scholarly journals Long-term trends of black carbon and sulphate aerosol in the Arctic: changes in atmospheric transport and source region emissions

2010 ◽  
Vol 10 (19) ◽  
pp. 9351-9368 ◽  
Author(s):  
D. Hirdman ◽  
J. F. Burkhart ◽  
H. Sodemann ◽  
S. Eckhardt ◽  
A. Jefferson ◽  
...  
Keyword(s):  
Black Carbon ◽  
Atmospheric Circulation ◽  
Atmospheric Transport ◽  
Particle Dispersion ◽  
Downward Trend ◽  
The Arctic ◽  
Northern Eurasia ◽  
Source Regions ◽  
Long Term Trends

Abstract. As a part of the IPY project POLARCAT (Polar Study using Aircraft, Remote Sensing, Surface Measurements and Models, of Climate, Chemistry, Aerosols and Transport) and building on previous work (Hirdman et al., 2010), this paper studies the long-term trends of both atmospheric transport as well as equivalent black carbon (EBC) and sulphate for the three Arctic stations Alert, Barrow and Zeppelin. We find a general downward trend in the measured EBC concentrations at all three stations, with a decrease of −2.1±0.4 ng m−3 yr−1 (for the years 1989–2008) and −1.4±0.8 ng m−3 yr−1 (2002–2009) at Alert and Zeppelin respectively. The decrease at Barrow is, however, not statistically significant. The measured sulphate concentrations show a decreasing trend at Alert and Zeppelin of −15±3 ng m−3 yr−1 (1985–2006) and −1.3±1.2 ng m−3 yr−1 (1990–2008) respectively, while there is no trend detectable at Barrow. To reveal the contribution of different source regions on these trends, we used a cluster analysis of the output of the Lagrangian particle dispersion model FLEXPART run backward in time from the measurement stations. We have investigated to what extent variations in the atmospheric circulation, expressed as variations in the frequencies of the transport from four source regions with different emission rates, can explain the long-term trends in EBC and sulphate measured at these stations. We find that the long-term trend in the atmospheric circulation can only explain a minor fraction of the overall downward trend seen in the measurements of EBC (0.3–7.2%) and sulphate (0.3–5.3%) at the Arctic stations. The changes in emissions are dominant in explaining the trends. We find that the highest EBC and sulphate concentrations are associated with transport from Northern Eurasia and decreasing emissions in this region drive the downward trends. Northern Eurasia (cluster: NE, WNE and ENE) is the dominant emission source at all Arctic stations for both EBC and sulphate during most seasons. In wintertime, there are indications that the EBC emissions from the eastern parts of Northern Eurasia (ENE cluster) have increased over the last decade.

scholarly journals Long-term trends of black carbon and sulphate aerosol in the Arctic: changes in atmospheric transport and source region emissions

2010 ◽  
Vol 10 (5) ◽  
pp. 12133-12184 ◽  
Author(s):  
D. Hirdman ◽  
J. F. Burkhart ◽  
H. Sodemann ◽  
S. Eckhardt ◽  
A. Jefferson ◽  
...  
Keyword(s):  
Black Carbon ◽  
Atmospheric Circulation ◽  
Atmospheric Transport ◽  
Particle Dispersion ◽  
Downward Trend ◽  
The Arctic ◽  
Northern Eurasia ◽  
Source Regions ◽  
Long Term Trends

