scholarly journals Self-assembled plasmonics for angle-independent structural color displays with actively addressed black states

2020 ◽  
Vol 117 (24) ◽  
pp. 13350-13358 ◽  
Author(s):  
Daniel Franklin ◽  
Ziqian He ◽  
Pamela Mastranzo Ortega ◽  
Alireza Safaei ◽  
Pablo Cencillo-Abad ◽  
...  
Keyword(s):  
Physical Vapor Deposition ◽  
Film Growth ◽  
Liquid Crystal Display ◽  
Incident Light ◽  
Near Field ◽  
Strongly Coupled ◽  
Plasmonic Materials ◽  
Color Displays ◽  
Self Assembled ◽  
Saturated Color

Nanostructured plasmonic materials can lead to the extremely compact pixels and color filters needed for next-generation displays by interacting with light at fundamentally small length scales. However, previous demonstrations suffer from severe angle sensitivity, lack of saturated color, and absence of black/gray states and/or are impractical to integrate with actively addressed electronics. Here, we report a vivid self-assembled nanostructured system which overcomes these challenges via the multidimensional hybridization of plasmonic resonances. By exploiting the thin-film growth mechanisms of aluminum during ultrahigh vacuum physical vapor deposition, dense arrays of particles are created in near-field proximity to a mirror. The sub-10-nm gaps between adjacent particles and mirror lead to strong multidimensional coupling of localized plasmonic modes, resulting in a singular resonance with negligible angular dispersion and ∼98% absorption of incident light at a desired wavelength. The process is compatible with arbitrarily structured substrates and can produce wafer-scale, diffusive, angle-independent, and flexible plasmonic materials. We then demonstrate the unique capabilities of the strongly coupled plasmonic system via integration with an actively addressed reflective liquid crystal display with control over black states. The hybrid display is readily programmed to display images and video.

Three-Dimensional Finite-Difference Time-Domain Method Modeling of Nanowire Optical Probe

2014 ◽  
Vol 602-605 ◽  
pp. 3359-3362
Author(s):  
Chun Li Zhu ◽  
Jing Li
Keyword(s):  
Finite Difference ◽  
Time Domain ◽  
Finite Difference Time Domain ◽  
Incident Light ◽  
Near Field ◽  
Three Dimensional ◽  
Polarization Direction ◽  
Near Field Imaging ◽  
Difference Time ◽  
Field Imaging

In this paper, output near fields of nanowires with different optical and structure configurations are calculated by using the three-dimensional finite-difference time-domain (3D FDTD) method. Then a nanowire with suitable near field distribution is chosen as the probe for scanning dielectric and metal nanogratings. Scanning results show that the resolution in near-field imaging of dielectric nanogratings can be as low as 80nm, and the imaging results are greatly influenced by the polarization direction of the incident light. Compared with dielectric nanogratings, metal nanogratings have significantly enhanced resolutions when the arrangement of gratings is perpendicular to the polarization direction of the incident light due to the enhancement effect of the localized surface plasmons (SPs). Results presented here could offer valuable references for practical applications in near-field imaging with nanowires as optical probes.

scholarly journals Fabrication of New Liquid Crystal Device Using Layer-by-Layer Thin Film Process

Processes ◽  
2018 ◽  
Vol 6 (8) ◽  
pp. 108 ◽  
Author(s):  
Gitae Moon ◽  
Wonjun Jang ◽  
Intae Son ◽  
Hyun Cho ◽  
Yong Park ◽  
...  
Keyword(s):  
Liquid Crystal ◽  
Indium Tin Oxide ◽  
Film Growth ◽  
Mechanical Stability ◽  
Liquid Crystal Display ◽  
Layer By Layer ◽  
Transparent Electrodes ◽  
Ito Electrode ◽  
Display Performance ◽  
Layer Thin Film

