scholarly journals Characterization of a boreal convective boundary layer and its impact on atmospheric chemistry during HUMPPA-COPEC-2010

2012 ◽  
Vol 12 (19) ◽  
pp. 9335-9353 ◽  
Author(s):  
H. G. Ouwersloot ◽  
J. Vilà-Guerau de Arellano ◽  
A. C. Nölscher ◽  
M. C. Krol ◽  
L. N. Ganzeveld ◽  
...  

Abstract. We studied the atmospheric boundary layer (ABL) dynamics and the impact on atmospheric chemistry during the HUMPPA-COPEC-2010 campaign. We used vertical profiles of potential temperature and specific moisture, obtained from 132 radio soundings, to determine the main boundary layer characteristics during the campaign. We propose a classification according to several main ABL prototypes. Further, we performed a case study of a single day, focusing on the convective boundary layer, to analyse the influence of the dynamics on the chemical evolution of the ABL. We used a mixed layer model, initialized and constrained by observations. In particular, we investigated the role of large scale atmospheric dynamics (subsidence and advection) on the ABL development and the evolution of chemical species concentrations. We find that, if the large scale forcings are taken into account, the ABL dynamics are represented satisfactorily. Subsequently, we studied the impact of mixing with a residual layer aloft during the morning transition on atmospheric chemistry. The time evolution of NOx and O3 concentrations, including morning peaks, can be explained and accurately simulated by incorporating the transition of the ABL dynamics from night to day. We demonstrate the importance of the ABL height evolution for the representation of atmospheric chemistry. Our findings underscore the need to couple the dynamics and chemistry at different spatial scales (from turbulence to mesoscale) in chemistry-transport models and in the interpretation of observational data.

2012 ◽  
Vol 12 (6) ◽  
pp. 13619-13665 ◽  
Author(s):  
H. G. Ouwersloot ◽  
J. Vilà-Guerau de Arellano ◽  
A. C. Nölscher ◽  
M. C. Krol ◽  
L. N. Ganzeveld ◽  
...  

Abstract. We studied the atmospheric boundary layer (ABL) dynamics and the impact on atmospheric chemistry during the HUMPPA-COPEC-2010 campaign. We used vertical profiles of potential temperature and specific moisture, obtained from 132 radio soundings, to determine the main boundary layer characteristics during the campaign. We propose a classification according to several main ABL prototypes. Further, we performed a case study of a single day characterized as a convective boundary layer to analyse the influence of the dynamics on the chemical evolution of the ABL, using a systematic analysis that can easily be extended to other periods during HUMPPA-COPEC-2010. We used a mixed layer model, initialized and constrained by observations. In particular, we investigated the role of large scale atmospheric dynamics (subsidence and advection) on the ABL development and the evolution of chemical species concentrations. We find that, if the large scale forcings are taken into account, the ABL dynamics are represented satisfactorily. Subsequently, we studied the impact of mixing with a residual layer aloft during the morning transition on atmospheric chemistry. The time evolution of NOx and O3 concentrations, including morning peaks, can be explained and accurately simulated by incorporating the transition of the ABL dynamics from night to day. We demonstrate the importance of the ABL height evolution for the representation of atmospheric chemistry. Our findings underscore the need to couple the dynamics and chemistry at different spatial scales (from turbulence to mesoscale) in chemistry-transport models and in the interpretation of observational data.


Atmosphere ◽  
2018 ◽  
Vol 9 (3) ◽  
pp. 102 ◽  
Author(s):  
Stefano Serafin ◽  
Bianca Adler ◽  
Joan Cuxart ◽  
Stephan De Wekker ◽  
Alexander Gohm ◽  
...  

