scholarly journals Radiative Impacts of Aerosols During COVID-19 Lockdown Period Over the Indian Region

2021 ◽  
Vol 9 ◽  
Author(s):  
Rohini L. Bhawar ◽  
Suvarna Fadnavis ◽  
Vinay Kumar ◽  
P. R. C. Rahul ◽  
Tushar Sinha ◽  
...  

The COVID-19 lockdown restrictions influenced global atmospheric aerosols. We report aerosol variations over India using multiple remote sensing datasets [Moderate Resolution Imaging Spectroradiometer (MODIS), Ozone Monitoring Instrument (OMI), Cloud-Aerosol Lidar, and Infrared Pathfinder (CALIPSO)], and model reanalysis [Copernicus Atmosphere Monitoring Service (CAMS)] during the lockdown implemented during the COVID-19 pandemic outbreak period from March 25 to April 14, 2020. Our analysis shows that, during this period, MODIS and CALIPSO showed a 30–40% reduction in aerosol optical depth (AOD) over the Indo-Gangetic Plain (IGP) with respect to decadal climatology (2010–2019). The absorbing aerosol index and dust optical depth measurements also showed a notable reduction over the Indian region, highlighting less emission of anthropogenic dust and also a reduced dust transport from West Asia during the lockdown period. On the contrary, central India showed an ∼12% AOD enhancement. CALIPSO measurements revealed that this increase was due to transported biomass burning aerosols. Analysis of MODIS fire data product and CAMS fire fluxes (black carbon, SO2, organic carbon, and nitrates) showed intense fire activity all over India but densely clustered over central India. Thus, we show that the lockdown restrictions implemented at the government level have significantly improved the air quality over northern India but fires offset its effects over central India. The biomass-burning aerosols formed a layer near 2–4 km (AOD 0.08–0.1) that produced heating at 3–4 K/day and a consequent negative radiative forcing at the surface of ∼−65 W/m2 (±40 W/m2) over the central Indian region.

2021 ◽  
Author(s):  
Kanishtha Dubey ◽  
Shubha Verma

<p>The study investigates the chemical composition and source of aerosol origin at a semi-urban (Kharagpur–Kgp) and urban (Kolkata–Kol) region during the period February 2015 to January 2016 and September 2010 to August 2011 respectively. Major water-soluble inorganic aerosols (WSII) were determined using Ion chromatography and carbonaceous aerosols (CA) using OC–EC analyser. A multivariate factor analysis Positive Matrix Factorization (PMF) was used in resolving source of aerosols at the study locations. Seasonal analysis of WSII at Kgp and Kol indicated relative dominance of calcium at both the places followed by sodium, chloride, and magnesium ions. Non-sea salt potassium (nss–K<sup>+</sup>), a biomass burning tracer was found higher at Kol than at Kgp. Sum of secondary aerosols sulphate (SO<sub>4</sub><sup>2-</sup>), nitrate (NO<sub>3</sub><sup>-</sup>) and ammonium (NH<sub>4</sub><sup>+</sup>) was higher at Kol than Kgp with relative concentration of SO<sub>4</sub><sup>2-</sup> being higher than NO<sub>3</sub><sup>-</sup> at Kgp which was vice-versa at Kol. Examination of carbonaceous aerosols showed three times higher concentration of organic carbon (OC) than elemental carbon (EC) with monthly mean of OC/EC ratio > 2, indicating likely formation of secondary organic carbon formation. Seasonal influence of biomass burning inferred from nss–K<sup>+</sup> (OC/EC) ratio relationship indicated dissimilarity in seasonality of biomass burning at Kgp (Kol). PMF resolved sources for Kgp constituted of secondary aerosol emissions, biomass burning, fugitive dust, marine aerosols, crustal dust and emissions from brick kilns while for Kol factors constituted of burning of waste, resuspended paved road dust, coal combustion, sea spray aerosols, vehicular emissions and biomass burning.</p>


Atmosphere ◽  
2018 ◽  
Vol 9 (10) ◽  
pp. 405 ◽  
Author(s):  
Shreemat Shrestha ◽  
Murray Peel ◽  
Graham Moore

