scholarly journals Ultrafast Deep-Ultraviolet Laser-Induced Voltage Response of Pyrite

Micromachines ◽  
2021 ◽  
Vol 12 (12) ◽  
pp. 1555
Author(s):  
Xuecong Liu ◽  
Yudong Li ◽  
Haoqiang Wu ◽  
Yawen Yu ◽  
Honglei Zhan ◽  
...  
Keyword(s):  
Laser Energy ◽  
Low Cost ◽  
Response Speed ◽  
Voltage Response ◽  
Induced Voltage ◽  
High Concentration ◽  
Uv Photodetectors ◽  
Practical Applications ◽  
Production Processes ◽  
Deep Ultraviolet

Ultrafast, high-sensitivity deep-ultraviolet (UV) photodetectors are crucial for practical applications, including optical communication, ozone layer monitoring, flame detection, etc. However, fast-response UV photodetectors based on traditional materials suffer from issues of expensive production processes. Here, we focused on pyrite with simultaneously cheap production processes and ultrafast response speed. Nanoseconds photovoltaic response was observed under UV pulsed laser irradiation without an applied bias at room temperature. In addition, the response time of the laser-induced voltage (LIV) signals was ~20 ns, which was the same as the UV laser pulse width. The maximum value of the responsivity is 0.52 V/mJ and the minimum value of detectivity was about to ~1.4 × 1013 Jones. When there exists nonuniform illumination, a process of diffusion occurs by which the carriers migrate from the region of high concentration toward the region of low concentration. The response speed is limited by a factor of the diffusion of the carriers. With an increment in laser energy, the response speed of LIV is greatly improved. The high response speed combined with low-cost fabrication makes these UV photodetectors highly attractive for applications in ultrafast detection.

scholarly journals Solar-blind deep-ultraviolet photodetectors based on solution-synthesized quasi-2D Te nanosheets

Nanophotonics ◽  
2020 ◽  
Vol 9 (8) ◽  
pp. 2459-2466 ◽  
Author(s):  
Rui Cao ◽  
Ye Zhang ◽  
Huide Wang ◽  
Yonghong Zeng ◽  
Jinlai Zhao ◽  
...  
Keyword(s):  
Response Speed ◽  
Fast Response ◽  
Pollution Monitoring ◽  
Practical Applications ◽  
Ambient Exposure ◽  
Photoelectric Properties ◽  
Solar Blind ◽  
Deep Ultraviolet ◽  
Viable Approach ◽  
Ultraviolet Photodetectors

AbstractSolar-blind deep ultraviolet (DUV) photodetectors with high responsivity (R) and fast response speed are crucial for practical applications in astrophysical analysis, environmental pollution monitoring, and communication. Recently, 2D tellurium has emerged as a potential optoelectronic material because of its excellent photoelectric properties. In this study, solar-blind DUV photodetectors are demonstrated based on solution-synthesized and air-stable quasi-2D Te nanosheets (Te NSs). An R of 6.5 × 104 A/W at 261 nm and an external quantum efficiency (EQE) of higher than 2.26 × 106% were obtained, which are highest among most other 2D material-based solar-blind DUV photodetectors. Moreover, the photoelectric performance of the quasi-2D Te-based photodetector exhibited good stability even after ambient exposure for 90 days without any encapsulation. These results indicate that quasi-2D Te NSs provide a viable approach for developing solar-blind DUV photodetectors with ultrahigh R and EQE.

scholarly journals Application of Deep Learning in Integrated Pest Management: A Real-Time System for Detection and Diagnosis of Oilseed Rape Pests

2019 ◽  
Vol 2019 ◽  
pp. 1-14 ◽  
Author(s):  
Yong He ◽  
Hong Zeng ◽  
Yangyang Fan ◽  
Shuaisheng Ji ◽  
Jianjian Wu
Keyword(s):  
Deep Learning ◽  
Integrated Pest Management ◽  
Pest Management ◽  
Real Time ◽  
Oilseed Rape ◽  
Data Augmentation ◽  
Low Cost ◽  
Response Speed ◽  
Original Model ◽  
Real Time System

