scholarly journals Fluorescence lidar observations of wildfire smoke inside cirrus: A contribution to smoke-cirrus – interaction research

2021 ◽  
Author(s):  
Igor Veselovskii ◽  
Qiaoyun Hu ◽  
Albert Ansmann ◽  
Philippe Goloub ◽  
Thierry Podvin ◽  
...  

Abstract. A remote sensing method, based on fluorescence lidar measurements, that allows to detect and to quantify the smoke content in upper troposphere and lower stratosphere (UTLS) is presented. The unique point of this approach is that, smoke and cirrus properties are observed in the same air volume simultaneously. In the article, we provide results of fluorescence and multiwavelength Mie-Raman lidar measurements performed at ATOLL observatory from Laboratoire d’Optique Atmosphérique, University of Lille, during strong smoke episodes in the summer and autumn seasons of 2020. The aerosol fluorescence was induced by 355 nm laser radiation and the fluorescence backscattering was measured in a single spectral channel, centered at 466 nm of 44 nm width. To estimate smoke properties, such as number, surface area and volume concentration, the conversion factors, which link the fluorescence backscattering and the smoke microphysical properties, are derived from the synergy of multiwavelength Mie-Raman and fluorescence lidar observations. Based on two case studies, we demonstrate that the fluorescence lidar technique provides possibility to estimate the smoke surface area concentration within freshly formed cirrus layers. This value was used in smoke INP parameterization scheme to predict ice crystal number concentrations in cirrus generation cells.

2021 ◽  
Vol 21 (17) ◽  
pp. 13397-13423 ◽  
Author(s):  
Ronny Engelmann ◽  
Albert Ansmann ◽  
Kevin Ohneiser ◽  
Hannes Griesche ◽  
Martin Radenz ◽  
...  

Abstract. An advanced multiwavelength polarization Raman lidar was operated aboard the icebreaker Polarstern during the MOSAiC (Multidisciplinary drifting Observatory for the Study of Arctic Climate) expedition to continuously monitor aerosol and cloud layers in the central Arctic up to 30 km height. The expedition lasted from September 2019 to October 2020 and measurements were mostly taken between 85 and 88.5∘ N. The lidar was integrated into a complex remote-sensing infrastructure aboard the Polarstern. In this article, novel lidar techniques, innovative concepts to study aerosol–cloud interaction in the Arctic, and unique MOSAiC findings will be presented. The highlight of the lidar measurements was the detection of a 10 km deep wildfire smoke layer over the North Pole region between 7–8 km and 17–18 km height with an aerosol optical thickness (AOT) at 532 nm of around 0.1 (in October–November 2019) and 0.05 from December to March. The dual-wavelength Raman lidar technique allowed us to unambiguously identify smoke as the dominating aerosol type in the aerosol layer in the upper troposphere and lower stratosphere (UTLS). An additional contribution to the 532 nm AOT by volcanic sulfate aerosol (Raikoke eruption) was estimated to always be lower than 15 %. The optical and microphysical properties of the UTLS smoke layer are presented in an accompanying paper (Ohneiser et al., 2021). This smoke event offered the unique opportunity to study the influence of organic aerosol particles (serving as ice-nucleating particles, INPs) on cirrus formation in the upper troposphere. An example of a closure study is presented to explain our concept of investigating aerosol–cloud interaction in this field. The smoke particles were obviously able to control the evolution of the cirrus system and caused low ice crystal number concentration. After the discussion of two typical Arctic haze events, we present a case study of the evolution of a long-lasting mixed-phase cloud layer embedded in Arctic haze in the free troposphere. The recently introduced dual-field-of-view polarization lidar technique was applied, for the first time, to mixed-phase cloud observations in order to determine the microphysical properties of the water droplets. The mixed-phase cloud closure experiment (based on combined lidar and radar observations) indicated that the observed aerosol levels controlled the number concentrations of nucleated droplets and ice crystals.


2015 ◽  
Vol 15 (1) ◽  
pp. 1171-1191 ◽  
Author(s):  
D. Shin ◽  
D. Müller ◽  
K. Lee ◽  
S. Shin ◽  
Y. J. Kim ◽  
...  

