scholarly journals Effects of Ocean Ecosystem on Marine Aerosol-Cloud Interaction

2010 ◽  
Vol 2010 ◽  
pp. 1-13 ◽  
Author(s):  
Nicholas Meskhidze ◽  
Athanasios Nenes
Keyword(s):  
Aerosol Optical Depth ◽  
Optical Depth ◽  
Cloud Condensation Nuclei ◽  
Multiple Time ◽  
Surface Ocean ◽  
Microphysical Properties ◽  
Microphysical Parameters ◽  
The Difference ◽  
Ocean Ecosystem ◽  
Positive Correlations

Using satellite data for the surface ocean, aerosol optical depth (AOD), and cloud microphysical parameters, we show that statistically significant positive correlations exist between ocean ecosystem productivity, the abundance of submicron aerosols, and cloud microphysical properties over different parts of the remote oceans. The correlation coefficient for remotely sensed surface chlorophyllaconcentration ([Chl-a]) and liquid cloud effective radii over productive areas of the oceans varies between−0.2and−0.6. Special attention is given to identifying (and addressing) problems from correlation analysis used in the previous studies that can lead to erroneous conclusions. A new approach (using the difference between retrieved AOD and predicted sea salt aerosol optical depth,AODdiff) is developed to explore causal links between ocean physical and biological systems and the abundance of cloud condensation nuclei (CCN) in the remote marine atmosphere. We have found that over multiple time periods, 550 nmAODdiff(sensitive to accumulation mode aerosol, which is the prime contributor to CCN) correlates well with [Chl-a] over the productive waters of the Southern Ocean. Since [Chl-a] can be used as a proxy of ocean biological productivity, our analysis demonstrates the role of ocean ecology in contributing CCN, thus shaping the microphysical properties of low-level marine clouds.

scholarly journals High lightning activity in maritime clouds near Mexico

2012 ◽  
Vol 12 (17) ◽  
pp. 8055-8072 ◽  
Author(s):  
B. Kucienska ◽  
G. B. Raga ◽  
R. Romero-Centeno
Keyword(s):  
Aerosol Optical Depth ◽  
Optical Depth ◽  
Cloud Condensation Nuclei ◽  
Meridional Wind ◽  
Lightning Activity ◽  
Wind Component ◽  
Inter Tropical Convergence Zone ◽  
High Rainfall ◽  
Wind Variability ◽  
Monthly Distribution

Abstract. Lightning activity detected by the World Wide Lightning Location Network (WWLLN) over oceanic regions adjacent to Mexico is often as high as that observed over the continent. In order to explore the possible causes of the observed high flash density over those regions, the relationships between lightning, rainfall, vertical hydrometeor profiles, latent heating, wind variability and aerosol optical depth are analyzed. The characteristics of lightning and precipitation over four oceanic zones adjacent to Mexican coastlines are contrasted against those over the continent. The number of flashes per rainfall over some coastal maritime regions is found to be higher than over the continent. The largest number of flashes per rainfall is observed during the biomass burning season. In addition, we compare two smaller areas of the Tropical Pacific Ocean: one located within the Inter-Tropical Convergence Zone and characterized by high rainfall and weak lightning activity and the other one influenced by a continental wind jet and characterized by high rainfall and strong lightning activity. During the rainy season, the monthly distribution of lightning within the region influenced by the continental wind jet is contrary to that of rainfall. Moreover, the monthly variability of lightning is very similar to the variability of the meridional wind component and it is also related to the variability of aerosol optical depth. The analysis suggests that the high lightning activity observed over coastal Pacific region is linked to the continental cloud condensation nuclei advected over the ocean. Analysis of daily observations indicates that the greatest lightning density is observed for moderate values of the aerosol optical depth, between 0.2 and 0.35.

scholarly journals Assessment of nocturnal aerosol optical depth from lunar photometry at the Izaña high mountain observatory

2017 ◽  
Vol 10 (8) ◽  
pp. 3007-3019 ◽  
Author(s):  
África Barreto ◽  
Roberto Román ◽  
Emilio Cuevas ◽  
Alberto J. Berjón ◽  
A. Fernando Almansa ◽  
...  
Keyword(s):  
Aerosol Optical Depth ◽  
Optical Depth ◽  
High Mountain ◽  
Moon Phase ◽  
Stable Conditions ◽  
Lunar Observations ◽  
The Common ◽  
The Difference ◽  
Single Night ◽  
Calibration Techniques

