scholarly journals Light Scattering by Single Natural Ice Crystals

2006 ◽  
Vol 63 (5) ◽  
pp. 1513-1525 ◽  
Author(s):  
Valery Shcherbakov ◽  
Jean-François Gayet ◽  
Brad Baker ◽  
Paul Lawson

Abstract During the South Pole Ice Crystal Experiment, angular scattering intensities (ASIs) of single ice crystals formed in natural conditions were measured for the first time with the polar nephelometer instrument. The microphysical properties of the ice crystals were simultaneously obtained with a cloud particle imager. The observations of the scattering properties of numerous ice crystals reveal high variability of the ASIs in terms of magnitude and distribution over scattering angles. To interpret observed ASI features, lookup tables were computed with a modified ray tracing code, which takes into account the optical geometry of the polar nephelometer. The numerical simulations consider a wide range of input parameters for the description of the ice crystal properties (particle orientation, aspect ratio, surface roughness, and internal inclusions). A new model of surface roughness, which assumes the Weibull statistics, was proposed. The simulations reproduce the overwhelming majority of the observed ASIs features and trace very well the quasi-specular reflection from crystal facets. The discrepancies observed between the model and the experimental data correspond to the rays, which pass through the ice crystal and are scattered toward the backward angles. This feature may be attributed to the internal structure of the ice crystals that should be considered in modeling refinements.

2020 ◽  
Vol 13 (3) ◽  
pp. 1273-1285 ◽  
Author(s):  
Thomas Kuhn ◽  
Sandra Vázquez-Martín

Abstract. Accurate predictions of snowfall require good knowledge of the microphysical properties of the snow ice crystals and particles. Shape is an important parameter as it strongly influences the scattering properties of the ice particles, and thus their response to remote sensing techniques such as radar measurements. The fall speed of ice particles is another important parameter for both numerical forecast models as well as representation of ice clouds and snow in climate models, as it is responsible for the rate of removal of ice from these models. We describe a new ground-based in situ instrument, the Dual Ice Crystal Imager (D-ICI), to determine snow ice crystal properties and fall speed simultaneously. The instrument takes two high-resolution pictures of the same falling ice particle from two different viewing directions. Both cameras use a microscope-like setup resulting in an image pixel resolution of approximately 4 µm pixel−1. One viewing direction is horizontal and is used to determine fall speed by means of a double exposure. For this purpose, two bright flashes of a light-emitting diode behind the camera illuminate the falling ice particle and create this double exposure, and the vertical displacement of the particle provides its fall speed. The other viewing direction is close-to-vertical and is used to provide size and shape information from single-exposure images. This viewing geometry is chosen instead of a horizontal one because shape and size of ice particles as viewed in the vertical direction are more relevant than these properties viewed horizontally, as the vertical fall speed is more strongly influenced by the vertically viewed properties. In addition, a comparison with remote sensing instruments that mostly have a vertical or close-to-vertical viewing geometry is favoured when the particle properties are measured in the same direction. The instrument has been tested in Kiruna, northern Sweden (67.8∘ N, 20.4∘ E). Measurements are demonstrated with images from different snow events, and the determined snow ice crystal properties are presented.


2014 ◽  
Vol 14 (22) ◽  
pp. 12357-12371 ◽  
Author(s):  
N. B. Magee ◽  
A. Miller ◽  
M. Amaral ◽  
A. Cumiskey

Abstract. Here we show high-magnification images of hexagonal ice crystals acquired by environmental scanning electron microscopy (ESEM). Most ice crystals were grown and sublimated in the water vapor environment of an FEI-Quanta-200 ESEM, but crystals grown in a laboratory diffusion chamber were also transferred intact and imaged via ESEM. All of these images display prominent mesoscopic topography including linear striations, ridges, islands, steps, peaks, pits, and crevasses; the roughness is not observed to be confined to prism facets. The observations represent the most highly magnified images of ice surfaces yet reported and expand the range of conditions in which rough surface features are known to be conspicuous. Microscale surface topography is seen to be ubiquitously present at temperatures ranging from −10 °C to −40 °C, in supersaturated and subsaturated conditions, on all crystal facets, and irrespective of substrate. Despite the constant presence of surface roughness, the patterns of roughness are observed to be dramatically different between growing and sublimating crystals, and transferred crystals also display qualitatively different patterns of roughness. Crystals are also demonstrated to sometimes exhibit inhibited growth in moderately supersaturated conditions following exposure to near-equilibrium conditions, a phenomenon interpreted as evidence of 2-D nucleation. New knowledge about the characteristics of these features could affect the fundamental understanding of ice surfaces and their physical parameterization in the context of satellite retrievals and cloud modeling. Links to supplemental videos of ice growth and sublimation are provided.


