scholarly journals How much is particulate matter near the ground influenced by upper-level processes within and above the PBL? A summertime case study in Milan (Italy) evidences the distinctive role of nitrate

2015 ◽  
Vol 15 (5) ◽  
pp. 2629-2649 ◽  
Author(s):  
G. Curci ◽  
L. Ferrero ◽  
P. Tuccella ◽  
F. Barnaba ◽  
F. Angelini ◽  
...  
Keyword(s):  
Particulate Matter ◽  
Vertical Mixing ◽  
Ground Level ◽  
Lower Atmosphere ◽  
Aerosol Layer ◽  
Dynamical Processes ◽  
Aerosol Mass ◽  
Short Period ◽  
Important Player ◽  
Upper Level

Abstract. Chemical and dynamical processes lead to the formation of aerosol layers in the upper planetary boundary layer (PBL) and above it. Through vertical mixing and entrainment into the PBL these layers may contribute to the ground-level particulate matter (PM); however, to date a quantitative assessment of such a contribution has not been carried out. This study investigates this aspect by combining chemical and physical aerosol measurements with WRF/Chem (Weather Research and Forecasting with Chemistry) model simulations. The observations were collected in the Milan urban area (northern Italy) during the summer of 2007. The period coincided with the passage of a meteorological perturbation that cleansed the lower atmosphere, followed by a high-pressure period favouring pollutant accumulation. Lidar observations revealed the formation of elevated aerosol layers and evidence of their entrainment into the PBL. We analysed the budget of ground-level PM2.5 (particulate matter with an aerodynamic diameter less than 2.5 μm) with the help of the online meteorology–chemistry WRF/Chem model, focusing in particular on the contribution of upper-level processes. Our findings show that an important player in determining the upper-PBL aerosol layer is particulate nitrate, which may reach higher values in the upper PBL (up to 30% of the aerosol mass) than in the lower PBL. The nitrate formation process is predicted to be largely driven by the relative-humidity vertical profile, which may trigger efficient aqueous nitrate formation when exceeding the ammonium nitrate deliquescence point. Secondary PM2.5 produced in the upper half of the PBL may contribute up to 7–8 μg m−3 (or 25%) to ground-level concentrations on an hourly basis. The residual aerosol layer above the PBL is also found to potentially play a large role, which may occasionally contribute up to 10–12 μg m−3 (or 40%) to hourly ground-level PM2.5 concentrations during the morning hours. Although the results presented here refer to one relatively short period in one location, this study highlights the importance of considering the interplay between chemical and dynamical processes occurring within and above the PBL when interpreting ground-level aerosol observations.

scholarly journals How much is particulate matter near the ground influenced by upper level processes within and above the PBL? A summertime case study in Milan (Italy)

2014 ◽  
Vol 14 (19) ◽  
pp. 26403-26461 ◽  
Author(s):  
G. Curci ◽  
L. Ferrero ◽  
P. Tuccella ◽  
F. Barnaba ◽  
F. Angelini ◽  
...  
Keyword(s):  
Particulate Matter ◽  
Vertical Mixing ◽  
Ground Level ◽  
Lower Atmosphere ◽  
Aerosol Layer ◽  
Dynamical Processes ◽  
Aerosol Mass ◽  
Important Player ◽  
Upper Level

