scholarly journals Dynamics of the Great Oxidation Event from a 3D photochemical-climate model

2021 ◽  
Author(s):  
Adam Yassin Jaziri ◽  
Benjamin Charnay ◽  
Franck Selsis ◽  
Jérémy Leconte ◽  
Franck Lefèvre
Keyword(s):  
Temperature Dependence ◽  
Atmospheric Circulation ◽  
Climate Model ◽  
Ozone Layer ◽  
Oxygen Level ◽  
Great Oxidation Event ◽  
Atmospheric Instability ◽  
Major Shift ◽  
Rapid Transition ◽  
Methane Concentrations

Abstract. From the Archean toward the Proterozoic, the Earth's atmosphere underwent a major shift from anoxic to oxic conditions, around 2.4 to 2.1 Gyr, known as the Great Oxidation Event (GOE). This rapid transition may be related to an atmospheric instability caused by the formation of the ozone layer. Previous works were all based on 1D photochemical models. Here, we revisit the GOE with a 3D photochemical-climate model to investigate the possible impact of the atmospheric circulation and the coupling between the climate and the dynamics of the oxidation. We show that the diurnal, seasonal and transport variations do not bring significant changes compared to 1D models. Nevertheless, we highlight a temperature dependence for atmospheric photochemical losses. A cooling during the late Archean could then have favored the triggering of the oxygenation. In addition, we show that the Huronian glaciations, which took place during the GOE, could have introduced a fluctuation in the evolution of the oxygen level. Finally, we show that the oxygen overshoot which is expected to have occurred just after the GOE, was likely accompanied by a methane overshoot. Such high methane concentrations could have had climatic consequences and could have played a role in the dynamics of the Huronian glaciations.

The response of stratospheric ozone and dynamics to changes in atmospheric oxygen

2021 ◽  
Author(s):  
Iga Józefiak ◽  
Timofei Sukhodolov ◽  
Tatiana Egorova ◽  
Eugene Rozanov ◽  
Gabriel Chiodo ◽  
...  
Keyword(s):  
Molecular Oxygen ◽  
Climate Model ◽  
Atmospheric Oxygen ◽  
Stratospheric Ozone ◽  
Ozone Layer ◽  
Self Healing ◽  
Oxygen Level ◽  
Meridional Transport ◽  
Regional Patterns ◽  
Total Column Ozone

<p>Photolysis of molecular oxygen (O<sub>2</sub>) maintains the stratospheric ozone layer, protecting living organisms on Earth by absorbing harmful ultraviolet radiation. The atmospheric oxygen level has not always been constant, and has been held responsible for species extinctions via a thinning of the ozone layer in the past. On paleo-climate timescales, it ranged between 10 and 35% depending on the level of photosynthetic activity of plants and oceans. Previous estimates, however, showed highly uncertain ozone (O<sub>3</sub>) <sub></sub>responses to atmospheric O<sub>2</sub> changes, including monotonic positive or negative correlations, or displaying a maximum in O<sub>3 </sub>column around a certain oxygen level. Motivated by these discrepancies we reviewed how the ozone layer responds to atmospheric oxygen changes by means of a state-of-the-art chemistry-climate model (CCM). We used the CCM SOCOL-AERv2 to assess the ozone layer sensitivity to past and potential future concentrations of atmospheric oxygen varying from 5 to 40 %. Our findings are at odds with previous studies: we find that the current mixing ratio of O<sub>2</sub>, 21 %, indeed maximizes the O<sub>3</sub> layer thickness and, thus, represents an optimal state for life on Earth. In the model, any alteration in atmospheric oxygen would result globally in less total column ozone and, therefore, more UV reaching the troposphere. Total ozone column in low-latitude regions is less sensitive to the changes, because of the “self-healing” effect, i.e. more UV entering lower levels, where O<sub>2</sub> photolyzes, can partly compensate the O<sub>3</sub> lack higher up. Mid- and high-latitudes, however, are characterized by ±20 DU ozone hemispheric redistributions even for small (±5 %) variations in O<sub>2</sub> content. Additional regional patterns result from the hemispheric asymmetry of meridional transport pathways via the Brewer-Dobson circulation (BDC). We will discuss the different ozone responses resulting from changes in the BDC. These effects are further modulated by the influence of ozone on stratospheric temperatures and thus on the BDC. Lower O<sub>2 </sub>cases result in a deceleration of the BDC. This renders the relation between ozone and molecular oxygen changes non-linear on both global and regional scales.</p>