The assessment of direct radiative forcing due to atmospheric aerosols (ADRF) in the Indo Gangetic Plain (IGP), which is a food basket of south Asia, is important for measuring the effect of atmospheric aerosols on the terrestrial ecosystem and for assessing the effect of aerosols on crop production in the region. Existing comprehensive analytical models to estimate ADRF require a large number of input parameters and high processing time. In this context, here, we develop a simple model to estimate daily ADRF at any location on the surface of the IGP through multiple regressions of AErosol RObotic NETwork (AERONET) aerosol optical depth (AOD) and atmospheric water vapour using data from 2002 to 2015 at 10 stations in the IGP. The goodness of fit of the model is indicated by an adjusted R2 value of 0.834. The Jackknife method of deleting one group (station data) was employed to cross validate and study the stability of the regression model. It was found to be robust with an adjusted R2 fluctuating between 0.813 and 0.842. In order to use the year-round ADRF model for locations beyond the AERONET stations in the IGP, AOD, and atmospheric water vapour products from MODIS Aqua and Terra were compared against AERONET station data and they were found to be similar. Using MODIS Aqua and Terra products as input, the year-round ADRF regression was evaluated at the IGP AERONET stations and found to perform well with Pearson correlation coefficients of 0.66 and 0.65, respectively. Using ADRF regression model with MODIS inputs allows for the estimation of ADRF across the IGP for assessing the aerosol impact on ecosystem and crop production.


2012 ◽  
Vol 12 (11) ◽  
pp. 5129-5145 ◽  
Author(s):  
O. E. García ◽  
J. P. Díaz ◽  
F. J. Expósito ◽  
A. M. Díaz ◽  
O. Dubovik ◽  
...  

Abstract. The shortwave radiative forcing (ΔF) and the radiative forcing efficiency (ΔFeff) of natural and anthropogenic aerosols have been analyzed using estimates of radiation both at the Top (TOA) and at the Bottom Of Atmosphere (BOA) modeled based on AERONET aerosol retrievals. Six main types of atmospheric aerosols have been compared (desert mineral dust, biomass burning, urban-industrial, continental background, oceanic and free troposphere) in similar observational conditions (i.e., for solar zenith angles between 55° and 65°) in order to compare the nearly same solar geometry. The instantaneous ΔF averages obtained vary from −122 ± 37 Wm−2 (aerosol optical depth, AOD, at 0.55 μm, 0.85 ± 0.45) at the BOA for the mixture of desert mineral dust and biomass burning aerosols in West Africa and −42 ± 22 Wm−2 (AOD = 0.9 ± 0.5) at the TOA for the pure mineral dust also in this region up to −6 ± 3 Wm−2 and −4 ± 2 Wm−2 (AOD = 0.03 ± 0.02) at the BOA and the TOA, respectively, for free troposphere conditions. This last result may be taken as reference on a global scale. Furthermore, we observe that the more absorbing aerosols are overall more efficient at the BOA in contrast to at the TOA, where they backscatter less solar energy into the space. The analysis of the radiative balance at the TOA shows that, together with the amount of aerosols and their absorptive capacity, it is essential to consider the surface albedo of the region on which they are. Thus, we document that in regions with high surface reflectivity (deserts and snow conditions) atmospheric aerosols lead to a warming of the Earth-atmosphere system.


1970 ◽  
Vol 8 (3) ◽  
pp. 11-24 ◽  
Author(s):  
Deepti Sharma ◽  
Manjit Singh ◽  
Darshan Singh

The present study deals with impact of post-harvest biomass burning on aerosol characteristics over Patiala (Lat: 30.33°N; Long: 76.4°E), Punjab state, India during 2008-09, using ground based and satellite data. Results of Aerosol Optical Depth (AOD) measurements using MICROTOPS II show significant variations with highest AOD500 ≈2.65 in October 2008 and ≈1.71 in November 2009. The maximum monthly mean values of angstrom parameters “α” and “β” are 1.13±0.16 and 0.39±0.20, respectively. Daily averaged values of Black Carbon (BC) mass concentration during day time show significant variations (8-18μg/m³) yielding SSA varying from 0.76-0.88 during highly turbid days and 0.95-0.97 during less turbid days. During highly turbid days, the estimated atmospheric radiative forcing using SBDART varies from +43.0 to +86.5Wm-2 suggesting high BC concentration in the atmosphere associated with paddy residue burning in the fields. DOI: http://dx.doi.org/10.3126/jie.v8i3.5927 JIE 2011; 8(3): 11-24


