scholarly journals Microphysical variability in southeast Pacific Stratocumulus clouds: synoptic conditions and radiative response

2010 ◽  
Vol 10 (13) ◽  
pp. 6255-6269 ◽  
Author(s):  
D. Painemal ◽  
P. Zuidema
Keyword(s):  
Boundary Layer ◽  
Cloud Droplet ◽  
Static Stability ◽  
Radiative Properties ◽  
Free Troposphere ◽  
Subtropical Anticyclone ◽  
Lower Cloud ◽  
Synoptic Conditions ◽  
Southeast Pacific ◽  
Stratocumulus Clouds

Abstract. Synoptic and satellite-derived cloud property variations for the southeast Pacific stratocumulus region associated with changes in coastal satellite-derived cloud droplet number concentrations (Nd) are explored. MAX and MIN Nd composites are defined by the top and bottom terciles of daily area-mean Nd values over the Arica Bight, the region with the largest mean oceanic Nd, for the five October months of 2001, 2005, 2006, 2007 and 2008. The ability of the satellite retrievals to capture composite differences is assessed with ship-based data. Nd and ship-based accumulation mode aerosol concentrations (Na) correlate well (r = 0.65), with a best-fit aerosol activation value dln Nddln Na of 0.56 for pixels with Nd>50 cm−3. The adiabatically-derived MODIS cloud depths also correlate well with the ship-based cloud depths (r=0.7), though are consistently higher (mean bias of almost 60 m). The MAX-Nd composite is characterized by a weaker subtropical anticyclone and weaker winds both at the surface and the lower free troposphere than the MIN-Nd composite. The MAX-Nd composite clouds over the Arica Bight are thinner than the MIN-Nd composite clouds, have lower cloud tops, lower near-coastal cloud albedos, and occur below warmer and drier free tropospheres (as deduced from radiosondes and NCEP Reanalysis). CloudSat radar reflectivities indicate little near-coastal precipitation. The co-occurrence of more boundary-layer aerosol/higher Nd within a more stable atmosphere suggests a boundary layer source for the aerosol, rather than the free troposphere. The MAX-Nd composite cloud thinning extends offshore to 80° W, with lower cloud top heights out to 95° W. At 85° W, the top-of-atmosphere shortwave fluxes are significantly higher (~50%) for the MAX-Nd composite, with thicker, lower clouds and higher cloud fractions than for the MIN-Nd composite. The change in Nd at this location is small (though positive), suggesting that the MAX-MIN Nd composite differences in radiative properties primarily reflects synoptic changes. Circulation anomalies and a one-point spatial correlation map reveal a weakening of the 850 hPa southerly winds decreases the free tropospheric cold temperature advection. The resulting increase in the static stability along 85° W is highly correlated to the increased cloud fraction, despite accompanying weaker free tropospheric subsidence.

scholarly journals Synoptically-induced variability in the microphysical properties of the South East Pacific stratocumulus deck

2009 ◽  
Vol 9 (6) ◽  
pp. 25523-25564 ◽  
Author(s):  
D. Painemal ◽  
P. Zuidema
Keyword(s):  
Boundary Layer ◽  
Cloud Droplet ◽  
Static Stability ◽  
Meridional Flow ◽  
Free Troposphere ◽  
Subtropical Anticyclone ◽  
Microphysical Properties ◽  
Cloud Properties ◽  
Highly Correlated ◽  
Cloud Tops

