scholarly journals Dome effect of black carbon and its key influencing factors: a one-dimensional modelling study

2018 ◽  
Vol 18 (4) ◽  
pp. 2821-2834 ◽  
Author(s):  
Zilin Wang ◽  
Xin Huang ◽  
Aijun Ding

Abstract. Black carbon (BC) has been identified to play a critical role in aerosol–planetary boundary layer (PBL) interaction and further deterioration of near-surface air pollution in megacities, which has been referred to as the “dome effect”. However, the impacts of key factors that influence this effect, such as the vertical distribution and aging processes of BC, as well as the underlying land surface, have not been quantitatively explored yet. Here, based on available in situ measurements of meteorology and atmospheric aerosols together with the meteorology–chemistry online coupled model WRF-Chem, we conduct a set of parallel simulations to quantify the roles of these factors in influencing the BC dome effect and surface haze pollution. Furthermore, we discuss the main implications of the results to air pollution mitigation in China. We found that the impact of BC on the PBL is very sensitive to the altitude of aerosol layer. The upper-level BC, especially that near the capping inversion, is more essential in suppressing the PBL height and weakening the turbulent mixing. The dome effect of BC tends to be significantly intensified as BC mixed with scattering aerosols during winter haze events, resulting in a decrease in PBL height by more than 15 %. In addition, the dome effect is more substantial (up to 15 %) in rural areas than that in the urban areas with the same BC loading, indicating an unexpected regional impact of such an effect to air quality in countryside. This study indicates that China's regional air pollution would greatly benefit from BC emission reductions, especially those from elevated sources from chimneys and also domestic combustion in rural areas, through weakening the aerosol–boundary layer interactions that are triggered by BC.

2017 ◽  
Author(s):  
Zilin Wang ◽  
Xin Huang ◽  
Aijun Ding

Abstract. Black carbon (BC) has been identified to play a critical role in aerosol-planet boundary layer (PBL) interaction and further deterioration of near-surface air pollution in megacities, which has been named as its dome effect. However, the impacts of key factors that influence this effect, such as the vertical distribution and aging processes of BC, and also the underlying land surface, have not been quantitatively explored yet. Here, based on available in-situ measurements of meteorology and atmospheric aerosols together with the meteorology-chemistry online coupled model, WRF-Chem, we conduct a set of parallel simulations to quantify the roles of these factors in influencing the BC's dome effect and surface haze pollution, and discuss the main implications of the results to air pollution mitigation in China. We found that the impact of BC on PBL is very sensitive to the altitude of aerosol layer. The upper level BC, especially those near the capping inversion, is more essential in suppressing the PBL height and weakening the turbulence mixing. The dome effect of BC tends to be significantly intensified as BC aerosol mixed with scattering aerosols during winter haze events, resulting in a decrease of PBL height by more than 25 %. In addition, the dome effect is more substantial (up to 15 %) in rural areas than that in the urban areas with the same BC loading, indicating an unexpected regional impact of such kind of effect to air quality in countryside. This study suggests that China's regional air pollution would greatly benefit from BC emission reductions, especially those from the elevated sources from the chimneys and also the domestic combustions in rural areas, through weakening the aerosol-boundary layer interactions that triggered by BC.


2020 ◽  
Author(s):  
Benjamin Fersch ◽  
Alfonso Senatore ◽  
Bianca Adler ◽  
Joël Arnault ◽  
Matthias Mauder ◽  
...  

