scholarly journals Global and regional trends in aerosol optical depth based on remote sensing products and pollutant emission estimates between 2000 and 2009

2010 ◽  
Vol 10 (12) ◽  
pp. 30731-30776 ◽  
Author(s):  
A. de Meij ◽  
A. Pozzer ◽  
J. Lelieveld

Abstract. This study evaluates global and regional aerosol optical depth (AOD) trends in view of aerosol (precursor) emission changes between 2000 and 2009. We use AOD products from MODIS, MISR and AERONET, and emission estimates from the EMEP, REAS and IPCC inventories. First we compare trends in global Level 3 AOD products of MODIS, MISR and AERONET (Level 2). We find generally negative trends over Europe and North America, whereas over South and East Asia they are mostly positive. The negative trends over parts of Europe and North-East America appear to be significant. Second, we analyze MODIS Level 2 AODs for three selected regions with good data coverage (Central Mediterranean, North-East America and East Asia) and compare with Level 3 products. This corroborates that the 2000–2009 AOD trend over the Central Mediterranean is negative and corresponds well with the MODIS Level 3 analysis. Also for North-East America the trend is generally negative and in agreement with MODIS Level 3 products. For East Asia the trends derived from Level 2 products are mostly positive and correspond with the MODIS Level 3 results. Over Europe, the trends in aerosol single scattering albedo, as derived from MISR data, appear to be positive (declining solar radiation absorption), whereas this is not the case over the USA, though these data are not yet validated. Third we compare trends in AOD with emission changes of SO2, NOx, NH3 and black carbon. We associate the downward trends in AOD over Europe and North America with decreasing emissions of SO2, NOx, and other criteria pollutants, and consequently declining aerosol concentrations. Over East Asia the MODIS Level 2 trends are generally positive, consistent with increasing pollutant emissions by fossil energy use and growing industrial and urban activities. It appears that SO2 emission changes dominate the AOD trends, although especially in Asia NOx emissions may become increasingly important. Our results suggest that solar brightening due to decreasing SO2 emissions and resulting downward AOD trends over Europe may have weakened in the 2000s compared to the 1990s.

2015 ◽  
Vol 15 (23) ◽  
pp. 33897-33929 ◽  
Author(s):  
H. Lee ◽  
O. V. Kalashnikova ◽  
K. Suzuki ◽  
A. Braverman ◽  
M. J. Garay ◽  
...  

Abstract. The Multi-angle Imaging SpectroRadiometer (MISR) Joint Aerosol (JOINT_AS) Level 3 product provides a global, descriptive summary of MISR Level 2 aerosol optical depth (AOD) and aerosol type information for each month between March 2000 and the present. Using Version 1 of JOINT_AS, which is based on the operational (Version 22) MISR Level 2 aerosol product, this study analyzes, for the first time, characteristics of observed and simulated distributions of AOD for three broad classes of aerosols: non-absorbing, absorbing, and non-spherical – near or downwind of their major source regions. The statistical moments (means, standard deviations, and skewnesses) and distributions of AOD by components derived from the JOINT_AS are compared with results from the SPectral RadIatioN-TrAnSport (SPRINTARS) model, a chemistry transport model (CTM) with very high spatial and temporal resolution. Overall, the AOD distributions of combined MISR aerosol types show good agreement with those from SPRINTARS. Marginal distributions of AOD for each aerosol type in both MISR and SPRINTARS show considerable high positive skewness, which indicates the importance of including extreme AOD events when comparing satellite retrievals with models. The MISR JOINT_AS product will greatly facilitate comparisons between satellite observations and model simulations of aerosols by type.


2013 ◽  
Vol 13 (2) ◽  
pp. 675-692 ◽  
Author(s):  
J. A. Ruiz-Arias ◽  
J. Dudhia ◽  
C. A. Gueymard ◽  
D. Pozo-Vázquez

Abstract. The daily Level-3 MODIS aerosol optical depth (AOD) product is a global daily spatial aggregation of the Level-2 MODIS AOD (10-km spatial resolution) into a regular grid with a resolution of 1° × 1°. It offers interesting characteristics for surface solar radiation and numerical weather modeling applications. However, most of the validation efforts so far have focused on Level-2 products and only rarely on Level 3. In this contribution, we compare the Level-3 Collection 5.1 MODIS AOD dataset from the Terra satellite available since 2000 against observed daily AOD values at 550 nm from more than 500 AERONET ground stations around the globe. Overall, the mean error of the dataset is 0.03 (17%, relative to the mean ground-observed AOD), with a root mean square error of 0.14 (73%, relative to the same), but these errors are also found highly dependent on geographical region. We propose new functions for the expected error of the Level-3 AOD, as well as for both its mean error and its standard deviation. Additionally, we investigate the role of pixel count vis-à-vis the reliability of the AOD estimates, and also explore to what extent the spatial aggregation from Level 2 to Level 3 influences the total uncertainty in the Level-3 AOD. Finally, we use a radiative transfer model to investigate how the Level-3 AOD uncertainty propagates into the calculated direct normal and global horizontal irradiances.