Abstract. As a part of the IPY project POLARCAT (Polar Study using Aircraft, Remote Sensing, Surface Measurements and Models, of Climate, Chemistry, Aerosols and Transport) and building on previous work (Hirdman et al., 2010), this paper studies the long-term trends of both atmospheric transport as well as equivalent black carbon (EBC) and sulphate for the three Arctic stations Alert, Barrow and Zeppelin. We find a general downward trend in the measured EBC concentrations at all three stations, with a decrease of −2.1±0.4 ng m−3 yr−1 (for the years 1989–2008) and −1.4±0.8 ng m−3 yr−1 (2002–2009) at Alert and Zeppelin respectively. The decrease at Barrow is, however, not statistically significant. The measured sulphate concentrations show a decreasing trend at Alert and Zeppelin of −15±3 ng m−3 yr−1 (1985–2006) and −1.3±1.2 ng m−3 yr−1 (1990–2008) respectively, while the trend at Barrow is unclear. To reveal the influence of different source regions on these trends, we used a cluster analysis of the output of the Lagrangian particle dispersion model FLEXPART run backward in time from the measurement stations. We have investigated to what extent variations in the atmospheric circulation, expressed as variations in the frequencies of the transport from four source regions with different emission rates, can explain the long-term trends in EBC and sulphate measured at these stations. We find that the long-term trend in the atmospheric circulation can only explain a minor fraction of the overall downward trend seen in the measurements of EBC (0.3–7.2%) and sulphate (0.3–5.3%) at the Arctic stations. The changes in emissions are dominant in explaining the trends. We find that the highest EBC and sulphate concentrations are associated with transport from Northern Eurasia and decreasing emissions in this region drive the downward trends. Northern Eurasia (cluster: NE, WNE and ENE) is the dominant emission source at all Arctic stations for both EBC and sulphate during most seasons. In wintertime, there are indications that the EBC emissions from the eastern parts of Northern Eurasia (ENE cluster) have increased over the last decade.

scholarly journals Pan-Arctic seasonal cycles and long-term trends of aerosol properties from ten observatories

2021 ◽  
Author(s):  
Julia Schmale ◽  
Sangeeta Sharma ◽  
Stefano Decesari ◽  
Jakob Pernov ◽  
Andreas Massling ◽  
...  
Keyword(s):  
Black Carbon ◽  
Methanesulfonic Acid ◽  
The Arctic ◽  
Anthropogenic Emissions ◽  
Natural Sources ◽  
Arctic Haze ◽  
Long Term Trends ◽  
Aerosol Properties ◽  
Natural Aerosol

Abstract. Even though the Arctic is remote, aerosol properties observed there are strongly influenced by anthropogenic emissions from outside the Arctic. This is particularly true for the so-called Arctic haze season (January through April). In summer (June through September), when atmospheric transport patterns change, and precipitation is more frequent, local Arctic, i.e. natural sources of aerosols and precursors, play an important role. Over the last decades, significant reductions in anthropogenic emissions have taken place. At the same time a large body of literature shows evidence that the Arctic is undergoing fundamental environmental changes due to climate forcing, leading to enhanced emissions by natural processes that may impact aerosol properties. In this study, we analyze nine aerosol chemical species and four particle optical properties from ten Arctic observatories (Alert, Gruvebadet, Kevo, Pallas, Summit, Thule, Tiksi, Barrow, Villum, Zeppelin) to understand changes in anthropogenic and natural aerosol contributions. Variables include equivalent black carbon, particulate sulfate, nitrate, ammonium, methanesulfonic acid, sodium, iron, calcium and potassium, as well as scattering and absorption coefficients, single scattering albedo and scattering Ångström exponent. First, annual cycles are investigated, which despite anthropogenic emission reductions still show the Arctic haze phenomenon. Second, long-term trends are studied using the Mann-Kendall Theil-Sen slope method. We find in total 28 significant trends over full station records, i.e. spanning more than a decade, compared to 17 significant decadal trends. The majority of significantly declining trends is from anthropogenic tracers and occurred during the haze period, driven by emission changes between 1990 and 2000. For the summer period, no uniform picture of trends has emerged. Twenty-one percent of trends, i.e. eleven out of 57, are significant, and of those five are positive and six are negative. Negative trends include not only anthropogenic tracers such as equivalent black carbon at Kevo, but also natural indicators such as methanesulfonic acid and non-sea salt calcium at Alert. Positive trends are observed for sulfate at Zeppelin and Gruvebadet. No clear evidence of a significant change in the natural aerosol contribution can be observed yet. However, testing the sensitivity of the Mann-Kendall Theil-Sen method, we find that monotonic changes of around 5 % per year in an aerosol property are needed to detect a significant trend within one decade. This highlights that long-term efforts well beyond a decade are needed to capture smaller changes. It is particularly important to understand the ongoing natural changes in the Arctic, where interannual variability can be high, such as with forest fire emissions and their influence on the aerosol population. To investigate the climate-change induced influence on the aerosol population and the resulting climate feedback, long-term observations of tracers more specific to natural sources are needed, as well as of particle microphysical properties such as size distributions, which can be used to identify changes in particle populations which are not well captured by mass-oriented methods such as bulk chemical composition.