<p>The land surface and the atmospheric boundary layer are closely intertwined with respect to the exchange of water, trace gases and energy. Nonlinear feedback and scale dependent mechanisms are obvious by observations and theories. Modeling instead is often narrowed to single compartments of the terrestrial system or bound to traditional viewpoints of definite scientific disciplines. Coupled terrestrial hydrometeorological modeling systems attempt to overcome these limitations to achieve a better integration of the processes relevant for regional climate studies and local area weather prediction. We examine the ability of the hydrologically enhanced version of the Weather Research and Forecasting Model (WRF-Hydro) to reproduce the regional water cycle by means of a two-way coupled approach and assess the impact of hydrological coupling with respect to a traditional regional atmospheric model setting. It includes the observation-based calibration of the hydrological model component (offline WRF-Hydro) and a comparison of the classic WRF and the fully coupled WRF-Hydro models both with identical calibrated parameter settings for the land surface model (Noah-MP). The simulations are evaluated based on extensive observations at the pre-Alpine Terrestrial Environmental Observatory (TERENO Pre-Alpine) for the Ammer (600 km²) and Rott (55 km²) river catchments in southern Germany, covering a five month period (Jun–Oct 2016).</p><p>The sensitivity of 7 land surface parameters is tested using the <em>Latin-Hypercube One-factor-At-a-Time</em> (LH-OAT) method and 6 sensitive parameters are subsequently optimized for 6 different subcatchments, using the Model-Independent <em>Parameter Estimation and Uncertainty Analysis software</em> (PEST).</p><p>The calibration of the offline WRF-Hydro leads to Nash-Sutcliffe efficiencies between 0.56 and 0.64 and volumetric efficiencies between 0.46 and 0.81 for the six subcatchments. The comparison of classic WRF and fully coupled WRF-Hydro shows only tiny alterations for radiation and precipitation but considerable changes for moisture- and energy fluxes. By comparison with TERENO Pre-Alpine observations, the fully coupled model slightly outperforms the classic WRF with respect to evapotranspiration, sensible and ground heat flux, near surface mixing ratio, temperature, and boundary layer profiles of air temperature. The subcatchment-based water budgets show uniformly directed variations for evapotranspiration, infiltration excess and percolation whereas soil moisture and precipitation change randomly.</p>


2020 ◽  
Vol 20 (8) ◽  
pp. 4575-4592 ◽  
Author(s):  
Dandan Zhao ◽  
Guangjing Liu ◽  
Jinyuan Xin ◽  
Jiannong Quan ◽  
Yuesi Wang ◽  
...  

Abstract. Under a high atmospheric oxidization capacity, the synergistic effect of the physicochemical processes in the atmospheric boundary layer (ABL) caused summer haze pollution in Beijing. The southern and southwestern areas, generally 60–300 km away from Beijing, were seriously polluted in contrast to Beijing, which remained clean. Southerly winds moving faster than 20–30 km h−1 since the early morning primarily caused haze pollution initiation. The PM2.5 (particulate matter with a dynamic equivalent diameter smaller than 2.5 µm) level increased to 75 µg m−3 over several hours during the daytime, which was simultaneously affected by the ABL structure. Additionally, the O3 concentration was quite high during the daytime (250 µg m−3), corresponding to a high atmospheric oxidation capacity. Much sulfate and nitrate were produced through active atmospheric chemical processes, with sulfur oxidation ratios (SORs) up to ∼0.76 and nitrogen oxidation ratios (NORs) increasing from 0.09 to 0.26, which further facilitated particulate matter (PM) level enhancement. However, the increase in sulfate was mainly linked to southerly transport. At midnight, the PM2.5 concentration sharply increased from 75 to 150 µg m−3 over 4 h and remained at its highest level until the next morning. Under an extremely stable ABL structure, secondary aerosol formation dominated by nitrate was quite intense, driving the haze pollution outbreak. The PM levels in the southern and southeastern areas of Beijing were significantly lower than those in Beijing at this time, even below air quality standards; thus, the contribution of pollution transport had almost disappeared. With the formation of a nocturnal stable boundary layer (NSBL) at an altitude ranging from 0–0.3 km, the extremely low turbulence kinetic energy (TKE) ranging from 0 to 0.05 m2 s−2 inhibited the spread of particles and moisture, ultimately resulting in elevated near-surface PM2.5 and relative humidity (∼90 %) levels. Due to the very high humidity and ambient oxidization capacity, NOR rapidly increased from 0.26 to 0.60, and heterogeneous hydrolysis reactions at the moist particle surface were very notable. The nitrate concentration steeply increased from 11.6 to 57.8 µg m−3, while the sulfate and organics concentrations slightly increased by 6.1 and 3.1 µg m−3, respectively. With clean and strong winds passing through Beijing, the stable ABL dissipated with the potential temperature gradient becoming negative and the ABL height (ABLH) increasing to ∼2.5 km. The high turbulence activity with a TKE ranging from 3 to 5 m2 s−2 notably promoted pollution diffusion. The self-cleaning capacity of the atmosphere is commonly responsible for air pollution dispersion. However, reducing the atmospheric oxidization capacity, through strengthening collaborative control of nitrogen oxide (NOx) and volatile organic compounds (VOCs), as well as continuously deepening regional joint air pollution control, is urgent.


