Rainfall Investigation by Means of Marine In Situ Gamma-ray Spectrometry in Ligurian Sea, Mediterranean Sea, Italy

Marine in situ gamma-ray spectrometry was utilized for a rainfall study at the W1M3A observing system in Ligurian Sea, Mediterranean Sea, Italy. From 7 June to 10 October 2016, underwater total gamma-ray counting rate (TCR) and the activity concentration of radon daughters 214Pb, 214Bi and potassium 40K were continuously monitored along with ambient noise and meteorological parameters. TCR was proven as a good rainfall indicator as radon daughters’ fallout resulted in increased levels of marine radioactivity during and 2–3 h after the rainfall events. Cloud origin significantly affects TCR and radon progenies variations, as aerial mass trajectories, which extend upon terrestrial areas, result in higher increments. TCR and radon progenies concentrations revealed an increasing non-linear trend with rainfall height and intensity. 40K was proven to be an additional radio-tracer as its dilution was associated with rainfall height. 40K variations combined with 214Bi measurements can be used to investigate the mixing of rain- and seawater. In comparison with measurements in the atmosphere, the application of marine in situ gamma-ray spectrometry for precipitation investigation provided important advantages: allows quantitative measurement of the radionuclides; 40K can be used, along with radon daughters, as a radio-tracer; the mixing of rain- and seawater can be associated with meteorological parameters.

Radon daughter removal from PTFE surfaces and its application in liquid xenon detectors

Long-lived radon daughters are a critical background source in experiments searching for low-energy rare events. Originating from radon in ambient air, radioactive polonium, bismuth and lead isotopes plate-out on materials that are later employed in the experiment. In this paper, we examine cleaning procedures for their capability to remove radon daughters from PTFE surfaces, a material often used in liquid xenon TPCs. We find a large difference between the removal efficiency obtained for the decay chains of $$^{222}$$ 222 Rn and $$^{220}$$ 220 Rn. This indicates that the plate-out mechanism has an effect on the cleaning success. While the long-lived $$^{222}$$ 222 Rn daughters can be reduced by a factor of 2, the removal of $$^{220}$$ 220 Rn daughters is up to 10 times more efficient depending on the treatment. Furthermore, the impact of a nitric acid based PTFE cleaning on the liquid xenon purity is investigated in a small-scale liquid xenon TPC.

The LUX-ZEPLIN (LZ) radioactivity and cleanliness control programs

LUX-ZEPLIN (LZ) is a second-generation direct dark matter experiment with spin-independent WIMP-nucleon scattering sensitivity above $${1.4 \times 10^{-48}}\, {\hbox {cm}}^{2}$$ 1.4 × 10 - 48 cm 2 for a WIMP mass of $${40}\, \hbox {GeV}/{\hbox {c}}^{2}$$ 40 GeV / c 2 and a $${1000}\, \hbox {days}$$ 1000 days exposure. LZ achieves this sensitivity through a combination of a large $${5.6}\, \hbox {t}$$ 5.6 t fiducial volume, active inner and outer veto systems, and radio-pure construction using materials with inherently low radioactivity content. The LZ collaboration performed an extensive radioassay campaign over a period of six years to inform material selection for construction and provide an input to the experimental background model against which any possible signal excess may be evaluated. The campaign and its results are described in this paper. We present assays of dust and radon daughters depositing on the surface of components as well as cleanliness controls necessary to maintain background expectations through detector construction and assembly. Finally, examples from the campaign to highlight fixed contaminant radioassays for the LZ photomultiplier tubes, quality control and quality assurance procedures through fabrication, radon emanation measurements of major sub-systems, and bespoke detector systems to assay scintillator are presented.

A technology of drinking water decontamination from radon and its decay products

Underground water is one of the main sources of radon for households. This article focuses on the estimation and removal of radon from underground water using the technology and inorganic sorbents developed by EKSORB Ltd., Russia for liquid radioactive waste treatment in the nuclear power industry. The article presents the results of tests of a system for the removal of radon and radon daughters from water patented by EKSORB. This is achieved by filtering water through RATZIR sorbent, followed by periodic load regeneration. Over a period of three years, the plant is successful in removing radon from the water that had an initial radon content of approximately 1500 Bq/L to less than 60 Bq/L, without releasing radon to indoor/outdoor air.

Radon Gas Profiles and Exposure Estimates in the Perama Cave, Greece

An investigation of atmospheric radon levels in the Perama Cave, North-western Greece, has been carried out using CR-39 detectors. The detectors were placed at various locations along the guided cave pathway and exposed during different sampling periods. Mean concentrations amounting to 925±418 and 1311±352 Bq m-3 were recorded in the summer and winter months, respectively. The quantification of effective doses from radon daughters' inhalation was important, as the Perama Cave is one of the most popular in Greece, attracting more than 85,000 tourists per year. Due to the short duration of the guided tour along the cave, exposure of tourists was found to be insignificant, lying below 5.1 μSv per visit. Permanent cave guides receive doses ranging from 4.2 to 5.9 mSv y-1. Considering the ICRP-65 recommendation that action levels in dwellings and workplaces should be set between 3 and 10 mSv y-1 untertaking remedial measures to reduce the exposure of cave staff may be appropriate.

Gamma spectroscopy methodology for large amounts of environmental samples in Sweden 30 years after the Chernobyl accident

In a Swedish citizen science project, more than 200 elementary school classes participated in collecting fungi, soil samples, and droppings from deer and wild boar, from all over Sweden. The samples have been sent to a laboratory at Uppsala University where they are being analyzed through gamma spectroscopy with a shielded HPGe detector. The main objective is to scan the samples for 137Cs from the Chernobyl accident and compare the data with measurements from 1986, but uptake of naturally occuring radionuclides like 40K and radon daughters will also be determined. Together with the soil samples, transfer factors will be derived, and correlations for these factors will be sought for different species of fungi and soil types. The potential for correlating the results with different biological processes will also be investigated, in part through the collected animal droppings. This is a work in progress where the present status of the experimental setup and methodology are presented. Issues with the initial approach for corrections are discussed and preliminary results are presented.

Vertical distribution of 137Cs and natural radioactivity in core sediments of Thermaikos Gulf, northwestern Aegean Sea

Sub-superficial sediments have been collected from the Thermaikos Gulf, located in the NW Aegean Sea, in order to determine sedimentation rates using vertical distributions of 137Cs and 210Pb. In addition measurements of the characteristic radionuclides of the 238U and 232Th natural series has also been performed to better understand the transport and the sedimentation process in a marine environment, which is strongly influenced by the main North Greece rivers. The sedimentation rates of the five selected cores using the two methods were consistent and varied from 0.20 ± 0.01 till 0.30 ± 0.02 cm y-1. The mean sedimentation rates derived with both methods are enhanced during the last ten years compared to previous values at the studied region by one order of magnitude, due to human implications. The activity concentration of the 238U decay products does not exhibit variation along the depth. The activities of 226Ra are enhanced (~30 %) compared to the activities of radon daughters (214Pb, 214Bi) especially at the surface layer. The results of the correlation between 232Th decay products and 40K indicate that there is positive correlation between their averaged activities. The good proportionality between 232Th and 40K concentrations may be attributed to the fact that thorium is a particularly insoluble element in water.