scholarly journals Modelling changes in secondary inorganic aerosol formation and nitrogen deposition in Europe from 2005 to 2030

2021 ◽  
Author(s):  
Jan Eiof Jonson ◽  
Hilde Fagerli ◽  
Thomas Scheuschner ◽  
Svetlana Tsyro
Keyword(s):  
Critical Loads ◽  
Fine Particles ◽  
Regional Scale ◽  
Ammonia Emission ◽  
Ammonia Emissions ◽  
Aerosol Formation ◽  
European Continent ◽  
Reduced Nitrogen ◽  
Inorganic Aerosol ◽  
Oxidised Nitrogen

Abstract. Secondary inorganic PM2.5 particles are formed from SOx, NOx and ammonia emissions, through the formation of either ammonium sulphate or ammonium nitrate. EU limits and WHO guidelines for PM2.5 levels are frequently exceeded in Europe, in particular in the winter months. In addition the critical loads for eutrophication are exceeded in most of the European continent. Further reductions in ammonia emissions and other PM precursors beyond the 2030 requirements could alleviate some of the health burden from fine particles, and also reduce the deposition of nitrogen to vulnerable ecosystems. Using the regional scale EMEP/MSC-W model, we have studied the effects of year 2030 ammonia emissions on PM2.5 concentrations and depositions of nitrogen in Europe in the light of present (2017) and past (2005) conditions. Our calculations show that in Europe the formation of PM2.5 from ammonia to a large extent is limited by the ratio between the emissions of ammonia on one hand, and SOx plus NOx, on the other hand. As the ratio of ammonia to SOx and NOx is increasing, the potential to further curb PM2.5 levels through reductions in ammonia emissions is decreasing. Here we show that per gram of ammonia emissions mitigated, the resulting reductions in PM2.5 levels simulated using 2030 emissions are about a factor of 2.6 lower than when 2005 emissions are used. However, this ratio is lower in winter, thus further reductions in the ammonia emissions in winter may have similar potentials as SOx and NOx in curbing PM2.5 levels in this season. Following the expected reductions of ammonia emission, depositions of reduced nitrogen should also decrease in Europe. However, as the reductions in NOx emission are larger than for ammonia, the fraction of total nitrogen (reduced plus oxidised nitrogen) deposited as reduced nitrogen is increasing and may exceed 60 % in most of Europe by 2030. Thus the potential for future reductions in the exceedances of critical loads for eutrophication in Europe will mainly rely on the ability to reduce ammonia emissions.

AMMONIA EMISSION FROM ANIMAL PRODUCTION IN POLAND ON A REGIONAL SCALE

2019 ◽  
Vol XXI (2) ◽  
pp. 117-124 ◽  
Author(s):  
Zuzanna Jarosz ◽  
Antoni Faber
Keyword(s):  
Regional Scale ◽  
Agricultural Practices ◽  
Spatial Differentiation ◽  
Farming System ◽  
Animal Production ◽  
Ammonia Emission ◽  
Animal Nutrition ◽  
Poultry Production ◽  
Ammonia Emissions ◽  
National Centre

The aim of the study was to present ammonia emissions from animal production on a regional scale in 2016. Emission estimates in particular regions were based on methodology developed by EEA in 2016 and applied in Poland by The National Centre for Emissions Management (NCEM). The conducted analyses were based on the size of livestock population, farming system and emission factors at every stage of manure management. The analysis showed substantial spatial differentiation of ammonia emissions from animal production. Voivodships that accounted for the biggest share in emissions from cattle farming were as follows: Mazowieckie, Podlaskie and Wielkopolskie. Estimated emissions in these voivodships amounted to: 47.4, 32.8 and 21.7 Gg NH3, respectively. The highest levels of ammonia emissions from pig production were identified in the region of Wielkopolska. Ammonia emissions in this voivodship amounted to 16.2 Gg NH3. The Wielkopolska region is also distinguished by the highest ammonia emissions from poultry production. The emissions equaled 11.4 Gg NH3 and accounted for 24.1% of total emissions in this region. The realization of reduction commitments for ammonia imposed by the NEC Directive depends on the introduction of a set of changes in livestock production: regarding the housing method, animal nutrition, fertilizer storage and application as well as dissemination of good agricultural practices aiming at ammonia emission reduction.

