scholarly journals Identification of the Aerosol Types over Athens, Greece: The Influence of Air-Mass Transport

2010 ◽  
Vol 2010 ◽  
pp. 1-15 ◽  
Author(s):  
D. G. Kaskaoutis ◽  
P. G. Kosmopoulos ◽  
H. D. Kambezidis ◽  
P. T. Nastos

Aerosol optical depth at 550 nm () and fine-mode (FM) fraction data from Terra-MODIS were obtained over the Greater Athens Area covering the period February 2000–December 2005. Based on both and FM values three main aerosol types have been discriminated corresponding to urban/industrial aerosols, clean maritime conditions, and coarse-mode, probably desert dust, particles. Five main sectors were identified for the classification of the air-mass trajectories, which were further used in the analysis of the ( and FM data for the three aerosol types). The HYSPLIT model was used to compute back trajectories at three altitudes to investigate the relation between -FM and wind sector depending on the altitude. The accumulation of local pollution is favored in spring and corresponds to air masses at lower altitudes originating from Eastern Europe and the Balkan. Clean maritime conditions are rare over Athens, limited in the winter season and associated with air masses from the Western or Northwestern sector. The coarse-mode particles origin seems to be more complicated proportionally to the season. Thus, in summer the Northern sector dominates, while in the other seasons, and especially in spring, the air masses belong to the Southern sector enriched with Saharan dust aerosols.

2020 ◽  
Vol 237 ◽  
pp. 02018 ◽  
Author(s):  
Dominika Szczepanik ◽  
Eleni Tetoni ◽  
Dongxiang Wang ◽  
Iwona S. Stachlewska

This paper presents preliminary results of using an extended POLIPHON method for separation of dust and non-dust aerosol backscatter coefficient, applied on a case study of 9th August 2013. That day, long-range transport of mineral dust over EARLINET-ACTRIS lidar site in Warsaw was observed with the 8-channel PollyXT-UW lidar. The dust particles were also observed by the Cloud-Aerosol Lidar with Orthogonal Polarization (CALIOP) on board the CALIPSO satellite. The backward trajectories calculated using the HYSPLIT model confirmed the air-mass transport from Northern Africa. Results yield possible dust separation for the mixture of dust with other aerosol types, such as pollution, marine type, etc.


2014 ◽  
Vol 142 (11) ◽  
pp. 4207-4229 ◽  
Author(s):  
Robert M. Rauber ◽  
Matthew K. Macomber ◽  
David M. Plummer ◽  
Andrew A. Rosenow ◽  
Greg M. McFarquhar ◽  
...  

Abstract Data from airborne W-band radar, thermodynamic fields from the Weather Research and Forecasting (WRF) Model, and air parcel back trajectories from the Hybrid Single-Particle Lagrangian Integrated Trajectory (HYSPLIT) model are used to investigate the finescale reflectivity, vertical motion, and airmass structure of the comma head of a winter cyclone that produced 15–25 cm of snow across the U.S. Midwest on 29–30 January 2010. The comma head consisted of three vertically stacked air masses: from bottom to top, an arctic air mass of Canadian origin, a moist cloud-bearing air mass of Gulf of Mexico origin, and a drier air mass originating mostly at low altitudes over Baja California and the Mexican Plateau. The drier air mass capped the entire comma head and significantly influenced precipitation distribution and type across the storm, limiting cloud depth on the warm side, and creating instability with respect to ice-saturated ascent, cloud-top generating cells, and a seeder–feeder process on the cold side. Convective generating cells with depths of 1.5–3.0 km and vertical air velocities of 1–3 m s−1 were ubiquitous atop the cold side of the comma head. The airmass boundaries within the comma head lacked the thermal contrast commonly observed along fronts in other sectors of extratropical cyclones. The boundary between the Gulf and Canadian air masses, although quite distinct in terms of precipitation distribution, wind, and moisture, was marked by almost no horizontal thermal contrast at the time of observation. The higher-altitude airmass boundary between the Gulf of Mexico and Baja air masses also lacked thermal contrast, with the less-stable Baja air mass overriding the stable Gulf of Mexico air.


2019 ◽  
Vol 19 (6) ◽  
pp. 3557-3578 ◽  
Author(s):  
Martin Osborne ◽  
Florent F. Malavelle ◽  
Mariana Adam ◽  
Joelle Buxmann ◽  
Jaqueline Sugier ◽  
...  

