scholarly journals Reply to “Comment on ‘Rethinking the Lower Bound on Aerosol Radiative Forcing’”

2017 ◽  
Vol 30 (16) ◽  
pp. 6585-6589 ◽  
Author(s):  
Bjorn Stevens ◽  
Stephanie Fiedler
Keyword(s):  
Twentieth Century ◽  
Lower Bound ◽  
Radiative Forcing ◽  
Climate Models ◽  
Anthropogenic Aerosols ◽  
Anthropogenic Aerosol ◽  
Aerosol Radiative Forcing ◽  
Clear Sky ◽  
The North ◽  
Aerosol Forcing

Kretzschmar et al., in a comment in 2017, use the spread in the output of aerosol–climate models to argue that the models refute the hypothesis (presented in a paper by Stevens in 2015) that for the mid-twentieth-century warming to be consistent with observations, then the present-day aerosol forcing, [Formula: see text] must be less negative than −1 W m−2. The main point of contention is the nature of the relationship between global SO2 emissions and [Formula: see text] In contrast to the concave (log-linear) relationship used by Stevens and in earlier studies, whereby [Formula: see text] becomes progressively less sensitive to SO2 emissions, some models suggest a convex relationship, which would imply a less negative lower bound. The model that best exemplifies this difference, and that is most clearly in conflict with the hypothesis of Stevens, does so because of an implausible aerosol response to the initial rise in anthropogenic aerosol precursor emissions in East and South Asia—already in 1975 this model’s clear-sky reflectance from anthropogenic aerosol over the North Pacific exceeds present-day estimates of the clear-sky reflectance by the total aerosol. The authors perform experiments using a new (observationally constrained) climatology of anthropogenic aerosols to further show that the effects of changing patterns of aerosol and aerosol precursor emissions during the late twentieth century have, for the same global emissions, relatively little effect on [Formula: see text] These findings suggest that the behavior Kretzschmar et al. identify as being in conflict with the lower bound in Stevens arises from an implausible relationship between SO2 emissions and [Formula: see text] and thus provides little basis for revising this lower bound.

scholarly journals MACv2-SP: a parameterization of anthropogenic aerosol optical properties and an associated Twomey effect for use in CMIP6

2017 ◽  
Vol 10 (1) ◽  
pp. 433-452 ◽  
Author(s):  
Bjorn Stevens ◽  
Stephanie Fiedler ◽  
Stefan Kinne ◽  
Karsten Peters ◽  
Sebastian Rast ◽  
...  
Keyword(s):  
Optical Properties ◽  
Radiative Forcing ◽  
Industrial Emissions ◽  
Max Planck ◽  
Aerosol Optical Properties ◽  
Anthropogenic Aerosol ◽  
Aerosol Radiative Forcing ◽  
Clear Sky ◽  
Aerosol Forcing ◽  
Aerosol Radiative

Abstract. A simple plume implementation of the second version (v2) of the Max Planck Institute Aerosol Climatology, MACv2-SP, is described. MACv2-SP provides a prescription of anthropogenic aerosol optical properties and an associated Twomey effect. It was created to provide a harmonized description of post-1850 anthropogenic aerosol radiative forcing for climate modeling studies. MACv2-SP has been designed to be easy to implement, change and use, and thereby enable studies exploring the climatic effects of different patterns of aerosol radiative forcing, including a Twomey effect. MACv2-SP is formulated in terms of nine spatial plumes associated with different major anthropogenic source regions. The shape of the plumes is fit to the Max Planck Institute Aerosol Climatology, version 2, whose present-day (2005) distribution is anchored by surface-based observations. Two types of plumes are considered: one predominantly associated with biomass burning, the other with industrial emissions. These differ in the prescription of their annual cycle and in their optical properties, thereby implicitly accounting for different contributions of absorbing aerosol to the different plumes. A Twomey effect for each plume is prescribed as a change in the host model's background cloud-droplet population density using relationships derived from satellite data. Year-to-year variations in the amplitude of the plumes over the historical period (1850–2016) are derived by scaling the plumes with associated national emission sources of SO2 and NH3. Experiments using MACv2-SP are performed with the Max Planck Institute Earth System Model. The globally and annually averaged instantaneous and effective aerosol radiative forcings are estimated to be −0.6 and −0.5 W m−2, respectively. Forcing from aerosol–cloud interactions (the Twomey effect) offsets the reduction of clear-sky forcing by clouds, so that the net effect of clouds on the aerosol forcing is small; hence, the clear-sky forcing, which is more readily measurable, provides a good estimate of the total aerosol forcing.