Abstract. This work is a first approach to correct the systematic errors observed in the aerosol optical depth (AOD) retrieved at nighttime using lunar photometry and calibration techniques dependent on the lunar irradiance model. To this end, nocturnal AOD measurements were performed in 2014 using the CE318-T master Sun–sky–lunar photometer (lunar Langley calibrated) at the Izaña high mountain observatory. This information has been restricted to 59 nights characterized as clean and stable according to lidar vertical profiles. A phase angle dependence as well as an asymmetry within the Moon's cycle of the Robotic Lunar Observatory (ROLO) model could be deduced from the comparison in this 59-night period of the CE318-T calibration performed by means of the lunar Langley calibration and the calibration performed every single night by means of the common Langley technique. Nocturnal AOD has also been compared in the same period with a reference AOD based on daylight AOD extracted from the AErosol RObotic NETwork (AERONET) at the same station. Considering stable conditions, the difference ΔAODfit, between AOD from lunar observations and the linearly interpolated AOD (the reference) from daylight data, has been calculated. The results show that ΔAODfit values are strongly affected by the Moon phase and zenith angles. This dependency has been parameterized using an empirical model with two independent variables (Moon phase and zenith angles) in order to correct the AOD for these residual dependencies. The correction of this parameterized dependency has been checked at four stations with quite different environmental conditions (Izaña, Lille, Carpentras and Dakar) showing a significant reduction of the AOD dependence on phase and zenith angles and an improved agreement with daylight reference data. After the correction, absolute AOD differences for day–night–day clean and stable transitions remain below 0.01 for all wavelengths.

scholarly journals Daytime aerosol optical depth above low-level clouds is similar to that in adjacent clear skies at the same heights: airborne observation above the southeast Atlantic

2020 ◽  
Author(s):  
Yohei Shinozuka ◽  
Meloë S. Kacenelenbogen ◽  
Sharon P. Burton ◽  
Steven G. Howell ◽  
Paquita Zuidema ◽  
...  
Keyword(s):  
Aerosol Optical Depth ◽  
Optical Depth ◽  
Wavelength Dependence ◽  
Single Scattering ◽  
Airborne Lidar ◽  
Aerosol Layer ◽  
Low Level ◽  
Satellite Retrieval ◽  
Biomass Burning Aerosol ◽  
The Difference

Abstract. To help satellite retrieval of aerosols and studies of their radiative effects, we demonstrate that daytime 532 nm aerosol optical depth over low-level clouds is similar to that in neighboring clear skies at the same heights in recent airborne lidar and sunphotometer observations above the southeast Atlantic. The mean AOD difference is between 0 and −0.01, when comparing the two sides, each up to 20 km wide, of cloud edges. The difference is not statistically significant according to a paired t-test. Systematic differences in the wavelength dependence of AOD and in situ single scattering albedo are also minute. These results hold regardless of the vertical distance between cloud top and aerosol layer bottom. AOD aggregated over ~ 2° grid boxes for each of September 2016, August 2017 and October 2018 also shows little correlation with the presence of low-level clouds. We posit that a satellite retrieval artifact is entirely responsible for a previous finding of generally smaller AOD over clouds (Chung et al., 2016), at least for the region and season of our study. Our results also suggest that the same values can be assumed for the intensive properties of free-tropospheric biomass-burning aerosol regardless of whether clouds exist below.

scholarly journals High temporal resolution estimates of columnar aerosol microphysical parameters from spectrum of aerosol optical depth by linear estimation: application to long-term AERONET and star-photometry measurements

2015 ◽  
Vol 8 (8) ◽  
pp. 3117-3133 ◽  
Author(s):  
D. Pérez-Ramírez ◽  
I. Veselovskii ◽  
D. N. Whiteman ◽  
A. Suvorina ◽  
M. Korenskiy ◽  
...  
Keyword(s):  
Aerosol Optical Depth ◽  
Optical Depth ◽  
Temporal Resolution ◽  
High Temporal Resolution ◽  
Linear Estimation ◽  
Night Time ◽  
Microphysical Properties ◽  
Fine Mode ◽  
Using Data ◽  
Aerosol Types

Abstract. This work deals with the applicability of the linear estimation technique (LE) to invert spectral measurements of aerosol optical depth (AOD) provided by AERONET CIMEL sun photometers. The inversion of particle properties using only direct-sun AODs allows the evaluation of parameters such as effective radius (reff) and columnar volume aerosol content (V) with significantly better temporal resolution than the operational AERONET algorithm which requires both direct sun and sky radiance measurements. Sensitivity studies performed demonstrate that the constraints on the range of the inversion are very important to minimize the uncertainties, and therefore estimates of reff can be obtained with uncertainties less than 30 % and of V with uncertainties below 40 %. The LE technique is applied to data acquired at five AERONET sites influenced by different aerosol types and the retrievals are compared with the results of the operational AERONET code. Good agreement between the two techniques is obtained when the fine mode predominates, while for coarse mode cases the LE results systematically underestimate both reff and V. The highest differences are found for cases where no mode predominates. To minimize these biases, correction functions are developed using the multi-year database of observations at selected sites, where the AERONET retrieval is used as the reference. The derived corrections are tested using data from 18 other AERONET stations offering a range of aerosol types. After correction, the LE retrievals provide better agreement with AERONET for all the sites considered. Finally, the LE approach developed here is applied to AERONET and star-photometry measurements in the city of Granada (Spain) to obtain day-to-night time evolution of columnar aerosol microphysical properties.