scholarly journals A trajectory analysis of atmospheric transport of black carbon aerosols to Canadian High Arctic in winter and spring (1990–2005)

2010 ◽  
Vol 10 (2) ◽  
pp. 2221-2244 ◽  
Author(s):  
L. Huang ◽  
S. L. Gong ◽  
S. Sharma ◽  
D. Lavoué ◽  
C. Q. Jia
Keyword(s):  
Regression Model ◽  
Black Carbon ◽  
North American ◽  
Emission Intensity ◽  
Atmospheric Transport ◽  
High Arctic ◽  
The Arctic ◽  
Canadian High Arctic ◽  
Near Surface ◽  
Annual Variations

Abstract. Black carbon (BC) particles accumulated in the Arctic troposphere and deposited over snow have significant effects on radiative forcing of the Arctic regional climate. Applying cluster analysis technique on 10-day backward trajectories, transport pathways affecting Alert (82.5° N, 62.5° W), Nunavut in Canada are identified in this work, along with the associated transport frequency. Based on the atmospheric transport frequency and the estimated BC emission intensity from surrounding regions, a linear regression model is constructed to investigate the inter-annual variations of BC observed at Alert in January and April, representative of winter and spring respectively, between 1990 and 2005. Strong correlations are found between BC concentrations predicted with the regression model and measured at Alert for both seasons (R2 equals 0.77 and 0.81 for winter and spring, respectively). Results imply that atmospheric transport and BC emission are the major contributors to the inter-annual variations in BC concentrations observed at Alert in the cold seasons for the 16-year period. Based on the regression model the relative contributions of regional BC emissions affecting Alert are attributed to the Eurasian sector, composed of the European Union and the former USSR, and the North American sector. Considering both seasons, the model suggests that Eurasia is the major contributor to the near-surface BC levels at the Canadian High Arctic site with an average contribution of over 85% during the 16-year period. In winter, the atmospheric transport of BC aerosols from Eurasia is found to be even more predominant with a multi-year average of 94%. The model estimates smaller contribution from the Eurasian sector in spring (70%) than that in winter. It is also found that the change in Eurasian contributions depends mainly on the reduction of emission intensity, while the changes in both emission and atmospheric transport contributed to the inter-annual variation of North American contributions.

scholarly journals Increase in Aerosol Black Carbon in the 2000s over Ny-Ålesund in the Summer

2015 ◽  
Vol 73 (1) ◽  
pp. 251-262 ◽  
Author(s):  
Liqi Chen ◽  
Wei Li ◽  
Jianqiong Zhan ◽  
Jianjun Wang ◽  
Yuanhui Zhang ◽  
...  
Keyword(s):  
Temporal Variation ◽  
Black Carbon ◽  
Atmospheric Circulation ◽  
Yellow River ◽  
The Arctic ◽  
Radiative Energy ◽  
Back Trajectory ◽  
Significant Implication ◽  
Svalbard Archipelago ◽  
Local Emissions

Abstract To investigate the concentrations, sources, and temporal variations of atmospheric black carbon (BC) in the summer Arctic, routine ground-level observations of BC by optical absorption were made in the summer from 2005 to 2008 at the Chinese Arctic “Yellow River” Station (78°55′N, 11°56′E) at Ny-Ålesund on the island of Spitsbergen in the Svalbard Archipelago. Methods of the ensemble empirical-mode decomposition analysis and back-trajectory analysis were employed to assess temporal variation embedded in the BC datasets and airmass transport patterns. The 10th-percentile and median values of BC concentrations were 7.2 and 14.6 ng m−3, respectively, and hourly average BC concentrations ranged from 2.5 to 54.6 ng m−3. A gradual increase was found by 4 ng m−3 a−1. This increase was not seen in the Zeppelin Station and it seemed to contrast with the prevalent conception of generally decreasing BC concentration since 1989 in the Arctic. Factors responsible for this increase such as changes in emissions and atmospheric transport were taken into consideration. The result indicated that BC from local emissions was mostly responsible for the observed increase from 2005 to 2008. BC temporal variation in the summer was controlled by the atmospheric circulation, which presented a significant 6–14-day variation and coherent with 1–3- and 2–5-day and longer cycle variation. Although the atmospheric circulation changes from 2005 to 2008, there was not a marked trend in long-range transportation of BC. This study suggested that local emissions might have significant implication for the regional radiative energy balance at Ny-Ålesund.