Abstract. Chemical and dynamical processes yield to the formation of aerosol layers in the upper planetary boundary layer (PBL) and above it. Through vertical mixing and entrainment into the PBL these layers may contribute to the ground-level particulate matter (PM), but a quantitative assessment of such contribution is still missing. This study investigates this aspect combining chemical and physical aerosol measurements with WRF/Chem model simulations. The observations were collected in the Milan urban area (Northern Italy) during summer of 2007. The period coincided with the passage of a meteorological perturbation that cleansed the lower atmosphere, followed by a high pressure period that favoured pollutant accumulation. Lidar observations reveal the formation of elevated aerosol layers and show evidences of their entrainment into the PBL. We analyze the budget of ground-level PM2.5 (particulate matter with aerodynamic diameter less than 2.5 μm with the help of the online meteorology-chemistry WRF/Chem model, with particular focus on the contribution of upper level processes. We find that an important player in determining the upper PBL aerosol layer is particulate nitrate, which may reach higher values in the upper PBL (up to 30% of the aerosol mass) than the lower. The nitrate formation process is predicted to be largely driven by the relative humidity vertical profile, that may trigger efficient aqueous nitrate formation when exceeding the ammonium nitrate deliquescence point. Secondary PM2.5 produced in the upper half of the PBL may contribute up to 7–8 μg m−3 (or 25%) to ground level concentrations on hourly basis. A large potential role is also found to be played by the residual aerosol layer above the PBL, which may occasionally contribute up to 10–12 μg m−3 (or 40%) to hourly ground level PM2.5 concentrations during the morning. This study highlights the importance of considering the interplay between chemical and dynamical processes occurring within and above the PBL when interpreting ground level aerosol observations.

scholarly journals A low-cost monitor for simultaneous measurement of fine particulate matter and aerosol optical depth – Part 1: Specifications and testing

2019 ◽  
Vol 12 (10) ◽  
pp. 5431-5441 ◽  
Author(s):  
Eric A. Wendt ◽  
Casey W. Quinn ◽  
Daniel D. Miller-Lionberg ◽  
Jessica Tryner ◽  
Christian L'Orange ◽  
...  
Keyword(s):  
Particulate Matter ◽  
Aerosol Optical Depth ◽  
Optical Depth ◽  
Low Cost ◽  
Fine Particulate Matter ◽  
Ground Level ◽  
Aerosol Mass ◽  
Fine Particulate ◽  
The Cost ◽  
Equivalent Method

Abstract. Globally, fine particulate matter (PM2.5) air pollution is a leading contributor to death, disease, and environmental degradation. Satellite-based measurements of aerosol optical depth (AOD) are used to estimate PM2.5 concentrations across the world, but the relationship between satellite-estimated AOD and ground-level PM2.5 is uncertain. Sun photometers measure AOD from the Earth's surface and are often used to improve satellite data; however, reference-grade photometers and PM2.5 monitors are expensive and rarely co-located. This work presents the development and validation of the aerosol mass and optical depth (AMOD) sampler, an inexpensive and compact device that simultaneously measures PM2.5 mass and AOD. The AMOD utilizes a low-cost light-scattering sensor in combination with a gravimetric filter measurement to quantify ground-level PM2.5. Aerosol optical depth is measured using optically filtered photodiodes at four discrete wavelengths. Field validation studies revealed agreement within 10 % for AOD values measured between co-located AMOD and AErosol RObotics NETwork (AERONET) monitors and for PM2.5 mass measured between co-located AMOD and EPA Federal Equivalent Method (FEM) monitors. These results demonstrate that the AMOD can quantify AOD and PM2.5 accurately at a fraction of the cost of existing reference monitors.

Flow Patterns at the Ends of a Street Canyon: Measurements from the Joint Urban 2003 Field Experiment

2008 ◽  
Vol 47 (5) ◽  
pp. 1413-1426 ◽  
Author(s):  
Suhas U. Pol ◽  
Michael J. Brown
Keyword(s):  
Street Canyon ◽  
Vertical Mixing ◽  
Ground Level ◽  
Flow Patterns ◽  
Unidirectional Flow ◽  
Sonic Anemometers ◽  
Wide Range ◽  
Upper Level ◽  
Joint Urban 2003 Experiment ◽  
Wind Vane

Abstract During the Joint Urban 2003 experiment held in Oklahoma City, Oklahoma, an east–west-running street canyon was heavily instrumented with wind sensors. In this paper, the flow patterns at the street canyon ends are investigated by looking at sonic anemometers placed near ground level and tethersonde wind vane systems operated in “ladder” mode that were suspended over the sides of the buildings on each side of the street. For southerly flow conditions, the street-level wind sensors often showed what appeared to be a horizontally rotating “corner” or “end” vortex existing at each end of the street canyon near the intersections. It was found that this vortex flow pattern appeared for a wide range of upper-level wind directions but then changed to purely unidirectional flow for wind directions that were outside this range. The tethersonde wind vane measurements show that this vortexlike flow regime occasionally existed through the entire depth of the street canyon. The horizontal extent of the end vortex into the street canyon was found to be different at each end of the street. Under high-wind conditions, the mean wind patterns in the street did not vary appreciably during the day and night. The end vortex may be important in the dispersal of airborne contaminants, acting to enhance lateral and vertical mixing.

