◽  
Treatment Strategies ◽  
Annual Review ◽  
Publication Date ◽  
Preserved Ejection Fraction ◽  
Reduced Ejection Fraction ◽  
Patients With Heart Failure ◽  
Prevalence Of Obesity

Approximately half of all patients with heart failure (HF) have a preserved ejection fraction, and the prevalence is growing rapidly given the aging population in many countries and the rising prevalence of obesity, diabetes, and hypertension. Functional capacity and quality of life are severely impaired in heart failure with preserved ejection fraction (HFpEF), and morbidity and mortality are high. In striking contrast to HF with reduced ejection fraction, there are few effective treatments currently identified for HFpEF, and these are limited to decongestion by diuretics, promotion of a healthy active lifestyle, and management of comorbidities. Improved phenotyping of subgroups within the overall HFpEF population might enhance individualization of treatment. This review focuses on the current understanding of the pathophysiologic mechanisms underlying HFpEF and treatment strategies for this complex syndrome. Expected final online publication date for the Annual Review of Medicine, Volume 73 is January 2022. Please see http://www.annualreviews.org/page/journal/pubdates for revised estimates.

Electronic, Ionic, and Mixed Conduction in Polymeric Systems

2021 ◽  
Vol 51 (1) ◽  
Author(s):  
Elayne M. Thomas ◽  
Phong H. Nguyen ◽  
Seamus D. Jones ◽  
Michael L. Chabinyc ◽  
Rachel A. Segalman
Keyword(s):  
Materials Science ◽  
Transport Coefficients ◽  
Polymeric Materials ◽  
Annual Review ◽  
Publication Date ◽  
Energy Storage Devices ◽  
Polymeric Systems ◽  
Storage Devices ◽  
Technological Advances ◽  
Performance Benchmark

Polymers that simultaneously transport electrons and ions are paramount to drive the technological advances necessary for next-generation electrochemical devices, including energy storage devices and bioelectronics. However, efforts to describe the motion of ions or electrons separately within polymeric systems become inaccurate when both species are present. Herein, we highlight the basic transport equations necessary to rationalize mixed transport and the multiscale materials properties that influence their transport coefficients. Potential figures of merit that enable a suitable performance benchmark in mixed conducting systems independent of end application are discussed. Practical design and implementation of mixed conducting polymers require an understanding of the evolving nature of structure and transport with ionic and electronic carrier density to capture the dynamic disorder inherent in polymeric materials. Expected final online publication date for the Annual Review of Materials Science, Volume 51 is July 2021. Please see http://www.annualreviews.org/page/journal/pubdates for revised estimates.

Chemistry Under Shock Conditions

2021 ◽  
Vol 51 (1) ◽  
Author(s):  
Brenden W. Hamilton ◽  
Michael N. Sakano ◽  
Chunyu Li ◽  
Alejandro Strachan
Keyword(s):  
Materials Science ◽  
Low Frequency ◽  
Annual Review ◽  
Publication Date ◽  
Energy Localization ◽  
Ambient Conditions ◽  
Static Loads ◽  
Nonequilibrium Conditions ◽  
Life On Earth ◽  
Modes Coupling

Shock loading takes materials from ambient conditions to extreme conditions of temperature and nonhydrostatic stress on picosecond timescales. In molecular materials the fast loading results in temporary nonequilibrium conditions with overheated low-frequency modes and relatively cold, high-frequency, intramolecular modes; coupling the shock front with the material's microstructure and defects results in energy localization in hot spots. These processes can conspire to lead to a material response not observed under quasi-static loads. This review focuses on chemical reactions induced by dynamical loading, the understanding of which requires bringing together materials science, shock physics, and condensed matter chemistry. Recent progress in experiments and simulations holds the key to the answer of long-standing grand challenges with implications for the initiation of detonation and life on Earth. Expected final online publication date for the Annual Review of Materials Science, Volume 51 is August 2021. Please see http://www.annualreviews.org/page/journal/pubdates for revised estimates.