2021 ◽  
Vol 21 (11) ◽  
pp. 9253-9268
Author(s):  
Zhuozhi Shu ◽  
Yubao Liu ◽  
Tianliang Zhao ◽  
Junrong Xia ◽  
Chenggang Wang ◽  
...  

Abstract. Deep basins create uniquely favorable conditions for causing air pollution, and the Sichuan Basin (SCB) in Southwest China is such a basin featuring frequent heavy pollution. A wintertime heavy haze pollution event in the SCB was studied with conventional and intensive observation data and the WRF-Chem model to explore the 3D distribution of PM2.5 to understand the impact of regional pollutant emissions, basin circulations associated with plateaus, and downwind transport to the adjacent areas. It was found that the vertical structure of PM2.5 over the SCB was characterized by a remarkable hollow sandwiched by high PM2.5 layers at heights of 1.5–3 km and a highly polluted near-surface layer. The southwesterlies over the Tibetan Plateau (TP) and Yunnan-Guizhou Plateau (YGP) resulted in a lee vortex over the SCB, which helped form and maintain heavy PM2.5 pollution. The basin PM2.5 was lifted into the free troposphere and transported outside of the SCB. At the bottom of the SCB, high PM2.5 concentrations were mostly located in the northwestern and southern regions. Due to the blocking effect of the plateau terrain on the northeasterly winds, PM2.5 gradually increased from northeast to southwest in the basin. In the lower free troposphere, the high PM2.5 centers were distributed over the northwestern and southwestern SCB areas, as well as the central SCB region. For this event, the regional emissions from the SCB contributed 75.4 %–94.6 % to the surface PM2.5 concentrations in the SCB. The SCB emissions were the major source of PM2.5 over the eastern regions of the TP and the northern regions of the YGP, with contribution rates of 72.7 % and 70.5 %, respectively, during the dissipation stage of heavy air pollution over the SCB, which was regarded as the major pollutant source affecting atmospheric environment changes in Southwest China.


2021 ◽  
Vol 21 (11) ◽  
pp. 8637-8654
Author(s):  
Na Zhao ◽  
Xinyi Dong ◽  
Kan Huang ◽  
Joshua S. Fu ◽  
Marianne Tronstad Lund ◽  
...  