Abstract. Synoptic variations associated with changes in satellite-derived cloud droplet number concentrations (Nd) for the southeast Pacific stratocumulus deck were examined using a composite analysis applied to daily values from the five October months of 2001, 2005, 2006, 2007 and 2008. MAX and MIN Nd composites were defined by the top and bottom terciles of daily area-mean Nd values over the Arica Bight, the region with the largest mean oceanic Nd. Nd and ship-based accumulation mode aerosol concentrations (Na) correlate well (r=0.65), with a best-fit aerosol activation value dln Nddln Na of 0.53 for pixels with Nd>50 cm−3. The adiabatically-derived MODIS cloud depths also correlate well with the ship-based cloud depths (r=0.7), though are consistently higher (mean bias of almost 60 m). The MAX-Nd composite is characterized by a weaker subtropical anticyclone and weaker winds both at the surface and the lower free troposphere than the MIN-Nd composite. The MAX-Nd composite clouds over the Arica Bight are thinner than the MIN-Nd composite clouds, have lower cloud tops, and occur within warmer, drier free tropospheres (as deduced from radiosondes) that imply greater coastal subsidence. The cloud thinning compensates radiatively for increased reflectance from increases in Nd, most apparent near the coast. CloudSat radar reflectivities do not imply significant aerosol scavenging by precipitation near the coast, indicating that variability in wind transport contributes to the aerosol variability. The co-occurrence of more boundary-layer aerosol/higher Nd within a more stable atmosphere suggests a boundary layer source for the aerosol, rather than the free troposphere. Along 85° W, the top-of-atmosphere shortwave fluxes are significantly higher (~50%) for the MAX-Nd composite than for the MIN-Nd composite, with thicker clouds and higher cloud fractions. The change in Nd at this location is small (though positive), so that the composite difference primarily reflects synoptic changes. A one-point spatial correlation map reveals anomalous northerly winds at 850 hPa account for an anomalous warm temperature advection. The increase in the static stability along 85° W is highly correlated to the increased cloud fraction, despite accompanying weaker free tropospheric subsidence. This synoptic impact on offshore cloud properties is arguably our most radiatively important finding, and draws attention to the free tropospheric meridional flow as a meteorological control.

scholarly journals Southeast Pacific stratocumulus clouds, precipitation and boundary layer structure sampled along 20° S during VOCALS-REx

2010 ◽  
Vol 10 (21) ◽  
pp. 10639-10654 ◽  
Author(s):  
C. S. Bretherton ◽  
R. Wood ◽  
R. C. George ◽  
D. Leon ◽  
G. Allen ◽  
...  
Keyword(s):  
Boundary Layer ◽  
Liquid Water ◽  
Vertical Structure ◽  
Layer Structure ◽  
Cloud Droplet ◽  
Free Troposphere ◽  
Liquid Water Path ◽  
Typical Structure ◽  
Southeast Pacific ◽  
Over The Top

Abstract. Multiplatform airborne, ship-based, and land-based observations from 16 October–15 November 2008 during the VOCALS Regional Experiment (REx) are used to document the typical structure of the Southeast Pacific stratocumulus-topped boundary layer and lower free troposphere on a~transect along 20° S between the coast of Northern Chile and a buoy 1500 km offshore. Strong systematic gradients in clouds, precipitation and vertical structure are modulated by synoptically and diurnally-driven variability. The boundary layer is generally capped by a strong (10–12 K), sharp inversion. In the coastal zone, the boundary layer is typically 1 km deep, fairly well mixed, and topped by thin, nondrizzling stratocumulus with accumulation-mode aerosol and cloud droplet concentrations exceeding 200 cm−3. Far offshore, the boundary layer depth is typically deeper (1600 m) and more variable, and the vertical structure is usually decoupled. The offshore stratocumulus typically have strong mesoscale organization, much higher peak liquid water paths, extensive drizzle, and cloud droplet concentrations below 100 cm−3, sometimes with embedded pockets of open cells with lower droplet concentrations. The lack of drizzle near the coast is not just a microphysical response to high droplet concentrations; smaller cloud depth and liquid water path than further offshore appear comparably important. Moist boundary layer air is heated and mixed up along the Andean slopes, then advected out over the top of the boundary layer above adjacent coastal ocean regions. Well offshore, the lower free troposphere is typically much drier. This promotes strong cloud-top radiative cooling and stronger turbulence in the clouds offshore. In conjunction with a slightly cooler free troposphere, this may promote stronger entrainment that maintains the deeper boundary layer seen offshore. Winds from ECMWF and NCEP operational analyses have an rms difference of only 1 m s−1 from collocated airborne leg-mean observations in the boundary layer and 2 m s−1 above the boundary layer. This supports the use of trajectory analysis for interpreting REx observations. Two-day back-trajectories from the 20° S transect suggest that eastward of 75° W, boundary layer (and often free-tropospheric) air has usually been exposed to South American coastal aerosol sources, while at 85° W, neither boundary-layer or free-tropospheric air has typically had such contact.

scholarly journals Assessing regional scale predictions of aerosols, marine stratocumulus, and their interactions during VOCALS-REx using WRF-Chem

