The impact of model grid zooming on tracer transport in the 1999/2000 Arctic polar vortex

Abstract. We have used a 3D chemistry transport model to evaluate the transport of HF and CH4 in the stratosphere during the Arctic winter of 1999/2000. Several model experiments were carried out with the use of a zoom algorithm to investigate the effect of different horizontal resolutions. Balloon-borne and satellite-borne observations of HF and CH4 were used to test the model. In addition, air mass descent rates within the polar vortex were calculated and compared to observations. Outside the vortex the model results agree well with the observations, but inside the vortex the model underestimates the observed vertical gradient in HF and CH4, even when the highest available resolution (1°×1°) is applied. The calculated diabatic descent rates agree with observations above potential temperature levels of 450 K. These model results suggest that too strong mixing through the vortex edge could be a plausible cause for the model discrepancies, associated with the calculated mass fluxes, although other reasons are also discussed. Based on our model experiments we conclude that a global 6°×9° resolution is too coarse to represent the polar vortex, whereas the higher resolutions, 3°×2° and 1°×1°, yield similar results, even with a 6°×9° resolution in the tropical region.

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The impact of model grid zooming on tracer transport in the 1999/2000 Arctic polar vortex

Atmospheric Chemistry and Physics ◽

10.5194/acp-3-1833-2003 ◽

2003 ◽

Vol 3 (5) ◽

pp. 1833-1847 ◽

Cited By ~ 11

Author(s):

M. M. P. van den Broek ◽

M. K. van Aalst ◽

A. Bregman ◽

M. Krol ◽

J. Lelieveld ◽

...

Keyword(s):

Transport Model ◽

Potential Temperature ◽

Polar Vortex ◽

Vertical Gradient ◽

The Arctic ◽

Strong Mixing ◽

Tropical Region ◽

Tracer Transport ◽

Model Experiments ◽

The Impact

Abstract. We have used a 3D chemistry transport model to evaluate the transport of HF and CH4 in the stratosphere during the Arctic winter of 1999/2000. Several model experiments were carried out with the use of a zoom algorithm to investigate the effect of different horizontal resolutions. Balloon-borne and satellite-borne observations of HF and CH4 were used to test the model. In addition, air mass descent rates within the polar vortex were calculated and compared to observations. Outside the vortex the model results agree well with the observations, but inside the vortex the model underestimates the observed vertical gradient in HF and CH4, even when the highest available resolution (1º x 1º) is applied. The calculated diabatic descent rates agree with observations above potential temperature levels of 450 K. These model results suggest that too strong mixing through the vortex edge could be a plausible cause for the model discrepancies, associated with the calculated mass fluxes, although other reasons are also discussed. Based on our model experiments we conclude that a global 6º x 9º resolution is too coarse to represent the polar vortex, whereas the higher resolutions, 3º x 2º and 1º x 1º, yield similar results, even with a 6º x 9º resolution in the tropical region.

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A Match-based approach to the estimation of polar stratospheric ozone loss using Aura Microwave Limb Sounder observations

Atmospheric Chemistry and Physics ◽

10.5194/acp-15-9945-2015 ◽

2015 ◽

Vol 15 (17) ◽

pp. 9945-9963 ◽

Cited By ~ 21

Author(s):

N. J. Livesey ◽

M. L. Santee ◽

G. L. Manney

Keyword(s):

