scholarly journals How does the UKESM1 climate model produce its cloud-aerosol forcing in the North Atlantic?

2020 ◽  
Author(s):  
Daniel P. Grosvenor ◽  
Kenneth S. Carslaw

Abstract. Climate variability in the North Atlantic influences processes such as hurricane activity and droughts. Global model simulations have identified aerosol-cloud interactions (ACIs) as an important driver of sea surface temperature variability via surface aerosol forcing. However, ACIs are a major cause of uncertainty in climate forcing, therefore caution is needed in interpreting the results from coarse resolution, highly parameterized global models. Here we separate and quantify the components of the surface shortwave effective radiative forcing (ERF) due to aerosol in the atmosphere-only version of the UK Earth System Model (UKESM1) and evaluate the cloud properties and their radiative effects against observations. We focus on a northern region of the North Atlantic (NA) where stratocumulus clouds dominate (denoted the northern NA region) and a southern region where trade cumulus and broken stratocumlus dominate (southern NA region). Aerosol forcing was diagnosed using a pair of simulations in which the meteorology is approximately fixed via nudging to analysis; one simulation has pre-industrial (PI) and one has present-day (PD) aerosol emissions. Contributions to the surface ERF from changes in cloud fraction (fc), in-cloud liquid water path (LWPic) and droplet number concentration (Nd) were quantified. Over the northern NA region increases in Nd and LWPic dominate the forcing. This is likely because the high fc there precludes further large increases in fc and allows cloud brightening to act over a larger region. Over the southern NA region increases in fc dominate due to the suppression of rain by the additional aerosols. Aerosol-driven increases in macrophysical cloud properties (LWPic and fc) will rely on the response of the boundary layer parameterization, along with input from the cloud microphysics scheme, which are highly uncertain processes. Model gridboxes with low-altitude clouds present in both the PI and PD dominate the forcing in both regions. In the northern NA the brightening of completely overcast low cloud scenes (100 % cloud cover, likely stratocumlus) contributes the most, whereas in the southern NA the creation of clouds with fc of around 20 % from clear skies in the PI was the largest single contributor, suggesting that trade cumulus clouds are created in response to increases in aerosol. The creation of near-overcast clouds was also important there. The correct spatial pattern, coverage and properties of clouds are important for determining the magnitude of aerosol forcing so we also assess the realism of the modelled PD clouds against satellite observations. We find that the model reproduces the spatial pattern of all the observed cloud variables well, but that there are biases. The shortwave top-of-the-atmosphere (SWTOA) flux is overestimated by 5.8 % in the northern NA region and 1.7 % in the southern NA, which we attribute mainly to positive biases in low-altitude fc. Nd is too low by −20.6 % in the northern NA and too high by by 21.5 % in the southern NA, but does not contribute greatly to the main SWTOA biases. Cloudy-sky liquid water path mainly shows biases north of Scandinavia that reach up to between 50 and 100 % and dominate the SWTOA bias in that region. The large contribution to aerosol forcing in the UKESM1 model from highly uncertain macrophysical adjustments suggests that further targeted observations are needed to assess rain formation processes, how they depend on aerosols and the model response to precipitation in order to reduce uncertainty in climate projections.

2020 ◽  
Vol 20 (24) ◽  
pp. 15681-15724
Author(s):  
Daniel P. Grosvenor ◽  
Kenneth S. Carslaw