Indium tin oxide (ITO) transparent electrodes are troubled with high cost and poor mechanical stability. In this study, layer-by-layer (LBL)-processed thin films with single-walled carbon nanotubes (SWNTs) exhibited high transparency and electrical conductivity as a candidate for ITO replacement. The repetitive deposition of polycations and stabilized SWNTs with a negative surfactant exhibits sufficiently linear film growth and high optoelectronic performance to be used as transparent electrodes for vertically aligned (VA) liquid crystal display (LCD) cells. The LC molecules were uniformly aligned on the all of the prepared LBL electrodes. VA LCD cells with SWNT LBL electrodes exhibited voltage-transmittance (V-T) characteristics similar to those with the conventional ITO electrodes. Although the response speeds were slower than the LCD cell with the ITO electrode, as the SWNT layers increased, the display performance was closer to the LCD cells with conventional ITO electrode. This work demonstrated the good optoelectronic performance and alignment compatibility with LC molecules of the SWNT LBL assemblies, which are potential alternatives to ITO films as transparent electrodes for LCDs.

Lateral Coupling of Self-Assembled Quantum Dots Studied by Near-Field Spectroscopy

1999 ◽  
Vol 571 ◽  
Author(s):  
H.D. Robinson ◽  
B.B. Goldberg ◽  
J.L. Merz
Keyword(s):  
Quantum Dots ◽  
Additional Data ◽  
High Spatial Resolution ◽  
Large Fraction ◽  
Near Field ◽  
Localized States ◽  
Emission Lines ◽  
Lateral Coupling ◽  
Self Assembled ◽  
Density Regime

ABSTRACTLateral coupling between separate quantum dots has been observed in a system of In0.55A10.45As self-assembled quantum dots. The experiment was performed by taking photoluminescence excitation (PLE) spectra in the optical near-field at 4.2 K. The high spatial resolution afforded by the near-field technique allows us to resolve individual dots in a density regime where interactions between neighboring dots become apparent. In the PLE spectra, narrow resonances are observed in the emission lines of individual dots. A large fraction of these resonances occur simultaneously in several emission lines, originating from different quantum dots. This is evidence of interdot scattering of carriers, which additional data show to be mediated by localized states at energies below the wetting layer exciton energy. A very rich phonon spectrum generated by the complicated interfaces between barrier and dot material is also evident in the data.

scholarly journals Generation of Charged Ti Nanoparticles and Their Deposition Behavior with a Substrate Bias during RF Magnetron Sputtering

Coatings ◽  
2020 ◽  
Vol 10 (5) ◽  
pp. 443
Author(s):  
Ji-Hye Kwon ◽  
Du-Yun Kim ◽  
Nong-Moon Hwang
Keyword(s):  
Electron Microscopy ◽  
Vapor Deposition ◽  
Physical Vapor Deposition ◽  
Film Growth ◽  
Film Deposition ◽  
Calculated Density ◽  
X Ray ◽  
Positively Charged ◽  
Made In ◽  
Ti Films

This study is based on the film growth by non-classical crystallization, where charged nanoparticles (NPs) are the building block of film deposition. Extensive studies about the generation of charged NPs and their contribution to film deposition have been made in the chemical vapor deposition (CVD) process. However, only a few studies have been made in the physical vapor deposition (PVD) process. Here, the possibility for Ti films to grow by charged Ti NPs was studied during radio frequency (RF) sputtering using Ti target. After the generation of charged Ti NPs was confirmed, their influence on the film quality was investigated. Charged Ti NPs were captured on amorphous carbon membranes with the electric bias of −70 V, 0 V, +5 V, +15 V and +30 V and examined by transmission electron microscopy (TEM). The number density of the Ti NPs decreased with increasing positive bias, which showed that some of Ti NPs were positively charged and repelled by the positively biased TEM membrane. Ti films were deposited on Si substrates with the bias of −70 V, 0 V and +30 V and analyzed by TEM, field-emission scanning electron microscopy (FESEM), X-ray diffraction (XRD) and X-ray reflectivity (XRR). The film deposited at −70 V had the highest thickness of 180 nm, calculated density of 4.974 g/cm3 and crystallinity, whereas the film deposited at +30 V had the lowest thickness of 92 nm, calculated density of 3.499 g/cm3 and crystallinity. This was attributed to the attraction of positively charged Ti NPs to the substrate at −70 V and to the landing of only small-sized neutral Ti NPs on the substrate at +30 V. These results indicate that the control of charged NPs is necessary to obtain a high quality thin film at room temperature.