scholarly journals Vertical Wind Shear Modulates Particulate Matter Pollutions: A Perspective from Radar Wind Profiler Observations in Beijing, China

2020 ◽  
Vol 12 (3) ◽  
pp. 546 ◽  
Author(s):  
Ying Zhang ◽  
Jianping Guo ◽  
Yuanjian Yang ◽  
Yu Wang ◽  
Steve Yim
Keyword(s):  
Particulate Matter ◽  
Air Quality ◽  
Wind Shear ◽  
Strong Dependence ◽  
Vertical Mixing ◽  
Vertical Wind Shear ◽  
Ground Level ◽  
Vertical Wind ◽  
Wind Profiler ◽  
Northerly Wind

Vertical wind shear (VWS) is one of the key meteorological factors in modulating ground-level particulate matter with an aerodynamic diameter of 2.5 µm or less (PM2.5). Due to the lack of high-resolution vertical wind measurements, how the VWS affects ground-level PM2.5 remains highly debated. Here we employed the wind profiling observations from the fine-time-resolution radar wind profiler (RWP), together with hourly ground-level PM2.5 measurements, to explore the wind features in the planetary boundary layer (PBL) and their association with aerosols in Beijing for the period from December 1, 2018, to February 28, 2019. Overall, southerly wind anomalies almost dominated throughout the whole PBL or even beyond the PBL under polluted conditions during the course of a day, as totally opposed to the northerly wind anomalies in the PBL under clean conditions. Besides, the ground-level PM2.5 pollution exhibited a strong dependence on the VWS. A much weaker VWS was observed in the lower part of the PBL under polluted conditions, compared with that under clean conditions, which could be due to the strong ground-level PM2.5 accumulation induced by weak vertical mixing in the PBL. Notably, weak northbound transboundary PM2.5 pollution mainly appeared within the PBL, where relatively small VWS dominated. Above the PBL, strong northerlies winds also favored the long-range transport of aerosols, which in turn deteriorated the air quality in Beijing as well. This was well corroborated by the synoptic-scale circulation and backward trajectory analysis. Therefore, we argued here that not only the wind speed in the vertical but the VWS were important for the investigation of aerosol pollution formation mechanism in Beijing. Also, our findings offer wider insights into the role of VWS from RWP in modulating the variation of PM2.5, which deserves explicit consideration in the forecast of air quality in the future.

scholarly journals A low-cost monitor for measurement of fine particulate matter and aerosol optical depth. Part 1: Specifications and testing

2019 ◽  
Author(s):  
Eric A. Wendt ◽  
Casey W. Quinn ◽  
Daniel D. Miller-Lionberg ◽  
Jessica Tryner ◽  
Christian L'Orange ◽  
...  
Keyword(s):  
Particulate Matter ◽  
Aerosol Optical Depth ◽  
Optical Depth ◽  
Low Cost ◽  
Fine Particulate Matter ◽  
Ground Level ◽  
Aerosol Mass ◽  
Fine Particulate ◽  
The Cost ◽  
Equivalent Method