Abstract. On 15–16 October 2017, ex-hurricane Ophelia passed to the west of the British Isles, bringing dust from the Sahara and smoke from Portuguese forest fires that was observable to the naked eye and reported in the UK's national press. We report here detailed observations of this event using the UK operational lidar and sun-photometer network, established for the early detection of aviation hazards, including volcanic ash. We also use ECMWF ERA5 wind field data and MODIS imagery to examine the aerosol transport. The observations, taken continuously over a period of 30 h, show a complex picture, dominated by several different aerosol layers at different times and clearly correlated with the passage of different air masses associated with the intense cyclonic system. A similar evolution was observed at several sites, with a time delay between them explained by their different location with respect to the storm and associated meteorological features. The event commenced with a shallow dust layer at 1–2 km in altitude and culminated in a deep and complex structure that lasted ∼12 h at each site over the UK, correlated with the storm's warm sector. For most of the time, the aerosol detected was dominated by mineral dust mixtures, as highlighted by depolarisation measurements, but an intense biomass burning aerosol (BBA) layer was observed towards the end of the event, lasting around 3 h at each site. The aerosol optical depth at 355 nm (AOD355) during the whole event ranged from 0.2 to 2.9, with the larger AOD correlated to the intense BBA layer. Such a large AOD is unprecedented in the UK according to AERONET records for the last 20 years. The Raman lidars permitted the measurement of the aerosol extinction coefficient at 355 nm, the particle linear depolarisation ratio (PLDR), and the lidar ratio (LR) and made the separation of the dust (depolarising) aerosol from other aerosol types possible. A specific extinction has also been computed to provide an estimate of the atmospheric concentration of both aerosol types separately, which peaked at 420±200 µg m−3 for the dust and 558±232 µg m−3 for the biomass burning aerosols. Back trajectories computed using the Numerical Atmospheric-dispersion Modelling Environment (NAME) were used to identify the sources and strengthen the conclusions drawn from the observations. The UK network represents a significant expansion of the observing capability in northern Europe, with instruments evenly distributed across Great Britain, from Camborne in Cornwall to Lerwick in the Shetland Islands, and this study represents the first attempt to demonstrate its capability and validate the methods in use. Its ultimate purpose will be the detection and quantification of volcanic plumes, but the present study clearly demonstrates the advanced capabilities of the network.


2020 ◽  
Author(s):  
Claire Ryder ◽  
Eleanor Highwood ◽  
Adrian Walser ◽  
Petra Walser ◽  
Anne Philipp ◽  
...  

<p>Mineral dust is an important component of the climate system, interacting with radiation, clouds, and biogeochemical systems and impacting atmospheric circulation, air quality, aviation, and solar energy generation. These impacts are sensitive to dust particle size distribution (PSD), yet models struggle or even fail to represent coarse (diameter (<span><em>d</em></span>) <span>>2.5</span> <span>µ</span>m) and giant (<span><em>d</em>>20</span> <span>µ</span>m) dust particles and the evolution of the PSD with transport. Here we examine three state-of-the-art airborne observational datasets, all of which measured the full size range of dust (<span><em>d</em>=0.1</span> to <span>>100</span> <span>µ</span>m) at different stages during transport with consistent instrumentation. We quantify the presence and evolution of coarse and giant particles and their contribution to optical properties using airborne observations over the Sahara (from the Fennec field campaign) and in the Saharan Air Layer (SAL) over the tropical eastern Atlantic (from the AER-D field campaign).</p><p>Observations show significantly more abundant coarse and giant dust particles over the Sahara compared to the SAL: effective diameters of up to 20 <span>µ</span>m were observed over the Sahara compared to 4 <span>µ</span>m in the SAL. Excluding giant particles over the Sahara results in significant underestimation of mass concentration (40 %), as well as underestimates of both shortwave and longwave extinction (18 % and 26 %, respectively, from scattering calculations), while the effects in the SAL are smaller but non-negligible. The larger impact on longwave extinction compared to shortwave implies a bias towards a radiative cooling effect in dust models, which typically exclude giant particles and underestimate coarse-mode concentrations.</p><p>A compilation of the new and published effective diameters against dust age since uplift time suggests that two regimes of dust transport exist. During the initial 1.5 d, both coarse and giant particles are rapidly deposited. During the subsequent 1.5 to 10 d, PSD barely changes with transport, and the coarse mode is retained to a much greater degree than expected from estimates of gravitational sedimentation alone. The reasons for this are unclear and warrant further investigation in order to improve dust transport schemes and the associated radiative effects of coarse and giant particles in models.</p><p>This work has been recently published in ACP (Ryder, C. L., Highwood, E. J., Walser, A., Seibert, P., Philipp, A., and Weinzierl, B.: Coarse and giant particles are ubiquitous in Saharan dust export regions and are radiatively significant over the Sahara, Atmos. Chem. Phys., 19, 15353–15376, https://doi.org/10.5194/acp-19-15353-2019, 2019).</p>