scholarly journals Anthropogenic aerosol forcing under the Shared Socioeconomic Pathways

2019 ◽  
Author(s):  
Marianne T. Lund ◽  
Gunnar Myhre ◽  
Bjørn H. Samset
Keyword(s):  
Air Pollution ◽  
Radiative Forcing ◽  
Global Climate ◽  
Radiative Transfer Model ◽  
Transfer Model ◽  
Air Pollution Control ◽  
Anthropogenic Aerosols ◽  
Anthropogenic Aerosol ◽  
Aerosol Radiative Forcing ◽  
Aerosol Forcing

Abstract. Emissions of anthropogenic aerosols are expected to change drastically over the coming decades, with potentially significant climate implications. Using the most recent generation of harmonized emission scenarios, the Shared Socioeconomic Pathways (SSPs) as input to a global chemistry transport and radiative transfer model, we provide estimates of the projected future global and regional burdens and radiative forcing of anthropogenic aerosols under three different levels of air pollution control: strong (SSP1), medium (SSP2) and weak (SSP3). We find that the broader range of future air pollution emission trajectories spanned by the SSPs compared to previous scenarios translates into total aerosol forcing estimates in 2100 relative to 1750 ranging from −0.04 W m−2 in SSP1-1.9 to −0.51 W m−2 in SSP3-7.0. Compared to our 1750–2015 estimate of −0.61 W m−2, this shows that depending on the success of air pollution policies over the coming decades, aerosol radiative forcing may weaken by nearly 95 % or remain close to the pre-industrial to present-day level. In all three scenarios there is a positive forcing in 2100 relative to 2015, from 0.51 W m−2 in SSP1-1.9 to 0.04 W m−2 in SSP3-7.0. Results also demonstrate significant differences across regions and scenarios, especially in South Asia and Africa. While rapid weakening of the negative aerosol forcing following effective air quality policies will unmask more of the greenhouse gas-induced global warming, slow progress on mitigating air pollution will significantly enhance the atmospheric aerosol levels and risk to human health. In either case, the resulting impacts on regional and global climate can be significant.

scholarly journals A Limited Role for Unforced Internal Variability in Twentieth-Century Warming

2019 ◽  
Vol 32 (16) ◽  
pp. 4893-4917 ◽  
Author(s):  
Karsten Haustein ◽  
Friederike E. L. Otto ◽  
Victor Venema ◽  
Peter Jacobs ◽  
Kevin Cowtan ◽  
...  
Keyword(s):  
Twentieth Century ◽  
Surface Temperature ◽  
Radiative Forcing ◽  
Low Frequency ◽  
Internal Variability ◽  
External Forcing ◽  
Anthropogenic Aerosol ◽  
Transient Climate Response ◽  
The North ◽  
Aerosol Forcing