Stratospheric Ozone ◽

Potential Temperature ◽

Polar Vortex ◽

Rate Of Change ◽

The Arctic ◽

Air Mass ◽

Ozone Loss ◽

Chemical Destruction ◽

Induced Changes ◽

The Impact

Abstract. The well-established "Match" approach to quantifying chemical destruction of ozone in the polar lower stratosphere is applied to ozone observations from the Microwave Limb Sounder (MLS) on NASA's Aura spacecraft. Quantification of ozone loss requires distinguishing transport- and chemically induced changes in ozone abundance. This is accomplished in the Match approach by examining cases where trajectories indicate that the same air mass has been observed on multiple occasions. The method was pioneered using ozonesonde observations, for which hundreds of matched ozone observations per winter are typically available. The dense coverage of the MLS measurements, particularly at polar latitudes, allows matches to be made to thousands of observations each day. This study is enabled by recently developed MLS Lagrangian trajectory diagnostic (LTD) support products. Sensitivity studies indicate that the largest influence on the ozone loss estimates are the value of potential vorticity (PV) used to define the edge of the polar vortex (within which matched observations must lie) and the degree to which the PV of an air mass is allowed to vary between matched observations. Applying Match calculations to MLS observations of nitrous oxide, a long-lived tracer whose expected rate of change is negligible on the weekly to monthly timescales considered here, enables quantification of the impact of transport errors on the Match-based ozone loss estimates. Our loss estimates are generally in agreement with previous estimates for selected Arctic winters, though indicating smaller losses than many other studies. Arctic ozone losses are greatest during the 2010/11 winter, as seen in prior studies, with 2.0 ppmv (parts per million by volume) loss estimated at 450 K potential temperature (~ 18 km altitude). As expected, Antarctic winter ozone losses are consistently greater than those for the Arctic, with less interannual variability (e.g., ranging between 2.3 and 3.0 ppmv at 450 K). This study exemplifies the insights into atmospheric processes that can be obtained by applying the Match methodology to a densely sampled observation record such as that from Aura MLS.

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A study of polar ozone depletion based on sequential assimilation of satellite data from the ENVISAT/MIPAS and Odin/SMR instruments

Atmospheric Chemistry and Physics ◽

10.5194/acp-7-899-2007 ◽

2007 ◽

Vol 7 (3) ◽

pp. 899-911 ◽

Cited By ~ 16

Author(s):

J. D. Rösevall ◽

D. P. Murtagh ◽

J. Urban ◽

A. K. Jones

Keyword(s):

Satellite Data ◽

Ozone Depletion ◽

Transport Model ◽

Potential Temperature ◽

Polar Vortex ◽

Solar Irradiation ◽

The Arctic ◽

Ozone Data ◽

The Antarctic ◽

Polar Ozone

Abstract. The objective of this study is to demonstrate how polar ozone depletion can be mapped and quantified by assimilating ozone data from satellites into the wind driven transport model DIAMOND, (Dynamical Isentropic Assimilation Model for OdiN Data). By assimilating a large set of satellite data into a transport model, ozone fields can be built up that are less noisy than the individual satellite ozone profiles. The transported fields can subsequently be compared to later sets of incoming satellite data so that the rates and geographical distribution of ozone depletion can be determined. By tracing the amounts of solar irradiation received by different air parcels in a transport model it is furthermore possible to study the photolytic reactions that destroy ozone. In this study, destruction of ozone that took place in the Antarctic winter of 2003 and in the Arctic winter of 2002/2003 have been examined by assimilating ozone data from the ENVISAT/MIPAS and Odin/SMR satellite-instruments. Large scale depletion of ozone was observed in the Antarctic polar vortex of 2003 when sunlight returned after the polar night. By mid October ENVISAT/MIPAS data indicate vortex ozone depletion in the ranges 80–100% and 70–90% on the 425 and 475 K potential temperature levels respectively while the Odin/SMR data indicates depletion in the ranges 70–90% and 50–70%. The discrepancy between the two instruments has been attributed to systematic errors in the Odin/SMR data. Assimilated fields of ENVISAT/MIPAS data indicate ozone depletion in the range 10–20% on the 475 K potential temperature level, (~19 km altitude), in the central regions of the 2002/2003 Arctic polar vortex. Assimilated fields of Odin/SMR data on the other hand indicate ozone depletion in the range 20–30%.

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Key aspects of stratospheric tracer modeling

Atmospheric Chemistry and Physics Discussions ◽

10.5194/acpd-6-4375-2006 ◽

2006 ◽

Vol 6 (3) ◽

pp. 4375-4414 ◽

Cited By ~ 1

Author(s):

B. Bregman ◽

E. Meijer ◽

R. Scheele

Keyword(s):

