scholarly journals Key aspects of stratospheric tracer modeling

2006 ◽  
Vol 6 (3) ◽  
pp. 4375-4414 ◽  
Author(s):  
B. Bregman ◽  
E. Meijer ◽  
R. Scheele

Abstract. This study describes key aspects of global chemistry-transport models and the impact on stratospheric tracer transport. We concentrate on global models that use assimilated winds from numerical weather predictions, but the results also apply to tracer transport in general circulation models. We examined grid resolution, numerical diffusion and dispersion of the winds fields, the meteorology update time intervals, update frequency, and time interpolation. For this study we applied the three-dimensional chemistry-transport Tracer Model version 5 (TM5) and a trajectory model and performed several diagnoses focusing on different transport regimes. Covering different time and spatial scales, we examined (1) polar vortex dynamics during the Arctic winter, (2) the large-scale stratospheric meridional circulation, and (3) air parcel dispersion in the tropical lower stratosphere. Tracer distributions inside the Arctic polar vortex show considerably worse agreement with observations when the model grid resolution in the polar region is reduced to avoid numerical instability. Using time interpolated winds improve the tracer distributions only marginally. Considerable improvement is found when the update frequency of the assimilated winds is increased from 6 to 3h, both in the large-scale tracer distribution and the polar regions. It further reduces in particular the vertical dispersion of air parcels in the tropical lower stratosphere. The results in this study demonstrates significant progress in the use of assimilated meteorology in chemistry-transport models, which is important for both short- and long-term integrations.

2006 ◽  
Vol 6 (12) ◽  
pp. 4529-4543 ◽  
Author(s):  
B. Bregman ◽  
E. Meijer ◽  
R. Scheele

Abstract. This study describes key aspects of global chemistry-transport models and their impact on stratospheric tracer transport. We concentrate on global models that use assimilated winds from numerical weather predictions, but the results also apply to tracer transport in general circulation models. We examined grid resolution, numerical diffusion, air parcel dispersion, the wind or mass flux update frequency, and time interpolation. The evaluation is performed with assimilated meteorology from the "operational analyses or operational data" (OD) from the European Centre for Medium-Range Weather Forecasts (ECMWF). We also show the effect of the mass flux update frequency using the ECMWF 40-year re-analyses (ERA40). We applied the three-dimensional chemistry-transport Tracer Model version 5 (TM5) and a trajectory model and performed several diagnoses focusing on different transport regimes. Covering different time and spatial scales, we examined (1) polar vortex dynamics during the Arctic winter, (2) the large-scale stratospheric meridional circulation, and (3) air parcel dispersion in the tropical lower stratosphere. Tracer distributions inside the Arctic polar vortex show considerably worse agreement with observations when the model grid resolution in the polar region is reduced to avoid numerical instability. The results are sensitive to the diffusivity of the advection. Nevertheless, the use of a computational cheaper but diffusive advection scheme is feasible for tracer transport when the horizontal grid resolution is equal or smaller than 1 degree. The use of time interpolated winds improves the tracer distributions, particularly in the middle and upper stratosphere. Considerable improvement is found both in the large-scale tracer distribution and in the polar regions when the update frequency of the assimilated winds is increased from 6 to 3 h. It considerably reduces the vertical dispersion of air parcels in the tropical lower stratosphere. Strong horizontal dispersion is not necessarily an indication of poor wind quality, as observations indicate. Moreover, the generally applied air parcel dispersion calculations should be interpreted with care, given the strong sensitivity of dispersion with altitude. The results in this study provide a guideline for stratospheric tracer modeling using assimilated winds. They further demonstrate significant progress in the use of assimilated meteorology in chemistry-transport models, relevant for both short- and long-term integrations.