AbstractThe early twentieth-century warming (EW; 1910–45) and the mid-twentieth-century cooling (MC; 1950–80) have been linked to both internal variability of the climate system and changes in external radiative forcing. The degree to which either of the two factors contributed to EW and MC, or both, is still debated. Using a two-box impulse response model, we demonstrate that multidecadal ocean variability was unlikely to be the driver of observed changes in global mean surface temperature (GMST) after AD 1850. Instead, virtually all (97%–98%) of the global low-frequency variability (>30 years) can be explained by external forcing. We find similarly high percentages of explained variance for interhemispheric and land–ocean temperature evolution. Three key aspects are identified that underpin the conclusion of this new study: inhomogeneous anthropogenic aerosol forcing (AER), biases in the instrumental sea surface temperature (SST) datasets, and inadequate representation of the response to varying forcing factors. Once the spatially heterogeneous nature of AER is accounted for, the MC period is reconcilable with external drivers. SST biases and imprecise forcing responses explain the putative disagreement between models and observations during the EW period. As a consequence, Atlantic multidecadal variability (AMV) is found to be primarily controlled by external forcing too. Future attribution studies should account for these important factors when discriminating between externally forced and internally generated influences on climate. We argue that AMV must not be used as a regressor and suggest a revised AMV index instead [the North Atlantic Variability Index (NAVI)]. Our associated best estimate for the transient climate response (TCR) is 1.57 K (±0.70 at the 5%–95% confidence level).

Comment on “Rethinking the Lower Bound on Aerosol Radiative Forcing”

2017 ◽  
Vol 30 (16) ◽  
pp. 6579-6584 ◽  
Author(s):  
Jan Kretzschmar ◽  
Marc Salzmann ◽  
Johannes Mülmenstädt ◽  
Olivier Boucher ◽  
Johannes Quaas
Keyword(s):  
Radiative Forcing ◽  
Climate Models ◽  
Coupled Model ◽  
Warming Trend ◽  
Anthropogenic Aerosols ◽  
Aerosol Radiative Forcing ◽  
Aerosol Forcing ◽  
Interesting Study ◽  
Log Linear ◽  
Negative Formula

In an influential and interesting study, Stevens (2015) suggested that the global and also Northern Hemispheric warming during the early industrial period implies that the effective radiative forcing [Formula: see text] by anthropogenic aerosols in the year 2000 compared to 1850 cannot be more negative than −1.0 W m−2. Here results from phase 5 of the Coupled Model Intercomparison Project are analyzed and it is shown that there is little relationship between [Formula: see text] and the warming trend in the early industrial period in comprehensive climate models. In particular, some models simulate a warming in the early industrial period despite a strong (very negative) [Formula: see text]. The reason for this difference in results is that the global-mean log-linear scaling of [Formula: see text] with anthropogenic sulfur dioxide emissions introduced and used by Stevens tends to produce a substantially larger aerosol forcing compared to climate models in the first half of the twentieth century, when SO2 emissions were concentrated over smaller regions. In turn, it shows smaller (less negative) [Formula: see text] in the recent period with comparatively more widespread SO2 emissions.

scholarly journals Influence of future air pollution mitigation strategies on total aerosol radiative forcing

2008 ◽  
Vol 8 (21) ◽  
pp. 6405-6437 ◽  
Author(s):  
S. Kloster ◽  
F. Dentener ◽  
J. Feichter ◽  
F. Raes ◽  
J. van Aardenne ◽  
...  
Keyword(s):  
Air Pollution ◽  
Radiative Forcing ◽  
Mitigation Strategies ◽  
Radiation Budget ◽  
Anthropogenic Aerosol ◽  
Aerosol Radiative Forcing ◽  
Pollution Mitigation ◽  
Aerosol Forcing ◽  
Future Air Pollution ◽  
Aerosol Radiative