Large Scale ◽

Lower Stratosphere ◽

Polar Vortex ◽

Grid Resolution ◽

The Arctic ◽

Tracer Transport ◽

Transport Models ◽

Key Aspects ◽

The Impact ◽

Update Frequency

Abstract. This study describes key aspects of global chemistry-transport models and the impact on stratospheric tracer transport. We concentrate on global models that use assimilated winds from numerical weather predictions, but the results also apply to tracer transport in general circulation models. We examined grid resolution, numerical diffusion and dispersion of the winds fields, the meteorology update time intervals, update frequency, and time interpolation. For this study we applied the three-dimensional chemistry-transport Tracer Model version 5 (TM5) and a trajectory model and performed several diagnoses focusing on different transport regimes. Covering different time and spatial scales, we examined (1) polar vortex dynamics during the Arctic winter, (2) the large-scale stratospheric meridional circulation, and (3) air parcel dispersion in the tropical lower stratosphere. Tracer distributions inside the Arctic polar vortex show considerably worse agreement with observations when the model grid resolution in the polar region is reduced to avoid numerical instability. Using time interpolated winds improve the tracer distributions only marginally. Considerable improvement is found when the update frequency of the assimilated winds is increased from 6 to 3h, both in the large-scale tracer distribution and the polar regions. It further reduces in particular the vertical dispersion of air parcels in the tropical lower stratosphere. The results in this study demonstrates significant progress in the use of assimilated meteorology in chemistry-transport models, which is important for both short- and long-term integrations.

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STRATAQ: A three-dimensional Chemical Transport Model of the stratosphere

Annales Geophysicae ◽

10.5194/angeo-20-847-2002 ◽

2002 ◽

Vol 20 (6) ◽

pp. 847-862

Author(s):

B. Grassi ◽

G. Redaelli ◽

G. Visconti

Keyword(s):

Middle Atmosphere ◽

Transport Model ◽

Three Dimensional ◽

Polar Vortex ◽

Chemical Transport ◽

Heterogeneous Reactions ◽

The Arctic ◽

Chemical Transport Model ◽

Time Space ◽

The Impact

Abstract. A three-dimensional (3-D) Chemical Transport Model (CTM) of the stratosphere has been developed and used for a test study of the evolution of chemical species in the arctic lower stratosphere during winter 1996/97. This particular winter has been chosen for testing the model’s capabilities for its remarkable dynamical situation (very cold and strong polar vortex) along with the availability of sparse chlorine, HNO3 and O3 data, showing also very low O3 values in late March/April. Due to those unusual features, the winter 1996/97 can be considered an excellent example of the impact of both dynamics and heterogeneous reactions on the chemistry of the stratosphere. Model integration has been performed from January to March 1997 and the resulting long-lived and short-lived tracer fields compared with available measurements. The model includes a detailed gas phase chemical scheme and a parameterization of the heterogeneous reactions occurring on liquid aerosol and polar stratospheric cloud (PSC) surfaces. The transport is calculated using a semi-lagrangian flux scheme, forced by meteorological analyses. In such form, the STRATAQ CTM model is suitable for short-term integrations to study transport and chemical evolution related to "real" meteorological situations. Model simulation during the chosen winter shows intense PSC formation, with noticeable local HNO3 capture by PSCs, and the activation of vortex air leading to chlorine production and subsequent O3 destruction. The resulting model fields show generally good agreement with satellite data (MLS and TOMS), although the available observations, due to their limited number and time/space sparse nature, are not enough to effectively constraint the model. In particular, the model seems to perform well in reproducing the rapid processing of air inside the polar vortex on PSC converting reservoir species in active chlorine. In addition, it satisfactorily reproduces the morphology of the continuous O3 decline as shown by the satellite during the investigated period, with a tendency, however, to underestimate the total column values inside the polar vortex during late winter. As possible causes of this model/observation difference we suggest an incorrect estimation of the vertical transport and of the tropospheric contribution.Key words. Atmospheric composition and structure (Middle atmosphere-composition and chemistry) Meterology and atmospheric dynamics (middle atmosphere dynamics)

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A Match-based approach to the estimation of polar stratospheric ozone loss using Aura Microwave Limb Sounder observations

Atmospheric Chemistry and Physics Discussions ◽

10.5194/acpd-15-10041-2015 ◽

2015 ◽

Vol 15 (7) ◽

pp. 10041-10083 ◽

Cited By ~ 2

Author(s):

