scholarly journals Sources of anions in aerosols in northeast Greenland during late winter

2013 ◽  
Vol 13 (3) ◽  
pp. 1569-1578 ◽  
Author(s):  
M. Fenger ◽  
L. L. Sørensen ◽  
K. Kristensen ◽  
B. Jensen ◽  
Q. T. Nguyen ◽  
...  
Keyword(s):  
Sea Ice ◽  
Long Range ◽  
Atmospheric Aerosols ◽  
Fine Particles ◽  
Chemical Properties ◽  
High Arctic ◽  
Early Spring ◽  
Water Soluble ◽  
The Arctic ◽  
Late Winter

Abstract. The knowledge of climate effects of atmospheric aerosols is associated with large uncertainty, and a better understanding of their physical and chemical properties is needed, especially in the Arctic environment. The objective of the present study is to improve our understanding of the processes affecting the composition of aerosols in the high Arctic. Therefore size-segregated aerosols were sampled at a high Arctic site, Station Nord (Northeast Greenland), in March 2009 using a Micro Orifice Uniform Deposit Impactor. The aerosol samples were extracted in order to analyse three water-soluble anions: chloride, nitrate and sulphate. The results are discussed based on possible chemical and physical transformations as well as transport patterns. The total concentrations of the ions at Station Nord were 53–507 ng m−3, 2–298 ng m−3 and 535–1087 ng m−3 for chloride (Cl−), nitrate (NO3−) and sulphate (SO42−), respectively. The aerosols in late winter/early spring, after polar sunrise, are found to be a mixture of long-range transported and regional to local originating aerosols. Fine particles, smaller than 1 μm, containing SO42−, Cl− and NO3−, are hypothesized to originate from long-range transport, where SO42− is by far the dominating anion accounting for 50–85% of the analyzed mass. The analysis suggests that Cl− and NO3− in coarser particles (> 1.5 μm) originate from local/regional sources. Under conditions where the air mass is transported over sea ice at high wind speeds, very coarse particles (> 18 μm) are observed, and it is hypothesized that frost flowers on the sea ice are a source of the very coarse nitrate particles.

scholarly journals Sources of anions in aerosols in northeast Greenland during late winter

2012 ◽  
Vol 12 (6) ◽  
pp. 14813-14836 ◽  
Author(s):  
M. Fenger ◽  
L. L. Sørensen ◽  
K. Kristensen ◽  
B. Jensen ◽  
Q. T. Nquyen ◽  
...  
Keyword(s):  
Sea Ice ◽  
Long Range ◽  
Atmospheric Aerosols ◽  
Fine Particles ◽  
Chemical Properties ◽  
High Arctic ◽  
Early Spring ◽  
Water Soluble ◽  
The Arctic ◽  
Late Winter

Abstract. The knowledge of climate effects of atmospheric aerosols is associated with large uncertainty, and a better understanding of their physical and chemical properties is needed, especially in the Arctic environment. The objective of the present study is to improve our understanding of the processes affecting the composition of the aerosols in the high Arctic. Therefore size-segregated aerosols were sampled at a high Arctic site, Station Nord (Northeast Greenland), in March 2009 using a Micro Orifice Uniform Deposit Impactor. The aerosol samples were extracted in order to analyze the three water-soluble anions: chloride, nitrate and sulphate. The results are discussed based on possible chemical and physical transformations as well as transport patterns. The total concentrations of the ions at Station Nord were 53–507 ng m−3, 2–298 ng m−3 and 535–1087 ng m−3 for chloride (Cl−), nitrate (NO3-) and sulphate (SO42−), respectively. The aerosols in late winter/early spring, after polar sunrise, are found to be a mixture of long-range transported and regional to local originating aerosols. Fine particles, smaller than 1 μm, containing SO42−, Cl− and NO3−, are hypothesized to originate from long-range transport, where SO42− is by far the dominating anion accounting for 50–85% of the analyzed mass. The analysis suggests that Cl− and NO3− in coarser particles (>1.5 μm) originate from local/regional sources. Under conditions where the air mass is transported over sea-ice at high wind speeds, very coarse particles (>18 μm) are observed and it is hypothesized that frost flowers on the sea ice is a source of very coarse chloride particles in the Arctic.

scholarly journals Chemical Fractionation of Trace Elements in Arctic PM10 Samples

Atmosphere ◽  
2021 ◽  
Vol 12 (9) ◽  
pp. 1152
Author(s):  
Eleonora Conca ◽  
Mery Malandrino ◽  
Agnese Giacomino ◽  
Paolo Inaudi ◽  
Annapaola Giordano ◽  
...  
Keyword(s):  
Sequential Extraction ◽  
Long Range ◽  
Extraction Procedure ◽  
Early Spring ◽  
Transport Processes ◽  
Sequential Extraction Procedure ◽  
The Arctic ◽  
Long Range Transport ◽  
Late Winter ◽  
Range Transport