2014 ◽  
Vol 7 (10) ◽  
pp. 10249-10292 ◽  
Author(s):  
A. Korolev ◽  
P. R. Field

Abstract. Shattering presents a serious obstacle to current airborne in-situ methods of characterizing the microphysical properties of ice clouds. Small shattered fragments result from the impact of natural ice crystals with the forward parts of aircraft-mounted measurement probes. The presence of these shattered fragments may result in a significant overestimation of the measured concentration of small ice crystals, contaminating the measurement of the ice particle size distribution (PSD). One method of identifying shattered particles is to use an interarrival time algorithm. This method is based on the assumption that shattered fragments form spatial clusters that have short interarrival times between particles, relative to natural particles, when they pass through the sample volume of the probe. The interarrival time algorithm is a successful technique for the classification of shattering artifacts and natural particles. This study assesses the limitations and efficiency of the interarrival time algorithm. The analysis has been performed using simultaneous measurements of 2-D optical array probes with the standard and antishattering "K-tips" collected during the Airborne Icing Instrumentation Experiment (AIIE). It is shown that the efficiency of the algorithm depends on ice particle size, concentration and habit. Additional numerical simulations indicate that the effectiveness of the interarrival time algorithm to eliminate shattering artifacts can be significantly restricted in some cases. Improvements to the interarrival time algorithm are discussed.


2019 ◽  
Author(s):  
Thomas Kuhn ◽  
Sandra Vázquez-Martín

Abstract. Accurate predictions of snowfall require good knowledge of the microphysical properties of the snow ice crystals and particles. Shape is an important parameter as it influences strongly the scattering properties of the ice particles, and thus their response to remote sensing techniques such as radar measurements. The fall speed of ice particles is another important parameter for both numerical forecast models as well as representation of ice clouds and snow in climate models, as it is responsible for the rate of removal of ice from these models. We describe a new ground-based in-situ instrument, the Dual Ice Crystal Imager (D-ICI), to determine snow ice crystal properties and fall speed simultaneously. The instrument takes two high-resolution pictures of the same falling ice particle from two different viewing directions. Both cameras use a microscope-like set-up resulting in an image pixel resolution of approximately 4 μm/pixel. One viewing direction is horizontal and is used to determine fall speed by means of a double exposure. For this purpose, two bright flashes of a light emitting diode behind the camera illuminate the falling ice particle and create this double exposure and the vertical displacement of the particle provides its fall speed. The other viewing direction is close to vertical and is used to provide size and shape information from single-exposure images. This viewing geometry is chosen instead of a horizontal one because shape and size of ice particles as viewed in the vertical direction are more relevant than these properties viewed horizontally as the vertical fall speed is more strongly influenced by the vertically viewed properties. In addition, a comparison with remote sensing instruments that mostly have a vertical or close to vertical viewing geometry is favoured when the particle properties are measured in the same direction. The instrument has been tested in Kiruna, northern Sweden (67.8° N, 20.4° E). Measurements are demonstrated with images from different snow events, and the determined snow ice crystal properties are presented.


2014 ◽  
Vol 14 (6) ◽  
pp. 8393-8418 ◽  
Author(s):  
N. B. Magee ◽  
A. Miller ◽  
M. Amaral ◽  
A. Cumiskey

Abstract. Here we show high-magnification images of hexagonal ice crystals acquired by Environmental Scanning Electron Microscopy (ESEM). Most ice crystals were grown and sublimated in the water vapor environment of an FEI-Quanta-200 ESEM, but crystals grown in a laboratory diffusion chamber were also transferred intact and imaged via ESEM. All of these images display prominent mesoscopic topography including linear striations, ridges, islands, steps, peaks, pits, and crevasses; the roughness is not observed to be confined to prism facets. The observations represent the most highly magnified images of ice surfaces yet reported and expand the range of conditions where the rough surface features are known to be conspicuous. Microscale surface topography is seen to be ubiquitously present at temperatures ranging from −10 °C to −40 °C, at super-saturated and sub-saturated conditions, on all crystal facets, and irrespective of substrate. Despite the constant presence of surface roughness, the patterns of roughness are observed to be dramatically different between growing and sublimating crystals, and transferred crystals also display qualitatively different patterns of roughness. Crystals are also demonstrated to sometimes exhibit inhibited growth in moderately supersaturated conditions following exposure to near-equilibrium conditions, a phenomena interpreted as evidence of 2-D nucleation. New knowledge of the characteristics of these features could affect the fundamental understanding of ice surfaces and their physical parameterization in the context of satellite retrievals and cloud modeling. Links to Supplement videos of ice growth and sublimation are provided.