Abstract. Climate variability in the North Atlantic influences processes such as hurricane activity and droughts. Global model simulations have identified aerosol–cloud interactions (ACIs) as an important driver of sea surface temperature variability via surface aerosol forcing. However, ACIs are a major cause of uncertainty in climate forcing; therefore, caution is needed in interpreting the results from coarse-resolution, highly parameterized global models. Here, we separate and quantify the components of the surface shortwave effective radiative forcing (ERF) due to aerosol in the atmosphere-only version of the UK Earth System Model (UKESM1) and evaluate the cloud properties and their radiative effects against observations. We focus on a northern region of the North Atlantic (NA) where stratocumulus clouds dominate (denoted the northern NA region) and a southern region where trade cumulus and broken stratocumulus dominate (southern NA region). Aerosol forcing was diagnosed using a pair of simulations in which the meteorology is approximately fixed via nudging to analysis; one simulation has pre-industrial (PI) and one has present-day (PD) aerosol emissions. This model does not include aerosol effects within the convective parameterization (but aerosol does affect the clouds associated with detrainment) and so it should be noted that the representation of aerosol forcing for convection is incomplete. Contributions to the surface ERF from changes in cloud fraction (fc), in-cloud liquid water path (LWPic) and droplet number concentration (Nd) were quantified. Over the northern NA region, increases in Nd and LWPic dominate the forcing. This is likely because the already-high fc there reduces the chances of further large increases in fc and allows cloud brightening to act over a larger region. Over the southern NA region, increases in fc dominate due to the suppression of rain by the additional aerosols. Aerosol-driven increases in macrophysical cloud properties (LWPic and fc) will rely on the response of the boundary layer parameterization, along with input from the cloud microphysics scheme, which are highly uncertain processes. Model grid boxes with low-altitude clouds present in both the PI and PD dominate the forcing in both regions. In the northern NA, the brightening of completely overcast low cloud scenes (100 % cloud cover, likely stratocumulus) contributes the most, whereas in the southern NA the creation of clouds with fc of around 20 % from clear skies in the PI was the largest single contributor, suggesting that trade cumulus clouds are created in response to increases in aerosol. The creation of near-overcast clouds was also important there. The correct spatial pattern, coverage and properties of clouds are important for determining the magnitude of aerosol forcing, so we also assess the realism of the modelled PD clouds against satellite observations. We find that the model reproduces the spatial pattern of all the observed cloud variables well but that there are biases. The shortwave top-of-the-atmosphere (SWTOA) flux is overestimated by 5.8 % in the northern NA region and 1.7 % in the southern NA, which we attribute mainly to positive biases in low-altitude fc. Nd is too low by −20.6 % in the northern NA and too high by 21.5 % in the southern NA but does not contribute greatly to the main SWTOA biases. Cloudy-sky liquid water path mainly shows biases north of Scandinavia that reach between 50 % and 100 % and dominate the SWTOA bias in that region. The large contribution to aerosol forcing in the UKESM1 model from highly uncertain macrophysical adjustments suggests that further targeted observations are needed to assess rain formation processes, how they depend on aerosols and the model response to precipitation in order to reduce uncertainty in climate projections.


2021 ◽  
Author(s):  
Pedro Jiménez-Guerrero ◽  
Nuno Ratola

AbstractThe atmospheric concentration of persistent organic pollutants (and of polycyclic aromatic hydrocarbons, PAHs, in particular) is closely related to climate change and climatic fluctuations, which are likely to influence contaminant’s transport pathways and transfer processes. Predicting how climate variability alters PAHs concentrations in the atmosphere still poses an exceptional challenge. In this sense, the main objective of this contribution is to assess the relationship between the North Atlantic Oscillation (NAO) index and the mean concentration of benzo[a]pyrene (BaP, the most studied PAH congener) in a domain covering Europe, with an emphasis on the effect of regional-scale processes. A numerical simulation for a present climate period of 30 years was performed using a regional chemistry transport model with a 25 km spatial resolution (horizontal), higher than those commonly applied. The results show an important seasonal behaviour, with a remarkable spatial pattern of difference between the north and the south of the domain. In winter, higher BaP ground levels are found during the NAO+ phase for the Mediterranean basin, while the spatial pattern of this feature (higher BaP levels during NAO+ phases) moves northwards in summer. These results show deviations up to and sometimes over 100% in the BaP mean concentrations, but statistically significant signals (p<0.1) of lower changes (20–40% variations in the signal) are found for the north of the domain in winter and for the south in summer.