Abstract. Globally, fine particulate matter (PM2.5) air pollution is a leading contributor to death, disease, and environmental degradation. Satellite-based measurements of aerosol optical depth (AOD) are used to estimate PM2.5 concentrations across the world, but the relationship between satellite-estimated AOD and ground-level PM2.5 is uncertain. Sun photometers measure AOD from the Earth's surface and are often used to improve satellite data; however, reference-grade photometers and PM2.5 monitors are expensive and rarely co-located. This work presents the development and validation of the Aerosol Mass and Optical Depth (AMOD) sampler, an inexpensive and compact device that simultaneously measures PM2.5 mass and AOD and was designed specifically to be used in citizen science campaigns. The AMOD utilizes a low-cost light-scattering sensor in combination with a gravimetric filter measurement to quantify ground-level PM2.5. Aerosol optical depth is measured using optically filtered photodiodes at four discrete wavelengths. Field validation studies revealed agreement within 10 % for AOD values measured between co-located AMOD and AErosol RObotics NETwork (AERONET) monitors and for PM2.5 mass measured between co-located AMOD and EPA Federal Equivalent Method (FEM) monitors. These results demonstrate that the AMOD can quantify AOD and PM2.5 accurately at a fraction of the cost of existing reference monitors.

scholarly journals Spatial Analysis (Measurements at Heights of 10 m and 20 m above Ground Level) of the Concentrations of Particulate Matter (PM10, PM2.5, and PM1.0) and Gaseous Pollutants (H2S) on the University Campus: A Case Study

Atmosphere ◽  
2021 ◽  
Vol 12 (1) ◽  
pp. 62
Author(s):  
Robert Cichowicz ◽  
Maciej Dobrzański
Keyword(s):  
Spatial Distribution ◽  
Hydrogen Sulfide ◽  
Particulate Matter ◽  
Air Quality ◽  
Spatial Analysis ◽  
Ground Level ◽  
Leeward Side ◽  
High Concentration ◽  
Above Ground Level ◽  
High Concentrations

Spatial analysis of the distribution of particulate matter PM10, PM2.5, PM1.0, and hydrogen sulfide (H2S) gas pollution was performed in the area around a university library building. The reasons for the subject matter were reports related to the perceptible odor characteristic of hydrogen sulfide and a general poor assessment of air quality by employees and students. Due to the area of analysis, it was decided to perform measurements at two heights, 10 m and 20 m above ground level, using measuring equipment attached to a DJI Matrice 600 unmanned aerial vehicle (UAV). The aim of the measurements was air quality assessment and investigate the convergence of the theory of air flow around the building with the spatial distribution of air pollutants. Considerable differences of up to 63% were observed in the concentrations of pollutants measured around the building, especially between opposite sides, depending on the direction of the wind. To explain these differences, the theory of aerodynamics was applied to visualize the probable airflow in the direction of the wind. A strong convergence was observed between the aerodynamic model and the spatial distribution of pollutants. This was evidenced by the high concentrations of dust in the areas of strong turbulence at the edges of the building and on the leeward side. The accumulation of pollutants was also clearly noticeable in these locations. A high concentration of H2S was recorded around the library building on the side of the car park. On the other hand, the air turbulence around the building dispersed the gas pollution, causing the concentration of H2S to drop on the leeward side. It was confirmed that in some analyzed areas the permissible concentration of H2S was exceeded.

scholarly journals Wind Energy Meteorology: Insight into Wind Properties in the Turbine-Rotor Layer of the Atmosphere from High-Resolution Doppler Lidar

2013 ◽  
Vol 94 (6) ◽  
pp. 883-902 ◽  
Author(s):  
Robert M. Banta ◽  
Yelena L. Pichugina ◽  
Neil D. Kelley ◽  
R. Michael Hardesty ◽  
W. Alan Brewer
Keyword(s):  
Wind Energy ◽  
Ground Level ◽  
Turbine Rotor ◽  
Energy Industry ◽  
Doppler Lidar ◽  
Near Surface ◽  
Surface Measurements ◽  
Wind Measurements ◽  
Upper Level ◽  
Insight Into

Addressing the need for high-quality wind information aloft in the layer occupied by turbine rotors (~30–150 m above ground level) is one of many significant challenges facing the wind energy industry. Without wind measurements at heights within the rotor sweep of the turbines, characteristics of the flow in this layer are unknown for wind energy and modeling purposes. Since flow in this layer is often decoupled from the surface, near-surface measurements are prone to errant extrapolation to these heights, and the behavior of the near-surface winds may not reflect that of the upper-level flow.

