total scattering
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2021 ◽  
Vol 7 (1) ◽  
pp. 2
Author(s):  
Kenichi Kato ◽  
Kazuya Shigeta

The total scattering method, which is based on measurements of both Bragg and diffuse scattering on an equal basis, has been still challenging even by means of synchrotron X-rays. This is because such measurements require a wide coverage in scattering vector Q, high Q resolution, and a wide dynamic range for X-ray detectors. There is a trade-off relationship between the coverage and resolution in Q, whereas the dynamic range is defined by differences in X-ray response between detector channels (X-ray response non-uniformity: XRNU). XRNU is one of the systematic errors for individual channels, while it appears to be a random error for different channels. In the present study, taking advantage of the randomness, the true sensitivity for each channel has been statistically estimated. Results indicate that the dynamic range of microstrip modules (MYTHEN, Dectris, Baden-Daettwil, Switzerland), which have been assembled for a total scattering measurement system (OHGI), has been successfully restored from 104 to 106. Furthermore, the correction algorithm has been optimized to increase time efficiencies. As a result, the correcting time has been reduced from half a day to half an hour, which enables on-demand correction for XRNU according to experimental settings. High-precision X-ray total scattering measurements, which has been achieved by a high-accuracy detector system, have demonstrated valence density studies from powder and PDF studies for atomic displacement parameters.


2021 ◽  
pp. 117590
Author(s):  
Devon Drey ◽  
Eric O'Quinn ◽  
Sarah Finkeldei ◽  
Joerg Neuefeind ◽  
Maik Lang

2021 ◽  
Vol 77 (6) ◽  
pp. 611-636
Author(s):  
Robert J. Koch ◽  
Nikolaj Roth ◽  
Yiu Liu ◽  
Oleh Ivashko ◽  
Ann-Christin Dippel ◽  
...  

Data reduction and correction steps and processed data reproducibility in the emerging single-crystal total-scattering-based technique of three-dimensional differential atomic pair distribution function (3D-ΔPDF) analysis are explored. All steps from sample measurement to data processing are outlined using a crystal of CuIr2S4 as an example, studied in a setup equipped with a high-energy X-ray beam and a flat-panel area detector. Computational overhead as pertains to data sampling and the associated data-processing steps is also discussed. Various aspects of the final 3D-ΔPDF reproducibility are explicitly tested by varying the data-processing order and included steps, and by carrying out a crystal-to-crystal data comparison. Situations in which the 3D-ΔPDF is robust are identified, and caution against a few particular cases which can lead to inconsistent 3D-ΔPDFs is noted. Although not all the approaches applied herein will be valid across all systems, and a more in-depth analysis of some of the effects of the data-processing steps may still needed, the methods collected herein represent the start of a more systematic discussion about data processing and corrections in this field.


2021 ◽  
Vol 28 (5) ◽  
Author(s):  
V. I. Mankovsky ◽  
E. V. Mankovskaya ◽  
◽  

Purpose. The aim of the work is to study relationships between the parameters of the light volume scattering functions based on the data of their measurements in the Mediterranean Sea surface waters. Methods and Results. The data of measurements of the light volume scattering functions in the water samples taken in a few regions of the southern Mediterranean Sea, namely from the Strait of Gibraltar to the Levant Sea, as well as in the central part of the Aegean Sea and near the Dardanelles Strait (May, 1998) were used. The following parameters of the volume scattering functions were calculated: total scattering coefficient, and asymmetry and variation coefficients. The maximum and minimum values of the scattering coefficient were 0.21 and 0.09 m–1, respectively; and those for the asymmetry coefficient – 77.8 and 33.9. The variation coefficient of the angle scattering coefficients changed within 35–79%, its maximum and minimum values fell on the angles 7.5° and 162.5°, respectively. Obtained were the relations between the variation coefficient and the scattering angle, the asymmetry coefficient and the scattering coefficient, and the angle scattering coefficients and the total scattering coefficient. All of them possess high (more than 0.9) correlation coefficients. The coefficient value (51.7%) at the angle 2° does not correspond to general relation of the variation coefficient to the scattering angle. This fact is explained by different contributions of coarse and fine suspended matter to the light volume scattering function. At the angle 2°, the main contribution is made by a coarse (organic) suspended matter, whereas at the angles exceeding 7.5° – by a fine (mineral) suspension. Conclusions. The values of the variation coefficient of the angle scattering coefficient at the angles equal to 2° and exceeding 7.5° demonstrate variability of the coarse and fine suspended matter in the Mediterranean Sea, respectively. The equation for the relation between the asymmetry coefficient of the light volume scattering functions and the total scattering coefficient obtained for the Mediterranean Sea waters is close to the analogous one obtained for the Atlantic Ocean tropical waters. The angle 3.5° is optimal for determining the total scattering coefficient using the angle scattering coefficient for the Mediterranean Sea functions.


2021 ◽  
Vol 54 (5) ◽  
pp. 1542-1545
Author(s):  
Peter F. Peterson ◽  
David A. Keen

Errors and ambiguities in the article by Peterson, Olds, McDonnell & Page [J. Appl. Cryst. (2021), 54, 317–332] are corrected and clarified, respectively.


2021 ◽  
Vol 263 (3) ◽  
pp. 3511-3522
Author(s):  
Linwei Zhuo ◽  
Feruza Amirkulova

Metamaterials are engineered composites that can achieved electromagnetic and mechanical properties that do not exist in natural materials by rearranging their structures. Due to the complexity of the objective functions, it is difficult to find the globally optimized solutions in metameterial design. This talk outlines a gradient-based optimization with generative networks that can search for the globally optimized cloaking devices over a wide range of parameters. The GLO-Net[1] model was developed originally for one-dimensional nano-photonic metagratings is generalized in this work to design two-dimensional broadband acoustic cloaking devices by perturbing positions of each scatterer in planar configuration of cylindrical scatterers. Such optimized cloaking devices can efficiently suppress the total scattering cross section to the minimum at certain parameters over range of wavenumbers. During training each iteration, a generative model generates a batch of metamaterials and compute the total scattering cross section and its gradients using an in-house built multiple scattering MATLAB solver. To evaluate our approach, we compare our obtained results with fmincon in MATLAB. Reference: [1] Jiaqi Jiang and Jonathan A. Fan. Simulator-based training of generative neural networks for the inverse design of metasurfaces. Nanophotonics, 9(5):1059-1069, nov 2019.


2021 ◽  
Vol 77 (a1) ◽  
pp. a270-a270
Author(s):  
Katharine Page ◽  
Peter Metz ◽  
Thomas Huegle ◽  
George Renich ◽  
Van Graves ◽  
...  
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