scholarly journals Atmospheric transport of persistent semi-volatile organic chemicals to the Arctic and cold condensation in the mid-troposphere – Part 2: 3-D modeling of episodic atmospheric transport

2010 ◽  
Vol 10 (15) ◽  
pp. 7315-7324 ◽  
Author(s):  
L. Zhang ◽  
J. Ma ◽  
C. Tian ◽  
Y. Li ◽  
H. Hung
Keyword(s):  
Atmospheric Circulation ◽  
Atmospheric Transport ◽  
The Arctic ◽  
Organic Chemicals ◽  
High Latitudes ◽  
Volatile Organic ◽  
Volatile Organic Chemicals ◽  
Cold Condensation ◽  
Condensation Effect ◽  
Modeling Study

Abstract. Two 3-dimensional global atmospheric transport models for persistent organic pollutants (POPs) have been employed to investigate the association between the large-scale atmospheric motions and poleward transports of persistent semi-volatile organic chemicals (SVOCs). We examine the modeled daily air concentration of α- and γ-hexachlorocyclohexane (HCH) over a period from 1997 through 1999 during which a number of episodic atmospheric transport events were detected in this modeling study. These events provide modeling evidence for improving the interpretation on the cold condensation effect and poleward atmospheric transport of SVOCs in the mid-troposphere. Two episodic transport events of γ-HCH (lindane) to the high Arctic (80–90° N), one from Asian and another from Eurasian sources, are reported in this paper. Both events suggest that the episodic atmospheric transports occurring in the mid-troposphere (e.g. from 3000 m to 5500 m height) are driven by atmospheric horizontal and vertical motions. The association of the transport events with atmospheric circulation is briefly discussed. Strong southerly winds, forced by the evolution of two semi-permanent high pressure systems over mid-high latitudes in the Northern Hemisphere, play an important role in the long-range transport (LRT) of HCHs to the high latitudes from its sources. Being consistent with the cold condensation effect and poleward atmospheric transport in a mean meridional atmospheric circulation simulated by a 2-D atmospheric transport model, as reported by the first part of this study, this modeling study indicates that cold condensation is likely occurring more intensively in the mid-troposphere where rapid declining air temperature results in condensed phase of the chemical over and near its source regions and where stronger winds convey the chemical more rapidly to the polar region during the episodic poleward atmospheric transport events.

Comparison of the Long-Term Trends of the Largest Waves in the Ice-Free Arctic Waters From Different Reanalysis Products

2018 ◽  
Author(s):  
Takuji Waseda ◽  
Takehiko Nose ◽  
Adrean Webb
Keyword(s):  
Arctic Ocean ◽  
The Arctic ◽  
Extreme Value Analysis ◽  
Positive Trend ◽  
Value Analysis ◽  
The Arctic Ocean ◽  
Ship Route ◽  
Long Term Trends ◽  
Horizontal Grid

The long-term trends of the expected largest waves in the ice-free Arctic waters from Laptev to Beaufort Seas was studied analyzing the ERA-interim reanalysis from 1979 to 2016. The analysis showed that the positive trend is largest in October and increased almost 70 cm in 38 years. For ships navigating the Northern Ship Route, it is important to know what the possible largest waves to expect during its cruise. In view of conducting the extreme value analysis, the uncertainty of the largest wave needs to be validated. However, the observation in the Arctic Ocean is limited. We, therefore, rely on the reanalysis wave products in the Arctic Ocean, whose uncertainty is yet to be determined. ERA-Interim and ERA-5 are compared in the Laptev, the East Siberian, Chukchi and Beaufort Seas. The comparison is relevant as the two products differ in its horizontal grid resolution and availability of the satellite altimeter significant wave height data assimilation. During 2010–2016 when the ERA5 is available, only a small difference from ERA-Interim was detected in the mean. However, the expected largest waves in the domain tended to be large for the ERA-5, 8% normalized bias. The tendency was quite similar with a high correlation of 0.98.