2021 ◽  
Author(s):  
Vasilis Margaritis ◽  
Nikolaos Hatzianastassiou ◽  
Marios Bruno Korras Carraca ◽  
Maria Gavrouzou

<p>After the outbreak of SARS-CoV-2 in December 2019 and its spread worldwide in the following months and seasons, the governments around the world were forced, one by one, to impose lockdown measures in their countries during the ‘Covid Year’ of 2020, trying to slowdown or even stop the spread of the virus. These nationwide lockdowns, included measures that led to the reduction of human movement, such as transportation, in urban areas, while they also diminished the industrial activity. Since transportation and industrial activity are among the major sources of emission of anthropogenic aerosols, it is possible that a change, namely a decrease, of the atmospheric aerosol loading is observed during the year 2020. </p><p>In this study, we examine and quantify the possible effect of worldwide Covid19-related lockdowns on air quality, and more specifically on the aerosol optical depth, which is a good measure of aerosol loading. The analysis is done at global scale using Collection 6.1 Level-3 daily 1°x1° latitude-longitude gridded spectral Aerosol Optical Depth (AOD) data from Moderate Resolution Imaging Spectroradiometer (MODIS) on AQUA satellite during the period 2003-2020. We assess the possible anomaly in AOD values during 2020 by comparing their annual, seasonal and monthly mean values with the corresponding climatological ones for the period 2003-2019. A trend analysis is also performed using time series of deseasonalized AOD anomalies during the period 2003-2020. Special emphasis is given to specific great urban areas, as well as to areas where stricter measures were taken for limiting the virus’ spread. For these areas of interest, a further analysis using higher resolution (10km x 10km) MODIS Level-2  AOD data was made in order to capture local changes in AOD that could be hindered by the coarser resolution Level-3 data. Finally, for these regions, the AOD changes estimated using MODIS Level-2 data are intercompared with the corresponding ones using data from local AERONET (AErosol RObotic NETwork) stations. Preliminary results show a clear reduction in AOD values, mainly starting from April 2020 and becoming more clear in late spring and early summer (May and June) of 2020.</p>


2020 ◽  
Vol 12 (17) ◽  
pp. 2847 ◽  
Author(s):  
Pawan Gupta ◽  
Lorraine A. Remer ◽  
Falguni Patadia ◽  
Robert C. Levy ◽  
Sundar A. Christopher

The state-of-art satellite observations of atmospheric aerosols over the last two decades from NASA’s Moderate Resolution Imaging Spectroradiometer (MODIS) instruments have been extensively utilized in climate change and air quality research and applications. The operational algorithms now produce Level 2 aerosol data at varying spatial resolutions (1, 3, and 10 km) and Level 3 data at 1 degree. The local and global applications have benefited from the coarse resolution gridded data sets (i.e., Level 3, 1 degree), as it is easier to use since data volume is low, and several online and offline tools are readily available to access and analyze the data with minimal computing resources. At the same time, researchers who require data at much finer spatial scales have to go through a challenging process of obtaining, processing, and analyzing larger volumes of data sets that require high-end computing resources and coding skills. Therefore, we created a high spatial resolution (high-resolution gridded (HRG), 0.1 × 0.1 degree) daily and monthly aerosol optical depth (AOD) product by combining two MODIS operational algorithms, namely Deep Blue (DB) and Dark Target (DT). The new HRG AODs meet the accuracy requirements of Level 2 AOD data and provide either the same or more spatial coverage on daily and monthly scales. The data sets are provided in daily and monthly files through open an Ftp server with python scripts to read and map the data. The reduced data volume with an easy to use format and tools to access the data will encourage more users to utilize the data for research and applications.


2016 ◽  
Vol 16 (10) ◽  
pp. 6627-6640 ◽  
Author(s):  
Huikyo Lee ◽  
Olga V. Kalashnikova ◽  
Kentaroh Suzuki ◽  
Amy Braverman ◽  
Michael J. Garay ◽  
...  