2011 ◽  
Vol 11 (23) ◽  
pp. 11951-11975 ◽  
Author(s):  
Q. Yang ◽  
J. D. Fast ◽  
H. Wang ◽  
R. C. Easter ◽  
H. Morrison ◽  
...  
Keyword(s):  
Boundary Layer ◽  
Optical Properties ◽  
Cloud Droplet ◽  
Energy Fluxes ◽  
Microphysics Scheme ◽  
Marine Stratocumulus ◽  
Aerosol Cloud ◽  
Southeast Pacific ◽  
Temperature And Humidity ◽  
Stratocumulus Clouds

Abstract. This study assesses the ability of the recent chemistry version (v3.3) of the Weather Research and Forecasting (WRF-Chem) model to simulate boundary layer structure, aerosols, stratocumulus clouds, and energy fluxes over the Southeast Pacific Ocean. Measurements from the VAMOS Ocean-Cloud-Atmosphere-Land Study Regional Experiment (VOCALS-REx) and satellite retrievals (i.e., products from the MODerate resolution Imaging Spectroradiometer (MODIS), Clouds and Earth's Radiant Energy System (CERES), and GOES-10) are used for this assessment. The Morrison double-moment microphysics scheme is newly coupled with interactive aerosols in the model. The 31-day (15 October–16 November 2008) WRF-Chem simulation with aerosol-cloud interactions (AERO hereafter) is also compared to a simulation (MET hereafter) with fixed cloud droplet number concentrations in the microphysics scheme and simplified cloud and aerosol treatments in the radiation scheme. The well-simulated aerosol quantities (aerosol number, mass composition and optical properties), and the inclusion of full aerosol-cloud couplings lead to significant improvements in many features of the simulated stratocumulus clouds: cloud optical properties and microphysical properties such as cloud top effective radius, cloud water path, and cloud optical thickness. In addition to accounting for the aerosol direct and semi-direct effects, these improvements feed back to the simulation of boundary-layer characteristics and energy budgets. Particularly, inclusion of interactive aerosols in AERO strengthens the temperature and humidity gradients within the capping inversion layer and lowers the marine boundary layer (MBL) depth by 130 m from that of the MET simulation. These differences are associated with weaker entrainment and stronger mean subsidence at the top of the MBL in AERO. Mean top-of-atmosphere outgoing shortwave fluxes, surface latent heat, and surface downwelling longwave fluxes are in better agreement with observations in AERO, compared to the MET simulation. Nevertheless, biases in some of the simulated meteorological quantities (e.g., MBL temperature and humidity) and aerosol quantities (e.g., underestimations of accumulation mode aerosol number) might affect simulated stratocumulus and energy fluxes over the Southeastern Pacific, and require further investigation. The well-simulated timing and outflow patterns of polluted and clean episodes demonstrate the model's ability to capture daily/synoptic scale variations of aerosol and cloud properties, and suggest that the model is suitable for studying atmospheric processes associated with pollution outflow over the ocean. The overall performance of the regional model in simulating mesoscale clouds and boundary layer properties is encouraging and suggests that reproducing gradients of aerosol and cloud droplet concentrations and coupling cloud-aerosol-radiation processes are important when simulating marine stratocumulus over the Southeast Pacific.

scholarly journals Southeast Pacific stratocumulus clouds, precipitation and boundary layer structure sampled along 20 S during VOCALS-REx

2010 ◽  
Vol 10 (6) ◽  
pp. 15921-15962 ◽  
Author(s):  
C. S. Bretherton ◽  
R. Wood ◽  
R. C. George ◽  
D. Leon ◽  
G. Allen ◽  
...  
Keyword(s):  
Boundary Layer ◽  
Liquid Water ◽  
Vertical Structure ◽  
Layer Structure ◽  
Cloud Droplet ◽  
Free Troposphere ◽  
Liquid Water Path ◽  
Typical Structure ◽  
Southeast Pacific ◽  
Over The Top