Abstract. We apply different aerosol and aerosol precursor emission scenarios reflecting possible future control strategies for air pollution in the ECHAM5-HAM model, and simulate the resulting effect on the Earth's radiation budget. We use two opposing future mitigation strategies for the year 2030: one in which emission reduction legislation decided in countries throughout the world are effectively implemented (current legislation; CLE 2030) and one in which all technical options for emission reductions are being implemented independent of their cost (maximum feasible reduction; MFR 2030). We consider the direct, semi-direct and indirect radiative effects of aerosols. The total anthropogenic aerosol radiative forcing defined as the difference in the top-of-the-atmosphere radiation between 2000 and pre-industrial times amounts to −2.00 W/m2. In the future this negative global annual mean aerosol radiative forcing will only slightly change (+0.02 W/m2) under the "current legislation" scenario. Regionally, the effects are much larger: e.g. over Eastern Europe radiative forcing would increase by +1.50 W/m2 because of successful aerosol reduction policies, whereas over South Asia it would decrease by −1.10 W/m2 because of further growth of emissions. A "maximum feasible reduction" of aerosols and their precursors would lead to an increase of the global annual mean aerosol radiative forcing by +1.13 W/m2. Hence, in the latter case, the present day negative anthropogenic aerosol forcing could be more than halved by 2030 because of aerosol reduction policies and climate change thereafter will be to a larger extent be controlled by greenhouse gas emissions. We combined these two opposing future mitigation strategies for a number of experiments focusing on different sectors and regions. In addition, we performed sensitivity studies to estimate the importance of future changes in oxidant concentrations and the importance of the aerosol microphysical coupling within the range of expected future changes. For changes in oxidant concentrations caused by future air pollution mitigation, we do not find a significant effect for the global annual mean radiative aerosol forcing. In the extreme case of only abating SO2 or carbonaceous emissions to a maximum feasible extent, we find deviations from additivity for the radiative forcing over anthropogenic source regions up to 10% compared to an experiment abating both at the same time.

scholarly journals Anthropogenic aerosol forcing – insights from multiple estimates from aerosol-climate models with reduced complexity

2019 ◽  
Vol 19 (10) ◽  
pp. 6821-6841 ◽  
Author(s):  
Stephanie Fiedler ◽  
Stefan Kinne ◽  
Wan Ting Katty Huang ◽  
Petri Räisänen ◽  
Declan O'Donnell ◽  
...  
Keyword(s):  
Radiative Forcing ◽  
Climate Models ◽  
Coupled Model ◽  
Cloud Droplet ◽  
Internal Variability ◽  
Anthropogenic Aerosol ◽  
Aerosol Forcing ◽  
Effective Radiative Forcing ◽  
Absolute Magnitudes ◽  
Natural Aerosols

Abstract. This study assesses the change in anthropogenic aerosol forcing from the mid-1970s to the mid-2000s. Both decades had similar global-mean anthropogenic aerosol optical depths but substantially different global distributions. For both years, we quantify (i) the forcing spread due to model-internal variability and (ii) the forcing spread among models. Our assessment is based on new ensembles of atmosphere-only simulations with five state-of-the-art Earth system models. Four of these models will be used in the sixth Coupled Model Intercomparison Project (CMIP6; Eyring et al., 2016). Here, the complexity of the anthropogenic aerosol has been reduced in the participating models. In all our simulations, we prescribe the same patterns of the anthropogenic aerosol optical properties and associated effects on the cloud droplet number concentration. We calculate the instantaneous radiative forcing (RF) and the effective radiative forcing (ERF). Their difference defines the net contribution from rapid adjustments. Our simulations show a model spread in ERF from −0.4 to −0.9 W m−2. The standard deviation in annual ERF is 0.3 W m−2, based on 180 individual estimates from each participating model. This result implies that identifying the model spread in ERF due to systematic differences requires averaging over a sufficiently large number of years. Moreover, we find almost identical ERFs for the mid-1970s and mid-2000s for individual models, although there are major model differences in natural aerosols and clouds. The model-ensemble mean ERF is −0.54 W m−2 for the pre-industrial era to the mid-1970s and −0.59 W m−2 for the pre-industrial era to the mid-2000s. Our result suggests that comparing ERF changes between two observable periods rather than absolute magnitudes relative to a poorly constrained pre-industrial state might provide a better test for a model's ability to represent transient climate changes.

scholarly journals Comparison of Climate Response to Anthropogenic Aerosol versus Greenhouse Gas Forcing: Distinct Patterns

2016 ◽  
Vol 29 (14) ◽  
pp. 5175-5188 ◽  
Author(s):  
Hai Wang ◽  
Shang-Ping Xie ◽  
Qinyu Liu
Keyword(s):  
Northern Hemisphere ◽  
Radiative Forcing ◽  
Climate Model ◽  
East Asian Monsoon ◽  
Climate Response ◽  
Anthropogenic Aerosols ◽  
Anthropogenic Aerosol ◽  
Asian Monsoon Region ◽  
Surface Temperature Change ◽  
Aerosol Forcing