In this paper, we proposed an approach to detect oilseed rape pests based on deep learning, which improves the mean average precision (mAP) to 77.14%; the result increased by 9.7% with the original model. We adopt this model to mobile platform to let every farmer able to use this program, which will diagnose pests in real time and provide suggestions on pest controlling. We designed an oilseed rape pest imaging database with 12 typical oilseed rape pests and compared the performance of five models, SSD w/Inception is chosen as the optimal model. Moreover, for the purpose of the high mAP, we have used data augmentation (DA) and added a dropout layer. The experiments are performed on the Android application we developed, and the result shows that our approach surpasses the original model obviously and is helpful for integrated pest management. This application has improved environmental adaptability, response speed, and accuracy by contrast with the past works and has the advantage of low cost and simple operation, which are suitable for the pest monitoring mission of drones and Internet of Things (IoT).

scholarly journals Chemical Modification of Combusted Coal Gangue for U(VI) Adsorption: Towards a Waste Control by Waste Strategy

2021 ◽  
Vol 13 (15) ◽  
pp. 8421
Author(s):  
Yuan Gao ◽  
Jiandong Huang ◽  
Meng Li ◽  
Zhongran Dai ◽  
Rongli Jiang ◽  
...  
Keyword(s):  
Structural Analysis ◽  
High Efficiency ◽  
Low Cost ◽  
Chemical Activation ◽  
Cost Effective ◽  
Coal Gangue ◽  
Order Kinetic ◽  
Practical Applications ◽  
Detailed Structural Analysis ◽  
Alkaline Conditions

Uranium mining waste causes serious radiation-related health and environmental problems. This has encouraged efforts toward U(VI) removal with low cost and high efficiency. Typical uranium adsorbents, such as polymers, geopolymers, zeolites, and MOFs, and their associated high costs limit their practical applications. In this regard, this work found that the natural combusted coal gangue (CCG) could be a potential precursor of cheap sorbents to eliminate U(VI). The removal efficiency was modulated by chemical activation under acid and alkaline conditions, obtaining HCG (CCG activated with HCl) and KCG (CCG activated with KOH), respectively. The detailed structural analysis uncovered that those natural mineral substances, including quartz and kaolinite, were the main components in CCG and HCG. One of the key findings was that kalsilite formed in KCG under a mild synthetic condition can conspicuous enhance the affinity towards U(VI). The best equilibrium adsorption capacity with KCG was observed to be 140 mg/g under pH 6 within 120 min, following a pseudo-second-order kinetic model. To understand the improved adsorption performance, an adsorption mechanism was proposed by evaluating the pH of uranyl solutions, adsorbent dosage, as well as contact time. Combining with the structural analysis, this revealed that the uranyl adsorption process was mainly governed by chemisorption. This study gave rise to a utilization approach for CCG to obtain cost-effective adsorbents and paved a novel way towards eliminating uranium by a waste control by waste strategy.

scholarly journals Preparation and photocatalytic performance of metallic Nb0.9Ta0.1S2/2D-C3N4 composite

2020 ◽  
Vol 1 (1) ◽  
Author(s):  
Hanxiang Chen ◽  
Jianjian Yi ◽  
Zhao Mo ◽  
Yanhua Song ◽  
Wenshu Yang ◽  
...  
Keyword(s):  
Separation Efficiency ◽  
Low Cost ◽  
Metal Sulfide ◽  
Electron Hole ◽  
Practical Applications ◽  
Energy And Environment ◽  
Photocatalytic Application ◽  
Light Utilization ◽  
Ternary Metal ◽  
Key Issues

Abstract Photocatalysis technology has potential application in the field of energy and environment. How to expand visible light utilization and promote the separation efficiency of the carriers are the key issues for the high active photocatalysts preparation and future practical applications. In this work, a ternary metal sulfide Nb0.9Ta0.1S2 was prepared and used as an electron collector in the photocatalytic application. As a result, the generated electrons are quickly transferred to the surface of the composite to participate in the reaction. It was demonstrated that the photocatalytic activity of 2D-C3N4 was enhanced after the modification of Nb0.9Ta0.1S2. The Nb0.9Ta0.1S2/2D-C3N4 composite material was synthesized by solvothermal method. The composition of 5% Nb0.9Ta0.1S2/2D-C3N4 showed the highest H2 evolution rate of 1961.6 μmolg−1h−1, which was 6.6 times that of 2D-C3N4. The 15% Nb0.9Ta0.1S2/2D-C3N4 exhibited the best activity in Rhodamine B degradation rate of 97% in 2 h, which is 50% higher than that of 2D-C3N4. Nb0.9Ta0.1S2/2D-C3N4 can be used as electron trap to promote the effective separation of electron–hole pairs. This work provides benchmarks in exploring low-cost and efficient cocatalyst.