2020 ◽  
Vol 6 (29) ◽  
pp. eabb0425 ◽  
Author(s):  
Minhua Qin ◽  
Aiguo Dai ◽  
Wenjian Hua

Earth’s climate fluctuates considerably on decadal-multidecadal time scales, often causing large damages to our society and environment. These fluctuations usually result from internal dynamics, and many studies have linked them to internal climate modes in the North Atlantic and Pacific oceans. Here, we show that variations in volcanic and anthropogenic aerosols have caused in-phase, multidecadal SST variations since 1920 across all ocean basins. These forced variations resemble the Atlantic Multidecadal Oscillation (AMO) in time. Unlike the North Atlantic, where indirect and direct aerosol effects on surface solar radiation drive the multidecadal SST variations, over the tropical central and western Pacific atmospheric circulation response to aerosol forcing plays an important role, whereas aerosol-induced radiation change is small. Our new finding implies that AMO-like climate variations in Eurasia, North America, and other regions may be partly caused by the aerosol forcing, rather than being originated from the North Atlantic SST variations as previously thought.


2021 ◽  
Author(s):  
Jon Robson ◽  
Matthew Menary ◽  
Jonathan Gregory ◽  
Colin Jones ◽  
Bablu Sinha ◽  
...  

&lt;p&gt;Previous work has shown that anthropogenic aerosol emissions drive a strengthening in the Atlantic Meridional Overturning Circulation (AMOC) in CMIP6 historical simulations over ~1850-1985. However, the mechanisms driving the increase are not fully understood. Previously, forced AMOC changes have been linked to changes in surface heat fluxes, changes in salinity, and interhemispheric energy imbalances. Here we will show that across CMIP6 historical simulations there is a strong correlation between ocean heat loss from the subpolar North Atlantic and the forced change in the AMOC. Furthermore, the model spread in the surface heat flux change explains the spread of the AMOC response and is correlated with the strength of the models&amp;#8217; aerosol forcing.&amp;#160; However, the AMOC change is not strongly related to changes in downwelling surface shortwave radiation over the North Atlantic, showing that anthropogenic aerosols do not drive AMOC change through changes in the local surface radiation budget. Rather, by separating the models into those with &amp;#8216;strong&amp;#8217; and &amp;#8216;weak&amp;#8217; aerosol forcing, we show that aerosols appear to predominantly imprint their impact on the AMOC through changes in surface air temperature over the Northern Hemisphere and the consequent impact on latent and sensible heat flux. This thermodynamic driver (i.e. more heat loss from the North Atlantic) is enhanced both by the increase in the AMOC itself, which acts as a positive feedback, and by a response in atmospheric circulation.&amp;#160;&lt;/p&gt;


2020 ◽  
Vol 12 (3) ◽  
pp. 2121-2135
Author(s):  
Caroline A. Poulsen ◽  
Gregory R. McGarragh ◽  
Gareth E. Thomas ◽  
Martin Stengel ◽  
Matthew W. Christensen ◽  
...  

Abstract. We present version 3 (V3) of the Cloud_cci Along-Track Scanning Radiometer (ATSR) and Advanced ATSR (AATSR) data set. The data set was created for the European Space Agency (ESA) Cloud_cci (Climate Change Initiative) programme. The cloud properties were retrieved from the second ATSR (ATSR-2) on board the second European Remote Sensing Satellite (ERS-2) spanning 1995–2003 and the AATSR on board Envisat, which spanned 2002–2012. The data are comprised of a comprehensive set of cloud properties: cloud top height, temperature, pressure, spectral albedo, cloud effective emissivity, effective radius, and optical thickness, alongside derived liquid and ice water path. Each retrieval is provided with its associated uncertainty. The cloud property retrievals are accompanied by high-resolution top- and bottom-of-atmosphere shortwave and longwave fluxes that have been derived from the retrieved cloud properties using a radiative transfer model. The fluxes were generated for all-sky and clear-sky conditions. V3 differs from the previous version 2 (V2) through development of the retrieval algorithm and attention to the consistency between the ATSR-2 and AATSR instruments. The cloud properties show improved accuracy in validation and better consistency between the two instruments, as demonstrated by a comparison of cloud mask and cloud height with co-located CALIPSO data. The cloud masking has improved significantly, particularly in its ability to detect clear pixels. The Kuiper Skill score has increased from 0.49 to 0.66. The cloud top height accuracy is relatively unchanged. The AATSR liquid water path was compared with the Multisensor Advanced Climatology of Liquid Water Path (MAC-LWP) in regions of stratocumulus cloud and shown to have very good agreement and improved consistency between ATSR-2 and AATSR instruments. The correlation with MAC-LWP increased from 0.4 to over 0.8 for these cloud regions. The flux products are compared with NASA Clouds and the Earth's Radiant Energy System (CERES) data, showing good agreement within the uncertainty. The new data set is well suited to a wide range of climate applications, such as comparison with climate models, investigation of trends in cloud properties, understanding aerosol–cloud interactions, and providing contextual information for co-located ATSR-2/AATSR surface temperature and aerosol products. The following new digital identifier has been issued for the Cloud_cci ATSR-2/AATSRv3 data set: https://doi.org/10.5676/DWD/ESA_Cloud_cci/ATSR2-AATSR/V003 (Poulsen et al., 2019).