Abstract Spatial patterns of climate response to changes in anthropogenic aerosols and well-mixed greenhouse gases (GHGs) are investigated using climate model simulations for the twentieth century. The climate response shows both similarities and differences in spatial pattern between aerosol and GHG runs. Common climate response between aerosol and GHG runs tends to be symmetric about the equator. This work focuses on the distinctive patterns that are unique to the anthropogenic aerosol forcing. The tropospheric cooling induced by anthropogenic aerosols is locally enhanced in the midlatitude Northern Hemisphere with a deep vertical structure around 40°N, anchoring a westerly acceleration in thermal wind balance. The aerosol-induced negative radiative forcing in the Northern Hemisphere requires a cross-equatorial Hadley circulation to compensate interhemispheric energy imbalance in the atmosphere. Associated with a southward shift of the intertropical convergence zone, this interhemispheric asymmetric mode is unique to aerosol forcing and absent in GHG runs. Comparison of key climate response pattern indices indicates that the aerosol forcing dominates the interhemispheric asymmetric climate response in historical all-forcing simulations, as well as regional precipitation change such as the drying trend over the East Asian monsoon region. While GHG forcing dominates global mean surface temperature change, its effect is on par with and often opposes the aerosol effect on precipitation, making it difficult to detect anthropogenic change in rainfall from historical observations.

scholarly journals Dynamics of Asian Summer Monsoon Response to Anthropogenic Aerosol Forcing

2019 ◽  
Vol 32 (3) ◽  
pp. 843-858 ◽  
Author(s):  
Hai Wang ◽  
Shang-Ping Xie ◽  
Yu Kosaka ◽  
Qinyu Liu ◽  
Yan Du
Keyword(s):  
Summer Monsoon ◽  
Radiative Forcing ◽  
Asian Summer Monsoon ◽  
Atmospheric Response ◽  
Anthropogenic Aerosols ◽  
Anthropogenic Aerosol ◽  
Sst Cooling ◽  
Aerosol Forcing ◽  
Cooling Pattern ◽  
Asian Summer

Anthropogenic aerosols partially mask the greenhouse warming and cause the reduction in Asian summer monsoon precipitation and circulation. By decomposing the atmospheric change into the direct atmospheric response to radiative forcing and sea surface temperature (SST)-mediated change, the physical mechanisms for anthropogenic-aerosol-induced changes in the East Asian summer monsoon (EASM) and South Asian summer monsoon (SASM) are diagnosed. Using coupled and atmospheric general circulation models, this study shows that the aerosol-induced troposphere cooling over Asian land regions generates anomalous sinking motion between 20° and 40°N and weakens the EASM north of 20°N without SST change. The decreased EASM precipitation and the attendant wind changes are largely due to this direct atmospheric response to radiative forcing, although the aerosol-induced North Pacific SST cooling also contributes. The SST-mediated change dominates the aerosol-induced SASM response, with contributions from both the north–south interhemispheric SST gradient and the local SST cooling pattern over the tropical Indian Ocean. Specifically, with large meridional gradient, the zonal-mean SST cooling pattern is most important for the Asian summer monsoon response to anthropogenic aerosol forcing, resulting in a reorganization of the regional meridional atmospheric overturning circulation. While uncertainty in aerosol radiative forcing has been emphasized in the literature, our results show that the intermodel spread is as large in the SST effect on summer monsoon rainfall, calling for more research into the ocean–atmosphere coupling.

scholarly journals Reduced anthropogenic aerosol radiative forcing caused by biogenic new particle formation