Abstract. Black carbon (BC) emissions play an important role in regional climate change in the Arctic. It is necessary to pay attention to the impact of long-range transport from regions outside the Arctic as BC emissions from local sources in the Arctic were relatively small. The task force Hemispheric Transport of Air Pollution Phase 2 (HTAP2) set up a series of simulation scenarios to investigate the response of BC in a given region to different source regions. This study investigated the responses of Arctic BC concentrations and surface temperature to 20 % anthropogenic emission reductions from six regions in 2010 within the framework of HTAP2 based on ensemble modeling results. Emission reductions from East Asia (EAS) had the most (monthly contributions: 0.2–1.5 ng m−3) significant impact on the Arctic near-surface BC concentrations, while the monthly contributions from Europe (EUR), Middle East (MDE), North America (NAM), Russia–Belarus–Ukraine (RBU), and South Asia (SAS) were 0.2–1.0, 0.001–0.01, 0.1–0.3, 0.1–0.7, and 0.0–0.2 ng m−3, respectively. The responses of the vertical profiles of the Arctic BC to the six regions were found to be different due to multiple transport pathways. Emission reductions from NAM, RBU, EUR, and EAS mainly influenced the BC concentrations in the low troposphere of the Arctic, while most of the BC in the upper troposphere of the Arctic derived from SAS. The response of the Arctic BC to emission reductions in six source regions became less significant with the increase in the latitude. The benefit of BC emission reductions in terms of slowing down surface warming in the Arctic was evaluated by using absolute regional temperature change potential (ARTP). Compared to the response of global temperature to BC emission reductions, the response of Arctic temperature was substantially more sensitive, highlighting the need for curbing global BC emissions.


2021 ◽  
Author(s):  
Peter Huszar ◽  
Jan Karlický ◽  
Jana Marková ◽  
Tereza Nováková ◽  
Marina Liaskoni ◽  
...  

Abstract. Urban areas are hot-spots of intense emissions and they influence air-quality not only locally but on regional or even global scales. The impact of urban emissions over different scales depends on the dilution and chemical transformation of the urban plumes which are governed by the local and regional scale meteorological conditions. These are influenced by the presence of urbanized land-surface via the so called urban canopy meteorological forcing (UCMF). In this study, we investigate for selected central European cities (Berlin, Budapest, Munich, Prague, Vienna and Warsaw), how the urban emission impact (UEI) is modulated by the UCMF for present day climate conditions (2015–2016) using three regional climate-chemistry models: the regional climate models RegCM and WRF-Chem (its meteorological part), the chemistry transport model CAMx coupled to either RegCM and WRF and the “chemical” component of WRF-Chem. The UCMF was calculated by replacing the urbanized surface by rural one while the UEI was estimated by removing all anthropogenic emissions from the selected cities. We analyzed the urban emissions induced changes of near surface concentrations of NO2, O3 and PM2.5. We found increases of NO2 and PM2.5 concentrations over cities by 4–6 ppbv, and 4–6 μgm−3, respectively meaning that about 40–60 % and 20–40 % of urban concentrations of NO2 and PM2.5 are caused by local emissions and the rest is the result of emissions from surrounding rural areas. We showed that if UCMF is included, the UEI of these pollutants is about 40–60 % smaller, or in other words, the urban emission impact is overestimated if urban canopy effects are not taken into account. In case of ozone, models due to UEI usually predict decreases around −2 to −4 ppbv (about 10–20 %), which is again smaller if UCMF is considered (by about 60 %). We further showed that the impact on extreme (95th percentile) air-pollution is much stronger, as well as the modulation of UEI is larger for such situations. Finally, we evaluated the contribution of the urbanization induced modifications of vertical eddy-diffusion to the modulation of UEI, and found that it alone is able to explain the modelled decrease of the urban emission impact if the effects of UCMF are considered. In summary, our results showed that the meteorological changes resulting from urbanization have to be included in regional model studies if they intend to quantify the regional fingerprint of urban emissions. Ignoring these meteorological changes can lead to strong overestimation of UEI.


2019 ◽  
Author(s):  
Benjamin Fersch ◽  
Alfonso Senatore ◽  
Bianca Adler ◽  
Joël Arnault ◽  
Matthias Mauder ◽  
...  