scholarly journals Organic aerosol source apportionment by offline-AMS over a full year in Marseille

2017 ◽  
Author(s):  
Carlo Bozzetti ◽  
Imad El Haddad ◽  
Dalia Salameh ◽  
Kaspar Rudolf Daellenbach ◽  
Paola Fermo ◽  
...  
Keyword(s):  
Particulate Matter ◽  
Air Quality ◽  
Mediterranean Sea ◽  
Source Apportionment ◽  
Organic Aerosol ◽  
Aerodynamic Diameter ◽  
Aerosol Mass Spectrometer ◽  
Aerosol Mass ◽  
Aerosol Source

Abstract. We investigated the seasonal trends of OA sources affecting the air quality of Marseille (France) which is the largest harbor of the Mediterranean Sea. This was achieved by measurements of nebulized filter extracts using an aerosol mass spectrometer (offline-AMS). PM2.5 (particulate matter with an aerodynamic diameter

scholarly journals Indoor particulate matter measurement as a tool in the process of the implementation of Smoke-free Hospitals

2004 ◽  
Vol 61 (3) ◽  
Author(s):  
S. Nardini ◽  
R. Cagnin ◽  
G. Invernizzi ◽  
A. Ruprecht ◽  
R. Boffi ◽  
...  
Keyword(s):  
Particulate Matter ◽  
Real Time ◽  
Control Policy ◽  
National Standards ◽  
Portable Instrument ◽  
Aerosol Mass ◽  
Total Suspended Particles ◽  
European Code ◽  
Working Day ◽  
Indoor Particulate Matter

Aim of the study: There are International and National standards that requires hospitals and health premises to be smoke-free. According to recent data from Italy and other European Countries, smoking is a widespread habit in hospitals. To get smoke-free hospitals in an Italian region, we have adopted the European Code for smoke-free hospitals, which sets standards and provides instruments for its implementation. According to the Code, whenever possible, each step towards a smoke-free hospital, should be shared by all staff. As a mean for achieving this goal, in our region the certification of single units as smoke-free units has been chosen. For getting the certification, besides implementing the Code, we planned to use ETS (Environmental Tobacco Smoke) monitoring, as ETS should not be present in hospitals. As a marker of ETS we have chosen Particulate Matter (PM), as it can easily be measured in real-time with a portable instrument and, when other - even outdoor - sources of combustion can be ruled out, it is an accurate detector of cigarette smoke. Here the first experience of measuring PM in hospitals for monitoring ETS and certificating smoke-free health premises, is described. Materials and methods: PM measurements were carried out without any previous notification in different areas of two Network hospitals of the Veneto Region, during a single working day. A real time laser-operated aerosol mass analyser was used. Several classes of PM (PM1, PM2.5, PM7, PM10, TSP Total Suspended Particles) were measured. Results: Outdoor PM levels were found to be repeatedly lower than the annual official limits of 65 mcg/m3 and around the 24 hour official limits of 15 mcg/m3 [15 to 20 mcg/m3, with an overall mean (±SD) of 17.8 (1.9)] throughout the whole day. Very good indoor air quality was found in the operating theaters and isolation department, where PM2.5 concentrations were much lower than outdoor levels [1.6 (0.9) and 5.9 (0.6) mcg/m3, respectively]. No increase in PM pollution was found in the surveyed medical offices, halls and waiting rooms where smoking was positively forbidden [PM2.5 concentrations of 14.8 (2.2) and 12.9 (1.1) mcg/m3] except in a medical office and in two coffee rooms for staff only where high PM levels were recorded [PM2.5 58.7 (29.1), 27.0 (10.6) and 107.1 (47.8) mcg/m3] and an offence of smoking restrictions could be proved. Conclusions: The measurement of PM in hospital for monitoring ETS proved to be both feasible and sensible. PM measurements with a portable instrument can be used both for controlling the compliance with rules or chosen standards and for educating staff about smoking related hazards, thus gaining consensus for the implementation of the tobacco control policy. In our experience, PM measurement can be used as an aid inside all actions designed by the European Code for smoke-free hospitals.

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