Thermoelectrics by Computational Design: Progress and Opportunities

2021 ◽  
Vol 51 (1) ◽  
Author(s):  
Boris Kozinsky ◽  
David J. Singh
Keyword(s):  
First Principles ◽  
High Performance ◽  
Materials Science ◽  
Phonon Scattering ◽  
Transport Coefficients ◽  
Computational Design ◽  
Science Volume ◽  
Annual Review ◽  
Publication Date ◽  
Boltzmann Transport

The performance of thermoelectric materials is determined by their electrical and thermal transport properties that are very sensitive to small modifications of composition and microstructure. Discovery and design of next-generation materials are starting to be accelerated by computational guidance. We review progress and challenges in the development of accurate and efficient first-principles methods for computing transport coefficients and illustrate approaches for both rapid materials screening and focused optimization. Particularly important and challenging are computations of electron and phonon scattering rates that enter the Boltzmann transport equations, and this is where there are many opportunities for improving computational methods. We highlight the first successful examples of computation-driven discoveries of high-performance materials and discuss avenues for tightening the interaction between theoretical and experimental materials discovery and optimization. Expected final online publication date for the Annual Review of Materials Science, Volume 51 is August 2021. Please see http://www.annualreviews.org/page/journal/pubdates for revised estimates.

Emerging Capabilities for the High-Throughput Characterization of Structural Materials

2021 ◽  
Vol 51 (1) ◽  
Author(s):  
Daniel B. Miracle ◽  
Mu Li ◽  
Zhaohan Zhang ◽  
Rohan Mishra ◽  
Katharine M. Flores
Keyword(s):  
High Throughput ◽  
Materials Science ◽  
Structural Materials ◽  
Rapid Screening ◽  
Annual Review ◽  
Publication Date ◽  
Synthesis Methods ◽  
Alloy Development ◽  
Composition Gradients ◽  
Future Vision

Structural materials have lagged behind other classes in the use of combinatorial and high-throughput (CHT) methods for rapid screening and alloy development. The dual complexities of composition and microstructure are responsible for this, along with the need to produce bulk-like, defect-free materials libraries. This review evaluates recent progress in CHT evaluations for structural materials. High-throughput computations can augment or replace experiments and accelerate data analysis. New synthesis methods, including additive manufacturing, can rapidly produce composition gradients or arrays of discrete alloys-on-demand in bulk form, and new experimental methods have been validated for nearly all essential structural materials properties. The remaining gaps are CHT measurement of bulk tensile strength, ductility, and melting temperature and production of microstructural libraries. A search strategy designed for structural materials gains efficiency by performing two layers of evaluations before addressing microstructure, and this review closes with a future vision of the autonomous, closed-loop CHT exploration of structural materials. Expected final online publication date for the Annual Review of Materials Science, Volume 51 is August 2021. Please see http://www.annualreviews.org/page/journal/pubdates for revised estimates.

The Centrality of Child Maltreatment to Criminology

2021 ◽  
Vol 5 (1) ◽  
Author(s):  
Sarah A. Font ◽  
Reeve Kennedy
Keyword(s):  
Child Welfare ◽  
Child Maltreatment ◽  
Child Welfare System ◽  
Welfare System ◽  
Sufficient Evidence ◽  
Annual Review ◽  
Publication Date ◽  
Crime And Delinquency ◽  
Comprehensive Measurement

Despite sufficient evidence to conclude that maltreatment exposure affects the risk of crime and delinquency, we conclude that the magnitude and specificity of effects of child maltreatment on crime and delinquency and the mechanisms through which those effects operate remain poorly identified. Key challenges include insufficient attention to the overlap of child maltreatment with various forms of family dysfunction and adversity and a lack of comprehensive measurement of the multiple, often comorbid, forms of child maltreatment. We then consider the potential impacts of the child welfare system on the maltreatment–crime link. Because the child welfare system typically provides voluntary, short-term services of unknown quality, it likely neither increases nor reduces risks of delinquency and crime for most children who are referred or investigated. For the comparatively small (although nominally large and important) subset of children experiencing foster care, impacts on delinquency and crime likely vary by the quality of environments within and after their time in care—issues that, to date, have received too little attention. Expected final online publication date for the Annual Review of Criminology, Volume 5 is January 2022. Please see http://www.annualreviews.org/page/journal/pubdates for revised estimates.

scholarly journals Understanding and Responding to Health Literacy as a Social Determinant of Health

2020 ◽  
Vol 42 (1) ◽  
Author(s):  
Don Nutbeam ◽  
Jane E. Lloyd
Keyword(s):  
Health Literacy ◽  
Social Determinant ◽  
Literacy Intervention ◽  
Annual Review ◽  
Publication Date ◽  
Future Health ◽  
Transferable Skills ◽  
Low Health Literacy ◽  
Social Determinant Of Health

Evidence of a social gradient in health literacy has been found in all reported national population surveys. Health literacy is a midstream determinant of health but not a panacea for health inequities created by the maldistribution of opportunity and resources. It is possible to optimize the contribution health literacy makes in mediating the causes and effects of established social determinants of health. Existing interventions demonstrate the feasibility of improving health literacy among higher-risk populations, but research remains underdeveloped and effects on health inequity are largely untested. Future health literacy intervention research should focus on ( a) improving the quality of health communication that reaches a diversity of populations, especially by improving frontline professional skills and support; ( b) enabling people to develop transferable skills in accessing, understanding, analyzing, and applying health information; and ( c) ensuring that priority is proportionate to need by reaching and engaging the population groups who are disproportionately affected by low health literacy. Expected final online publication date for the Annual Review of Public Health, Volume 42 is April 1, 2021. Please see http://www.annualreviews.org/page/journal/pubdates for revised estimates.