2021 ◽  
Author(s):  
Philipp Richter ◽  
Mathias Palm ◽  
Christine Weinzierl ◽  
Hannes Griesche ◽  
Penny M. Rowe ◽  
...  

Abstract. A dataset of microphysical cloud parameters from optically thin clouds, retrieved from infrared spectral radiances measured in summer 2017 in the Arctic, is presented. Measurements were conducted using a mobile Fourier-transform infrared (FTIR) spectrometer which was carried by the RV Polarstern. This dataset contains retrieved optical depths and effective radii of ice and water, from which the liquid water path and ice water path are calculated. These water paths and the effective radii are compared with derived quantities from a combined cloud radar, lidar and microwave radiometer measurement synergy retrieval, called Cloudnet. Comparing the liquid water paths from the infrared retrieval and Cloudnet shows significant correlations with a standard deviation of 8.60 g · m−2. Although liquid water path retrievals from microwave radiometer data come with a uncertainty of at least 20 g · m−2, a significant correlation and a standard deviation of 5.32 g · m−2 between the results of clouds with a liquid water path of at most 20 g · m−2 retrieved from infrared spectra and results from Cloudnet can be seen. Therefore, despite its large uncertainty, the comparison with data retrieved from infrared spectra shows that optically thin clouds of the measurement campaign in summer 2017 can be observed well using microwave radiometers within the Cloudnet framework. Apart from this, the dataset of microphysical cloud properties presented here allows to perform calculations of the cloud radiative effects, when the Cloudnet data from the campaign are not available, which was from the 22nd July 2017 until the 19th August 2017. The dataset is published at Pangaea (Richter et al., 2021).


2011 ◽  
Vol 11 (6) ◽  
pp. 2893-2901 ◽  
Author(s):  
M. de la Torre Juárez ◽  
A. B. Davis ◽  
E. J. Fetzer

Abstract. Means, standard deviations, homogeneity parameters used in models based on their ratio, and the probability distribution functions (PDFs) of cloud properties from the MODerate resolution Infrared Spectrometer (MODIS) are estimated globally as function of averaging scale varying from 5 to 500 km. The properties – cloud fraction, droplet effective radius, and liquid water path – all matter for cloud-climate uncertainty quantification and reduction efforts. Global means and standard deviations are confirmed to change with scale. For the range of scales considered, global means vary only within 3% for cloud fraction, 7% for liquid water path, and 0.2% for cloud particle effective radius. These scale dependences contribute to the uncertainties in their global budgets. Scale dependence for standard deviations and generalized flatness are compared to predictions for turbulent systems. Analytical expressions are identified that fit best to each observed PDF. While the best analytical PDF fit to each variable differs, all PDFs are well described by log-normal PDFs when the mean is normalized by the standard deviation inside each averaging domain. Importantly, log-normal distributions yield significantly better fits to the observations than gaussians at all scales. This suggests a possible approach for both sub-grid and unified stochastic modeling of these variables at all scales. The results also highlight the need to establish an adequate spatial resolution for two-stream radiative studies of cloud-climate interactions.