N. J. Livesey ◽

M. L. Santee ◽

G. L. Manney

Keyword(s):

Stratospheric Ozone ◽

Potential Temperature ◽

Polar Vortex ◽

Rate Of Change ◽

The Arctic ◽

Ozone Loss ◽

Chemically Induced ◽

Chemical Destruction ◽

Induced Changes ◽

The Impact

Abstract. The well-established "Match" approach to quantifying chemical destruction of ozone in the polar lower stratosphere is applied to ozone observations from the Microwave Limb Sounder (MLS) on NASA's Aura spacecraft. Quantification of ozone loss requires distinguishing transport- and chemically induced changes in ozone abundance. This is accomplished in the Match approach by examining cases where trajectories indicate that the same airmass has been observed on multiple occasions. The method was pioneered using ozone sonde observations, for which hundreds of matched ozone observations per winter are typically available. The dense coverage of the MLS measurements, particularly at polar latitudes, allows matches to be made to thousands of observations each day. This study is enabled by recently developed MLS Lagrangian Trajectory Diagnostic (LTD) support products. Sensitivity studies indicate that the largest influence on the ozone loss estimates are the value of potential vorticity (PV) used to define the edge of the polar vortex (within which matched observations must lie) and the degree to which the PV of an airmass is allowed to vary between matched observations. Applying Match calculations to MLS observations of nitrous oxide, a long-lived tracer whose expected rate of change on these timescales is negligible, enables quantification of the impact of transport errors on the Match-based ozone loss estimates. Our loss estimates are generally in agreement with previous estimates for selected Arctic winters, though indicating smaller losses than many other studies. Arctic ozone losses are greatest during the 2010/11 winter, as seen in prior studies, with 2.0 ppmv (parts per million by volume) loss estimated at 450 K potential temperature. As expected, Antarctic winter ozone losses are consistently greater than those for the Arctic, with less interannual variability (e.g., ranging between 2.3 and 3.0 ppmv at 450 K). This study exemplifies the insights into atmospheric processes that can be obtained by applying the Match methodology to a densely sampled observation record such as that from Aura MLS.

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Chemical ozone loss and ozone mini-hole event during the Arctic winter 2010/2011 as observed by SCIAMACHY and GOME-2

Atmospheric Chemistry and Physics ◽

10.5194/acp-14-3247-2014 ◽

2014 ◽

Vol 14 (7) ◽

pp. 3247-3276 ◽

Cited By ~ 16

Author(s):

R. Hommel ◽

K.-U. Eichmann ◽

J. Aschmann ◽

K. Bramstedt ◽

M. Weber ◽

...

Keyword(s):

Transport Model ◽

Polar Vortex ◽

The Arctic ◽

Optical Absorption Spectroscopy ◽

Late Winter ◽

Total Column Ozone ◽

Bromine Oxide ◽

Ozone Loss ◽

Catalytic Cycles ◽

Total Column

Abstract. Record breaking loss of ozone (O3) in the Arctic stratosphere has been reported in winter–spring 2010/2011. We examine in detail the composition and transformations occurring in the Arctic polar vortex using total column and vertical profile data products for O3, bromine oxide (BrO), nitrogen dioxide (NO2), chlorine dioxide (OClO), and polar stratospheric clouds (PSC) retrieved from measurements made by SCIAMACHY (Scanning Imaging Absorption SpectroMeter for Atmospheric CHartography) on-board Envisat (Environmental Satellite), as well as total column ozone amount, retrieved from the measurements of GOME-2 (Global Ozone Monitoring Experiment) on MetOp-A (Meteorological Experimental Satellite). Similarly we use the retrieved data from DOAS (Differential Optical Absorption Spectroscopy) measurements made in Ny-Ålesund (78.55° N, 11.55° E). A chemical transport model (CTM) has been used to relate and compare Arctic winter–spring conditions in 2011 with those in the previous year. In late winter–spring 2010/2011 the chemical ozone loss in the polar vortex derived from SCIAMACHY observations confirms findings reported elsewhere. More than 70% of O3 was depleted by halogen catalytic cycles between the 425 and 525 K isentropic surfaces, i.e. in the altitude range ~16–20 km. In contrast, during the same period in the previous winter 2009/2010, a typical warm Arctic winter, only slightly more than 20% depletion occurred below 20 km, while 40% of O3 was removed above the 575 K isentrope (~23 km). This loss above 575 K is explained by the catalytic destruction by NOx descending from the mesosphere. In both Arctic winters 2009/2010 and 2010/2011, calculated O3 losses from the CTM are in good agreement to our observations and other model studies. The mid-winter 2011 conditions, prior to the catalytic cycles being fully effective, are also investigated. Surprisingly, a significant loss of O3 around 60%, previously not discussed in detail, is observed in mid-January 2011 below 500 K (~19 km) and sustained for approximately 1 week. The low O3 region had an exceptionally large spatial extent. The situation was caused by two independently evolving tropopause elevations over the Asian continent. Induced adiabatic cooling of the stratosphere favoured the formation of PSC, increased the amount of active chlorine for a short time, and potentially contributed to higher polar ozone loss later in spring.