scholarly journals A Survey on Deep Learning Based Methods and Datasets for Monocular 3D Object Detection

Electronics ◽  
2021 ◽  
Vol 10 (4) ◽  
pp. 517
Author(s):  
Seong-heum Kim ◽  
Youngbae Hwang
Keyword(s):  
Deep Learning ◽  
Object Detection ◽  
Low Cost ◽  
Detection Methods ◽  
Future Research ◽  
3D Object ◽  
Practical Applications ◽  
Depth Sensors ◽  
Significant Research ◽  
3D Object Detection

Owing to recent advancements in deep learning methods and relevant databases, it is becoming increasingly easier to recognize 3D objects using only RGB images from single viewpoints. This study investigates the major breakthroughs and current progress in deep learning-based monocular 3D object detection. For relatively low-cost data acquisition systems without depth sensors or cameras at multiple viewpoints, we first consider existing databases with 2D RGB photos and their relevant attributes. Based on this simple sensor modality for practical applications, deep learning-based monocular 3D object detection methods that overcome significant research challenges are categorized and summarized. We present the key concepts and detailed descriptions of representative single-stage and multiple-stage detection solutions. In addition, we discuss the effectiveness of the detection models on their baseline benchmarks. Finally, we explore several directions for future research on monocular 3D object detection.

Improved photocatalytic conversion of high−concentration ammonia in water by low−cost Cu/TiO2 and its mechanism study

Chemosphere ◽  
2021 ◽  
Vol 274 ◽  
pp. 129689
Author(s):  
Jianpei Feng ◽  
Xiaolei Zhang ◽  
Guan Zhang ◽  
Ji Li ◽  
Wei Song ◽  
...  
Keyword(s):  
Low Cost ◽  
Mechanism Study ◽  
High Concentration

scholarly journals Synthesis of poly (n-butyl acrylate) with tempo by nitroxide mediated polymerization method

2021 ◽  
pp. 096739112110245
Author(s):  
Amrita Sharma ◽  
PP Pande
Keyword(s):  
Butyl Acrylate ◽  
Low Cost ◽  
Polymerization Process ◽  
Polymerization Reaction ◽  
High Concentration ◽  
Acrylate Monomer ◽  
Controlled Polymerization ◽  
Acrylate Monomers ◽  
Nitroxide Mediated Polymerization ◽  
Polymerization Method

It has been observed that acrylate monomers are very difficult to polymerize with the low cost nitroxide catalyst 2,2,6,6-tetramethylpiperidinyl-1-oxyl (TEMPO). Therefore, costly acyclic nitroxides such as N-tert-butyl-N-(1-diethylphosphono-2,2-dimethyl)-N-oxyl, (SG1), 2,2,5-Trimethyl-4-phenyl-3-azahexane-3-nitroxide (TIPNO) and TIPNO derivatives have to be used for the polymerization of the acrylic acid derivatives. There are very few reports on the use of TEMPO-derivatives toward the polymerization of n-butyl acrylate. Generally different reducing agents viz. glucose, ascorbic acid, hydroxyacetone etc. have been used to destroy excess TEMPO during the polymerization reaction. The acrylate polymerizations fail in the presence of TEMPO due to the strong C–O bond formed between the acrylate chain end and nitroxide. To the best of our knowledge, no literature report is available on the use of TEMPO without reducing agent or high temperature initiators, toward the polymerization of n-butyl acrylate. The present study has been carried out with a view to re-examine the application of low cost nitroxide TEMPO, so that it can be utilized towards the polymerization of acrylate monomers (e.g. n-butyl acrylate). We have been able to polymerize n-butyl acrylate using the nitroxide TEMPO as initiator (via a macroinitiator). In this synthesis, a polystyrene macroinitiator was synthesized in the first step from TEMPO, after this TEMPO end-capped styrene macroinitiator (PSt-TEMPO) is used to polymerize n-butyl acrylate monomer. The amount of macroinitiator taken was varied from 0.05% to 50% by weight of n-butyl acrylate monomer. The polymerization was carried out at 120°C by bulk polymerization method. The experimental findings showed a gradual increase in molecular weight of the polymer formed and decrease in the polydispersity index (PDI) with increase in amount of PSt-TEMPO macroinitiator taken. In all experiments conversion was more than 80%. These results indicate that the polymerization takes place through controlled polymerization process. Effect of different solvents on polymerization has also been investigated. In the following experiments TEMPO capped styrene has been used as macroinitiator leading to the successful synthesis of poly n-Butyl acrylate. It has been found that styrene macroinitiator is highly efficient for the nitroxide mediated polymerization, even in very small concentration for the synthesis of poly n-butyl acrylate. High concentration of macroinitiator results in the formation of block copolymers of polystyrene and poly ( n-butyl acrylate) viz. polystyrene-block-poly-( n-butyl acrylate). The use of TEMPO toward controlled polymerization is of much importance, because it is the nitroxide commercially available at the lowest cost.