2003 ◽  
Vol 3 (2) ◽  
pp. 395-402 ◽  
Author(s):  
J.-U. Grooß ◽  
R. Müller

Abstract. Current stratospheric chemical model simulations underestimate substantially the large ozone loss rates that are derived for the Arctic from ozone sondes for January of some years. Until now, no explanation for this discrepancy has been found. Here, we examine the influence of intrusions of mid-latitude air into the polar vortex on these ozone loss estimates. This study focuses on the winter 1991/92, because during this winter the discrepancy between simulated and experimentally derived ozone loss rates is reported to be the largest. Also during the considered period the vortex was disturbed by a strong warming event with large-scale intrusions of mid-latitude air into the polar vortex, which is quite unusual for this time of the year. The study is based on simulations performed with the Chemical Lagrangian Model of the Stratosphere (CLaMS). Two methods for determination the ozone loss are investigated, the so-called vortex average approach and the Match method. The simulations for January 1992 show that the intrusions induce a reduction of vortex average ozone mixing ratio corresponding to a systematic offset of the ozone loss rate of about 12 ppb per day. This should be corrected for in the vortex average method. The simulations further suggest, that these intrusions do not cause a significant bias for the Match method due to effective quality control measures in the Match technique.


2005 ◽  
Vol 5 (2) ◽  
pp. 547-562 ◽  
Author(s):  
K. Krüger ◽  
U. Langematz ◽  
J. L. Grenfell ◽  
K. Labitzke

Abstract. The purpose of this study is to investigate horizontal transport processes in the winter stratosphere using data with a resolution relevant for chemistry and climate modeling. For this reason the Freie Universität Berlin Climate Middle Atmosphere Model (FUB-CMAM) with its model top at 83 km altitude, increased horizontal resolution T42 and the semi-Lagrangian transport scheme for advecting passive tracers is used. A new approach of this paper is the classification of specific transport phenomena within the stratosphere into tropical-subtropical streamers (e.g. Offermann et al., 1999) and polar vortex extrusions hereafter called polar vortex streamers. To investigate the role played by these large-scale structures on the inter-annual and seasonal variability of transport processes in northern mid-latitudes, the global occurrence of such streamers was calculated based on a 10-year model climatology, concentrating on the existence of the Arctic polar vortex. For the identification and counting of streamers, the new method of zonal anomaly was chosen. The analysis of the months October-May yielded a maximum occurrence of tropical-subtropical streamers during Arctic winter and spring in the middle and upper stratosphere. Synoptic maps revealed highest intensities in the subtropics over East Asia with a secondary maximum over the Atlantic in the northern hemisphere. Furthermore, tropical-subtropical streamers exhibited a higher occurrence than polar vortex streamers, indicating that the subtropical barrier is more permeable than the polar vortex barrier (edge) in the model, which is in good correspondence with observations (e.g. Plumb, 2002; Neu et al., 2003). Interesting for the total ozone decrease in mid-latitudes is the consideration of the lower stratosphere for tropical-subtropical streamers and the stratosphere above ~20 km altitude for polar vortex streamers, where strongest ozone depletion is observed at polar latitudes (WMO, 2003). In the lower stratosphere the FUB-CMAM simulated a climatological maximum of 10% occurrence of tropical-subtropical streamers over East-Asia/West Pacific and the Atlantic during early- and mid-winter. The results of this paper demonstrate that stratospheric streamers e.g. large-scale, tongue-like structures transporting tropical-subtropical and polar vortex air masses into mid-latitudes occur frequently during Arctic winter. They can therefore play a significant role on the strength and variability of the observed total ozone decrease at mid-latitudes and should not be neglected in future climate change studies.


2003 ◽  
Vol 3 (5) ◽  
pp. 1833-1847 ◽  
Author(s):  
M. M. P. van den Broek ◽  
M. K. van Aalst ◽  
A. Bregman ◽  
M. Krol ◽  
J. Lelieveld ◽  
...  

Abstract. We have used a 3D chemistry transport model to evaluate the transport of HF and CH4 in the stratosphere during the Arctic winter of 1999/2000. Several model experiments were carried out with the use of a zoom algorithm to investigate the effect of different horizontal resolutions. Balloon-borne and satellite-borne observations of HF and CH4 were used to test the model. In addition, air mass descent rates within the polar vortex were calculated and compared to observations. Outside the vortex the model results agree well with the observations, but inside the vortex the model underestimates the observed vertical gradient in HF and CH4, even when the highest available resolution (1º x 1º) is applied. The calculated diabatic descent rates agree with observations above potential temperature levels of 450 K. These model results suggest that too strong mixing through the vortex edge could be a plausible cause for the model discrepancies, associated with the calculated mass fluxes, although other reasons are also discussed. Based on our model experiments we conclude that a global 6º x 9º resolution is too coarse to represent the polar vortex, whereas the higher resolutions, 3º x 2º and 1º x 1º, yield similar results, even with a 6º x 9º resolution in the tropical region.


