scholarly journals Laser-Inscribed Stress-Induced Birefringence of Sapphire

Nanomaterials ◽  
2019 ◽  
Vol 9 (10) ◽  
pp. 1414 ◽  
Author(s):  
Hua Fan ◽  
Meguya Ryu ◽  
Reo Honda ◽  
Junko Morikawa ◽  
Zhen-Ze Li ◽  
...  
Keyword(s):  
Bessel Beam ◽  
Laser Pulses ◽  
Visible Spectral Range ◽  
Vortex Generation ◽  
Cross Sectional ◽  
Optical Elements ◽  
High Birefringence ◽  
Self Organized ◽  
Fs Laser ◽  
Spatially Varying

Birefringence of 3 × 10 - 3 is demonstrated inside cross-sectional regions of 100 μ m, inscribed by axially stretched Bessel-beam-like fs-laser pulses along the c-axis inside sapphire. A high birefringence and retardance of λ / 4 at mid-visible spectral range (green) can be achieved using stretched beams with axial extension of 30–40 μ m. Chosen conditions of laser-writing ensure that there are no formations of self-organized nano-gratings. This method can be adopted for creation of polarization optical elements and fabrication of spatially varying birefringent patterns for optical vortex generation.

scholarly journals All Femtosecond Optical Pump and X-Ray Probe: Holey-Axicon for Free Electron Laser

2020 ◽  
Author(s):  
Vijayakumar Anand ◽  
Jovan Maksimovic ◽  
Tomas Katkus ◽  
Soon Hock Ng ◽  
Orestas Ulcinas ◽  
...  
Keyword(s):  
Free Electron ◽  
Free Electron Laser ◽  
Optical Axis ◽  
Bessel Beam ◽  
X Rays ◽  
Temporal Dimension ◽  
Optical Elements ◽  
Optical Pump ◽  
X Ray ◽  
Fs Laser

We put forward a co-axial pump(optical)-probe(X-rays) experimental concept and show performance of the optical component. A Bessel beam generator with a central 100 micrometers-diameter hole (on the optical axis) was fabricated using femtosecond (fs) laser structuring inside a silica plate. This flat-axicon optical element produces a needle-like axial intensity distribution which can be used for the optical pump pulse. The fs-X-ray free electron laser (X-FEL) beam of sub-1 micrometer diameter can be introduced through the central hole along the optical axis onto a target as a probe. Different realisations of optical pump are discussed. Such optical elements facilitate alignment of ultra-short fs-pulses in space and time and can be used in light-matter interaction experiments at extreme energy densities on the surface and in the volume of targets. Full advantage of ultra-short 10 fs X-FEL probe pulses with fs-pump(optical) opens an unexplored temporal dimension of phase transitions and the fastest laser-induced rates of material heating and quenching. A wider field of applications of fs-laser-enabled structuring of materials and design of specific optical elements for astrophotonics is presented.

Nanoscale Heat Transport in Self-Organized Ge Clusters on Si(001)

2012 ◽  
Vol 1456 ◽  
Author(s):  
Tim Frigge ◽  
Annika Kalus ◽  
Friedrich Klasing ◽  
Martin Kammler ◽  
Anja Hanisch-Blicharski ◽  
...  
Keyword(s):  
Laser Pulses ◽  
Transient Temperature ◽  
Equivalent Thickness ◽  
Time Resolved ◽  
Pump Probe ◽  
Nanoscale Heat Transport ◽  
Self Organized ◽  
Transmission Electron ◽  
Fs Laser ◽  
Cooling Behavior

ABSTRACTUltrafast time resolved transmission electron diffraction (TED) in a reflection geometry was used to study the cooling behavior of self-organized, well defined nanoscale germanium hut and dome clusters on Si(001). The clusters were heated in a pump-probe scheme by fs-laser pulses. The resulting transient temperature rise was then determined from the drop in diffraction intensity caused by the Debye-Waller effect. From a cooling time of τ =177 ps we estimated a strongly reduced heat transfer compared with homogeneous films of equivalent thickness.

scholarly journals Few Percent Efficient Polarization-Sensitive Conversion in Nonlinear Plasmonic Interactions Inside Oligomeric Gold Structures