The exchange of heat, momentum, and mass in the atmosphere over mountainous terrain is controlled by synoptic-scale dynamics, thermally driven mesoscale circulations, and turbulence. This article reviews the key challenges relevant to the understanding of exchange processes in the mountain boundary layer and outlines possible research priorities for the future. The review describes the limitations of the experimental study of turbulent exchange over complex terrain, the impact of slope and valley breezes on the structure of the convective boundary layer, and the role of intermittent mixing and wave–turbulence interaction in the stable boundary layer. The interplay between exchange processes at different spatial scales is discussed in depth, emphasizing the role of elevated and ground-based stable layers in controlling multi-scale interactions in the atmosphere over and near mountains. Implications of the current understanding of exchange processes over mountains towards the improvement of numerical weather prediction and climate models are discussed, considering in particular the representation of surface boundary conditions, the parameterization of sub-grid-scale exchange, and the development of stochastic perturbation schemes.


2018 ◽  
Vol 75 (7) ◽  
pp. 2317-2336 ◽  
Author(s):  
Bowen Zhou ◽  
Shiwei Sun ◽  
Kai Yao ◽  
Kefeng Zhu

Abstract Turbulent mixing in the daytime convective boundary layer (CBL) is carried out by organized nonlocal updrafts and smaller local eddies. In the upper mixed layer of the CBL, heat fluxes associated with nonlocal updrafts are directed up the local potential temperature gradient. To reproduce such countergradient behavior in parameterizations, a class of planetary boundary layer schemes adopts a countergradient correction term in addition to the classic downgradient eddy-diffusion term. Such schemes are popular because of their simple formulation and effective performance. This study reexamines those schemes to investigate the physical representations of the gradient and countergradient (GCG) terms, and to rebut the often-implied association of the GCG terms with heat fluxes due to local and nonlocal (LNL) eddies. To do so, large-eddy simulations (LESs) of six idealized CBL cases are performed. The GCG fluxes are computed a priori with horizontally averaged LES data, while the LNL fluxes are diagnosed through conditional sampling and Fourier decomposition of the LES flow field. It is found that in the upper mixed layer, the gradient term predicts downward fluxes in the presence of positive mean potential temperature gradient but is compensated by the upward countergradient correction flux, which is larger than the total heat flux. However, neither downward local fluxes nor larger-than-total nonlocal fluxes are diagnosed from LES. The difference reflects reduced turbulence efficiency for GCG fluxes and, in terms of physics, conceptual deficiencies in the GCG representation of CBL heat fluxes.


2020 ◽  
Vol 77 (2) ◽  
pp. 435-442
Author(s):  
John Thuburn ◽  
Georgios A. Efstathiou

Abstract We hypothesize that the convective atmospheric boundary layer is marginally stable when the damping effects of turbulence are taken into account. If the effects of turbulence are modeled as an eddy viscosity and diffusivity, then an idealized analysis based on the hypothesis predicts a well-known scaling for the magnitude of the eddy viscosity and diffusivity. It also predicts that the marginally stable modes should have vertical and horizontal scales comparable to the boundary layer depth. A more quantitative numerical linear stability analysis is presented for a realistic convective boundary layer potential temperature profile and is found to support the hypothesis.


2020 ◽  
Author(s):  
Jan Weinkaemmerer ◽  
Ivan Bašták Ďurán ◽  
Jürg Schmidli

<p>In the convective boundary layer over mountainous regions, the mean values and the fluxes of quantities like heat, mass, and momentum are strongly influenced by thermally induced flows. Several studies have pointed out that the enhanced warming of the air inside a valley can be explained by the valley-volume effect whereas the cross-valley circulation leads to a net export of heat to the free atmosphere. We are interested in the influence of an upper-level wind on the local circulations and the boundary-layer properties, both locally and in terms of the horizontal mean, as this aspect has not yet received much attention. LES are carried out over idealized, two-dimensional topographies using the CM1 numerical model. For the analysis, turbulent, mean-circulation, and large-scale contributions are systematically distinguished. Also, budget analyses are performed for the turbulence kinetic energy and the turbulent heat and mass flux. Based on the first results for periodic topographies, no crucial influence on the horizontally averaged heat-flux and temperature profile can be observed, even though the flow pattern of the thermal wind is qualitatively changed. In addition to that, the impact on moisture transport will be evaluated and simulations over different topographies as well as for different atmospheric conditions and surface properties will be presented.</p>


2013 ◽  
Vol 13 (12) ◽  
pp. 31527-31562 ◽  
Author(s):  
E. Blay-Carreras ◽  
D. Pino ◽  
A. Van de Boer ◽  
O. De Coster ◽  
C. Darbieu ◽  
...  