scholarly journals Effect of aerosol sub-grid variability on aerosol optical depth and cloud condensation nuclei: Implications for global aerosol modelling

2016 ◽  
Author(s):  
N. Weigum ◽  
N. Schutgens ◽  
P. Stier
Keyword(s):  
Aerosol Optical Depth ◽  
Optical Depth ◽  
Spatial Scales ◽  
Cloud Condensation Nuclei ◽  
Convective Transport ◽  
Condensation Nuclei ◽  
Gaseous Species ◽  
Climate Effects ◽  
Aerosol Model ◽  
The Impact

Abstract. A fundamental limitation of grid-based models is their inability to resolve variability on scales smaller than a grid box. Past research has shown that significant aerosol variability exists on scales smaller than these grid-boxes, which can lead to discrepancies in simulated aerosol climate effects between high and low resolution models. This study investigates the impact of neglecting sub-grid variability in present-day global microphysical aerosol models on aerosol optical depth (AOD) and cloud condensation nuclei (CCN). We introduce a novel technique to isolate the effect of aerosol variability from other sources of model variability by varying the resolution of aerosol and trace gas fields while maintaining a constant resolution in the rest of the model. We compare WRF-Chem runs in which aerosol and gases are simulated at 80 km and again at 10 km resolutions; in both simulations the other model components, such as meteorology and dynamics, are kept at the 10 km baseline resolution. We find that AOD is underestimated by 13 % and CCN is overestimated by 27 % when aerosol and gases are simulated at 80 km resolution compared to 10 km. Processes most affected by neglecting aerosol sub-grid variability are gas-phase chemistry and aerosol uptake of water through aerosol/gas equilibrium reactions. The inherent non-linearities in these processes result in large changes in aerosol parameters when aerosol and gaseous species are artificially mixed over large spatial scales. These changes in aerosol and gas concentrations are exaggerated by convective transport, which transports these altered concentrations to altitudes where their effect is more pronounced. These results demonstrate that aerosol variability can have a large impact on simulating aerosol climate effects, even when meteorology and dynamics are held constant. Future aerosol model development should focus on accounting for the effect of sub-grid variability on these processes at global scales in order to improve model predictions of the aerosol effect on climate.

scholarly journals OMI tropospheric NO<sub>2</sub> air mass factors over South America: effects of biomass burning aerosols

2015 ◽  
Vol 8 (9) ◽  
pp. 3831-3849 ◽  
Author(s):  
P. Castellanos ◽  
K. F. Boersma ◽  
O. Torres ◽  
J. F. de Haan
Keyword(s):  
Aerosol Optical Depth ◽  
Optical Depth ◽  
Biomass Burning ◽  
Radiative Transfer Model ◽  
Transfer Model ◽  
Air Mass ◽  
Cloud Parameters ◽  
Tropospheric No2 ◽  
The Difference ◽  
Aerosol Parameters