Author(s):  
Zepei Wu ◽  
Shuo Liu ◽  
Delong Zhao ◽  
Ling Yang ◽  
Zixin Xu ◽  
...  

AbstractCloud particles have different shapes in the atmosphere. Research on cloud particle shapes plays an important role in analyzing the growth of ice crystals and the cloud microphysics. To achieve an accurate and efficient classification algorithm on ice crystal images, this study uses image-based morphological processing and principal component analysis, to extract features of images and apply intelligent classification algorithms for the Cloud Particle Imager (CPI). Currently, there are mainly two types of ice-crystal classification methods: one is the mode parameterization scheme, and the other is the artificial intelligence model. Combined with data feature extraction, the dataset was tested on ten types of classifiers, and the highest average accuracy was 99.07%. The fastest processing speed of the real-time data processing test was 2,000 images/s. In actual application, the algorithm should consider the processing speed, because the images are in the order of millions. Therefore, a support vector machine (SVM) classifier was used in this study. The SVM-based optimization algorithm can classify ice crystals into nine classes with an average accuracy of 95%, blurred frame accuracy of 100%, with a processing speed of 2,000 images/s. This method has a relatively high accuracy and faster classification processing speed than the classic neural network model. The new method could be also applied in physical parameter analysis of cloud microphysics.


2016 ◽  
Vol 9 (8) ◽  
pp. 3817-3836 ◽  
Author(s):  
Naruki Hiranuma ◽  
Ottmar Möhler ◽  
Gourihar Kulkarni ◽  
Martin Schnaiter ◽  
Steffen Vogt ◽  
...  

Abstract. Separation of particles that play a role in cloud activation and ice nucleation from interstitial aerosols has become necessary to further understand aerosol-cloud interactions. The pumped counterflow virtual impactor (PCVI), which uses a vacuum pump to accelerate the particles and increase their momentum, provides an accessible option for dynamic and inertial separation of cloud elements. However, the use of a traditional PCVI to extract large cloud hydrometeors is difficult mainly due to its small cut-size diameters (< 5 µm). Here, for the first time we describe a development of an ice-selecting PCVI (IS-PCVI) to separate ice in controlled mixed-phase cloud system based on the particle inertia with the cut-off diameter  ≥  10 µm. We also present its laboratory application demonstrating the use of the impactor under a wide range of temperature and humidity conditions. The computational fluid dynamics simulations were initially carried out to guide the design of the IS-PCVI. After fabrication, a series of validation laboratory experiments were performed coupled with the Aerosol Interaction and Dynamics in the Atmosphere (AIDA) expansion cloud simulation chamber. In the AIDA chamber, test aerosol particles were exposed to the ice supersaturation conditions (i.e., RHice > 100 %), where a mixture of droplets and ice crystals was formed during the expansion experiment. In parallel, the flow conditions of the IS-PCVI were actively controlled, such that it separated ice crystals from a mixture of ice crystals and cloud droplets, which were of diameter  ≥  10 µm. These large ice crystals were passed through the heated evaporation section to remove the water content. Afterwards, the residuals were characterized with a suite of online and offline instruments downstream of the IS-PCVI. These results were used to assess the optimized operating parameters of the device in terms of (1) the critical cut-size diameter, (2) the transmission efficiency and (3) the counterflow-to-input flow ratio. Particle losses were characterized by comparing the residual number concentration to the rejected interstitial particle number concentration. Overall results suggest that the IS-PCVI enables inertial separation of particles with a volume-equivalent particle size in the range of  ~ 10–30 µm in diameter with small inadvertent intrusion (~  5 %) of unwanted particles.


2016 ◽  
Author(s):  
Naruki Hiranuma ◽  
Ottmar Möhler ◽  
Gourihar Kulkarni ◽  
Martin Schnaiter ◽  
Steffen Vogt ◽  
...  