Sensors ◽  
2020 ◽  
Vol 21 (1) ◽  
pp. 59
Author(s):  
Nikolay Busleev ◽  
Sergey Kudryashov ◽  
Irina Saraeva ◽  
Pavel Danilov ◽  
Andrey Rudenko ◽  
...  
Keyword(s):  
Plasmon Resonance ◽  
Laser Pulses ◽  
Visible Range ◽  
Oligomeric Structure ◽  
Self Organized ◽  
Electromagnetic Interactions ◽  
Nanoscale Characterization ◽  
Fs Laser ◽  
The Individual ◽  
Anti Stokes

The backscattering spectra of a 500 nm thick gold film, which was excited near the 525 nm transverse localized plasmon resonance of its constituent, self-organized, vertically-aligned nanorods by normally incident 515 nm, 300 fs laser pulses with linear, radial, azimuthal and circular polarizations, revealed a few-percent conversion into Stokes and anti-Stokes side-band peaks. The investigation of these spectral features based on the nanoscale characterization of the oligomeric structure and numerical simulations of its backscattering response indicated nonlinear Fano-like plasmonic interactions, particularly the partially degenerate four-wave mixing comprised by the visible-range transverse plasmon resonance of the individual nanorods and an IR-range collective mode of the oligomeric structure. Such oligomeric structures in plasmonic films may greatly enhance inner nonlinear electromagnetic interactions and inner near-IR hotspots, paving the way for their engineered IR tunability for broad applications in chemosensing and biosensing.

scholarly journals Crystallization of optically thick amorphous silicon films by near-IR femtosecond laser processing

2020 ◽  
Author(s):  
Kirill Bronnikov ◽  
Alexander Dostovalov ◽  
Artem Cherepakhin ◽  
Eugeny Mitsai ◽  
Alexander Nepomniaschiy ◽  
...  
Keyword(s):  
Femtosecond Laser ◽  
Amorphous Silicon ◽  
Laser Pulses ◽  
Femtosecond Laser Pulses ◽  
Visible Spectral Range ◽  
Ir Radiation ◽  
Optical Elements ◽  
Near Ir ◽  
Lateral Crystallization ◽  
Si Films

Amorphous silicon (α-Si) film present an inexpensive and promising material for optoelectronic and nanophotonic applications. Its basic optical and optoelectronic properties are known to be improved via phase transition from amorphous to polycrystalline phase. Infrared femtosecond laser radiation can be considered as a promising nondestructive and facile way to drive uniform in-depth and lateral crystallization of α-Si films that are typically opaque in UV-visible spectral range. However, so far only a few studies reported on utilization of near-IR radiation for laser-induced crystallization of α-Si providing no information regarding optical properties of the resultant polycrystalline Si films. The present work demonstrates efficient and gentle single-pass crystallization of α-Si films induced by their direct irradiation with near-IR femtosecond laser pulses coming at sub-MHz repetition rate. Comprehensive analysis of morphology and composition of laser-annealed films by atomic-force microscopy, optical, micro-Raman and energy-dispersive X-ray spectroscopy, as well as numerical modeling of optical spectra, confirmed efficient crystallization of α-Si and high-quality of the obtained films. Moreover, we highlight localized laser-driven crystallization of α-Si as a promising way for optical information encryption, anti-counterfeiting and fabrication of micro-optical elements.

Characterization of Rh/Si multilayer structure by HREM and HAADF

1992 ◽  
Vol 50 (1) ◽  
pp. 122-123
Author(s):  
Y. Cheng ◽  
J. Liu ◽  
M.B. Stearns ◽  
D.G. Steams
Keyword(s):  
Normal Incidence ◽  
High Resolution Electron Microscopy ◽  
X Rays ◽  
Beam Direction ◽  
Cross Sectional ◽  
Optical Elements ◽  
Resolution Electron ◽  
Point To Point ◽  
Better Than