Abstract. Biomass burning is an important and uncertain source of aerosols and NOx (NO + NO2) to the atmosphere. Satellite observations of tropospheric NO2 are essential for characterizing this emissions source, but inaccuracies in the retrieval of NO2 tropospheric columns due to the radiative effects of aerosols, especially light-absorbing carbonaceous aerosols, are not well understood. It has been shown that the O2–O2 effective cloud fraction and pressure retrieval is sensitive to aerosol optical and physical properties, including aerosol optical depth (AOD). Aerosols implicitly influence the tropospheric air mass factor (AMF) calculations used in the NO2 retrieval through the effective cloud parameters used in the independent pixel approximation. In this work, we explicitly account for the effects of biomass burning aerosols in the Ozone Monitoring Instrument (OMI) tropospheric NO2 AMF calculation for cloud-free scenes. We do so by including collocated aerosol extinction vertical profile observations from the CALIOP instrument, and aerosol optical depth (AOD) and single scattering albedo (SSA) retrieved by the OMI near-UV aerosol algorithm (OMAERUV) in the DISAMAR radiative transfer model. Tropospheric AMFs calculated with DISAMAR were benchmarked against AMFs reported in the Dutch OMI NO2 (DOMINO) retrieval; the mean and standard deviation of the difference was 0.6 ± 8 %. Averaged over three successive South American biomass burning seasons (2006–2008), the spatial correlation in the 500 nm AOD retrieved by OMI and the 532 nm AOD retrieved by CALIOP was 0.6, and 68 % of the daily OMAERUV AOD observations were within 30 % of the CALIOP observations. Overall, tropospheric AMFs calculated with observed aerosol parameters were on average 10 % higher than AMFs calculated with effective cloud parameters. For effective cloud radiance fractions less than 30 %, or effective cloud pressures greater than 800 hPa, the difference between tropospheric AMFs based on implicit and explicit aerosol parameters is on average 6 and 3 %, respectively, which was the case for the majority of the pixels considered in our study; 70 % had cloud radiance fraction below 30 %, and 50 % had effective cloud pressure greater than 800 hPa. Pixels with effective cloud radiance fraction greater than 30 % or effective cloud pressure less than 800 hPa corresponded with stronger shielding in the implicit aerosol correction approach because the assumption of an opaque effective cloud underestimates the altitude-resolved AMF; tropospheric AMFs were on average 30–50 % larger when aerosol parameters were included, and for individual pixels tropospheric AMFs can differ by more than a factor of 2. The observation-based approach to correcting tropospheric AMF calculations for aerosol effects presented in this paper depicts a promising strategy for a globally consistent aerosol correction scheme for clear-sky pixels.

Lidar Measurements for Comparison of Atmospheric Aerosol Extinction and Scattering Properties over Lanzhou, China

2011 ◽  
Vol 137 ◽  
pp. 256-261 ◽  
Author(s):  
Xian Jie Cao ◽  
Lei Zhang ◽  
Xiao Jing Quan ◽  
Bi Zhou ◽  
Jing Bao ◽  
...  
Keyword(s):  
Aerosol Optical Depth ◽  
Optical Depth ◽  
Extinction Coefficient ◽  
Atmospheric Aerosol ◽  
Aerosol Extinction ◽  
Vertical Profiles ◽  
Lidar Measurements ◽  
The Difference ◽  
Aerosol Extinction Coefficient ◽  
Semi Arid

The aerosol comparison experiment was conducted in the Semi-Arid Climate and Environment Observatory of Lanzhou University since March to April 2007 with the measurements of two micro-pulse lidars MPL-4B and CE370-2. In the paper, the differences of aerosol extinction coefficient and optical depth retrieved from the observations of MPL-4B and CE370-2 are analyzed, and the results show: the aerosol extinction coefficient retrieved from the observation of MPL-4B is in general smaller than that from CE370-2, and the difference mainly exists in the low layer, while their trends of vertical profiles agree well; the aerosol optical depths from the observations of MPL-4B and CE370-2 correlate linearly rather well with the coefficient of 0.71, and the aerosol optical depth retrieved from the measurement of MPL-4B is less than that from CE370-2 in whole.

scholarly journals Climatological Aspects of Aerosol Physical Characteristics in Tunisia Deduced from Sun Photometric Measurements

2012 ◽  
Vol 2012 ◽  
pp. 1-11 ◽  
Author(s):  
Mabrouk Chaâbane ◽  
Chafai Azri ◽  
Khaled Medhioub
Keyword(s):  
Aerosol Optical Depth ◽  
Optical Depth ◽  
Climatic Data ◽  
Weather Patterns ◽  
Annual Variations ◽  
Microphysical Properties ◽  
Atmospheric Turbidity ◽  
Long Time ◽  
Photometric Measurements ◽  
Aerosol Emissions

Atmospheric and climatic data measured at Thala site (Tunisia) for a long-time period (1977–2001) are used to analyse the monthly, seasonal, and annual variations of the aerosol optical depth at 1 μm wavelength. We have shown that aerosol and microphysical properties and the dominating aerosol types depend on seasons. A comparison of the seasonal cycle of aerosol optical characteristics at Thala site showed that the contribution of long-range transported particles is expected to be larger in summer as a consequence of the weather stability typical of this season. Also, the winter decrease in atmospheric turbidity may result from increases in relative humidity and decreases in temperature, leading to increased particle size and mass and increased fall and deposition velocities. The spring and autumn weather patterns usually carry fine dust and sand particles for the desert area to Thala region. The annual behaviour of the aerosol optical depth recorded a period of stead increase started in 1986 until 2001. Trends in atmospheric turbidity after 1988 could be explained other ways by the contribution of the eruption of Mount Pinatubo in 1991 and by local or regional changes in climate or in aerosol emissions.

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