2019 ◽  
Author(s):  
Caroline A. Poulsen ◽  
Gregory R. Mcgarragh ◽  
Gareth E. Thomas ◽  
Martin Stengel ◽  
Matthew W. Christiensen ◽  
...  

Abstract. We present version 3 (V3) of the Cloud_cci ATSR-2/AATSR dataset. The dataset was created for the European Space Agency (ESA) Cloud_cci (Climate Change Initiative) program. The cloud properties were retrieved from the second Along- Track Scanning Radiometer (ATSR-2) on board the second European Remote Sensing Satellite (ERS-2) spanning 1995–2003 and the Advanced ATSR (AATSR) on board Envisat, which spanned 2002–2012. The data comprises a comprehensive set of cloud properties: cloud top height, temperature, pressure, spectral albedo, cloud effective emissivity, effective radius and optical thickness alongside derived liquid and ice water path. Each retrieval is provided with its associated uncertainty. The cloud property retrievals are accompanied by high-resolution top and bottom-of-atmosphere short- and long-wave fluxes that have been derived from the retrieved cloud properties using a radiative transfer model. The fluxes were generated for all-sky and clear-sky conditions. V3 differs from the previous version 2 (V2) through development of the retrieval algorithm and attention to the consistency between the ATSR-2 and AATSR instruments. The cloud properties show improved accuracy in validation and better consistency between the two instruments, as demonstrated by a comparison of cloud mask and cloud height with collocated CALIPSO data. The cloud masking has improved significantly, particularly the ability to detect clear pixels The Kuiper Skill score has increased from .49 to .66. The cloud top height accuracy is relatively unchanged. The AATSR liquid water path was compared with the Multisensor Advanced Climatology of Liquid Water Path (MAC-LWP) in regions of stratocumulous cloud and shown to have very good agreement and improved consistency between ATSR-2 and AATSR instruments, the Correlation with MAC-LWP increase from .4 to over .8 for these cloud regions. The flux products are compared with NASA Clouds and the Earth’s Radiant Energy System (CERES) data, showing good agreement within the uncertainty. The new dataset is well suited to a wide range of climate applications, such as comparison with climate models, investigation of trends in cloud properties, understanding aerosol-cloud interactions, and providing contextual information for collocated ATSR-2/AATSR surface temperature and aerosol products. For the Cloud_cci ATSR-2/AATSRv3 dataset a new digital identifier has been issued: https://doi.org/10.5676/DWD/ESA_Cloud_cci/ATSR2-AATSR/V003 Poulsen et al. (2019).


2013 ◽  
Vol 26 (11) ◽  
pp. 3823-3845 ◽  
Author(s):  
Axel Lauer ◽  
Kevin Hamilton

Abstract Clouds are a key component of the climate system affecting radiative balances and the hydrological cycle. Previous studies from the Coupled Model Intercomparison Project phase 3 (CMIP3) showed quite large biases in the simulated cloud climatology affecting all GCMs as well as a remarkable degree of variation among the models that represented the state of the art circa 2005. Here the progress that has been made in recent years is measured by comparing mean cloud properties, interannual variability, and the climatological seasonal cycle from the CMIP5 models with satellite observations and with results from comparable CMIP3 experiments. The focus is on three climate-relevant cloud parameters: cloud amount, liquid water path, and cloud radiative forcing. The comparison shows that intermodel differences are still large in the Coupled Model Intercomparison Project phase 5 (CMIP5) simulations, and reveals some small improvements of particular cloud properties in some regions in the CMIP5 ensemble over CMIP3. In CMIP5 there is an improved agreement of the modeled interannual variability of liquid water path and of the modeled longwave cloud forcing over mid- and high-latitude oceans with observations. However, the differences in the simulated cloud climatology from CMIP3 and CMIP5 are generally small, and there is very little to no improvement apparent in the tropical and subtropical regions in CMIP5. Comparisons of the results from the coupled CMIP5 models with their atmosphere-only versions run with observed SSTs show remarkably similar biases in the simulated cloud climatologies. This suggests the treatments of subgrid-scale cloud and boundary layer processes are directly implicated in the poor performance of current GCMs in simulating realistic cloud fields.


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