Abstract. Separation of particles that play a role in cloud activation and ice nucleation from interstitial aerosols has become necessary to further understand aerosol-cloud interactions. The pumped counterflow virtual impactor (PCVI), which uses a vacuum pump to accelerate the particles and increase their momentum, provides an accessible option for dynamic and inertial separation of cloud elements. However, the use of a traditional PCVI to extract large size cloud hydrometeors is difficult mainly due to its small cut-size diameters (< 5 µm). Here, for the first time we describe a development of an ice-selecting PCVI (IS-PCVI) to separate ice in the controlled mixed-phase cloud system based on the particle inertia with the cut-off diameter > 10 µm. We also present its laboratory application demonstrating the use of the impactor under a wide range of temperature and humidity conditions. The computational fluid dynamics (CFD) simulations were initially carried out to guide the design of the IS-PCVI. After fabrication, a series of validation laboratory experiments were performed coupled with the Aerosol Interaction and Dynamics in the Atmosphere (AIDA) expansion cloud simulation chamber. In the AIDA chamber, test aerosol particles were exposed to the ice supersaturation conditions (i.e., RHice > 100 %), where a mixture of droplets and ice crystals was formed during the expansion experiment. In parallel, the flow conditions of the IS-PCVI were actively controlled, such that it separated ice crystals from a mixture of ice crystals and cloud droplets, which were of size ≥ 10 µm. These large ice crystals were passed through the heated evaporation section to remove the water content. Afterwards, the residuals were characterized with a suite of online and offline instruments downstream of the IS-PCVI. These results were used to assess the optimized operating parameters of the device in terms of (1) the critical cut-size diameter, (2) the transmission efficiency and (3) the counterflow-to-input flow ratio. Particle losses were characterized by comparing the residual number concentration to the rejected interstitial particle number concentration. Overall results suggest that the IS-PCVI enables inertial separation of particles with a volume-equivalent particle size in the range of ~ 10–30 µm in diameter with small inadvertent intrusion (~ 5 %) of unwanted particles.


2017 ◽  
Vol 56 (2) ◽  
pp. 433-453 ◽  
Author(s):  
Oliver Schlenczek ◽  
Jacob P. Fugal ◽  
Gary Lloyd ◽  
Keith N. Bower ◽  
Thomas W. Choularton ◽  
...  

AbstractDuring the Cloud and Aerosol Characterization Experiment (CLACE) 2013 field campaign at the High Altitude Research Station Jungfraujoch, Switzerland, optically thin pure ice clouds and ice crystal precipitation were measured using holographic and other in situ particle instruments. For cloud particles, particle images, positions in space, concentrations, and size distributions were obtained, allowing one to extract size distributions classified by ice crystal habit. Small ice crystals occurring under conditions with a vertically thin cloud layer above and a stratocumulus layer approximately 1 km below exhibit similar properties in size and crystal habits as Antarctic/Arctic diamond dust. Also, ice crystal precipitation stemming from midlevel clouds subsequent to the diamond dust event was observed with a larger fraction of ice crystal aggregates when compared with the diamond dust. In another event, particle size distributions could be derived from mostly irregular ice crystals and aggregates, which likely originated from surface processes. These particles show a high spatial and temporal variability, and it is noted that size and habit distributions have only a weak dependence on the particle number concentration. Larger ice crystal aggregates and rosette shapes of some hundred microns in maximum dimension could be sampled as a precipitating cirrostratus cloud passed the site. The individual size distributions for each habit agree well with lognormal distributions. Fitted parameters to the size distributions are presented along with the area-derived ice water content, and the size distributions are compared with other measurements of pure ice clouds made in the Arctic and Antarctic.


2015 ◽  
Vol 8 (2) ◽  
pp. 761-777 ◽  
Author(s):  
A. Korolev ◽  
P. R. Field

Abstract. Shattering presents a serious obstacle to current airborne in situ methods of characterizing the microphysical properties of ice clouds. Small shattered fragments result from the impact of natural ice crystals with the forward parts of aircraft-mounted measurement probes. The presence of these shattered fragments may result in a significant overestimation of the measured concentration of small ice crystals, contaminating the measurement of the ice particle size distribution (PSD). One method of identifying shattered particles is to use an inter-arrival time algorithm. This method is based on the assumption that shattered fragments form spatial clusters that have short inter-arrival times between particles, relative to natural particles, when they pass through the sample volume of the probe. The inter-arrival time algorithm is a successful technique for the classification of shattering artifacts and natural particles. This study assesses the limitations and efficiency of the inter-arrival time algorithm. The analysis has been performed using simultaneous measurements of two-dimensional (2-D) optical array probes with the standard and antishattering "K-tips" collected during the Airborne Icing Instrumentation Experiment (AIIE). It is shown that the efficiency of the algorithm depends on ice particle size, concentration and habit. Additional numerical simulations indicate that the effectiveness of the inter-arrival time algorithm to eliminate shattering artifacts can be significantly restricted in some cases. Improvements to the inter-arrival time algorithm are discussed. It is demonstrated that blind application of the inter-arrival time algorithm cannot filter out all shattered aggregates. To mitigate against the effects of shattering, the inter-arrival time algorithm should be used together with other means, such as antishattering tips and specially designed algorithms for segregation of shattered artifacts and natural particles.


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