scholarly journals Characterizing polar atmospheres and their effect on Rayleigh-scattering optical depth

2010 ◽  
Vol 115 (D2) ◽  
Author(s):  
Claudio Tomasi ◽  
Boyan Petkov ◽  
Robert S. Stone ◽  
Elena Benedetti ◽  
Vito Vitale ◽  
...  
2013 ◽  
Vol 70 (1) ◽  
pp. 317-329 ◽  
Author(s):  
M. Sikand ◽  
J. Koskulics ◽  
K. Stamnes ◽  
B. Hamre ◽  
J. J. Stamnes ◽  
...  

Abstract Microphysical and radiative measurements in boundary layer mixed-phase clouds (MPCs), consisting of ice crystals and liquid droplets, have been analyzed. These cloud measurements were collected during a May–June 2008 tethered-balloon campaign in Ny-Ålesund, Norway, located at 78.9°N, 11.9°E in the High Arctic. The instruments deployed on the tethered-balloon platform included a radiometer, a cloud particle imager (CPI), and a meteorological package. To analyze the data, a radiative transfer model (RTM) was constructed with two cloud layers—consistent with the CPI data—embedded in a background Rayleigh scattering atmosphere. The mean intensities estimated from the radiometer measurements on the balloon were used in conjunction with the RTM to quantify the vertical structure of the MPC system, while the downward irradiances measured by an upward-looking ground-based radiometer were used to constrain the total cloud optical depth. The time series of radiometer and CPI data obtained while profiling the cloud system was used to estimate the time evolution of the liquid water and ice particle optical depths as well as the vertical location of the two cloud layers.


2018 ◽  
Vol 176 ◽  
pp. 08008
Author(s):  
Daniela Viviana Vlăduţescu ◽  
Stephen E. Schwartz ◽  
Dong Huang

Optically thin clouds have a strong radiative effect and need to be represented accurately in climate models. Cloud optical depth of thin clouds was retrieved using high resolution digital photography, lidar, and a radiative transfer model. The Doppler Lidar was operated at 1.5 μm, minimizing return from Rayleigh scattering, emphasizing return from aerosols and clouds. This approach examined cloud structure on scales 3 to 5 orders of magnitude finer than satellite products, opening new avenues for examination of cloud structure and evolution.


2021 ◽  
Author(s):  
Henri Diémoz ◽  
Anna Maria Siani ◽  
Stefano Casadio ◽  
Anna Maria Iannarelli ◽  
Giuseppe Rocco Casale ◽  
...  

Abstract. A re-evaluated data set of nitrogen dioxide (NO2) column densities over Rome for the years 1996 to 2017 is here presented. This long-term record is obtained from ground-based direct sun measurements with a MkIV Brewer spectrophotometer (#067), further reprocessed using a novel algorithm. Compared to the original Brewer algorithm, the new method includes updated NO2 absorption cross sections and Rayleigh scattering coefficients, and accounts for additional atmospheric compounds and instrumental artefacts, such as the spectral transmittance of the filters, the alignment of the wavelength scale and internal temperature. Moreover, long-term changes in the Brewer radiometric sensitivity are tracked using statistical methods for in-field calibration. The resulting series presents only few (about 30) periods with missing data longer than one week and features NO2 retrievals in more than 6100 days, covering nearly 80 % of the considered 20-year period. The high quality of the data is demonstrated by two independent comparisons. In a first intensive campaign, Brewer #067 is compared against another Brewer (#066), recently calibrated at the Izaña Atmospheric Observatory through the Langley method and there compared to reference instrumentation from the Network for the Detection of Atmospheric Composition Change (NDACC). Data from this campaign show a highly significant Pearson's correlation coefficient of 0.90 between the two series of slant column densities, slope 0.98 and offset 0.05 DU (1.3 × 1015 molec cm−2). The average bias between the vertical column densities is 0.03 DU (8.1 ×1014 molec cm−2), well within the combined uncertainty of both instruments. Brewer #067 is also independently compared with new-generation instrumentation, a co-located Pandora spectrometer (#117), over a 1-year long period (2016–2017) at Sapienza University of Rome, showing linear correlation indices above 0.96 between slant column densities, slope of 0.97 and offset of 0.02 DU (5.4 × 1014 molec cm−2). The average bias between vertical column densities is negligible (−0.002 DU or −5.4 × 1013 molec cm−2). This, incidentally, represents the first intercomparison of NO2 retrievals between a MkIV Brewer and a Pandora instrument. Owing to its accuracy and length, the Brewer data set collected in Rome can be useful for satellite cal/val exercises, comparison with photochemical models, and for better aerosol optical depth estimates (NO2 optical depth climatology). In addition, it can be employed to identify long-term trends in NO2 column densities over a metropolitan environment, during two decades witnessing important changes in environmental policies, emission loads and composition, and the effect of a worldwide economic recession, to offer just a few examples. The method can be replicated on the more than 80 MkIV spectrophotometers operating worldwide in the frame of the international Brewer network. The NO2 data set described in this manuscript can be freely accessed at https://doi.org/10.5281/zenodo.4715219 (Diémoz and Siani, 2021).