scholarly journals Early steps of the film growth mechanism in self-assembled multilayers of PAH and PSS on silica

2006 ◽  
Vol 288 (1-3) ◽  
pp. 26-35 ◽  
Author(s):  
J. Dejeu ◽  
L. Buisson ◽  
M.C. Guth ◽  
C. Roidor ◽  
F. Membrey ◽  
...  
Keyword(s):  
Growth Mechanism ◽  
Film Growth ◽  
Self Assembled

scholarly journals Near-field photochemical and radiation-induced chemical fabrication of nanopatterns of a self-assembled silane monolayer

2014 ◽  
Vol 5 ◽  
pp. 1441-1449 ◽  
Author(s):  
Ulrich Christian Fischer ◽  
Carsten Hentschel ◽  
Florian Fontein ◽  
Linda Stegemann ◽  
Christiane Hoeppener ◽  
...  
Keyword(s):  
Chemical Process ◽  
Oxygen Plasma ◽  
Near Field ◽  
General Concept ◽  
Photochemical Reactions ◽  
Self Assembled Monolayer ◽  
Photochemical Process ◽  
Radiation Induced ◽  
Oxygen Plasma Etching ◽  
Self Assembled

A general concept for parallel near-field photochemical and radiation-induced chemical processes for the fabrication of nanopatterns of a self-assembled monolayer (SAM) of (3-aminopropyl)triethoxysilane (APTES) is explored with three different processes: 1) a near-field photochemical process by photochemical bleaching of a monomolecular layer of dye molecules chemically bound to an APTES SAM, 2) a chemical process induced by oxygen plasma etching as well as 3) a combined near-field UV-photochemical and ozone-induced chemical process, which is applied directly to an APTES SAM. All approaches employ a sandwich configuration of the surface-supported SAM, and a lithographic mask in form of gold nanostructures fabricated through colloidal sphere lithography (CL), which is either exposed to visible light, oxygen plasma or an UV–ozone atmosphere. The gold mask has the function to inhibit the photochemical reactions by highly localized near-field interactions between metal mask and SAM and to inhibit the radiation-induced chemical reactions by casting a highly localized shadow. The removal of the gold mask reveals the SAM nanopattern.

β-Sn-based plasmonic materials and their near-field enhancement performance

2021 ◽  
Author(s):  
Ying-Wei Lu ◽  
Bin Li ◽  
Han-Han Wu ◽  
Liang Ren
Keyword(s):  
Near Field ◽  
Field Enhancement ◽  
Plasmonic Materials

Kinetic Monte Carlo Simulation of Metallic Nanoislands Grown by Physical Vapor Deposition

2011 ◽  
Vol 9 (1) ◽  
pp. 49-67 ◽  
Author(s):  
Abuhanif K. Bhuiyan ◽  
S. K. Dew ◽  
M. Stepanova
Keyword(s):  
Vapor Deposition ◽  
Physical Vapor Deposition ◽  
Kinetic Monte Carlo ◽  
Substrate Material ◽  
Film Deposition ◽  
Process Conditions ◽  
Control Factors ◽  
Critical Process Parameters ◽  
Self Assembled ◽  
Surface Morphologies

AbstractWe report kinetic Monte-Karlo (KMC) simulation of self-assembled synthesis of nanocrystals by physical vapor deposition (PVD), which is one of most flexible, efficient, and clean techniques to fabricate nanopatterns. In particular, self-assembled arrays of nanocrystals can be synthesized by PVD. However size, shape and density of self-assembled nanocrystals are highly sensitive to the process conditions such as duration of deposition, temperature, substrate material, etc. To efficiently synthesize nanocrystalline arrays by PVD, the process control factors should be understood in detail. KMC simulations of film deposition are an important tool for understanding the mechanisms of film deposition. In this paper, we report a KMC modeling that explicitly represents PVD synthesis of self-assembled nanocrystals. We study how varying critical process parameters such as deposition rate, duration, temperature, and substrate type affect the lateral 2D morphologies of self-assembled metallic islands on substrates, and compare our results with experimentally observed surface morphologies generated by PVD. Our simulations align well with experimental results reported in the literature.

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