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Record springtime stratospheric ozone depletion at 80°N in 2020

10.5194/egusphere-egu21-8892 ◽

2021 ◽

Author(s):

Ramina Alwarda ◽

Kristof Bognar ◽

Kimberly Strong ◽

Martyn Chipperfield ◽

Sandip Dhomse ◽

...

Keyword(s):

Ozone Depletion ◽

Transport Model ◽

Stratospheric Ozone ◽

Polar Vortex ◽

The Arctic ◽

Optical Absorption Spectroscopy ◽

Chemical Transport Model ◽

Polar Stratospheric Clouds ◽

Ozone Loss ◽

Stratospheric Clouds

The Arctic winter of 2019-2020 was characterized by an unusually persistent polar vortex and temperatures in the lower stratosphere that were consistently below the threshold for the formation of polar stratospheric clouds (PSCs). These conditions led to ozone loss that is comparable to the Antarctic ozone hole. Ground-based measurements from a suite of instruments at the Polar Environment Atmospheric Research Laboratory (PEARL) in Eureka, Canada (80.05&#176;N, 86.42&#176;W) were used to investigate chemical ozone depletion. The vortex was located above Eureka longer than in any previous year in the 20-year dataset and lidar measurements provided evidence of polar stratospheric clouds (PSCs) above Eureka. Additionally, UV-visible zenith-sky Differential Optical Absorption Spectroscopy (DOAS) measurements showed record ozone loss in the 20-year dataset, evidence of denitrification along with the slowest increase of NO2 during spring, as well as enhanced reactive halogen species (OClO and BrO). Complementary measurements of HCl and ClONO2 (chlorine reservoir species) from a Fourier transform infrared (FTIR) spectrometer showed unusually low columns that were comparable to 2011, the previous year with significant chemical ozone depletion. Record low values of HNO3 in the FTIR dataset are in accordance with the evidence of PSCs and a denitrified atmosphere. Estimates of chemical ozone loss were derived using passive ozone from the SLIMCAT offline chemical transport model to account for dynamical contributions to the stratospheric ozone budget.

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Extending the Modular Earth Submodel System (MESSy v2.54) model hierarchy: the ECHAM/MESSy IdeaLized (EMIL) model setup

Geoscientific Model Development ◽

10.5194/gmd-13-5229-2020 ◽

2020 ◽

Vol 13 (11) ◽

pp. 5229-5257

Author(s):

Hella Garny ◽

Roland Walz ◽

Matthias Nützel ◽

Thomas Birner

Keyword(s):

