A flexible, lightweight and stretchable all-solid-state supercapacitor based on warp-knitted stainless-steel mesh for wearable electronics

Highly conductive, flexible, stretchable and lightweight electrode substrates are essential to meet the future demand on supercapacitors for wearable electronics. However, it is difficult to achieve the above characteristics simultaneously. In this study, ultrafine stainless-steel fibers (with a diameter of ≈30 μm) are knitted into stainless-steel meshes (SSMs) with a diamond structure for the fabrication of textile stretchable electrodes and current collectors. The electrodes are fabricated by utilizing an electrodeposited three-dimensional network graphene framework and poly(3,4-ethylenedioxythiophene) (PEDOT) coating on the SSM substrates via a two-step electrodeposition process, which show a specific capacitance of 77.09 F g−1 (0.14 A g−1) and superb cycling stability (91% capacitance retention after 5000 cycles). Furthermore, the assembled flexible stretchable supercapacitor based on the PEDOT/reduced graphene oxide (RGO)@SSM electrodes exhibits an areal capacitance (53 mF cm−2 at 0.1 mA cm−2), a good cycling stability (≈73% capacitance retention after 5000 cycles), rate capability (36 mF cm−2 at 5 mA cm−2), stretchable stability (≈78% capacitance retention at 10% strain for 500 stretching cycles) and outstanding flexibility and stability under various bending deformations. The assembled supercapacitors can illuminate a thermometer and a light-emitting diode, demonstrating their potential application as stretchable supercapacitors. This simple and low-cost method developed for fabricating lightweight, stretchable and stable high-performance supercapacitors offers new opportunities for future stretchable electronic devices.

A Review of Fabrication Technologies for Carbon Electrode-Based Micro-Supercapacitors

The very fast evolution in wearable electronics drives the need for energy storage micro-devices, which have to be flexible. Micro-supercapacitors are of high interest because of their high power density, long cycle lifetime and fast charge and discharge. Recent developments on micro-supercapacitors focus on improving the energy density, overall electrochemical performance, and mechanical properties. In this review, the different types of micro-supercapacitors and configurations are briefly introduced. Then, the advances in carbon electrode materials are presented, including activated carbon, carbon nanotubes, graphene, onion-like carbon, and carbide-derived carbon. The different types of electrolytes used in studies on micro-supercapacitors are also treated, including aqueous, organic, ionic liquid, solid-state, and quasi-solid-state electrolytes. Furthermore, the latest developments in fabrication techniques for micro-supercapacitors, such as different deposition, coating, etching, and printing technologies, are discussed in this review on carbon electrode-based micro-supercapacitors.

Observation of localized magnetic plasmon skyrmions

Optical skyrmions have recently been constructed by tailoring vectorial near-field distributions through the interference of multiple surface plasmon polaritons, offering promising features for advanced information processing, transport and storage. Here, we provide experimental demonstration of electromagnetic skyrmions based on magnetic localized spoof plasmons (LSP) showing large topological robustness against continuous deformations, without stringent external interference conditions. By directly measuring the spatial profile of all three vectorial magnetic fields, we reveal multiple π-twist target skyrmion configurations mapped to multi-resonant near-equidistant LSP eigenmodes. The real-space skyrmion topology is robust against deformations of the meta-structure, demonstrating flexible skyrmionic textures for arbitrary shapes. The observed magnetic LSP skyrmions pave the way to ultra-compact and robust plasmonic devices, such as flexible sensors, wearable electronics and ultra-compact antennas.

Flexible Capacitive Pressure Sensors with Micro-Patterned Porous Dielectric Layer for Wearable Electronics

Highly sensitive soft sensors play key roles in flexible electronics, which therefore have attracted much attention in recent years. Herein, we report a flexible capacitive pressure sensor with high sensitivity by using engineered micro-patterned porous polydimethylsiloxane (PDMS) dielectric layer through an environmental-friendly fabrication procedure. The porous structure is formed by evaporation of emulsified water droplets during PDMS curing process, while the micro-patterned structure is obtained via molding on sandpaper. Impressively, this structure renders the capacitive sensor with a high sensitivity up to 143.5 MPa-1 at the pressure range of 0.068~150 kPa and excellent anti-fatigue performance over 20,000 cycles. Meanwhile, the sensor can distinguish different motions of the same person or different people doing the same action. Our work illustrates the promising application prospects of this flexible pressure sensor for the security field or human motion monitoring area.

In-situ Formation of Co3O4 Nanocrystals Embedded in Laser-Induced Graphene Foam for High-Energy Flexible Micro-supercapacitor

The cost-effective synthesis of flexible energy storage devices with high energy and power densities is a challenge in wearable electronics. Here, we report a facile, efficient, and scalable approach for...

Flexible Capacitive Pressure Sensors for Wearable Electronics

Flexible pressure sensors have attracted more and more attention recently due to their broad applications, such as electronic skin and wearable electronics for health monitoring. Among them, capacitive flexible pressure...

Ubiquitous clean and sustainable energy-driven self-rechargeable batteries realized by and used in organic electronics

Organic electronics have the advantages of low manufacturing cost, light weight, good flexibility, and good conformity to different surfaces. They are ideal for many emerging applications such as wearable electronics,...