In this study, the information potential of a two-step sequential extraction procedure was evaluated. For this purpose, first of all the elemental composition of Arctic PM10 samples collected in Ny-Ålesund (Svalbard Islands) from 28 February 2015 to 21 October 2015 was investigated. Enrichment Factors, Principal Component Analysis and Hierarchical Cluster Analysis were performed to identify PM10 sources and to understand the effects of short- and long-range transport processes. The investigation of the potential source areas was also aided by taking into account back-trajectories. Then, the sequential extraction procedure was applied to some of the samples in order to obtain more information on these sources. This approach allowed us to establish that most of the elements prevalently having an anthropogenic origin not only were present in higher concentrations, but they were also more easily extractable in late winter and early spring. This confirms the common statement that the anthropogenic portion of the elements present in a sample is generally loosely bound to the particulate matter structure, and so it is more easily extractable and releasable on the Arctic snowpack. Moreover, in the samples collected in late winter and early spring, even the elements prevalently having a crustal origin were more easily extractable, probably due to the particle size selection occurred during the long-range transport.

scholarly journals Observations and Simulations of Meteorological Conditions over Arctic Thick Sea Ice in Late Winter during the Transarktika 2019 Expedition

Atmosphere ◽  
2021 ◽  
Vol 12 (2) ◽  
pp. 174
Author(s):  
Günther Heinemann ◽  
Sascha Willmes ◽  
Lukas Schefczyk ◽  
Alexander Makshtas ◽  
Vasilii Kustov ◽  
...  
Keyword(s):  
Sea Ice ◽  
Climate Models ◽  
Climate Model ◽  
Regional Climate ◽  
Open Water ◽  
The Arctic ◽  
Late Winter ◽  
Good Representation ◽  
Hourly Temperature ◽  
Ice Model

The parameterization of ocean/sea-ice/atmosphere interaction processes is a challenge for regional climate models (RCMs) of the Arctic, particularly for wintertime conditions, when small fractions of thin ice or open water cause strong modifications of the boundary layer. Thus, the treatment of sea ice and sub-grid flux parameterizations in RCMs is of crucial importance. However, verification data sets over sea ice for wintertime conditions are rare. In the present paper, data of the ship-based experiment Transarktika 2019 during the end of the Arctic winter for thick one-year ice conditions are presented. The data are used for the verification of the regional climate model COSMO-CLM (CCLM). In addition, Moderate Resolution Imaging Spectroradiometer (MODIS) data are used for the comparison of ice surface temperature (IST) simulations of the CCLM sea ice model. CCLM is used in a forecast mode (nested in ERA5) for the Norwegian and Barents Seas with 5 km resolution and is run with different configurations of the sea ice model and sub-grid flux parameterizations. The use of a new set of parameterizations yields improved results for the comparisons with in-situ data. Comparisons with MODIS IST allow for a verification over large areas and show also a good performance of CCLM. The comparison with twice-daily radiosonde ascents during Transarktika 2019, hourly microwave water vapor measurements of first 5 km in the atmosphere and hourly temperature profiler data show a very good representation of the temperature, humidity and wind structure of the whole troposphere for CCLM.

scholarly journals Analysis of Arctic Spring Ozone Anomaly in the Phases of QBO and 11-year Solar Cycle for 1979–2011

2021 ◽  
Author(s):  
Yousuke Yamashita ◽  
Hideharu Akiyoshi ◽  
Masaaki Takahashi
Keyword(s):  
Solar Cycle ◽  
Climate Model ◽  
Polar Vortex ◽  
Reanalysis Data ◽  
Early Spring ◽  
The Arctic ◽  
Negative Anomaly ◽  
Late Winter ◽  
Quasi Biennial Oscillation ◽  
Biennial Oscillation

Arctic ozone amount in winter to spring shows large year-to-year variation. This study investigates Arctic spring ozone in relation to the phase of quasi-biennial oscillation (QBO)/the 11-year solar cycle, using satellite observations, reanalysis data, and outputs of a chemistry climate model (CCM) during the period of 1979–2011. For this duration, we found that the composite mean of the Northern Hemisphere high-latitude total ozone in the QBO-westerly (QBO-W)/solar minimum (Smin) phase is slightly smaller than those averaged for the QBO-W/Smax and QBO-E/Smax years in March. An analysis of a passive ozone tracer in the CCM simulation indicates that this negative anomaly is primarily caused by transport. The negative anomaly is consistent with a weakening of the residual mean downward motion in the polar lower stratosphere. The contribution of chemical processes estimated using the column amount difference between ozone and the passive ozone tracer is between 10–20% of the total anomaly in March. The lower ozone levels in the Arctic spring during the QBO-W/Smin years are associated with a stronger Arctic polar vortex from late winter to early spring, which is linked to the reduced occurrence of sudden stratospheric warming in the winter during the QBO-W/Smin years.