Abstract. Multiplatform airborne, ship-based, and land-based observations from 16 October–15 November 2008 during the VOCALS Regional Experiment (REx) are used to document the typical structure of the Southeast Pacific stratocumulus-topped boundary layer and lower free troposphere on a transect along 20° S between the coast of Northern Chile and a buoy 1500 km offshore. Strong systematic gradients in clouds, precipitation and vertical structure are modulated by synoptically and diurnally-driven variability. The boundary layer is generally capped by a strong (10–12 K), sharp inversion. In the coastal zone, the boundary layer is typically 1 km deep, fairly well mixed, and topped by thin, nondrizzling stratocumulus with haccumulation-mode aerosol and cloud droplet concentrations exceeding 200 cm−3. Far offshore, the boundary layer depth is typically deeper (1600 m) and more variable, and the vertical structure is usually decoupled. The offshore stratocumulus typically have strong mesoscale organization, much higher peak liquid water paths, extensive drizzle, and cloud droplet concentrations below 100 cm−3, sometimes with embedded pockets of open cells with lower droplet concentrations. The lack of drizzle near the coast is not just a microphysical response to high droplet concentrations; smaller cloud depth and liquid water path than further offshore appear comparably important. Moist boundary layer air is heated and mixed up along the Andean slopes, then advected out over the top of the boundary layer above adjacent coastal ocean regions. Well offshore, the lower free troposphere is typically much drier. This promotes strong cloud-top radiative cooling and stronger turbulence in the clouds offshore. In conjunction with a slightly cooler free troposphere, this may promote stronger entrainment that maintains the deeper boundary layer seen offshore. Winds from ECMWF and NCEP operational analyses have an rms difference of only 1 m s−1 from collocated airborne leg-mean observations in the boundary layer and 2 m s−1 above the boundary layer. This supports the use of trajectory analysis for interpreting REx observations. Two-day back-trajectories from the 20° S transect suggest that eastward of 75° W, boundary layer (and often free-tropospheric) air has usually been exposed to Chilean coastal aerosol sources, while at 85° W, neither boundary-layer or free-tropospheric air has typically had such contact.

Boundary Layer, Cloud, and Drizzle Variability in the Southeast Pacific Stratocumulus Regime

2008 ◽  
Vol 21 (23) ◽  
pp. 6191-6214 ◽  
Author(s):  
Efthymios Serpetzoglou ◽  
Bruce A. Albrecht ◽  
Pavlos Kollias ◽  
Christopher W. Fairall
Keyword(s):  
Boundary Layer ◽  
Layer Structure ◽  
Substantial Impact ◽  
Factors Affecting ◽  
Synoptic Conditions ◽  
Southeast Pacific ◽  
Boundary Layer Cloud ◽  
Similar Area ◽  
Earth’S Climate ◽  
Layer Cloud

Abstract The southeast Pacific stratocumulus regime is an important component of the earth’s climate system because of its substantial impact on albedo. Observational studies of this cloud regime have been limited, but during the past 5 yr, a series of cruises with research vessels equipped with in situ and remote sensing systems have provided unprecedented observations of boundary layer cloud and drizzle structures. These cruises started with the East Pacific Investigation of Climate (EPIC) 2001 field experiment, followed by cruises in a similar area in 2003 and 2004 [Pan-American Climate Studies (PACS) Stratus cruises]. The sampling from these three cruises provides a sufficient dataset to study the variability occurring over this region. This study compares observations from the 2004 cruise with those obtained during the previous two cruises. Observations from the ship provide information about boundary layer structure, fractional cloudiness, cloud depth, and drizzle characteristics. This study indicates more strongly decoupled boundary layers during the 2004 cruise than the well-mixed conditions that dominated the cloud and boundary layer structures during the EPIC cruise, and the highly variable conditions—sharp transitions from a solid stratus deck to broken-cloud and clear-sky periods—encountered during PACS Stratus 2003. Diurnal forcing and synoptic conditions are considered to be factors affecting these variations. A statistical evaluation of the macrophysical boundary layer, cloud, and drizzle properties is performed using the 5–6-day periods for which the research vessels remained stationed at the location of 20°S, 85°W during each cruise.

scholarly journals Wind speed response of marine non-precipitating stratocumulus clouds over a diurnal cycle in cloud-system resolving simulations

2016 ◽  
Vol 16 (9) ◽  
pp. 5811-5839 ◽  
Author(s):  
Jan Kazil ◽  
Graham Feingold ◽  
Takanobu Yamaguchi
Keyword(s):  
Boundary Layer ◽  
Wind Speed ◽  
Large Scale ◽  
Layer Growth ◽  
Radiative Properties ◽  
Cloud Base ◽  
Latent Heat Release ◽  
Marine Stratocumulus ◽  
Stratocumulus Clouds ◽  
Boundary Layer Growth