scholarly journals Effects of global ship emissions on European air pollution levels

2020 ◽  
Author(s):  
Jan Eiof Jonson ◽  
Michael Gauss ◽  
Michael Schulz ◽  
Jukka-Pekka Jalkanen ◽  
Hilde Fagerli
Keyword(s):  
Air Pollution ◽  
Sulfur Dioxide ◽  
Fine Particles ◽  
Regional Scale ◽  
Ozone Formation ◽  
Ship Emissions ◽  
Model Calculations ◽  
The World ◽  
Sensitivity Studies ◽  
Oxidised Nitrogen

Abstract. Ship emissions constitute a large, and so far poorly regulated, source of air pollution. Emissions are mainly clustered along major ship routes, both in open seas and close to densely populated shorelines. Major air pollutants emitted include sulfur dioxide, NOx and particles. Sulfur dioxide and NOx are both major contributors to the formation of secondary fine particles (PM2.5) and to acidification and eutrophication. In addition, NOx is a major precursor for ground-level ozone. This study is based on global and regional model calculations. The model runs are made with meteorology and emission data representative for year 2017, after the tightening of the SECA (Sulphur Emission Control Area) regulations in 2015, but before the global sulfur cap entering into force in 2020. We have also made model runs reducing sulfur emissions by 80 % corresponding to the 2020 requirements. This study is based on model sensitivity studies perturbing emissions from different sea areas: the Northern European SECA in the North Sea and the Baltic Sea, the Mediterranean Sea and the Black Sea, the Atlantic Ocean close to Europe, shipping in the rest of the world and finally all global ship emissions together. Sensitivity studies have also been made setting lower bounds on the effects of ship plumes on ozone formation. The results from the global and regional calculations are similar. Both global and regional scale calculations show that for PM2.5 and depositions of oxidised nitrogen and sulfur, the effects of ship emissions are much larger when emissions occur close to the shore than at open seas. In many coastal countries calculations show that shipping is responsible for 10 % or more of the controllable PM2.5 concentrations and depositions of oxidised nitrogen and sulphur. For ozone the lifetime in the atmosphere is much longer than for PM2.5, and the potential for ozone formation is much larger in otherwise pristine environments. We find considerable contributions from open sea shipping. As a result the largest contributions to ozone in several regions and countries are from rest of the world shipping.

scholarly journals Factors determining the formation of secondary inorganic aerosol: a case study in the Po Valley (Italy)

2013 ◽  
Vol 13 (4) ◽  
pp. 1927-1939 ◽  
Author(s):  
S. Squizzato ◽  
M. Masiol ◽  
A. Brunelli ◽  
S. Pistollato ◽  
E. Tarabotti ◽  
...  
Keyword(s):  
Regional Scale ◽  
Inorganic Ions ◽  
Weather Conditions ◽  
Water Soluble ◽  
Molar Ratio ◽  
Aerosol Formation ◽  
Po Valley ◽  
Inorganic Aerosol ◽  
One Year ◽  
Critical Regions

Abstract. Physicochemical properties of aerosol were investigated by analyzing the inorganic water soluble content in PM2.5 samples collected in the eastern part of the Po Valley (Italy). In this area the EU limits for many air pollutants are frequently exceeded as a consequence of local sources and regional-scale transport of secondary inorganic aerosol precursors. Nine PM2.5-bound major inorganic ions (F−, Cl−, NO3−, SO42−, Na+, NH4+, K+, Mg2+, Ca2+) were monitored over one year in three sites categorized as semi-rural background, urban background and industrial. The acidic properties of the PM2.5 were studied by applying the recently developed E-AIM thermodynamic model 4 (Extended Aerosol Thermodynamics Model). The experimental data were also examined in relation to the levels of gaseous precursors of secondary inorganic aerosol (SO2, NOx, NO, NO2) and on the basis of some environmental conditions having an effect on the secondary aerosols generation processes. A chemometric procedure using cluster analysis on experimental [NH4+]/[SO42−] molar ratio and NO3− concentration has been applied to determine the conditions needed for ammonium nitrate formation in different chemical environments. Finally, some considerations on the secondary inorganic aerosol formation and the most relevant weather conditions concerning the sulfate-nitrate-ammonium system were also discussed. The obtained results and discussion can help in understanding the secondary aerosol formation dynamics in the Po Valley, which is one of the most critical regions for air pollution in southern Europe.