High performance self-powered CuZnS/GaN UV photodetectors with ultrahigh on/off ratio (3 × 108)

2021 ◽  
Vol 9 (14) ◽  
pp. 4799-4807
Author(s):  
Yong Zhang ◽  
Weidong Song
Keyword(s):  
Chemical Bath Deposition ◽  
High Performance ◽  
Response Speed ◽  
Fast Response ◽  
Uv Photodetector ◽  
Uv Photodetectors ◽  
Simple Chemical ◽  
Self Powered

P-CuZnS/n-GaN UV photodetector is prepared by a simple chemical bath deposition, showing excellent self-powered properties, including ultrahigh on/off ratio (3 × 108), fast response speed (0.14/40 ms) and large detectivity of 3 × 1013 Jones.

scholarly journals Ruthenium Sensitizers and Their Applications in Dye-Sensitized Solar Cells

2012 ◽  
Vol 2012 ◽  
pp. 1-21 ◽  
Author(s):  
Yuancheng Qin ◽  
Qiang Peng
Keyword(s):  
Solar Cells ◽  
High Efficiency ◽  
Low Cost ◽  
Dye Sensitized Solar Cells ◽  
Ruthenium Complexes ◽  
Practical Applications ◽  
Photovoltaic Energy ◽  
Dye Sensitized ◽  
Sensitized Solar Cells ◽  
Excellent Stability

Dye-sensitized solar cells (DSSCs) have attracted considerable attention in recent years due to the possibility of low-cost conversion of photovoltaic energy. The DSSCs-based ruthenium complexes as sensitizers show high efficiency and excellent stability, implying potential practical applications. This review focuses on recent advances in design and preparation of efficient ruthenium sensitizers and their applications in DSSCs, including thiocyanate ruthenium sensitizers and thiocyanate-free ruthenium sensitizers.

The use and misuse of apparent resistivity in electromagnetic methods

Geophysics ◽  
1986 ◽  
Vol 51 (7) ◽  
pp. 1462-1471 ◽  
Author(s):  
Brian R. Spies ◽  
Dwight E. Eggers
Keyword(s):  
Apparent Resistivity ◽  
Early Time ◽  
Asymptotic Formulas ◽  
Voltage Response ◽  
Late Time ◽  
Induced Voltage ◽  
Resistivity Curve ◽  
Transient Electromagnetic ◽  
Electromagnetic Methods ◽  
Tem Method

Problems and misunderstandings arise with the concept of apparent resistivity when the analogy between an apparent resistivity computed from geophysical observations and the true resistivity structure of the subsurface is drawn too tightly. Several definitions of apparent resistivity are available for use in electromagnetic methods; however, those most commonly used do not always exhibit the best behavior. Many of the features of the apparent resistivity curve which have been interpreted as physically significant with one definition disappear when alternative definitions are used. It is misleading to compare the detection or resolution capabilities of different field systems or configurations solely on the basis of the apparent resistivity curve. For the in‐loop transient electromagnetic (TEM) method, apparent resistivity computed from the magnetic field response displays much better behavior than that computed from the induced voltage response. A comparison of “exact” and “asymptotic” formulas for the TEM method reveals that automated schemes for distinguishing early‐time and late‐time branches are at best tenuous, and those schemes are doomed to failure for a certain class of resistivity structures (e.g., the loop size is large compared to the layer thickness). For the magnetotelluric (MT) method, apparent resistivity curves defined from the real part of the impedance exhibit much better behavior than curves based on the conventional definition that uses the magnitude of the impedance. Results of using this new definition have characteristics similar to apparent resistivity obtained from time‐domain processing.

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