2002 ◽  
Vol 20 (12) ◽  
pp. 2105-2109 ◽  
Author(s):  
S. K. Satheesh

Abstract. It is now clearly understood that atmospheric aerosols have a significant impact on climate due to their important role in modifying the incoming solar and outgoing infrared radiation. The question of whether aerosol cools (negative forcing) or warms (positive forcing) the planet depends on the relative dominance of absorbing aerosols. Recent investigations over the tropical Indian Ocean have shown that, irrespective of the comparatively small percentage contribution in optical depth ( ~ 11%), soot has an important role in the overall radiative forcing. However, when the amount of absorbing aerosols such as soot are significant, aerosol optical depth and chemical composition are not the only determinants of aerosol climate effects, but the altitude of the aerosol layer and the altitude and type of clouds are also important. In this paper, the aerosol forcing in the presence of clouds and the effect of different surface types (ocean, soil, vegetation, and different combinations of soil and vegetation) are examined based on model simulations, demonstrating that aerosol forcing changes sign from negative (cooling) to positive (warming) when reflection from below (either due to land or clouds) is high.Key words. Atmospheric composition and structure (aerosols and particles) History of Geophysics (atmospheric sciences) Hydrology (anthropogenic effects)


2018 ◽  
Author(s):  
Nandita Singh ◽  
Tirthankar Banerjee ◽  
Made P. Raju ◽  
Karine Deboudt ◽  
Meytar Sorek-Hamer ◽  
...  

Abstract. The large-scale emissions of airborne particulates from burning of agricultural residues particularly over the upper Indo-Gangetic Plain (IGP) have often been associated with frequent formation of haze, adverse health impacts, modification in aerosol climatology and thereby aerosols impact on regional climate. In this study, short-term variations in aerosol climatology during extreme biomass burning emissions over IGP, and thereby to regional climate were investigated. Size-segregated particulate concentration was initially measured and submicron particles (PM1.1) were found to dominate particulate mass within the fine mode (PM2.1). Particulate bound water-soluble ions were mainly secondary in nature, primarily composed of sulfate and nitrate. There was evidence of gaseous NH3 dominating neutralization of acidic aerosol species (SO42−) in submicron particles, in contrast to crustal dominating neutralization in coarser particulates. Variation in black carbon mass ratio was found to be influenced by local sources, while sudden increase in concentration was consistent with high Delta-C, referring to biogenic emissions. Influence of biomass burning emissions were established using specific organic (levoglucosan), inorganic (K+ and NH4+) and satellite (UV Aerosol Index, UVAI) tracers. Levoglucosan was the most abundant within submicron particles (649±177 ng m−3), with a very high ratio (>50) against other anhydrosugars, indicating exclusive emissions from burning of agriculture residues. Temporal variations of all the tracers were consistent, while NH4+ was more closely associated to levoglucosan. Spatio-temporal distribution of aerosol and few trace gases (CO and NO2) were evaluated using both space-borne active and passive sensors, and a significant increase in columnar aerosol loading (AOD: 0.98) was evident during extreme biomass burning emissions, with presence of absorbing aerosols (UVAI > 1.5) having low aerosol layer height (~1.5 km). A strong intraseasonality in aerosol cross-sectional altitudinal profile was even noted from CALIPSO, referring dominance of smoke and polluted continental aerosols across IGP. Possible transport mechanism of biomass smoke was established using cluster analysis and concentration weighted of air mass back-trajectories. Short-wave aerosol radiative forcing (ARF) was further simulated considering intraseasonality in aerosol properties, which resulted in considerable increase of atmospheric ARF (135 Wm−2) and heating rate (4.3 K day−1) during extreme biomass burning emissions compared to non-dominating one (56 Wm−2, 1.8 K day−1). We therefore conclude that influence of biomass burning emissions on regional aerosol climatology must need to be studied in much finer scale to improve parameterization of aerosol/-climate model across the region.