Abstract. The land surface and the atmospheric boundary layer are closely intertwined with respect to the exchange of water, trace gases and energy. Nonlinear feedback and scale dependent mechanisms are obvious by observations and theories. Modeling instead is often narrowed to single compartments of the terrestrial system or largely bound to traditional disciplines. Coupled terrestrial hydrometeorological modeling systems attempt to overcome these limitations to achieve a better integration of the processes relevant for regional climate studies and local area weather prediction. This study examines the ability of the hydrologically enhanced version of the Weather Research and Forecasting Model (WRF-Hydro) to reproduce the regional water cycle by means of a two-way coupled approach and assesses the impact of hydrological coupling with respect to a traditional regional atmospheric model setting. It includes the observation-based calibration of the hydrological model component (offline WRF-Hydro) and a comparison of the classic WRF and the fully coupled WRF-Hydro models both with identical calibrated parameter settings for the land surface model (Noah-MP). The simulations are evaluated based on extensive observations at the preAlpine Terrestrial Environmental Observatory (TERENO-preAlpine) for the Ammer (600 km2) and Rott (55 km2) river catchments in southern Germany, covering a five month period (Jun–Oct 2016). The sensitivity of 7 land surface parameters is tested using the Latin-Hypercube One-factor-At-a-Time (LH-OAT) method and 6 sensitive parameters are subsequently optimized for 6 different subcatchments, using the Model-Independent Parameter Estimation and Uncertainty Analysis software (PEST). The calibration of the offline WRF-Hydro gives Nash-Sutcliffe efficiencies between 0.56 and 0.64 and volumetric efficiencies between 0.46 and 0.81 for the six subcatchments. The comparison of classic WRF and fully coupled WRF-Hydro, both using the calibrated parameters from the offline model, shows nominal alterations for radiation and precipitation but considerable changes for moisture- and heat fluxes. By comparison with TERENO-preAlpine observations, the fully coupled model slightly outperforms the classic WRF with respect to evapotranspiration, sensible and ground heat flux, near surface mixing ratio, temperature, and boundary layer profiles of air temperature. The subcatchment-based water budgets show uniformly directed variations for evapotranspiration, infiltration excess and percolation whereas soil moisture and precipitation change randomly.


2020 ◽  
Vol 20 (11) ◽  
pp. 6479-6493 ◽  
Author(s):  
Wenchao Han ◽  
Zhanqing Li ◽  
Fang Wu ◽  
Yuwei Zhang ◽  
Jianping Guo ◽  
...  

Abstract. The urban heat island intensity (UHII) is the temperature difference between urban areas and their rural surroundings. It is commonly attributed to changes in the underlying surface structure caused by urbanization. Air pollution caused by aerosol particles can affect the UHII through changing (1) the surface energy balance by the aerosol radiative effect (ARE) and (2) planetary-boundary-layer (PBL) stability and airflow intensity by modifying thermodynamic structure, which is referred to as the aerosol dynamic effect (ADE). By analyzing satellite data and ground-based observations collected from 2001 to 2010 at 35 cities in China and using the WRF-Chem model, we find that the impact of aerosols on UHII differs considerably: reducing the UHII in summer but increasing the UHII in winter. This seasonal contrast is proposed to be caused by the different strengths of the ARE and ADE between summer and winter. In summer, the ARE on UHII is dominant over the ADE, cooling down surface temperature more strongly in urban areas than in rural areas because of much higher aerosol loading, and offsets the urban heating, therefore weakening UHII. In winter, however, the ADE is more dominant, because aerosols stabilize the PBL more in the polluted condition, weakening the near-surface heat transport over urban areas in both vertical and horizontal directions. This means that the heat accumulated in urban areas is dispersed less effectively, and thus the UHII is enhanced. These findings shed new light on the impact of the interaction between urbanization-induced surface changes and air pollution on urban climate.


2020 ◽  
Vol 24 (5) ◽  
pp. 2457-2481 ◽  
Author(s):  
Benjamin Fersch ◽  
Alfonso Senatore ◽  
Bianca Adler ◽  
Joël Arnault ◽  
Matthias Mauder ◽  
...  