Abstract. The Multi-angle Imaging SpectroRadiometer (MISR) Joint Aerosol (JOINT_AS) Level 3 product has provided a global, descriptive summary of MISR Level 2 aerosol optical depth (AOD) and aerosol type information for each month over 16+ years since March 2000. Using Version 1 of JOINT_AS, which is based on the operational (Version 22) MISR Level 2 aerosol product, this study analyzes, for the first time, characteristics of observed and simulated distributions of AOD for three broad classes of aerosols: spherical nonabsorbing, spherical absorbing, and nonspherical – near or downwind of their major source regions. The statistical moments (means, standard deviations, and skewnesses) and distributions of AOD by components derived from the JOINT_AS are compared with results from two chemistry transport models (CTMs), the Goddard Chemistry Aerosol Radiation and Transport (GOCART) and SPectral RadIatioN-TrAnSport (SPRINTARS). Overall, the AOD distributions retrieved from MISR and modeled by GOCART and SPRINTARS agree with each other in a qualitative sense. Marginal distributions of AOD for each aerosol type in both MISR and models show considerable high positive skewness, which indicates the importance of including extreme AOD events when comparing satellite retrievals with models. The MISR JOINT_AS product will greatly facilitate comparisons between satellite observations and model simulations of aerosols by type.


2012 ◽  
Vol 12 (9) ◽  
pp. 23219-23260 ◽  
Author(s):  
J. A. Ruiz-Arias ◽  
J. Dudhia ◽  
C. A. Gueymard ◽  
D. Pozo-Vázquez

Abstract. The Level-3 MODIS aerosol optical depth (AOD) product offers interesting features for surface solar radiation and numerical weather modeling applications. Remarkably, the Collection 5.1 dataset extends over more than a decade, and provides daily values of AOD over a global regular grid of 1°×1° spatial resolution. However, most of the validation efforts so far have focused on Level-2 products (10-km, at original resolution) and only rarely on Level-3 (at aggregated spatial resolution of 1°×1°). In this contribution, we compare the Level-3 Collection 5.1 MODIS AOD dataset available since 2000 against observed daily AOD values at 550 nm from more than 500 AERONET ground stations around the globe. One aim of this study is to check the advisability of this MODIS dataset for surface shortwave solar radiation calculations using numerical weather models. Overall, the mean error of the dataset is 0.03 (17%, relative to the mean ground-observed AOD), with a root mean square error of 0.14 (73%, relative to the same), albeit these values are found highly dependent on geographical region. For AOD values below about 0.3 the expected error is found very similar to that of the Level-2 product. However, for larger AOD values, higher errors are found. Consequently, we propose new functions for the expected error of the Level-3 AOD, as well as for both its mean error and its standard deviation. Additionally, we investigate the role of pixel count vis-à-vis the reliability of the AOD estimates. Our results show that a higher pixel count does not necessarily turn into a more reliable AOD estimate. Therefore, we recommend to verify this assumption in the dataset at hand if the pixel count is meant to be used. We also explore to what extent the spatial aggregation from Level-2 to Level-3 influences the total uncertainty in the Level-3 AOD. In particular, we found that, roughly, half of the error might be attributable to Level-3 AOD sub-pixel variability. Finally, we use a~radiative transfer model to investigate how the Level-3 AOD uncertainty propagates into the calculated direct normal (DNI) and global horizontal (GHI) irradiances. Overall, results indicate that, for Level-3 AODs smaller than 0.5, the induced uncertainty in DNI due to the AOD uncertainty alone is below 15% on average, and below 5% for GHI (for a solar zenith angle of 30°. However, the uncertainty in AOD is highly spatially variable, and so is that in irradiance.


2012 ◽  
Vol 5 (2) ◽  
pp. 2169-2220 ◽  
Author(s):  
A. M. Sayer ◽  
N. C. Hsu ◽  
C. Bettenhausen ◽  
M.-J. Jeong ◽  
B. N. Holben ◽  
...  

Abstract. This study evaluates a new spectral aerosol optical depth (AOD) dataset derived from Sea-viewing Wide Field-of-view Sensor (SeaWiFS) measurements over land. First, the data are validated against Aerosol Robotic Network (AERONET) direct-sun AOD measurements, and found to compare well on a global basis. If only data with the highest quality flag are used, the correlation is 0.86 and 72% of matchups fall within an expected absolute uncertainty of 0.05 + 20% (for the wavelength of 550 nm). The quality is similar at other wavelengths and stable over the 13-yr (1997–2010) mission length. Performance tends to be better over vegetated, low-lying terrain with typical AOD of 0.3 or less, such as found over much of North America and Eurasia. Performance tends to be poorer for low-AOD conditions near backscattering geometries, where SeaWiFS overestimates AOD, or optically-thick cases of absorbing aerosol, where SeaWiFS tends to underestimate AOD. Second, the SeaWiFS data are compared with midvisible AOD derived from the Moderate Resolution Imaging Spectrometer (MODIS) and Multiangle Imaging Spectroradiometer (MISR). All instruments show similar spatial and seasonal distributions of AOD, although there are regional and seasonal offsets between them. At locations where AERONET data are available, these offsets are largely consistent with the known validation characteristics of each dataset. With the results of this study in mind, the SeaWiFS over-land AOD record is suitable for quantitative scientific use.