Shear Pleasure: The Structure, Formation, and Thermodynamics of Crystallographic Shear Phases

2021 ◽  
Vol 51 (1) ◽  
Author(s):  
Albert A. Voskanyan ◽  
Alexandra Navrotsky
Keyword(s):  
Materials Science ◽  
Defect Formation ◽  
Shear Plane ◽  
Annual Review ◽  
Publication Date ◽  
Future Directions ◽  
Extended Defect ◽  
Shear Structures ◽  
Crystallographic Shear ◽  
Exciting Area

A renaissance of interest in crystallographic shear structures and our recent work in this remarkable class of materials inspired this review. We first summarize the geometrical aspects of shear plane formation and possible transformations in ReO3, rutile, and perovskite-based structures. Then we provide a mechanistic overview of crystallographic shear formation, plane ordering, and propagation. Next we describe the energetics of planar defect formation and interaction, equilibria between point and extended defect structures, and thermodynamic stability of shear compounds. Finally, we emphasize the remaining challenges and propose future directions in this exciting area. Expected final online publication date for the Annual Review of Materials Science, Volume 51 is July 2021. Please see http://www.annualreviews.org/page/journal/pubdates for revised estimates.

Quantum Spin Liquids from a Materials Perspective

2021 ◽  
Vol 51 (1) ◽  
Author(s):  
Lucy Clark ◽  
Aly H. Abdeldaim
Keyword(s):  
Materials Science ◽  
Quantum Spin ◽  
Annual Review ◽  
Publication Date ◽  
Spin Liquids ◽  
Magnetic Systems ◽  
Quantum Spin Liquids ◽  
Interdisciplinary Field ◽  
Materials Research ◽  
Low Dimensional

Quantum spin liquids are unique quantum states of matter predicted to arise in low-dimensional, frustrated, and quantum magnetic systems. Compared with conventional ferromagnetic and antiferromagnetic states, quantum spin liquids are expected to display a variety of novel and exotic properties, making their realization in materials a highly appealing prospect. While an unambiguous realization of this long-sought-after state remains elusive, a growing number of materials candidates show promise in revealing the properties of quantum spin liquids. In this review, we present some of the key challenges and current opportunities in the synthesis, characterization, and understanding of quantum spin liquids from the perspective of the broad and interdisciplinary field of materials research. Expected final online publication date for the Annual Review of Materials Science, Volume 51 is August 2021. Please see http://www.annualreviews.org/page/journal/pubdates for revised estimates.

Looking Back, Looking Forward: Materials Science in Art, Archaeology, and Art Conservation

2021 ◽  
Vol 51 (1) ◽  
Author(s):  
Katherine T. Faber ◽  
Francesca Casadio ◽  
Admir Masic ◽  
Luc Robbiola ◽  
Marc Walton
Keyword(s):  
Cultural Heritage ◽  
Materials Science ◽  
Fine Arts ◽  
Life Cycles ◽  
Chemical Processes ◽  
Annual Review ◽  
Publication Date ◽  
Art Conservation ◽  
Sustainable Materials ◽  
Archaeological Objects

Cultural heritage materials, ranging from archaeological objects and sites to fine arts collections, are often characterized through their life cycle. In this review, the fundamentals and tools of materials science are used to explore such life cycles—first, via the origins of the materials and methods used to produce objects of function and artistry, and in some cases, examples of exceptional durability. The findings provide a window on our cultural heritage. Further, they inspire the design of sustainable materials for future generations. Also explored in this review are alteration phenomena over intervals as long as millennia or as brief as decades. Understanding the chemical processes that give rise to corrosion, passivation, or other degradation in chemical and physical properties can provide the foundation for conservation treatments. Finally, examples of characterization techniques that have been invented or enhanced to afford studies of cultural heritage materials, often nondestructively, are highlighted. Expected final online publication date for the Annual Review of Materials Science, Volume 51 is July 2021. Please see http://www.annualreviews.org/page/journal/pubdates for revised estimates.

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