Abstract. The land surface and the atmospheric boundary layer are closely intertwined with respect to the exchange of water, trace gases, and energy. Nonlinear feedback and scale-dependent mechanisms are obvious by observations and theories. Modeling instead is often narrowed to single compartments of the terrestrial system or bound to traditional viewpoints of definite scientific disciplines. Coupled terrestrial hydrometeorological modeling systems attempt to overcome these limitations to achieve a better integration of the processes relevant for regional climate studies and local-area weather prediction. This study examines the ability of the hydrologically enhanced version of the Weather Research and Forecasting model (WRF-Hydro) to reproduce the regional water cycle by means of a two-way coupled approach and assesses the impact of hydrological coupling with respect to a traditional regional atmospheric model setting. It includes the observation-based calibration of the hydrological model component (offline WRF-Hydro) and a comparison of the classic WRF and the fully coupled WRF-Hydro models both with identically calibrated parameter settings for the land surface model (Noah-Multiparametrization; Noah-MP). The simulations are evaluated based on extensive observations at the Terrestrial Environmental Observatories (TERENO) Pre-Alpine Observatory for the Ammer (600 km2) and Rott (55 km2) river catchments in southern Germany, covering a 5-month period (June–October 2016). The sensitivity of seven land surface parameters is tested using the Latin-Hypercube–One-factor-At-a-Time (LH-OAT) method, and six sensitive parameters are subsequently optimized for six different subcatchments, using the model-independent Parameter Estimation and Uncertainty Analysis software (PEST). The calibration of the offline WRF-Hydro gives Nash–Sutcliffe efficiencies between 0.56 and 0.64 and volumetric efficiencies between 0.46 and 0.81 for the six subcatchments. The comparison of the classic WRF and fully coupled WRF-Hydro models, both using the calibrated parameters from the offline model, shows only tiny alterations for radiation and precipitation but considerable changes for moisture and heat fluxes. By comparison with TERENO Pre-Alpine Observatory measurements, the fully coupled model slightly outperforms the classic WRF model with respect to evapotranspiration, sensible and ground heat flux, the near-surface mixing ratio, temperature, and boundary layer profiles of air temperature. The subcatchment-based water budgets show uniformly directed variations for evapotranspiration, infiltration excess and percolation, whereas soil moisture and precipitation change randomly.


2013 ◽  
Vol 14 (5) ◽  
pp. 1373-1400 ◽  
Author(s):  
Joseph A. Santanello ◽  
Sujay V. Kumar ◽  
Christa D. Peters-Lidard ◽  
Ken Harrison ◽  
Shujia Zhou

Abstract Land–atmosphere (LA) interactions play a critical role in determining the diurnal evolution of both planetary boundary layer (PBL) and land surface heat and moisture budgets, as well as controlling feedbacks with clouds and precipitation that lead to the persistence of dry and wet regimes. In this study, the authors examine the impact of improved specification of land surface states, anomalies, and fluxes on coupled Weather Research and Forecasting Model (WRF) forecasts during the summers of extreme dry (2006) and wet (2007) land surface conditions in the U.S. southern Great Plains. The improved land initialization and surface flux parameterizations are obtained through calibration of the Noah land surface model using the new optimization and uncertainty estimation subsystems in NASA's Land Information System (LIS-OPT/LIS-UE). The impact of the calibration on the 1) spinup of the land surface used as initial conditions and 2) the simulated heat and moisture states and fluxes of the coupled WRF simulations is then assessed. In addition, the sensitivity of this approach to the period of calibration (dry, wet, or average) is investigated. Results show that the offline calibration is successful in providing improved initial conditions and land surface physics for the coupled simulations and in turn leads to systematic improvements in land–PBL fluxes and near-surface temperature and humidity forecasts. Impacts are larger during dry regimes, but calibration during either primarily wet or dry periods leads to improvements in coupled simulations due to the reduction in land surface model bias. Overall, these results provide guidance on the questions of what, how, and when to calibrate land surface models for coupled model prediction.


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