scholarly journals Factors determining the formation of secondary inorganic aerosol: a case study in the Po Valley (Italy)

2012 ◽  
Vol 12 (7) ◽  
pp. 16377-16406 ◽  
Author(s):  
S. Squizzato ◽  
M. Masiol ◽  
A. Brunelli ◽  
S. Pistollato ◽  
E. Tarabotti ◽  
...  
Keyword(s):  
Ammonium Nitrate ◽  
Regional Scale ◽  
Inorganic Ions ◽  
Weather Conditions ◽  
Climatic Conditions ◽  
Water Soluble ◽  
Molar Ratio ◽  
Aerosol Formation ◽  
Po Valley ◽  
Inorganic Aerosol

Abstract. Physicochemical properties of aerosol were investigated by analyzing the inorganic water soluble content in PM2.5 samples collected in the eastern part of the Po Valley (Italy). In this area the EU limits for many air pollutants are frequently exceeded as a consequence of local sources and regional-scale transport of secondary inorganic aerosol precursors. Nine PM2.5-bound major inorganic ions (F-, Cl-, NO3-, SO42-, Na+, NH4+, K+, Mg2+, Ca2+) were monitored over one year in three sites categorized as semi-rural background, urban background and industrial. The acidic properties of the PM2.5 were studied by applying the recently developed E-AIM thermodynamic model 4. The experimental data were also examined in relation to the levels of gaseous precursors of SIA (SO2, NOx, NO, NO2) and on the basis of some environmental conditions having an effect on the secondary aerosols generation processes. A chemometric procedure using cluster analysis on experimental [NH4+]/[SO42-] molar ratio and NO3- concentration has been applied to determine the conditions needed for ammonium nitrate formation in different chemical environments. Finally, some considerations on the secondary inorganic aerosol formation and the most relevant weather conditions concerning the sulfate-nitrate-ammonium system were also discussed. The methods used can be easily applied to other environments to evaluate the physicochemical characteristics of aerosols and the climatic conditions necessary for the formation of ammonium sulfate and ammonium nitrate aerosols.

An Investigation on Aldehyde and Ammonia Emissions from a 4-Stroke Gasoline-Fueled Motorcycle. Ammonia Emission Reduction by using a SCR Catalyst

2013 ◽  
Author(s):  
Luiz Carlos Daemme ◽  
Renato de Arruda Penteado ◽  
Cláudio Furlan ◽  
Marcelo Errera ◽  
Fátima M. Z. Zotin
Keyword(s):  
Emission Reduction ◽  
Ammonia Emission ◽  
Ammonia Emissions ◽  
Scr Catalyst

Effects of ozone and relative humidity in secondary inorganic aerosol formation during haze events in Beijing, China

2021 ◽  
pp. 105855
Author(s):  
Pengkun Ma ◽  
Jiannong Quan ◽  
Xingcan Jia ◽  
Zhiheng Liao ◽  
Qianqian Wang ◽  
...  
Keyword(s):  
Relative Humidity ◽  
Aerosol Formation ◽  
Inorganic Aerosol ◽  
Beijing China

scholarly journals THE EFFECT OF DIFFERENT NEW BEDDING MATERIALS ON AMMONIA EMISSION FROM DAIRY COW SLURRY

AGROFOR ◽  
2020 ◽  
Vol 5 (3) ◽  
Author(s):  
Maarit HELLSTEDT ◽  
Hannu E.S. HAAPALA
Keyword(s):  
Dairy Cow ◽  
Volume Ratio ◽  
Renewable Resource ◽  
Ammonia Emission ◽  
Ammonia Emissions ◽  
Emission Rates ◽  
Canary Grass ◽  
Bedding Materials ◽  
By Products ◽  
Cow Slurry