2019 ◽  
Vol 99 ◽  
pp. 01006
Author(s):  
Sanaz Moghim ◽  
Reyhaneh Ramezanpoor

Atmospheric aerosols affect the Earth's climate, air quality, and thus human health. This study used the Aerosol Optical Depth (AOD) and the Ångström exponent to cluster different particle types over the Lake Urmia Basin. This classification found desert dust and marine (mixed with continental or local-pollution aerosols) as two main aerosol types over the region, while their sources are not well defined. Although different air masses and wind circulation over the study domain in varied months can help to distinguish aerosol sources, measurements are crucial for a complete evaluation.


2014 ◽  
Vol 14 (21) ◽  
pp. 11753-11773 ◽  
Author(s):  
C. Guirado ◽  
E. Cuevas ◽  
V. E. Cachorro ◽  
C. Toledano ◽  
S. Alonso-Pérez ◽  
...  

Abstract. More than 2 years of columnar atmospheric aerosol measurements (2006–2009) at the Tamanrasset site (22.79° N, 5.53° E, 1377 m a.s.l.), in the heart of the Sahara, are analysed. Aerosol Robotic Network (AERONET) level 2.0 data were used. The KCICLO (K is the name of a constant and ciclo means cycle in Spanish) method was applied to a part of the level 1.5 data series to improve the quality of the results. The annual variability of aerosol optical depth (AOD) and Ångström exponent (AE) has been found to be strongly linked to the convective boundary layer (CBL) thermodynamic features. The dry-cool season (autumn and winter) is characterized by a shallow CBL and very low mean turbidity (AOD ~ 0.09 at 440 nm, AE ~ 0.62). The wet-hot season (spring and summer) is dominated by high turbidity of coarse dust particles (AE ~ 0.28, AOD ~ 0.39 at 440 nm) and a deep CBL. The aerosol-type characterization shows desert mineral dust as the prevailing aerosol. Both pure Saharan dust and very clear sky conditions are observed depending on the season. However, several case studies indicate an anthropogenic fine mode contribution from the industrial areas in Libya and Algeria. The concentration weighted trajectory (CWT) source apportionment method was used to identify potential sources of air masses arriving at Tamanrasset at several heights for each season. Microphysical and optical properties and precipitable water vapour were also investigated.


2020 ◽  
Author(s):  
Yikun Yang ◽  
Chuanfeng Zhao ◽  
Quan Wang ◽  
Zhiyuan Cong ◽  
Xingchuan Yang ◽  
...  

Abstract. To better understand the aerosol properties over the Arctic, Antarctic, and Tibetan Plateau (TP), the aerosol optical properties were investigated using 13 years CALIPSO L3 data, and the back trajectories for air masses were also simulated using the Hybrid Single Particle Lagrangian Integrated Trajectory (HYSPLIT) model. The results show that the aerosol optical depth (AOD) has obvious spatial and seasonal variation characteristics, and the aerosol loading over Eurasia, Ross Sea, and South Asia is relatively large. The annual average AOD in the Arctic, Antarctic, and TP are 0.046, 0.025, and 0.098, respectively. The Arctic and Antarctic regions have larger AOD values in winter and spring, while the TP in spring and summer. There are no significant temporal trends of AOD anomalies in the three study regions. Clean marine and dust-related aerosols are the dominant types over ocean and land respectively in both the Arctic and Antarctic, while dust-related aerosol types have greater occurrence frequency (OF) over the TP. The OF of dust-related and elevated smoke is large for a broad range of heights, indicating that they are likely transported aerosols, while other types of aerosols mainly occurred at heights below 2 km in the Antarctic and Arctic. The maximum OF of dust-related aerosols mainly occurs at 6 km altitude over the TP. The analysis of back trajectories of the air masses shows large differences among different regions and seasons. The Arctic region is more vulnerable to mid-latitude pollutants than the Antarctic region, especially in winter and spring, while the air masses in the TP are mainly from the Iranian Plateau, Tarim Basin, and South Asia.


2006 ◽  
Vol 24 (3) ◽  
pp. 807-821 ◽  
Author(s):  
D. Balis ◽  
V. Amiridis ◽  
S. Kazadzis ◽  
A. Papayannis ◽  
G. Tsaknakis ◽  
...  