The Rh/Si multilayer (ML) thin films are promising optical elements for soft x-rays since they have a calculated normal incidence reflectivity of ∼60% at a x-ray wavelength of ∼13 nm. However, a reflectivity of only 28% has been attained to date for ML fabricated by dc magnetron sputtering. In order to determine the cause of this degraded reflectivity the microstructure of this ML was examined on cross-sectional specimens with two high-resolution electron microscopy (HREM and HAADF) techniques.Cross-sectional specimens were made from an as-prepared ML sample and from the same ML annealed at 298 °C for 1 and 100 hours. The specimens were imaged using a JEM-4000EX TEM operating at 400 kV with a point-to-point resolution of better than 0.17 nm. The specimens were viewed along Si [110] projection of the substrate, with the (001) Si surface plane parallel to the beam direction.

scholarly journals High laser induced damage threshold photoresists for nano-imprint and 3D multi-photon lithography

Nanophotonics ◽  
2021 ◽  
Vol 0 (0) ◽  
Author(s):  
Elmina Kabouraki ◽  
Vasileia Melissinaki ◽  
Amit Yadav ◽  
Andrius Melninkaitis ◽  
Konstantina Tourlouki ◽  
...  
Keyword(s):  
Nanoimprint Lithography ◽  
Three Dimensional ◽  
Damage Threshold ◽  
Laser Pulses ◽  
Intense Laser ◽  
Optical Elements ◽  
Photonic Circuits ◽  
Future Production ◽  
Intense Laser Pulses ◽  
Laser Induced Damage

Abstract Optics manufacturing technology is predicted to play a major role in the future production of integrated photonic circuits. One of the major drawbacks in the realization of photonic circuits is the damage of optical materials by intense laser pulses. Here, we report on the preparation of a series of organic–inorganic hybrid photoresists that exhibit enhanced laser-induced damage threshold. These photoresists showed to be candidates for the fabrication of micro-optical elements (MOEs) using three-dimensional multiphoton lithography. Moreover, they demonstrate pattern ability by nanoimprint lithography, making them suitable for future mass production of MOEs.

scholarly journals Laser-induced thermal grating spectroscopy based on femtosecond laser multi-photon absorption

2021 ◽  
Vol 11 (1) ◽  
Author(s):  
Maria Ruchkina ◽  
Dina Hot ◽  
Pengji Ding ◽  
Ali Hosseinnia ◽  
Per-Erik Bengtsson ◽  
...  
Keyword(s):  
Continuous Wave ◽  
Laser Pulses ◽  
Photon Absorption ◽  
Gas Flows ◽  
Single Shot ◽  
Photon Excitation ◽  
Fs Laser ◽  
Thermal Grating ◽  
Grating Spectroscopy ◽  
First Time

AbstractLaser-induced grating spectroscopy (LIGS) is for the first time explored in a configuration based on the crossing of two focused femtosecond (fs) laser pulses (800-nm wavelength) and a focused continuous-wave (cw) laser beam (532-nm wavelength). A thermal grating was formed by multi-photon absorption of the fs-laser pulses by $$\hbox {N}_{{2}}$$ N 2 with a pulse energy around 700 $$\upmu $$ μ J ($$\sim $$ ∼ 45 TW/$$\hbox {cm}^{2}$$ cm 2 ). The feasibility of this LIGS configuration was investigated for thermometry in heated nitrogen gas flows. The temperature was varied from room temperature up to 750 K, producing strong single-shot LIGS signals. A model based on the solution of the linearized hydrodynamic equations was used to extract temperature information from single-shot experimental data, and the results show excellent agreement with the thermocouple measurements. Furthermore, the fluorescence produced by the fs-laser pulses was investigated. This study indicates an 8-photon absorption pathway for $$\hbox {N}_{{2}}$$ N 2 in order to reach the $$\hbox {B}^{3}\Pi _{g}$$ B 3 Π g state from the ground state, and 8 + 5 photon excitation to reach the $$\hbox {B}^{2}\Sigma _{u}^{+}$$ B 2 Σ u + state of the $$\hbox {N}_{2}^{+}$$ N 2 + ion. At pulse energies higher than 1 mJ, the LIGS signal was disturbed due to the generation of plasma. Additionally, measurements in argon gas and air were performed, where the LIGS signal for argon shows lower intensity compared to air and $$\hbox {N}_{{2}}$$ N 2 .

scholarly journals “Perfect” Terahertz Vortex Beams Formed Using Diffractive Axicons and Prospects for Excitation of Vortex Surface Plasmon Polaritons