2016 ◽  
Vol 16 (23) ◽  
pp. 15371-15396 ◽  
Author(s):  
Gloria L. Manney ◽  
Zachary D. Lawrence

Abstract. The 2015/16 Northern Hemisphere winter stratosphere appeared to have the greatest potential yet seen for record Arctic ozone loss. Temperatures in the Arctic lower stratosphere were at record lows from December 2015 through early February 2016, with an unprecedented period of temperatures below ice polar stratospheric cloud thresholds. Trace gas measurements from the Aura Microwave Limb Sounder (MLS) show that exceptional denitrification and dehydration, as well as extensive chlorine activation, occurred throughout the polar vortex. Ozone decreases in 2015/16 began earlier and proceeded more rapidly than those in 2010/11, a winter that saw unprecedented Arctic ozone loss. However, on 5–6 March 2016 a major final sudden stratospheric warming ("major final warming", MFW) began. By mid-March, the mid-stratospheric vortex split after being displaced far off the pole. The resulting offspring vortices decayed rapidly preceding the full breakdown of the vortex by early April. In the lower stratosphere, the period of temperatures low enough for chlorine activation ended nearly a month earlier than that in 2011 because of the MFW. Ozone loss rates were thus kept in check because there was less sunlight during the cold period. Although the winter mean volume of air in which chemical ozone loss could occur was as large as that in 2010/11, observed ozone values did not drop to the persistently low values reached in 2011.We use MLS trace gas measurements, as well as mixing and polar vortex diagnostics based on meteorological fields, to show how the timing and intensity of the MFW and its impact on transport and mixing halted chemical ozone loss. Our detailed characterization of the polar vortex breakdown includes investigations of individual offspring vortices and the origins and fate of air within them. Comparisons of mixing diagnostics with lower-stratospheric N2O and middle-stratospheric CO from MLS (long-lived tracers) show rapid vortex erosion and extensive mixing during and immediately after the split in mid-March; however, air in the resulting offspring vortices remained isolated until they disappeared. Although the offspring vortices in the lower stratosphere survived longer than those in the middle stratosphere, the rapid temperature increase and dispersal of chemically processed air caused active chlorine to quickly disappear. Furthermore, ozone-depleted air from the lower-stratospheric vortex core was rapidly mixed with ozone rich air from the vortex edge and midlatitudes during the split. The impact of the 2016 MFW on polar processing was the latest in a series of unexpected events that highlight the diversity of potential consequences of sudden warming events for Arctic ozone loss.


2020 ◽  
Vol 12 (23) ◽  
pp. 3950
Author(s):  
Yu Shi ◽  
Valerii Shulga ◽  
Oksana Ivaniha ◽  
Yuke Wang ◽  
Oleksandr Evtushevsky ◽  
...  

In this paper, a comparison of the impact of major sudden stratospheric warmings (SSWs) in the Arctic in February 2018 (SSW1) and January 2019 (SSW2) on the mid-latitude mesosphere is given. The mesospheric carbon monoxide (CO) and zonal wind in these two major SSW events were observed at altitudes of 70–85 km using a microwave radiometer (MWR) at Kharkiv, Ukraine (50.0°N, 36.3°E). Data from ERA-Interim and MERRA-2 reanalyses and Aura Microwave Limb Sounder measurements were also used. It is shown that: (i) The differences between SSW1 and SSW2, in terms of local variability in zonal wind, temperature, and CO in the stratosphere and mesosphere, were clearly defined by the polar vortex (westerly in cyclonic circulation) and mid-latitude anticyclone (easterly) migrating over the MWR station, therefore; (ii) mesospheric intrusions of CO-rich air into the stratosphere over the Kharkiv region occurred only occasionally, (iii) the larger zonal wave 1–3 amplitudes before SSW1 were followed by weaker polar vortex recovery than that after SSW2, (iv) the strong vortex recovery after SSW2 was supported by earlier event timing (midwinter) favoring vortex cooling due to low solar irradiance and enhanced zonal circulation, and (v) vortex strengthening after SSW2 was accompanied by wave 1–3 amplification in March 2019, which was absent after SSW1. Finally, the influence of the large-scale circulation structures formed in individual major SSW events on the locally recorded characteristics of the atmosphere is discussed.