Dirty sea ice drives higher Mn concentrations in the Canada Basin

2021 ◽  
Author(s):  
Birgit Rogalla ◽  
Susan E. Allen ◽  
Manuel Colombo ◽  
Paul G. Myers ◽  
Kristin J. Orians
Keyword(s):  
Sea Ice ◽  
Long Range ◽  
Sediment Resuspension ◽  
Three Dimensional ◽  
Arctic Sea Ice ◽  
Canada Basin ◽  
The Arctic ◽  
Long Range Transport ◽  
Basin Surface ◽  
Range Transport

<p>The rapidly changing conditions of the Arctic sea ice system have cascading impacts on the biogeochemical cycles of the ocean. Sea ice transports sediments, nutrients, trace metals, pollutants, and gases from the extensive continental shelves into the more isolated central basins. However, it is difficult to assess the net contribution of this supply mechanism on nutrients in the surface ocean. In this study, we used Manganese (Mn), a micronutrient and tracer which can integrate source fluctuations in space and time, to understand the net impact of the long range transport of sea ice for Mn.</p><p>We developed a three-dimensional dissolved Mn model within a subdomain of the 1/12 degree Arctic and Northern Hemispheric Atlantic (ANHA12) configuration of NEMO centred on the Canadian Arctic Archipelago, and evaluated this model with in situ observations from the 2015 Canadian GEOTRACES cruises. The Mn model incorporates parameterizations for the contributions from river discharge, sediment resuspension, atmospheric deposition of aerosols directly to the ocean and via melt from sea ice, release of sediment from sea ice, and reversible scavenging, while the NEMO-TOP engine takes care of the advection and diffusion of the tracers. </p><p>Simulations with this model from 2002 to 2019 indicate that the majority of external Mn contributed annually to the Canada Basin surface is released by sediment from sea ice, much of which originates from the Siberian shelves. Reduced sea ice longevity in the Siberian shelf regions has been postulated to result in the disruption of the long range transport of sea ice by the transpolar drift. This reduced sea ice supply has the potential to decrease the Canada Basin Mn surface maximum and downstream Mn supply, with implications for other nutrients (such as Fe) contained in ice-rafted sediments as well. These results demonstrate some of the many changes to the biogeochemical supply mechanisms expected in the near-future in the Arctic Ocean and the subpolar seas.</p>

Lagrangian analysis of the northern polar vortex split in April 2020 during development of the Arctic ozone hole

2021 ◽  
Author(s):  
Jezabel Curbelo ◽  
Gang Chen ◽  
Carlos R. Mechoso
Keyword(s):  
Wave Train ◽  
Stratospheric Ozone ◽  
Polar Vortex ◽  
Early Spring ◽  
Ozone Hole ◽  
The Arctic ◽  
Late Winter ◽  
Lagrangian Analysis ◽  
The North ◽  
Vortex Split

<div>The evolution of the Northern Hemisphere stratosphere during late winter and early spring of 2020 was punctuated by outstanding events both in dynamics and tracer evolution. It provides an ideal case for study of the Lagrangian properties of the evolving flow and its connections with the troposphere. The events ranged from an episode of polar warming at upper levels in March, a polar vortex split into two cyclonic vortices at middle and lower levels in April, and a remarkably deep and persistent mass of ozone poor air within the westerly circulation throughout the period. The latter feature was particularly remarkable during 2020, which showed the lowest values of stratospheric ozone on record.</div><div> </div><div>We focus on the vortex split in April 2020 and we examine this split at middle as well as lower stratospheric levels, and the interactions that occurred between the resulting two vortices which determined the distribution of ozone among them. We also examine the connections among stratospheric and tropospheric events during the period.</div><div> </div><div>Our approach for analysis will be based on the application of Lagrangian tools to the flow field, based on following air parcels trajectories, examining barriers to the flow, and the activity and propagation of planetary waves. Our findings confirm the key role for the split played by a flow configuration with a polar hyperbolic trajectory and associated manifolds. A trajectory analysis illustrates the transport of ozone between the vortices during the split. We argue that these stratospheric events were linked to strong synoptic scale disturbances in the troposphere forming a wave train from the north Pacific to North America and Eurasia.</div><div><strong> </strong></div><div><strong>Reference:</strong><strong> </strong>J. Curbelo, G. Chen,  C. R. Mechoso. Multi-level analysis of the northern polar vortex split in April 2020 during development of the Arctic ozone hole. Earth and Space Science Open Archive. doi: 10.1002/essoar.10505516.1</div><div> </div><div><strong>Acknowledgements:</strong> NSF Grant AGS-1832842, RYC2018-025169 and EIN2019-103087.</div>