Abstract. We report on the first Raman lidar measurements of stratospheric aerosol layers in the upper troposphere and lower stratosphere over Korea. The data were taken with the multiwavelength aerosol Raman lidar at Gwangju (35.10° N, 126.53° E), Korea. The volcanic ash particles and gases were released around 12 June 2011 during the eruption of the Nabro volcano (13.37° N, 41.7° E) in Eritrea, east Africa. Forward trajectory computations show that the volcanic aerosols were advected from North Africa to East Asia. The first observation of the stratospheric aerosol layers over Korea was on 19 June 2011. The stratospheric aerosol layers appeared between 15 and 17 km height a.s.l. The aerosol layers' maximum value of the backscatter coefficient and the linear particle depolarization ratio at 532 nm were 1.5 ± 0.3 Mm−1 sr−1 and 2.2%, respectively. We found these values at 16.4 km height a.s.l. 44 days after this first observation, we observed the stratospheric aerosol layer again. We continuously probed the upper troposphere and lower stratosphere for this aerosol layer during the following 5 months, until December 2011. The aerosol layers typically occurred between 10 and 20 km height a.s.l. The stratospheric aerosol optical depth and the maximum backscatter coefficient at 532 nm decreased during these 5 months.


2019 ◽  
Vol 99 ◽  
pp. 02010
Author(s):  
Ronny Engelmann ◽  
Julian Hofer ◽  
Abduvosit N. Makhmudov ◽  
Holger Baars ◽  
Karsten Hanbuch ◽  
...  

During the 18-month Central Asian Dust Experiment we conducted continuous lidar measurements at the Physical Technical Institute of the Academy of Sciences of Tajikistan in Dushanbe between 2015 and 2016. Mineral dust plumes from various source regions have been observed and characterized in terms of their occurrence, and their optical and microphysical properties with the Raman lidar PollyXT. Currently a new container-based lidar system is constructed which will be installed for continuous long-term measurements in Dushanbe.


2013 ◽  
Vol 52 (11) ◽  
pp. 2235 ◽  
Author(s):  
Jörg Schmidt ◽  
Ulla Wandinger ◽  
Aleksey Malinka

2008 ◽  
Vol 25 (8) ◽  
pp. 1454-1462 ◽  
Author(s):  
Thierry Leblanc ◽  
I. Stuart McDermid ◽  
Robin A. Aspey

Abstract A new water vapor Raman lidar was recently built at the Table Mountain Facility (TMF) of the Jet Propulsion Laboratory (JPL) in California and more than a year of routine 2-h-long nighttime measurements 4–5 times per week have been completed. The lidar was designed to reach accuracies better than 5% anywhere up to 12-km altitude, and with the capability to measure water vapor mixing ratios as low as 1 to 10 ppmv near the tropopause and in the lower stratosphere. The current system is not yet fully optimized but has already shown promising results as water vapor profiles have been retrieved up to 18-km altitude. Comparisons with Vaisala RS92K radiosondes exhibit very good agreement up to at least 10 km. They also revealed a wet bias in the lidar profiles (or a dry bias in the radiosonde profiles), increasing with altitude and becoming significant near 10 km and large when approaching the tropopause. This bias cannot be explained solely by well-known too-dry measurements of the RS92K in the upper troposphere and therefore must partly originate in the lidar measurements. Excess signal due to residual fluorescence in the lidar receiver components is among the most likely candidates and is subject to ongoing investigation.


2009 ◽  
Vol 9 (22) ◽  
pp. 8799-8811 ◽  
Author(s):  
P. Di Girolamo ◽  
D. Summa ◽  
R.-F. Lin ◽  
T. Maestri ◽  
R. Rizzi ◽  
...  