2021 ◽  
Author(s):  
Sina Mehrdad ◽  
Khalil Karami ◽  
Dörthe Handorf ◽  
Johannes Quaas ◽  
Ines Höschel ◽  
...  

<p>The global warming has been observed to be more severe in the Arctic compared to the rest of the world. This enhanced warming i.e. Arctic Amplification is not just the result of local feedback processes in the Arctic. The stratospheric pathways of Arctic-midlatitude linkages and large-scale dynamical processes can contribute to the Arctic Amplification. The polar stratospheric dynamics crucially depends on the atmospheric waves at all scales. The winter polar vortex can be disturbed by gravity waves in the middle atmosphere. To investigate the sensitivity of the polar vortex dynamics, large-scale dynamical processes, and the stratospheric pathways of the Arctic-midlatitude linkages to the modification of gravity wave drag, we conduct sensitivity experiments using the global atmospheric model ICON-NWP (ICOsahedral Nonhydrostatic Model for Numerical Weather Prediction). These sensitivity experiments are performed by imposing a repeated annual cycle of the year 1986 for sea surface temperatures and sea ice as lower boundary conditions and for greenhouse gas concentrations as external forcing. This year is selected as both El-Nino Southern Oscillation and Pacific decadal oscillation were in their neutral phase and no explosive volcanic eruption has occurred. Hence, lower boundary and external forcing conditions in this year can serve as a useful proxy for the multi-year mean condition and an estimate of its internal variability. We performed simulations where in the control simulation the sub-grid parameterization scheme for both orographic and non-orographic gravity wave drags are switched on. The other two experiments are identical to the control simulation except that either orographic or non-orographic gravity wave drags are switched off.</p> <p>Recently, deep learning has extraordinarily progressed our ability to recognize complex patterns in big datasets. Deep neural networks have shown great capabilities to capture the dynamical process of the atmosphere. Applying deep learning algorithms on experiments’ results, the impact of gravity wave drag modifications on large-scale mechanisms of the Arctic Amplification will be analyzed. Special emphasis will be put on the effects of gravity wave drag modifications on the polar vortex dynamics.</p>


2016 ◽  
Author(s):  
Gloria L. Manney ◽  
Zachary D. Lawrence

Abstract. The 2015/16 Northern Hemisphere winter stratosphere appeared to have the greatest potential yet seen for record Arctic ozone loss. Temperatures in the Arctic lower stratosphere were at record lows from December 2015 through early February 2016, with an unprecedented period of temperatures below ice polar stratospheric cloud thresholds. Trace gas measurements from the Aura Microwave Limb Sounder (MLS) show that exceptional denitrification and dehydration, as well as extensive chlorine activation, occurred throughout the polar vortex. Ozone decreases in 2015/16 began earlier and proceeded more rapidly than those in 2010/11, a winter that saw unprecedented Arctic ozone loss. However, on 5–6 March 2016 a major final sudden stratospheric warming (“major final warming”, MFW) began. By mid-March, the mid-stratospheric vortex split after being displaced far off the pole. The resulting offspring vortices decayed rapidly preceding the full breakdown of the vortex by early April. In the lower stratosphere, the period of temperatures low enough for chlorine activation ended nearly a month earlier than that in 2011 because of the MFW. Ozone loss rates were thus kept in check because there was less sunlight during the cold period. And although the winter mean volume of air in which chemical ozone loss could occur was as large as that in 2010/11, net chemical ozone loss was considerably less. We use MLS trace gas measurements, as well as mixing and polar vortex diagnostics based on meteorological fields, to show how the timing and intensity of the MFW and its impact on transport and mixing halted chemical ozone loss. Our detailed characterization of the polar vortex breakdown includes investigations of individual offspring vortices and the origins and fate of air within them. Comparisons of mixing diagnostics with lower stratospheric N2O and middle stratospheric CO from MLS (long-lived tracers) show rapid vortex erosion and extensive mixing during and immediately after the split in mid-March; however, air in the resulting offspring vortices remained isolated until they disappeared. Although the offspring vortices in the lower stratosphere survived longer than those in the middle stratosphere, the rapid temperature increase and dispersal of chemically-processed air caused active chlorine to quickly disappear. Furthermore, ozone-depleted air from the lower stratospheric vortex core was rapidly mixed with ozone rich air from the vortex edge and midlatitudes during the split. The impact of the 2016 MFW on polar processing was the latest in a series of unexpected events that highlight the diversity of potential consequences of sudden warming events for Arctic ozone loss.