2013 ◽  
Vol 30 (5) ◽  
pp. 929-941 ◽  
Author(s):  
Hao Zhang ◽  
Bing Zhang ◽  
Dongmei Chen ◽  
Junsheng Li ◽  
Guangning Zhao

Abstract Beer’s attenuation law is the basis for the retrieval of aerosol optical depth (AOD) from sunphotometer data. However, the filter band function causes uncertainty during the retrieval of AOD from sunphotometer data, particularly for channels covering spectral regions of strong gas absorption. In this work, the uncertainty in AOD retrieval due to the filter band function is systematically analyzed by employing fine spectral absorption cross sections obtained from the Molecular Spectroscopy and Chemical Kinetics Group and the line-by-line radiative transfer model (LBLRTM). The uncertainty in AOD retrieval includes the uncertainty due to the wings of the filter band function in the ultraviolet (UV) region and errors in the optical depth calculation for Rayleigh scattering and absorption of O3, NO2, H2O, CH4, and CO2. The results showed that 1) the uncertainty of AOD retrieval by this method, which is called the approximate AOD retrieval method, might become large when the filter band function is not well designed, particularly in the UV region; 2) in the case of a large zenith observation condition, the errors will be nonnegligible if the Rayleigh scattering optical depth is calculated at a central wavelength without including filter band function; 3) the band-weighted absorption coefficients of O3 and NO2 remain nearly constant when the gas amounts change, except in the case of questionably designed band filters; and 4) these weak-absorption optical depths for H2O, CH4, and CO2 cannot be ignored in the 1020- or 1640-nm channels, where an optical depth error of 0.01−0.02 may be introduced.


2020 ◽  
Vol 86 (12) ◽  
pp. 767-774
Author(s):  
Wei Chen ◽  
Ge Song ◽  
Haozhong Wang ◽  
Haimeng Zhao ◽  
Jianfang Zhu ◽  
...  

Sky polarization patterns are a relatively new and interesting field of polarized remote sensing. However, most current research mainly focuses on Rayleigh scattering or different conditions of aerosol optical depth. In this study, the sky downward polarization patterns are calculated for both degree of linear polarization and angle of polarization with scattering and absorbing aerosol situations. When coarse-mode aerosol changes from scattering to absorbing, the decreasing trend in the sky downward degree-of-linear-polarization largely slows down when aerosol optical depth increases. For fine-mode aerosol, on the other hand, the change of pattern is not sensitive to the absorbing property of aerosol. Sky downward angle-of-polarization patterns for different levels of aerosol optical depth and aerosol modes are similar, with little change. The results suggest that in order to accurately use sky polarization for remote sensing or bionic navigation, it is necessary to characterize aerosol microphysical properties first, especially when coarse absorbing aerosol exists.


2019 ◽  
Vol 12 (8) ◽  
pp. 4309-4337 ◽  
Author(s):  
Emilio Cuevas ◽  
Pedro Miguel Romero-Campos ◽  
Natalia Kouremeti ◽  
Stelios Kazadzis ◽  
Petri Räisänen ◽  
...  