2017 ◽  
Author(s):  
Emmanouil Proestakis ◽  
Vassilis Amiridis ◽  
Eleni Marinou ◽  
Aristeidis K. Georgoulias ◽  
Stavros Solomos ◽  
...  

Abstract. We present a 3-D climatology of the desert dust distribution over South-East Asia derived using CALIPSO (Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observation) data. To distinguish desert dust from total aerosol load we apply a methodology developed in the framework of EARLINET (European Aerosol Research Lidar Network), the particle linear depolarization ratio and updated lidar ratio values suitable for Asian dust, on multiyear CALIPSO observations (01/2007–12/2015). The resulting dust product provides information on the horizontal and vertical distribution of dust aerosols over SE (South-East) Asia along with the seasonal transition of dust transport pathways. Persistent high D_AOD (Dust Aerosol Optical Depth) values, of the order of 0.6, are present over the arid and semi-arid desert regions. Dust aerosol transport (range, height and intensity) is subject to high seasonality, with highest values observed during spring for northern China (Taklimakan/Gobi deserts) and during summer over the Indian subcontinent (Thar Desert). Additionally we decompose the CALIPSO AOD (Aerosol Optical Depth) into dust and non-dust aerosol components to reveal the non-dust AOD over the highly industrialized and densely populated regions of SE Asia, where the non-dust aerosols yield AOD values of the order of 0.5. Furthermore, the CALIPSO-based short-term AOD and D_AOD time series and trends between 01/2007 and 12/2015 are calculated over SE Asia and over selected sub-regions. Positive trends are observed over northwest and east China and the Indian subcontinent, whereas over southeast China are mostly negative. The calculated AOD trends agree well with the trends derived from Aqua/MODIS (Moderate Resolution Imaging Spectroradiometer), although significant differences are observed over specific regions.


2006 ◽  
Vol 6 (3) ◽  
pp. 697-713 ◽  
Author(s):  
G. Pace ◽  
A. di Sarra ◽  
D. Meloni ◽  
S. Piacentino ◽  
P. Chamard

Abstract. Aerosol optical depth and Ångström exponent were obtained from multi filter rotating shadowband radiometer (MFRSR) observations carried out at the island of Lampedusa, in the Central Mediterranean, in the period July 2001–September 2003. The average aerosol optical depth at 495.7 nm, τ, is 0.24±0.14; the average Ångström exponent, α, is 0.86±0.63. The observed values of τ range from 0.03 to 1.13, and the values of α vary from −0.32 to 2.05, indicating a large variability in aerosol content and size. In cloud-free conditions, 36% of the airmasses come from Africa, 25% from Central-Eastern Europe, and 19% from Western France, Spain and the North Atlantic. In summer, 42% of the airmasses is of African origin. In almost all cases African aerosols display high values of τ and low values of α, typical of Saharan dust (average values of τ and α are 0.36 and 0.42, respectively). Particles originating from Central-Eastern Europe show relatively large average values of τ and α (0.23 and 1.5, respectively), while particles from Western France, Spain and the North Atlantic show the lowest average values of τ (0.15), and relatively small values of α (0.92). Intermediate values of α are often connected with relatively fast changes of the airmass originating sector, suggesting the contemporary presence of different types of particles in the air column. Clean marine conditions are rare at Lampedusa, and are generally associated with subsidence of the airmasses reaching the island. Average values of τ and α for clean marine conditions are 0.11 and 0.86, respectively. The largest values of α (about 2) were observed in August 2003, when large scale forest fires in Southern Europe produced consistent amounts of fine combustion particles, that were transported to the Central Mediterranean by a persistent high pressure system over Central Europe. Smoke particles in some cases mix with desert dust, producing intermediate values of α. The seasonal distribution of the meteorological patterns over the Mediterranean, the efficiency of the aerosol production mechanisms, and the variability of the particles' residence time produce a distinct seasonal cycle of aerosol optical depths and Ångström exponent values. Particles originating from all sectors show a summer maximum in aerosol optical depth. The summer increase in optical depth for European aerosols is linked with an increment in the values of α, that indicates an enhancement in the number of fine particles. The summer maximum of τ for African particles is associated with a weak reduction in the Ångström exponent, suggesting an increase in the total number of particles and a relatively more intense transport of large particles. The observations were classified according to the aerosol optical properties, and two main classes have been identified: desert dust and biomass burning/urban-industrial aerosols. Values of τ and α averaged over the whole observing period are 0.37 and 0.15 for desert dust, and 0.27 and 1.77 for urban-industrial/biomass burning aerosols.


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