Abstract. Raman lidar measurements performed in Potenza by the Raman lidar system BASIL in the presence of cirrus clouds are discussed. Measurements were performed on 6 September 2004 in the frame of the Italian phase of the EAQUATE Experiment. The major feature of BASIL is represented by its capability to perform high-resolution and accurate measurements of atmospheric temperature and water vapour, and consequently relative humidity, both in daytime and night-time, based on the application of the rotational and vibrational Raman lidar techniques in the UV. BASIL is also capable to provide measurements of the particle backscatter and extinction coefficient, and consequently lidar ratio (at the time of these measurements, only at one wavelength), which are fundamental to infer geometrical and microphysical properties of clouds. A case study is discussed in order to assess the capability of Raman lidars to measure humidity in presence of cirrus clouds, both below and inside the cloud. While air inside the cloud layers is observed to be always under-saturated with respect to water, both ice super-saturation and under-saturation conditions are found inside these clouds. Upper tropospheric moistening is observed below the lower cloud layer. The synergic use of the data derived from the ground based Raman Lidar and of spectral radiances measured by the NAST-I Airborne Spectrometer allows the determination of the temporal evolution of the atmospheric cooling/heating rates due to the presence of the cirrus cloud. Lidar measurements beneath the cirrus cloud layer have been interpreted using a 1-D cirrus cloud model with explicit microphysics. The 1-D simulations indicate that sedimentation-moistening has contributed significantly to the moist anomaly, but other mechanisms are also contributing. This result supports the hypothesis that the observed mid-tropospheric humidification is a real feature which is strongly influenced by the sublimation of precipitating ice crystals. Results illustrated in this study demonstrate that Raman lidars, like the one used in this study, can resolve the spatial and temporal scales required for the study of cirrus cloud microphysical processes and appear sensitive enough to reveal and quantify upper tropospheric humidification associated with cirrus cloud sublimation.


2017 ◽  
Author(s):  
Rodanthi-Elisavet Mamouri ◽  
Albert Ansmann

Abstract. We applied the recently introduced Polarization Lidar Photometer Networking (POLIPHON) technique for the first time to triple-wavelength polarization lidar measurements at 355, 532, and 1064 nm. The lidar observations were performed at Barbados during the Saharan Aerosol Long-Range Transport and Aerosol-Cloud-Interaction Experiment (SALTRACE) in the summer of 2014. POLIPHON comprises the traditional lidar technique to separate mineral dust and non-dust backscatter contributions and the new extended approach to separate even the dust backscatter component into fine and coarse dust fractions. We show that the traditional and the extended methods are compatible and lead to the same set of dust and non-dust profiles at simplified, less complex aerosol layering and mixing conditions as is the case over the remote tropical Atlantic. To derive dust mass concentration profiles from the lidar observations, trustworthy extinction-to-volume conversion factors are needed and obtained from an updated, extended AERONET sun photometer data analysis of the correlation of fine, coarse and total dust volume concentration with dust extinction coefficients for all three laser wavelengths. Conversion factors for pure marine aerosol conditions and continental anthropogenic aerosol situations are presented in addition. As an additional new feature of POLIPHON, the Raman-lidar method for particle extinction profiling is used to identify the aerosol type (marine or anthropogenic) of the non-dust aerosol fraction. The full POLIPHON methodology was successfully applied to a SALTRACE case and the results are discussed. We conclude that the 532 nm polarization lidar technique has many advantages in comparison to respective 355 and 1064 nm polarization lidar approaches and leads to most robust and accurate POLIPHON products.


2012 ◽  
Vol 5 (1) ◽  
pp. 17-36 ◽  
Author(s):  
T. Leblanc ◽  
I. S. McDermid ◽  
T. D. Walsh

Abstract. Recognizing the importance of water vapor in the upper troposphere and lower stratosphere (UTLS) and the scarcity of high-quality, long-term measurements, JPL began the development of a powerful Raman lidar in 2005 to try to meet these needs. This development was endorsed by the Network for the Detection of Atmospheric Composition Change (NDACC) and the validation program for the EOS-Aura satellite. In this paper we review the stages in the instrumental development, data acquisition and analysis, profile retrieval and calibration procedures of the lidar, as well as selected results from three validation campaigns: MOHAVE (Measurements of Humidity in the Atmosphere and Validation Experiments), MOHAVE-II, and MOHAVE 2009. In particular, one critical result from this latest campaign is the very good agreement (well below the reported uncertainties) observed between the lidar and the Cryogenic Frost-Point Hygrometer in the entire lidar range 3–20 km, with a mean bias not exceeding 2% (lidar dry) in the lower troposphere, and 3% (lidar moist) in the UTLS. Ultimately the lidar has demonstrated capability to measure water vapor profiles from ∼1 km above the ground to the lower stratosphere with a precision of 10% or better near 13 km and below, and an estimated accuracy of 5%. Since 2005, nearly 1000 profiles have been routinely measured, and since 2009, the profiles have typically reached 14 km for one-hour integration times and 1.5 km vertical resolution, and can reach 21 km for 6-h integration times using degraded vertical resolutions. These performance figures show that, with our present target of routinely running our lidar two hours per night, 4 nights per week, we can achieve measurements with a precision in the UTLS equivalent to that achieved if launching one CFH per month.


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