Abstract. A comprehensive comparison of more than 70 000 synchronous 1 min aerosol optical depth (AOD) data from three Global Atmosphere Watch precision-filter radiometers (GAW-PFR), traceable to the World AOD reference, and 15 Aerosol Robotic Network Cimel radiometers (AERONET-Cimel), calibrated individually with the Langley plot technique, was performed for four common or “near” wavelengths, 380, 440, 500 and 870 nm, in the period 2005–2015. The goal of this study is to assess whether, despite the marked technical differences between both networks (AERONET, GAW-PFR) and the number of instruments used, their long-term AOD data are comparable and consistent. The percentage of data meeting the World Meteorological Organization (WMO) traceability requirements (95 % of the AOD differences of an instrument compared to the WMO standards lie within specific limits) is >92 % at 380 nm, >95 % at 440 nm and 500 nm, and 98 % at 870 nm, with the results being quite similar for both AERONET version 2 (V2) and version 3 (V3). For the data outside these limits, the contribution of calibration and differences in the calculation of the optical depth contribution due to Rayleigh scattering and O3 and NO2 absorption have a negligible impact. For AOD >0.1, a small but non-negligible percentage (∼1.9 %) of the AOD data outside the WMO limits at 380 nm can be partly assigned to the impact of dust aerosol forward scattering on the AOD calculation due to the different field of view of the instruments. Due to this effect the GAW-PFR provides AOD values, which are ∼3 % lower at 380 nm and ∼2 % lower at 500 nm compared with AERONET-Cimel. The comparison of the Ångström exponent (AE) shows that under non-pristine conditions (AOD >0.03 and AE <1) the AE differences remain <0.1. This long-term comparison shows an excellent traceability of AERONET-Cimel AOD with the World AOD reference at 440, 500 and 870 nm channels and a fairly good agreement at 380 nm, although AOD should be improved in the UV range.


2017 ◽  
Vol 10 (2) ◽  
pp. 709-730 ◽  
Author(s):  
Jonas Witthuhn ◽  
Hartwig Deneke ◽  
Andreas Macke ◽  
Germar Bernhard

Abstract. The 19-channel rotating shadowband radiometer GUVis-3511 built by Biospherical Instruments provides automated shipborne measurements of the direct, diffuse and global spectral irradiance components without a requirement for platform stabilization. Several direct sun products, including spectral direct beam transmittance, aerosol optical depth, Ångström exponent and precipitable water, can be derived from these observations. The individual steps of the data analysis are described, and the different sources of uncertainty are discussed. The total uncertainty of the observed direct beam transmittances is estimated to be about 4 % for most channels within a 95 % confidence interval for shipborne operation. The calibration is identified as the dominating contribution to the total uncertainty. A comparison of direct beam transmittance with those obtained from a Cimel sunphotometer at a land site and a manually operated Microtops II sunphotometer on a ship is presented. Measurements deviate by less than 3 and 4 % on land and on ship, respectively, for most channels and in agreement with our previous uncertainty estimate. These numbers demonstrate that the instrument is well suited for shipborne operation, and the applied methods for motion correction work accurately. Based on spectral direct beam transmittance, aerosol optical depth can be retrieved with an uncertainty of 0.02 for all channels within a 95 % confidence interval. The different methods to account for Rayleigh scattering and gas absorption in our scheme and in the Aerosol Robotic Network processing for Cimel sunphotometers lead to minor deviations. Relying on the cross calibration of the 940 nm water vapor channel with the Cimel sunphotometer, the column amount of precipitable water can be estimated with an uncertainty of ±0.034 cm.


1997 ◽  
Vol 163 ◽  
pp. 461-464
Author(s):  
O. J. Dittmann

AbstractThe 3D transfer equation for polarized radiation is solved for several different model configurations. In the case of Rayleigh scattering the phasematrix is decomposed into a sum of matrix products to allow the use of operator splitting iteration schemes. For 30 slabs with constant extinction matrix and constant emission the emerging polarized fiuxe are calculated. We find that the optical depth and the scattering parameter can be fixed from observations even if only the fluxes are known. Specifying the extinction matrix our models can be applied to the inner regions of active galactic nuclei.


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