The role of sea ice for plastic pollution in the Arctic

2021 ◽  
Author(s):  
Ilka Peeken ◽  
Elisa Bergami ◽  
Ilaria Corsi ◽  
Benedikt Hufnagl ◽  
Christian Katlein ◽  
...  
Keyword(s):  
Sea Ice ◽  
Arctic Ocean ◽  
Long Range ◽  
Environmental Concern ◽  
Ice Cores ◽  
Atlantic Water ◽  
The Arctic ◽  
Polar Regions ◽  
Plastic Pollution ◽  
The Arctic Ocean

<p>Marine plastic pollution is a growing worldwide environmental concern as recent reports indicate that increasing quantities of litter disperse into secluded environments, including Polar Regions. Plastic degrades into smaller fragments under the influence of sunlight, temperature changes, mechanic abrasion and wave action resulting in small particles < 5mm called microplastics (MP). Sea ice cores, collected in the Arctic Ocean have so far revealed extremely high concentrations of very small microplastic particles, which might be transferred in the ecosystem with so far unknown consequences for the ice dependant marine food chain.  Sea ice has long been recognised as a transport vehicle for any contaminates entering the Arctic Ocean from various long range and local sources. The Fram Strait is hereby both, a major inflow gateway of warm Atlantic water, with any anthropogenic imprints and the major outflow region of sea ice originating from the Siberian shelves and carried via the Transpolar Drift. The studied sea ice revealed a unique footprint of microplastic pollution, which were related to different water masses and indicating different source regions. Climate change in the Arctic include loss of sea ice, therefore, large fractions of the embedded plastic particles might be released and have an impact on living systems. By combining modeling of sea ice origin and growth, MP particle trajectories in the water column as well as MPs long-range transport via particle tracking and transport models we get first insights  about the sources and pathways of MP in the Arctic Ocean and beyond and how this might affect the Arctic ecosystem.</p>

scholarly journals Concentrations of Cadmium, Copper, Lead and Zinc in Snow from Near Dye 3 in South Greenland

1988 ◽  
Vol 10 ◽  
pp. 193-197 ◽  
Author(s):  
E.W. Wolff ◽  
David A. Peel
Keyword(s):  
Heavy Metals ◽  
Early Spring ◽  
The Arctic ◽  
Late Winter ◽  
Limited Data ◽  
Crustal Component ◽  
Mean Values ◽  
Lead And Zinc ◽  
Gasoline Additive ◽  
Spring Maximum

Clean sampling and analysis procedures have been used to measure the concentrations of Al and four heavy metals in snow representing one year’s accumulation (1983-84) near Dye 3 in Greenland. Mean values were Al 17.5ng g−1, Cd 0.74 pg g−1, Cu 6.2 pg g−1, Pb 28 pg g−1 and Zn 27 pg g−1. Concentrations of the heavy metals are lower than previously reported at other Greenland sites for snowfall during the last 20 years. A distinct late-winter / early-spring maximum is seen for Al, Cu, Pb and Zn, in accord with other workers’ measurements of various species in the atmospheric aerosol in the Arctic. Cu appears to have a large crustal component, but Cd, Pb and Zn probably originate mainly from pollution. One explanation for the lower Pb values may be the considerable reduction in North American and European usage of Pb as a petrol (gasoline) additive during the last decade. These limited data emphasize the importance of obtaining a reliable century-long record of these metals in Greenland ice.

A Subice Suction Corer for Sampling Epontic Ice Algae

1988 ◽  
Vol 45 (3) ◽  
pp. 562-568 ◽  
Author(s):  
Harold E. Welch ◽  
Martin A. Bergmann ◽  
John K. Jorgenson ◽  
William Burton
Keyword(s):  
Sea Ice ◽  
Quantitative Assessment ◽  
Early Spring ◽  
Late Winter ◽  
First Year ◽  
Ice Algae ◽  
Sources Of Error

Standard SIPRE coring was compared with a new Subice Suction Corer and cores taken by diver for the quantitative assessment of epontic (subice) algae on first-year congelation sea ice at Resolute, N.W.T., Canada (≈75°N). The diver cores were probably most accurate but were slow and costly. SIPRE coring was as good as other techniques in late winter and early spring but gave progressively poorer (under) estimates as the season progressed, with up to 90% of the ice algae being lost from SIPRE cores by June. The Subice Suction Corer was fast, easy to operate, cheap, and gave results comparable with samples obtained by diving. Sources of error are discussed.

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