2003 ◽  
Vol 3 (3) ◽  
pp. 2261-2284
Author(s):  
M. M. P. van den Broek ◽  
M. K. van Aalst ◽  
A. Bregman ◽  
M. Krol ◽  
J. Lelieveld ◽  
...  

Abstract. We have used a 3D chemistry transport model to evaluate the transport of HF and CH4 in the stratosphere during the Arctic winter of 1999/2000. Several model experiments were carried out with the use of a zoom algorithm to investigate the effect of different horizontal resolutions. Balloon-borne and satellite-borne observations of HF and CH4 were used to test the model. In addition, air mass descent rates within the polar vortex were calculated and compared to observations. Outside the vortex the model results agree well with the observations, but inside the vortex the model underestimates the observed vertical gradient in HF and CH4, even when the highest available resolution (1°×1°) is applied. The calculated diabatic descent rates agree with observations above potential temperature levels of 450 K. These model results suggest that too strong mixing through the vortex edge could be a plausible cause for the model discrepancies, associated with the calculated mass fluxes, although other reasons are also discussed. Based on our model experiments we conclude that a global 6°×9° resolution is too coarse to represent the polar vortex, whereas the higher resolutions, 3°×2° and 1°×1°, yield similar results, even with a 6°×9° resolution in the tropical region.


Atmosphere ◽  
2021 ◽  
Vol 12 (4) ◽  
pp. 454
Author(s):  
Andrew R. Jakovlev ◽  
Sergei P. Smyshlyaev ◽  
Vener Y. Galin

The influence of sea-surface temperature (SST) on the lower troposphere and lower stratosphere temperature in the tropical, middle, and polar latitudes is studied for 1980–2019 based on the MERRA2, ERA5, and Met Office reanalysis data, and numerical modeling with a chemistry-climate model (CCM) of the lower and middle atmosphere. The variability of SST is analyzed according to Met Office and ERA5 data, while the variability of atmospheric temperature is investigated according to MERRA2 and ERA5 data. Analysis of sea surface temperature trends based on reanalysis data revealed that a significant positive SST trend of about 0.1 degrees per decade is observed over the globe. In the middle latitudes of the Northern Hemisphere, the trend (about 0.2 degrees per decade) is 2 times higher than the global average, and 5 times higher than in the Southern Hemisphere (about 0.04 degrees per decade). At polar latitudes, opposite SST trends are observed in the Arctic (positive) and Antarctic (negative). The impact of the El Niño Southern Oscillation phenomenon on the temperature of the lower and middle atmosphere in the middle and polar latitudes of the Northern and Southern Hemispheres is discussed. To assess the relative influence of SST, CO2, and other greenhouse gases’ variability on the temperature of the lower troposphere and lower stratosphere, numerical calculations with a CCM were performed for several scenarios of accounting for the SST and carbon dioxide variability. The results of numerical experiments with a CCM demonstrated that the influence of SST prevails in the troposphere, while for the stratosphere, an increase in the CO2 content plays the most important role.


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