2016 ◽  
Vol 113 (43) ◽  
pp. 12053-12058 ◽  
Author(s):  
Hamish Gordon ◽  
Kamalika Sengupta ◽  
Alexandru Rap ◽  
Jonathan Duplissy ◽  
Carla Frege ◽  
...  
Keyword(s):  
Radiative Forcing ◽  
Cloud Condensation Nuclei ◽  
Large Fraction ◽  
Particle Formation ◽  
Lower Atmosphere ◽  
Anthropogenic Aerosols ◽  
Anthropogenic Aerosol ◽  
Aerosol Radiative Forcing ◽  
Cloud Albedo ◽  
Aerosol Radiative

The magnitude of aerosol radiative forcing caused by anthropogenic emissions depends on the baseline state of the atmosphere under pristine preindustrial conditions. Measurements show that particle formation in atmospheric conditions can occur solely from biogenic vapors. Here, we evaluate the potential effect of this source of particles on preindustrial cloud condensation nuclei (CCN) concentrations and aerosol–cloud radiative forcing over the industrial period. Model simulations show that the pure biogenic particle formation mechanism has a much larger relative effect on CCN concentrations in the preindustrial atmosphere than in the present atmosphere because of the lower aerosol concentrations. Consequently, preindustrial cloud albedo is increased more than under present day conditions, and therefore the cooling forcing of anthropogenic aerosols is reduced. The mechanism increases CCN concentrations by 20–100% over a large fraction of the preindustrial lower atmosphere, and the magnitude of annual global mean radiative forcing caused by changes of cloud albedo since 1750 is reduced by 0.22 W m−2 (27%) to −0.60 W m−2. Model uncertainties, relatively slow formation rates, and limited available ambient measurements make it difficult to establish the significance of a mechanism that has its dominant effect under preindustrial conditions. Our simulations predict more particle formation in the Amazon than is observed. However, the first observation of pure organic nucleation has now been reported for the free troposphere. Given the potentially significant effect on anthropogenic forcing, effort should be made to better understand such naturally driven aerosol processes.

scholarly journals Comparison of Anthropogenic Aerosol Climate Effects among Three Climate Models with Reduced Complexity

Atmosphere ◽  
2019 ◽  
Vol 10 (8) ◽  
pp. 456 ◽  
Author(s):  
Xiangjun Shi ◽  
Wentao Zhang ◽  
Jiaojiao Liu
Keyword(s):  
Radiative Forcing ◽  
Climate Models ◽  
Reliable Estimate ◽  
Anthropogenic Aerosol ◽  
Climate Effects ◽  
Cloud Forcing ◽  
Radiative Forcings ◽  
Ensemble Simulations ◽  
Aerosol Forcing ◽  
The Difference

The same prescribed anthropogenic aerosol forcing was implemented into three climate models. The atmosphere components of these participating climate models were the GAMIL, ECHAM, and CAM models. Ensemble simulations were carried out to obtain a reliable estimate of anthropogenic aerosol effective radiative forcing (ERF). The ensemble mean ERFs from these three participating models with this aerosol forcing were −0.27, −0.63, and −0.54 W∙m−2. The model diversity in ERF is clearly reduced as compared with those based on the models’ own default approaches (−1.98, −0.21, and −2.22 W∙m−2). This is consistent with the design of this aerosol forcing. The modeled ERF can be decomposed into two basic components, i.e., the instantaneous radiative forcing (RF) from aerosol–radiation interactions (RFari) and the aerosol-induced changes in cloud forcing (△Fcloud*). For the three participating models, the model diversity in RFari (−0.21, −0.33, and −0.29 W∙m−2) could be constrained by reducing the differences in natural aerosol radiative forcings. However, it was difficult to figure out the reason for the model diversity in △Fcloud* (−0.05, −0.28, and −0.24 W∙m−2), which was the dominant source of the model diversity in ERF. The variability of modeled ERF was also studied. Ensemble simulations showed that the modeled RFs were very stable. The rapid adjustments (ERF − RF) had an important role to play in the quantification of the perturbation of ERF. Fortunately, the contribution from the rapid adjustments to the mean ERF was very small. This study also showed that we should pay attention to the difference between the aerosol climate effects we want and the aerosol climate effects we calculate.

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