Abstract. Observed and projected trends in large-scale wind speed over the oceans prompt the question: how do marine stratocumulus clouds and their radiative properties respond to changes in large-scale wind speed? Wind speed drives the surface fluxes of sensible heat, moisture, and momentum and thereby acts on cloud liquid water path (LWP) and cloud radiative properties. We present an investigation of the dynamical response of non-precipitating, overcast marine stratocumulus clouds to different wind speeds over the course of a diurnal cycle, all else equal. In cloud-system resolving simulations, we find that higher wind speed leads to faster boundary layer growth and stronger entrainment. The dynamical driver is enhanced buoyant production of turbulence kinetic energy (TKE) from latent heat release in cloud updrafts. LWP is enhanced during the night and in the morning at higher wind speed, and more strongly suppressed later in the day. Wind speed hence accentuates the diurnal LWP cycle by expanding the morning–afternoon contrast. The higher LWP at higher wind speed does not, however, enhance cloud top cooling because in clouds with LWP ⪆ 50 g m−2, longwave emissions are insensitive to LWP. This leads to the general conclusion that in sufficiently thick stratocumulus clouds, additional boundary layer growth and entrainment due to a boundary layer moistening arises by stronger production of TKE from latent heat release in cloud updrafts, rather than from enhanced longwave cooling. We find that large-scale wind modulates boundary layer decoupling. At nighttime and at low wind speed during daytime, it enhances decoupling in part by faster boundary layer growth and stronger entrainment and in part because shear from large-scale wind in the sub-cloud layer hinders vertical moisture transport between the surface and cloud base. With increasing wind speed, however, in decoupled daytime conditions, shear-driven circulation due to large-scale wind takes over from buoyancy-driven circulation in transporting moisture from the surface to cloud base and thereby reduces decoupling and helps maintain LWP. The total (shortwave + longwave) cloud radiative effect (CRE) responds to changes in LWP and cloud fraction, and higher wind speed translates to a stronger diurnally averaged total CRE. However, the sensitivity of the diurnally averaged total CRE to wind speed decreases with increasing wind speed.

Regional modelling of aerosol interaction with deep convection and the effect on new particle formation over Amazonia

2020 ◽  
Author(s):  
Xuemei Wang ◽  
Daniel Grosvenor ◽  
Hamish Gordon ◽  
Meinrat O. Andreae ◽  
Ken Carslaw
Keyword(s):  
Boundary Layer ◽  
Cloud Condensation Nuclei ◽  
Deep Convection ◽  
Particle Formation ◽  
Nucleation Mechanism ◽  
Transport Processes ◽  
Radiative Properties ◽  
Free Troposphere ◽  
New Particle Formation ◽  
New Particles

<p>It has been estimated that over 50% of the present-day global low-level cloud condensation nuclei (CCN) are formed from new particle formation (NPF), and that this process has a substantial effect on the radiative properties of shallow clouds (Gordon et al. 2017). In contrast, we have a very limited understanding of how NPF affects deep convective clouds. Deep clouds could interact strongly with NPF because they extend into the high free troposphere where most new particles are formed, and they are responsible for most of the vertical transport of the nucleating vapours. Andreae et al. (2018) hypothesised from ACRIDICON-CHUVA campaign that organic gas molecules are transported by deep convection to the upper troposphere where they are oxidised and produce new particles, which are then be entrained into the boundary layer and grow to CCN-relevent sizes.</p><p>Here we study the interaction of deep convection and NPF using the United Kingdom Chemistry and Aerosols (UKCA) model coupled with the Cloud-AeroSol Interacting Microphyics (CASIM) embedded in the regional configuration of UK Met Office Hadley Centre Global Environment Model (HadGEM3). We simulate several days over a 1000 km region of the Amazon at 4 km resolution. We then compare the regional model, which resolves cloud up- and downdrafts, with the global model with parameterised convection and low resolution.</p><p>Our simulations highlight three findings. Firstly, solely using a binary H<sub>2</sub>SO<sub>4</sub>-H<sub>2</sub>O nucleation mechanism strongly underestimates total aerosol concentrations compared to observations by a factor of 1.5-8 below 3 km over the Amazon. This points to the potential role of an additional nucleation mechanism, most likely involving biogenic compounds that occurs throughout more of the free troposphere. Secondly, deep convection transports insoluble gases such as DMS and monoterpenes vertically but not SO<sub>2</sub> or H<sub>2</sub>SO<sub>4</sub>. The time scale for DMS oxidation (~ 1 day) is much longer than for monoterpene (1-2 hours), which points to the importance of simulating biogenic nucleation over the Amazon in a cloud-resolving model, while lower-resolution global models may adequately capture DMS effects on H<sub>2</sub>SO<sub>4</sub> nucleation. Finally, we also examine the Andreae et al (2018) hypothesis of aerosol supply to the boundary layer by quantifying cloud-free and cloudy up- and downdraft transport. The transport of newly formed aerosols into the boundary layer is 8 times greater in cloud-free regions than in the clouds, but these transport processes are of similar magnitude for large aerosols.</p>

scholarly journals Large-Scale Atmospheric Forcing by Southeast Pacific Boundary Layer Clouds: A Regional Model Study*