Abstract. Observations, mixed-layer theory and the Dutch Large-Eddy Simulation model (DALES) are used to analyze the dynamics of the boundary layer during an intensive operational period (1 July 2011) of the Boundary Layer Late Afternoon and Sunset Turbulence campaign. Continuous measurements made by remote sensing and in situ instruments in combination with radio soundings, and measurements done by remotely piloted airplane systems and two aircrafts probed the vertical structure and the temporal evolution of the boundary layer during the campaign. The initial vertical profiles of potential temperature, specific humidity and wind, and the temporal evolution of the surface heat and moisture fluxes prescribed in the numerical simulations are inspired by some of these observations. The research focuses on the role played by the residual layer during the morning transition and by the large-scale subsidence on the evolution of the boundary layer. By using DALES, we show the importance of the dynamics of the boundary layer during the previous night in the development of the boundary layer at the morning. DALES numerical experiments including the residual layer are capable to model the observed sudden increase of the boundary-layer depth during the morning transition and the subsequent evolution of the boundary layer. The simulation shows a large increase of the entrainment buoyancy heat flux when the residual layer is incorporated into the mixed layer. We also examine how the inclusion of the residual layer above a shallow convective boundary layer modifies the turbulent kinetic energy budget. Large-scale subsidence mainly acts when the boundary layer is fully developed and, for the studied day, it is necessary to be considered to reproduce the afternoon observations. Additionally, we investigate how carbon dioxide (CO2) mixing ratio stored the previous night in the residual layer plays a fundamental role in the evolution of the CO2 mixing ratio during the following day.


2017 ◽  
Vol 17 (3) ◽  
pp. 1623-1640 ◽  
Author(s):  
Metodija M. Shapkalijevski ◽  
Huug G. Ouwersloot ◽  
Arnold F. Moene ◽  
Jordi Vilà-Guerau de Arrellano

Abstract. By characterizing the dynamics of a convective boundary layer above a relatively sparse and uniform orchard canopy, we investigated the impact of the roughness-sublayer (RSL) representation on the predicted diurnal variability of surface fluxes and state variables. Our approach combined numerical experiments, using an atmospheric mixed-layer model including a land-surface-vegetation representation, and measurements from the Canopy Horizontal Array Turbulence Study (CHATS) field experiment near Dixon, California. The RSL is parameterized using an additional factor in the standard Monin–Obukhov similarity theory flux-profile relationships that takes into account the canopy influence on the atmospheric flow. We selected a representative case characterized by southerly wind conditions to ensure well-developed RSL over the orchard canopy. We then investigated the sensitivity of the diurnal variability of the boundary-layer dynamics to the changes in the RSL key scales, the canopy adjustment length scale, Lc, and the β = u*/|U| ratio at the top of the canopy due to their stability and dependence on canopy structure. We found that the inclusion of the RSL parameterization resulted in improved prediction of the diurnal evolution of the near-surface mean quantities (e.g. up to 50 % for the wind velocity) and transfer (drag) coefficients. We found relatively insignificant effects on the modelled surface fluxes (e.g. up to 5 % for the friction velocity, while 3 % for the sensible and latent heat), which is due to the compensating effect between the mean gradients and the drag coefficients, both of which are largely affected by the RSL parameterization. When varying Lc (from 10 to 20 m) and β (from 0.25 to 0.4 m), based on observational evidence, the predicted friction velocity is found to vary by up to 25 % and the modelled surface-energy fluxes (sensible heat, SH, and latent heat of evaporation, LE) vary up to 2 and 9 %. Consequently, the boundary-layer height varies up to 6 %. Furthermore, our analysis indicated that to interpret the CHATS measurements above the canopy, the contributions of non-local effects such as entrainment, subsidence and the advection of heat and moisture over the CHATS site need to be taken into account.


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