2018 ◽  
Vol 18 (12) ◽  
pp. 8829-8848 ◽  
Author(s):  
Justyna Lisok ◽  
Anna Rozwadowska ◽  
Jesper G. Pedersen ◽  
Krzysztof M. Markowicz ◽  
Christoph Ritter ◽  
...  

Abstract. The aim of the presented study was to investigate the impact on the radiation budget of a biomass-burning plume, transported from Alaska to the High Arctic region of Ny-Ålesund, Svalbard, in early July 2015. Since the mean aerosol optical depth increased by the factor of 10 above the average summer background values, this large aerosol load event is considered particularly exceptional in the last 25 years. In situ data with hygroscopic growth equations, as well as remote sensing measurements as inputs to radiative transfer models, were used, in order to estimate biases associated with (i) hygroscopicity, (ii) variability of single-scattering albedo profiles, and (iii) plane-parallel closure of the modelled atmosphere. A chemical weather model with satellite-derived biomass-burning emissions was applied to interpret the transport and transformation pathways. The provided MODTRAN radiative transfer model (RTM) simulations for the smoke event (14:00 9 July–11:30 11 July) resulted in a mean aerosol direct radiative forcing at the levels of −78.9 and −47.0 W m−2 at the surface and at the top of the atmosphere, respectively, for the mean value of aerosol optical depth equal to 0.64 at 550 nm. This corresponded to the average clear-sky direct radiative forcing of −43.3 W m−2, estimated by radiometer and model simulations at the surface. Ultimately, uncertainty associated with the plane-parallel atmosphere approximation altered results by about 2 W m−2. Furthermore, model-derived aerosol direct radiative forcing efficiency reached on average −126 W m-2/τ550 and −71 W m-2/τ550 at the surface and at the top of the atmosphere, respectively. The heating rate, estimated at up to 1.8 K day−1 inside the biomass-burning plume, implied vertical mixing with turbulent kinetic energy of 0.3 m2 s−2.


2019 ◽  
Vol 19 (18) ◽  
pp. 11865-11886 ◽  
Author(s):  
Harshavardhana Sunil Pathak ◽  
Sreedharan Krishnakumari Satheesh ◽  
Ravi Shankar Nanjundiah ◽  
Krishnaswamy Krishna Moorthy ◽  
Sivaramakrishnan Lakshmivarahan ◽  
...  