2005 ◽  
Vol 18 (7) ◽  
pp. 934-951 ◽  
Author(s):  
Yuqing Wang ◽  
Shang-Ping Xie ◽  
Bin Wang ◽  
Haiming Xu
Keyword(s):  
Boundary Layer ◽  
Large Scale ◽  
Inversion Layer ◽  
Regional Model ◽  
Cloud Layer ◽  
Eastern Pacific ◽  
Radiative Effect ◽  
Boundary Layer Clouds ◽  
Southeast Pacific ◽  
Stratocumulus Clouds

Abstract A regional model is used to study the radiative effect of boundary layer clouds over the southeast Pacific on large-scale atmosphere circulation during August–October 1999. With the standard settings, the model simulates reasonably well the large-scale circulation over the eastern Pacific, precipitation in the intertropical convergence zone (ITCZ) north of the equator, and marine boundary layer stratocumulus clouds to the south. In a sensitivity experiment with the radiative effect of liquid clouds south of the equator over the eastern Pacific artificially removed, boundary layer clouds south of the equator almost disappear and precipitation in the ITCZ is reduced by 15%–20%, indicating that the stratocumulus clouds over the southeast Pacific have both local and cross-equatorial effects. Examination of the differences between the control and sensitivity experiments indicates that clouds exert a net diabatic cooling in the inversion layer. In response to this cloud-induced cooling, an in situ anomalous high pressure system develops in the boundary layer and an anomalous shallow meridional circulation develops in the lower troposphere over the equatorial eastern Pacific. At the lower branch of this shallow circulation, anomalous boundary layer southerlies blow from the boundary layer high toward the northern ITCZ where the air ascends. An anomalous returning flow (northerly) just above the cloud layer closes the shallow circulation. This low-level anomalous shallow circulation enhances the subsidence over the southeast Pacific above the cloud layer, helping to maintain boundary layer clouds and temperature inversion there. Meanwhile, the strengthened cross-equatorial flow near the surface enhances moisture convergence and convection in the ITCZ north of the equator. This in turn strengthens the local, deep Hadley circulation and hence the large-scale subsidence and boundary layer clouds over the southeast Pacific. This positive feedback therefore enhances the interhemispheric climate asymmetry over the tropical eastern Pacific.

scholarly journals Aircraft observations of aerosol, cloud, precipitation, and boundary layer properties in pockets of open cells over the southeast Pacific

2014 ◽  
Vol 14 (15) ◽  
pp. 8071-8088 ◽  
Author(s):  
C. R. Terai ◽  
C. S. Bretherton ◽  
R. Wood ◽  
G. Painter
Keyword(s):  
Boundary Layer ◽  
Cloud Condensation Nuclei ◽  
Surface Wind ◽  
Cloud Droplet ◽  
Cloud Base ◽  
Cold Pool ◽  
Accumulation Mode ◽  
Aerosol Cloud ◽  
Wide Range ◽  
Southeast Pacific