2021 ◽  
Vol 11 (2) ◽  
pp. 717
Author(s):  
Boris Knyazev ◽  
Valery Cherkassky ◽  
Oleg Kameshkov
Keyword(s):  
Surface Plasmon ◽  
Surface Plasmon Polaritons ◽  
Bessel Beam ◽  
Diffraction Theory ◽  
Terahertz Range ◽  
High Resistivity ◽  
Visible Range ◽  
Optical Elements ◽  
Scalar Diffraction ◽  
Plasmon Polaritons

Transformation of a Bessel beam by a lens results in the formation of a “perfect” vortex beam (PVB) in the focal plane of the lens. The PVB has a single-ring cross-section and carries an orbital angular momentum (OAM) equal to the OAM of the “parent” beam. PVBs have numerous applications based on the assumption of their ideal ring-type structure. For instance, we proposed using terahertz PVBs to excite vortex surface plasmon polaritons propagating along cylindrical conductors and the creation of plasmon multiplex communication lines in the future (Comput. Opt. 2019, 43, 992). Recently, we demonstrated the formation of PVBs in the terahertz range using a Bessel beam produced using a spiral binary silicon axicon (Phys. Rev. A 2017, 96, 023846). It was shown that, in that case, the PVB was not annular, but was split into nested spiral segments, which was obviously a consequence of the method of Bessel beam generation. The search for methods of producing perfect beams with characteristics approaching theoretically possible ones is a topical task. Since for the terahertz range, there are no devices like spatial modulators of light in the visible range, the main method for controlling the mode composition of beams is the use of diffractive optical elements. In this work, we investigated the characteristics of perfect beams, the parent beams being quasi-Bessel beams created by three types of diffractive phase axicons made of high-resistivity silicon: binary, kinoform, and “holographic”. The amplitude-phase distributions of the field in real perfect beams were calculated numerically in the approximation of the scalar diffraction theory. An analytical expression was obtained for the case of the binary axicon. It was shown that a distribution closest to an ideal vortex was obtained using a holographic axicon. The resulting distributions were compared with experimental and theoretical distributions of the evanescent field of a plasmon near the gold–zinc sulfide–air surface at different thicknesses of the dielectric layer, and recommendations for experiments were given.

scholarly journals Dual-shot dynamics and ultimate frequency of all-optical magnetic recording on GdFeCo

2021 ◽  
Vol 10 (1) ◽  
Author(s):  
Sicong Wang ◽  
Chen Wei ◽  
Yuanhua Feng ◽  
Hongkun Cao ◽  
Wenzhe Li ◽  
...  
Keyword(s):  
Magnetization Reversal ◽  
Energy Efficient ◽  
High Speed ◽  
Data Transfer ◽  
Laser Pulses ◽  
Time Resolved ◽  
All Optical ◽  
Fs Laser ◽  
High Speed Data ◽  
Natural Way

AbstractAlthough photonics presents the fastest and most energy-efficient method of data transfer, magnetism still offers the cheapest and most natural way to store data. The ultrafast and energy-efficient optical control of magnetism is presently a missing technological link that prevents us from reaching the next evolution in information processing. The discovery of all-optical magnetization reversal in GdFeCo with the help of 100 fs laser pulses has further aroused intense interest in this compelling problem. Although the applicability of this approach to high-speed data processing depends vitally on the maximum repetition rate of the switching, the latter remains virtually unknown. Here we experimentally unveil the ultimate frequency of repetitive all-optical magnetization reversal through time-resolved studies of the dual-shot magnetization dynamics in Gd27Fe63.87Co9.13. Varying the intensities of the shots and the shot-to-shot separation, we reveal the conditions for ultrafast writing and the fastest possible restoration of magnetic bits. It is shown that although magnetic writing launched by the first shot is completed after 100 ps, a reliable rewriting of the bit by the second shot requires separating the shots by at least 300 ps. Using two shots partially overlapping in space and minimally separated by 300 ps, we demonstrate an approach for GHz magnetic writing that can be scaled down to sizes below the diffraction limit.

Sign in / Sign up

Export Citation Format

Share Document