Abstract. Improving the accuracy of regional aerosol climate impact assessment calls for improvement in the accuracy of regional aerosol radiative effect (ARE) estimation. One of the most important means of achieving this is to use spatially homogeneous and temporally continuous datasets of critical aerosol properties, such as spectral aerosol optical depth (AOD) and single scattering albedo (SSA), which are the most important parameters for estimating aerosol radiative effects. However, observations do not provide the above; the space-borne observations though provide wide spatial coverage, are temporal snapshots and suffer from possible sensor degradation over extended periods. On the other hand, the ground-based measurements provide more accurate and temporally continuous data but are spatially near-point observations. Realizing the need for spatially homogeneous and temporally continuous datasets on one hand and the near non-existence of such data over the south Asian region (which is one of the regions where aerosols show large heterogeneity in most of their properties), construction of accurate gridded aerosol products by synthesizing the long-term space-borne and ground-based data has been taken up as an important objective of the South West Asian Aerosol Monsoon Interactions (SWAAMI), a joint Indo-UK field campaign, aiming at characterizing aerosol–monsoon links and their variabilities over the Indian region. In Part 1 of this two-part paper, we present spatially homogeneous gridded datasets of AOD and absorption aerosol optical depth (AAOD), generated for the first time over this region. These data products are developed by merging the highly accurate aerosol measurements from the dense networks of 44 (for AOD) and 34 (for AAOD) ground-based observatories of Aerosol Radiative Forcing over India NETwork (ARFINET) and AErosol RObotic NETwork (AERONET) spread across the Indian region, with satellite-retrieved AOD and AAOD, following statistical assimilation schemes. The satellite data used for AOD assimilation include AODs retrieved from MODerate Imaging Spectroradiometer (MODIS) and Multiangle Imaging SpectroRadiometer (MISR) over the same domain. For AAOD, the ground-based black carbon (BC) mass concentration measurements from the network of 34 ARFINET observatories and satellite-based (Kalpana-1, INSAT-3A) infrared (IR) radiance measurements are blended with gridded AAODs (500 nm, monthly mean) derived from Ozone Monitoring Instrument (OMI)-retrieved AAODs (at 354 and 388 nm). The details of the assimilation methods and the gridded datasets generated are presented in this paper. The merged gridded AOD and AAOD products thus generated are validated against the data from independent ground-based observatories, which were not used for the assimilation process but are representative of different subregions of the complex domain. This validation exercise revealed that the independent ground-based measurements are better confirmed by merged datasets than the respective satellite products. As ensured by assimilation techniques employed, the uncertainties in merged AODs and AAODs are significantly less than those in corresponding satellite products. These merged products also all exhibit important large-scale spatial and temporal features which are already reported for this region. Nonetheless, the merged AODs and AAODs are significantly different in magnitude from the respective satellite products. On the background of above-mentioned quality enhancements demonstrated by merged products, we have employed them for deriving the columnar SSA and analysed its spatiotemporal characteristics. The columnar SSA thus derived has demonstrated distinct seasonal variation over various representative subregions of the study domain. The uncertainties in the derived SSA are observed to be substantially less than those in OMI SSA. On the backdrop of these benefits, the merged datasets are employed for the estimation of regional aerosol radiative effects (direct), the results of which would be presented in a companion paper, Part 2 of this two-part paper.


2019 ◽  
Vol 11 (15) ◽  
pp. 1738 ◽  
Author(s):  
Chin-An Lin ◽  
Yi-Chun Chen ◽  
Chian-Yi Liu ◽  
Wei-Ting Chen ◽  
John H. Seinfeld ◽  
...  

Intense economic and industrial development in China has been accompanied by severe local air pollution, as well as in other downwind countries in East Asia. This study analyzes satellite observational data of sulfur dioxide (SO2), nitrogen dioxide (NO2), and aerosol optical depth (AOD) to explore the spatial distribution, long-term temporal variation, and correlation to meteorological conditions over this region over the period 2005–2015. SO2 and NO2 data are retrieved from the ozone monitoring instrument (OMI) onboard the National Aeronautics and Space Administration (NASA) Aura satellite, while AOD data are from the moderate-resolution imaging spectroradiometer (MODIS) onboard the NASA Aqua satellite. Spatial distributions of SO2, NO2, and AOD show the highest levels in the North China Plain (NCP), with hotspots also in Southeastern China (SC) and the Sichuan Basin (SB). Biomass burning also contributes to a high level of AOD in Southeast Asia in spring and in Equatorial Asia in fall. Considering the correlation of pollutant levels to meteorological conditions, monitoring data show that higher temperature and higher relative humidity (RH) favor the conversion of SO2 and NO2 to sulfate and nitrate aerosol, respectively. The impact of stronger lower tropospheric stability facilitates the accumulation of SO2 and NO2 in NCP and SC. Transport of SO2 and NO2 from intense source regions to relatively clean regions is highly influential over East Asia; such transport from the NCP leads to a considerable increase of pollutants in SC, SB, Taiwan Island (TW), and Taiwan Strait (TWS), particularly in winter. Aerosols generated by biomass burning in Southeast Asia and anthropogenic aerosol in SC are transported to TW and TWS and lead to the increase of AOD, with the highest levels of AOD in SC, TW, and TWS occurring in spring. Precipitation results in the removal of pollutants, especially in highly polluted regions, the effect of which is most significant in winter and spring.


Sign in / Sign up

Export Citation Format

Share Document