Abstract. Five pockets of open cells (POCs) are studied using aircraft flights from the VOCALS Regional Experiment (VOCALS-REx), conducted in October and November 2008 over the southeast Pacific Ocean. Satellite imagery from the geostationary satellite GOES-10 is used to distinguish POC areas, and measurements from the aircraft flights are used to compare aerosol, cloud, precipitation, and boundary layer conditions inside and outside of POCs. Conditions observed across individual POC cases are also compared. POCs are observed in boundary layers with a wide range of inversion heights (1250 to 1600 m) and surface wind speeds (5 to 11 m s−1) and show no remarkable difference from the observed surface and free-tropospheric conditions during the two months of the field campaign. In all cases, compared to the surrounding overcast region the POC boundary layer is more decoupled, supporting both thin stratiform and deeper cumulus clouds. Although cloud-base precipitation rates are higher in the POC than the overcast region in each case, a threshold precipitation rate that differentiates POC precipitation from overcast precipitation does not exist. Mean cloud-base precipitation rates in POCs can range from 1.7 to 5.8 mm d−1 across different POC cases. The occurrence of heavy drizzle (> 0 dBZ) lower in the boundary layer better differentiates POC precipitation from overcast precipitation, likely leading to the more active cold pool formation in POCs. Cloud droplet number concentration is at least a factor of 8 smaller in the POC clouds, and the ratio of drizzle water to cloud water in POC clouds is over an order of magnitude larger than that in overcast clouds, indicating an enhancement of collision–coalescence processes in POC clouds. Despite large variations in the accumulation-mode aerosol concentrations observed in the surrounding overcast region (65 to 324 cm−3), the accumulation-mode aerosol concentrations observed in the subcloud layer of all five POCs exhibit a much narrower range (24 to 40 cm−3), and cloud droplet concentrations within the cumulus updrafts originating in this layer reflect this limited variability. Above the POC subcloud layer exists an ultraclean layer with accumulation-mode aerosol concentrations < 5 cm−3, demonstrating that in-cloud collision–coalescence processes efficiently remove aerosols. The existence of the ultraclean layer also suggests that the major source of accumulation-mode aerosols, and hence of cloud condensation nuclei in POCs, is the ocean surface, while entrainment of free-tropospheric aerosols is weak. The measurements also suggest that at approximately 30 cm−3 a balance of surface source and coalescence scavenging sinks of accumulation-mode aerosols maintain the narrow range of observed subcloud aerosol concentrations.

scholarly journals Impacts of aerosol particles on the microphysical and radiative properties of stratocumulus clouds over the southeast Pacific Ocean

2013 ◽  
Vol 13 (5) ◽  
pp. 2541-2562 ◽  
Author(s):  
C. H. Twohy ◽  
J. R. Anderson ◽  
D. W. Toohey ◽  
M. Andrejczuk ◽  
A. Adams ◽  
...  
Keyword(s):  
Pacific Ocean ◽  
Aerosol Particles ◽  
Radiative Properties ◽  
Anthropogenic Sources ◽  
Small Contribution ◽  
Cloud Albedo ◽  
Wide Range ◽  
Southeast Pacific ◽  
Stratocumulus Clouds ◽  
Near Shore

Abstract. The southeast Pacific Ocean is covered by the world's largest stratocumulus cloud layer, which has a strong impact on ocean temperatures and climate in the region. The effect of anthropogenic sources of aerosol particles on the stratocumulus deck was investigated during the VOCALS field experiment. Aerosol measurements below and above cloud were made with a ultra-high sensitivity aerosol spectrometer and analytical electron microscopy. In addition to more standard in-cloud measurements, droplets were collected and evaporated using a counterflow virtual impactor (CVI), and the non-volatile residual particles were analyzed. Many flights focused on the gradient in cloud properties on an E-W track along 20° S from near the Chilean coast to remote areas offshore. Mean statistics, including their significance, from eight flights and many individual legs were compiled. Consistent with a continental source of cloud condensation nuclei, below-cloud accumulation-mode aerosol and droplet number concentration generally decreased from near shore to offshore. Single particle analysis was used to reveal types and sources of the enhanced particle number that influence droplet concentration. While a variety of particle types were found throughout the region, the dominant particles near shore were partially neutralized sulfates. Modeling and chemical analysis indicated that the predominant source of these particles in the marine boundary layer along 20° S was anthropogenic pollution from central Chilean sources, with copper smelters a relatively small contribution. Cloud droplets were smaller in regions of enhanced particles near shore. However, physically thinner clouds, and not just higher droplet number concentrations from pollution, both contributed to the smaller droplets. Satellite measurements were used to show that cloud albedo was highest 500–1000 km offshore, and actually slightly lower closer to shore due to the generally thinner clouds and lower liquid water paths there. Thus, larger scale forcings that impact cloud macrophysical properties, as well as enhanced aerosol particles, are important in determining cloud droplet size and cloud albedo. Differences in the size distribution of droplet residual particles and ambient aerosol particles were observed. By progressively excluding small droplets from the CVI sample, we were able to show that the larger drops, some of which may initiate drizzle, contain the largest aerosol particles. Geometric mean diameters of droplet residual particles were larger than those of the below-cloud and above cloud distributions. However, a wide range of particle sizes can act as droplet nuclei in these stratocumulus clouds. A detailed LES microphysical model was used to show that this can occur without invoking differences in chemical composition of cloud-nucleating particles.

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