Climate Model ◽

Polar Vortex ◽

Equilibrium Temperature ◽

Earth System ◽

Tracer Transport ◽

Dynamical Core ◽

Vortex Strength ◽

Model Hierarchy ◽

Model Setup ◽

The Impact

Abstract. As models of the Earth system grow in complexity, a need emerges to connect them with simplified systems through model hierarchies in order to improve process understanding. The Modular Earth Submodel System (MESSy) was developed to incorporate chemical processes into an Earth System model. It provides an environment to allow for model configurations and setups of varying complexity, and as of now the hierarchy ranges from a chemical box model to a fully coupled chemistry–climate model. Here, we present a newly implemented dry dynamical core model setup within the MESSy framework, denoted as ECHAM/MESSy IdeaLized (EMIL) model setup. EMIL is developed with the aim to provide an easily accessible idealized model setup that is consistently integrated in the MESSy model hierarchy. The implementation in MESSy further enables the utilization of diagnostic chemical tracers. The setup is achieved by the implementation of a new submodel for relaxation of temperature and horizontal winds to given background values, which replaces all other “physics” submodels in the EMIL setup. The submodel incorporates options to set the needed parameters (e.g., equilibrium temperature, relaxation time and damping coefficient) to functions used frequently in the past. This study consists of three parts. In the first part, test simulations with the EMIL model setup are shown to reproduce benchmarks provided by earlier dry dynamical core studies. In the second part, the sensitivity of the coupled troposphere–stratosphere dynamics to various modifications of the setup is studied. We find a non-linear response of the polar vortex strength to the prescribed meridional temperature gradient in the extratropical stratosphere that is indicative of a regime transition. In agreement with earlier studies, we find that the tropospheric jet moves poleward in response to the increase in the polar vortex strength but at a rate that strongly depends on the specifics of the setup. When replacing the idealized topography to generate planetary waves by mid-tropospheric wave-like heating, the response of the tropospheric jet to changes in the polar vortex is strongly damped in the free troposphere. However, near the surface, the jet shifts poleward at a higher rate than in the topographically forced simulations. Those results indicate that the wave-like heating might have to be used with care when studying troposphere–stratosphere coupling. In the third part, examples for possible applications of the model system are presented. The first example involves simulations with simplified chemistry to study the impact of dynamical variability and idealized changes on tracer transport, and the second example involves simulations of idealized monsoon circulations forced by localized heating. The ability to incorporate passive and chemically active tracers in the EMIL setup demonstrates the potential for future studies of tracer transport in the idealized dynamical model.

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Simulation of ash clouds after a Laacher See-type eruption

10.5194/egusphere-egu21-2314 ◽

2021 ◽

Author(s):

Ulrike Niemeier ◽

Felix Riede ◽

Claudia Timmreck

Keyword(s):

Explosive Volcanism ◽

Stratospheric Aerosol ◽

Radiative Heating ◽

The Arctic ◽

Current Evidence ◽

Aerosol Model ◽

Model Experiments ◽

North East ◽

Volcanic Cloud ◽

The Impact

The large explosive eruption of the Laacher See volcano c. 12,900 yrs BP marked the end of explosive volcanism in the East Eifel volcanic zone (Germany). We have reviewed the current evidence for the impact of the Laacher See Eruption (LSE) on the immediate and wider environment as recorded in a range of proxies with a series of interactive stratospheric aerosol model experiments. Recent studies about the climate impact of NH extratropical eruptions and new insights about the dating of the LSE warrant a return to this cataclysmic eruption and its potential influence on Northern Hemisphere climate. Rather detailed reconstructions of its eruption dynamics have been proposed. The eruption might have lasted several weeks or even months, most likely with an initial (~10h) intense early phase resulting in deposits over north-east Germany and the Baltic Sea, and a slightly later and weaker phase leaving deposits south of the volcano towards the Alps.Our interactive stratospheric aerosol model experiments are based on a reference LSE experiment with emission estimates of 20 Tg of sulfur dioxide (SO2) and 200 Tg of fine-ash, across two eruptive phases in May and June. Additional sensitivity experiments reflect the estimated range of uncertainty of the injection rate and altitude and, assess how the solar-absorptive heating from the 150 Tg of sub-micron ash emitted in the first eruptive phase changed the LSE cloud&#8217;s dispersion. Our simulations reveal that the heating of the ash likely played an important role in the transport of ash and sulfate. Depending on the altitude of the injection, our simulated volcanic cloud begins to rotate shortly after the eruption. This meso-cyclone, as well as the additional radiative heating of the fine ash then changes the dispersion of the cloud to be more southerly compared to dispersal estimated without fine-ash heating. Sulfate transport is similarly impacted by the heating of the ash, resulting in a stronger transport to low-latitudes, later arrival of the volcanic cloud in the Arctic regions and a longer lifetime compared to cases without injection of fine ash.

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