Abstract. High aerosol optical depth (AOD) values, larger than 0.6, are systematically observed in the Ultraviolet (UV) region both by sunphotometers and lidar systems over Greece during summertime. To study in more detail the characteristics and the origin of these high AOD values, a campaign took place in Greece in the frame of the PHOENICS (Particles of Human Origin Extinguishing Natural solar radiation In Climate Systems) and EARLINET (European Aerosol Lidar Network) projects during August–September of 2003, which included simultaneous sunphotometric and lidar measurements at three sites covering the north-south axis of Greece: Thessaloniki, Athens and Finokalia, Crete. Several events with high AOD values have been observed over the measuring sites during the campaign period, many of them corresponding to Saharan dust. In this paper we focused on the event of 30 and 31 August 2003, when a dust layer in the height range of 2000-5000 m, progressively affected all three stations. This layer showed a complex behavior concerning its spatial evolution and allowed us to study the changes in the optical properties of the desert dust particles along their transport due to aging and mixing with other types of aerosol. The extinction-to-backscatter ratio determined on the 30 August 2003 at Thessaloniki was approximately 50 sr, characteristic for rather spherical mineral particles, and the measured color index of 0.4 was within the typical range of values for desert dust. Mixing of the desert dust with other sources of aerosols resulted the next day in overall smaller and less absorbing population of particles with a lidar ratio of 20 sr. Mixing of polluted air-masses originating from Northern Greece and Crete and Saharan dust result in very high aerosol backscatter values reaching 7 Mm-1 sr-1 over Finokalia. The Saharan dust observed over Athens followed a different spatial evolution and was not mixed with the boundary layer aerosols mainly originating from local pollution.


2007 ◽  
Vol 7 (13) ◽  
pp. 3481-3495 ◽  
Author(s):  
J. Kusmierczyk-Michulec ◽  
G. De Leeuw ◽  
M. M. Moerman

Abstract. Sun photometer measurements at the AERONET station at the North Sea coast in The Hague (The Netherlands) provide a climatology of optical and physical aerosol properties for the area. Results are presented from the period January 2002 to July 2003. For the analysis and interpretation these data are coupled to chemical aerosol data from a nearby station of the Dutch National Air Quality Network. This network provides PM10 and black carbon concentrations. Meteorological conditions and air mass trajectories are also used. Due to the location close to the coast, the results are strongly dependent on wind direction, i.e. air mass trajectory. In general the aerosol optical properties are governed by industrial aerosol emitted form various industrial, agricultural and urban areas surrounding the site in almost all directions over land. For maritime air masses industrial aerosols are transported from over the North Sea, whereas very clean air is transported from the NW in clean polar air masses from the North Atlantic. In the winter the effect of the production of sea salt aerosol at high wind speeds is visible in the optical and physical aerosol data. In these cases fine and coarse mode radii are similar to those reported in the literature for marine aerosol. Relations are derived between the Ångström coefficients with both the fine/coarse mode fraction and the ratio of black carbon and PM10.


Atmosphere ◽  
2018 ◽  
Vol 9 (10) ◽  
pp. 374 ◽  
Author(s):  
Eliane Larroza ◽  
Philippe Keckhut ◽  
Jean-Luc Baray ◽  
Walter Nakaema ◽  
Hélène Vérèmes ◽  
...  

In this study, an air mass (containing a cirrus cloud) was detected by light detection and ranging (lidar) above São Paulo (Brazil) in June 2007 and tracked around the globe, thanks to Lagrangian calculations as well as ground-based and satellite observations. Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observation (CALIPSO) data were also used to provide locations of occurrence of cirrus around the globe and extract their respective macro physical parameters (altitude and temperature). An analysis of the air mass history based on Lagrangian trajectories reveals that water coming from the Equator is channelized through the southern subtropical jet for weeks. In this case, the back-trajectories showed that the cirrus cloud detected at São Paulo was a mixture of air masses from two different locations: (1) the active convective area located around the Equator, with transport into the upper troposphere that promotes cirrus cloud formation; and (2) the South Pacific Ocean, with transport that follows the subtropical jet stream (STJ). Air masses coming from equatorial convective regions are trapped by the jet, which contributes to maintaining the lifetime of the cirrus cloud for a few days. The cloud disappears near the African continent, due to a southern excursion and warmer temperatures, then reappears and is detected again by the lidar system in São Paulo after 12 days. The observed cloud is located at a similar altitude, revealing that sedimentation is small or compensated by radiative uplift.


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