Agriculture is the most significant source of Ammonia emission that causes e.g. loss of Nitrogen from agricultural systems. Manure is the main source of Ammonia emissions and causes losses in the nutrient cycles of agriculture as well as local odour nuisance. By using different bedding materials, it is possible to reduce both the Ammonia emissions and to improve the cycling of nutrient. Peat is known as an effective litter material but its use as a virtually non-renewable resource is questionable. Therefore, we need to find new bedding materials to replace peat. In this study, the effect of ten different industrial by-products, reeds and stalks to reduce Ammonia emissions was tested in laboratory in January 2020. Dairy cow slurry and bedding materials were mixed in a volume ratio of 4:1. The Ammonia emission was measured for two weeks once or twice a day. Measurements were performed with a photoacoustic method. The results show that all tested materials reduce the Ammonia emission from the cow slurry used. Interesting new materials to substitute peat are zero fiber and briquetted textile waste. Wheat bran, pellets made of reed canary grass and chopped bulrush had the best effect which is at the same level as that of peat. However, no statistically significant differences between the calculated emission rates were found.

scholarly journals REDUCTION OF AMMONIA EMISSIONS FROM THE COMPOSTING OF SLAUGHTERHOUSE SOLID WASTE USING ZEOLITE

2020 ◽  
Vol 3 (2) ◽  
pp. 164
Author(s):  
Rhenny Ratnawati ◽  
Sugito Sugito
Keyword(s):  
Solid Waste ◽  
High Capacity ◽  
Raw Material ◽  
Ammonia Emission ◽  
Ammonia Emissions ◽  
Impact Study ◽  
Aerobic Composting ◽  
Ammonia Gas ◽  
Gas Emissions ◽  
Composting Process

The process of aerobic composting the slaughterhouse (SH) solid waste generate ammonia emissions. Aim: The objective of this research to study the ability of the adsorbent to use zeolite to reduce ammonia gas emissions during the composting process of SH solid waste. Methodology and Results: Reduction of ammonia emission is conducted during the aerobic composting process which is 50 days. The raw material composition of the composting process used was 100% rumen contents, 60% rumen contents: 40% straw, 50% rumen contents: 50% straw, and 40% rumen contents: 60% straw. Zeolite used in the form of granular size 100 mesh. The result of the research showed that the level of release of ammonia gas emissions during the composting process could be reduced by zeolite. Conclusion, significance, and impact study: The efficiency of reducing ammonia gas emissions using zeolite adsorbents in the composting process of SH solid waste ranges from 98.09 - 99.40% on average. Zeolite is an adsorbent that has high adsorption power because it has many pores and has a high ion exchange high capacity and serves as an absorbent cation that can cause environmental pollution.

Satellite based county- to provincial-level ammonia emissions estimates

2021 ◽  
Author(s):  
Enrico Dammers ◽  
Mark Shephard ◽  
Evan White ◽  
Debora Griffin ◽  
Evan Chow ◽  
...  
Keyword(s):  
Western Europe ◽  
Satellite Observations ◽  
Ammonia Emission ◽  
Ammonia Emissions ◽  
Wind Fields ◽  
Spatially Resolved ◽  
Satellite Sensors ◽  
Cross Track ◽  
North Western

<p>While ammonia (NH3) at its current levels is known to be a hazard to environmental and human health, the atmospheric budget is still quite uncertain. This can largely be attributed to the short lifetime of ammonia in combination with an overall lack of (dense) in-situ measurement networks. The capability to observe ammonia distributions with satellites has opened new ways to study the atmospheric ammonia budget. Previous studies have demonstrated the capability of current ammonia satellite sensors to resolve emissions from point like sources, biomass burning, and constraining emission sources at a regional level with methods involving the use of air quality models.</p><p>In this study, we present the first spatially resolved ammonia emission estimates across the globe using a consistent methodology based solely on ammonia satellite observations from the Cross-track Infrared Sounder (CrIS) instrument and ECMWF ERA5 wind fields. The concept was evaluated for North Western Europe and demonstrated the ability to constrain annual emissions at county- to provincial-levels with most deviations within the bounds found in the error analysis. Furthermore, we show that for some regions the spatial patterns found in the satellite observations are consistent while others do not match the current inventories. Finally, the results indicate that the absolute emission levels tend to be underestimated for parts of the globe.</p>

Sign in / Sign up

Export Citation Format

Share Document