scholarly journals Wave Climate from Spectra and Its Connections with Local and Remote Wind Climate

2019 ◽  
Vol 49 (2) ◽  
pp. 543-559 ◽  
Author(s):  
Haoyu Jiang ◽  
Lin Mu
Keyword(s):  
Wind Field ◽  
Wave Climate ◽  
The Arctic ◽  
Target Point ◽  
Wave Spectra ◽  
Basin Scale ◽  
Long Term Trends ◽  
Wind Climate ◽  
Climate Systems

AbstractWind-generated waves can propagate over large distances. Therefore, wave spectra from a fixed point can record information about air–sea interactions in distant areas. In this study, the spectral wave climate for a point in the tropical eastern Pacific Ocean is computed. Several well-defined wave climate systems are observed in the mean wave spectrum. Significant seasonal cycling, long-term trends, and correlations with the Southern Oscillation, the Arctic Oscillation, and the Antarctic Oscillation are observed in the local wave spectra, showing abundant climatic information. Projections of wind vectors on the directions pointing to the target location are used to connect the spectral wave climate and basin-scale wind climate, because significant correlations are observed between the wave spectra and the wind projections of both local and remote wind systems. The origins of all the identified wave climate systems, including the westerlies and the trade winds in both hemispheres, are clearly shown in wind projection maps. Some of these origins are thousands of kilometers away from the target point, demonstrating the validity of this connection. Comparisons are made between wave spectra and the corresponding local and remote wind fields with respect to seasonal and interannual variability and long-term trends. The results show that each frequency and direction of ocean wave spectra at a certain location can be approximately linked to the wind field for a geographical area, implying that it is feasible to reconstruct spectral wave climates from observational wind field data and monitor wind climates from observational wave spectra geographically far away.

scholarly journals Atmospheric mercury observations from Antarctica: seasonal variation and source and sink region calculations

2012 ◽  
Vol 12 (7) ◽  
pp. 3241-3251 ◽  
Author(s):  
K. A. Pfaffhuber ◽  
T. Berg ◽  
D. Hirdman ◽  
A. Stohl
Keyword(s):  
Southern Hemisphere ◽  
Dispersion Model ◽  
Particle Dispersion ◽  
Atmospheric Mercury ◽  
The Arctic ◽  
Research Station ◽  
The Mean ◽  
The Antarctic ◽  
Source And Sink

Abstract. Long term atmospheric mercury measurements in the Southern Hemisphere are scarce and in Antarctica completely absent. Recent studies have shown that the Antarctic continent plays an important role in the global mercury cycle. Therefore, long term measurements of gaseous elemental mercury (GEM) were initiated at the Norwegian Antarctic Research Station, Troll (TRS) in order to improve our understanding of atmospheric transport, transformation and removal processes of GEM. GEM measurements started in February 2007 and are still ongoing, and this paper presents results from the first four years. The mean annual GEM concentration of 0.93 ± 0.19 ng m−3 is in good agreement with other recent southern-hemispheric measurements. Measurements of GEM were combined with the output of the Lagrangian particle dispersion model FLEXPART, for a statistical analysis of GEM source and sink regions. It was found that the ocean is a source of GEM to TRS year round, especially in summer and fall. On time scales of up to 20 days, there is little direct transport of GEM to TRS from Southern Hemisphere continents, but sources there are important for determining the overall GEM load in the Southern Hemisphere and for the mean GEM concentration at TRS. Further, the sea ice and marginal ice zones are GEM sinks in spring as also seen in the Arctic, but the Antarctic oceanic sink seems weaker. Contrary to the Arctic, a strong summer time GEM sink was found, when air originates from the Antarctic plateau, which shows that the summertime removal mechanism of GEM is completely different and is caused by other chemical processes than the springtime atmospheric mercury depletion events. The results were corroborated by an analysis of ozone source and sink regions.

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