Influence of atmospheric circulation variations on the ozone layer

2005 ◽  
Vol 26 (16) ◽  
pp. 3467-3478 ◽  
Author(s):  
E. A. Jadin ◽  
K. YA. Kondratyev ◽  
V. I. Bekoryukov ◽  
P. N. Vargin
Keyword(s):  
Atmospheric Circulation ◽  
Ozone Layer

scholarly journals Temperature-dependence of aerosol optical depth over the southeastern US

2016 ◽  
Author(s):  
Tero Mielonen ◽  
Anca Hienola ◽  
Thomas Kühn ◽  
Joonas Merikanto ◽  
Antti Lipponen ◽  
...  
Keyword(s):  
Temperature Dependence ◽  
Land Surface ◽  
Radiative Forcing ◽  
Climate Model ◽  
Biogenic Emissions ◽  
Anthropogenic Emissions ◽  
Model Estimate ◽  
Model Simulations ◽  
Southeastern Us ◽  
Biogenic Aerosols

Abstract. Previous studies have indicated that summer-time aerosol optical depths (AOD) over the southeastern US are dependent on temperature but the reason for this dependence and its radiative effects have so far been unclear. To quantify these effects we utilized AOD and land surface temperature (LST) products from the Advanced Along-Track Scanning Radiometer (AATSR) with observations of tropospheric nitrogen dioxide (NO2) column densities from the Ozone Monitoring Instrument (OMI). Furthermore, simulations of the global aerosol-climate model ECHAM-HAMMOZ have been used to identify the possible processes affecting aerosol loads and their dependence on temperature over the studied region. Our results showed that the level of AOD in the southeastern US is mainly governed by anthropogenic emissions but the observed temperature dependent behaviour is most likely originating from non-anthropogenic emissions. Model simulations indicated that biogenic emissions of volatile organic compounds (BVOC) can explain the observed temperature dependence of AOD. According to the remote sensing data sets, the non-anthropogenic contribution increases AOD by approximately 0.009 ± 0.018 K−1 while the modelled BVOC emissions increase AOD by 0.022 ± 0.002 K−1. Consequently, the regional direct radiative effect (DRE) of the non-anthropogenic AOD is −0.43 ± 0.88 W/m2/K and −0.17 ± 0.35 W/m2/K for clear- and all-sky conditions, respectively. The model estimate of the regional clear-sky DRE for biogenic aerosols is also in the same range: −0.86 ± 0.06 W/m2/K. These DRE values indicate significantly larger cooling than the values reported for other forested regions. Furthermore, the model simulations showed that biogenic emissions increased the number of biogenic aerosols with radius larger than 100 nm (N100, proxy for cloud condensation nuclei) by 28 % per one degree temperature increase. For the total N100, the corresponding increase was 4 % which implies that biogenic emissions could also have a small effect on indirect radiative forcing in this region.

scholarly journals Global stratospheric measurements of the isotopologues of methane from the Atmospheric Chemistry Experiment Fourier Transform Spectrometer

2015 ◽  
Vol 8 (10) ◽  
pp. 11171-11207
Author(s):  
E. M. Buzan ◽  
C. A. Beale ◽  
C. D. Boone ◽  
P. F. Bernath
Keyword(s):  
Fourier Transform ◽  
Atmospheric Chemistry ◽  
Climate Model ◽  
Fourier Transform Spectrometer ◽  
Atmospheric Methane ◽  
Community Climate Model ◽  
Atmospheric Sinks ◽  
Chemistry Experiment ◽  
Methane Concentrations ◽  
Balloon Measurements

Abstract. This paper presents an analysis of observations of methane and its two major isotopologues, CH3D and 13CH4 from the Atmospheric Chemistry Experiment (ACE) satellite between 2004 and 2013. Additionally, atmospheric methane chemistry is modeled using the Whole Atmospheric Community Climate Model (WACCM). ACE retrievals of methane extend from 6 km for all isotopologues to 75 km for 12CH4, 35 km for CH3D, and 50 km for 13CH4. While total methane concentrations retrieved from ACE agree well with the model, values of δD–CH4 and δ13C–CH4 show a bias toward higher δ compared to the model and balloon-based measurements. Calibrating δD and δ13C from ACE using WACCM in the troposphere gives improved agreement in δD in the stratosphere with the balloon measurements, but values of δ13C still disagree. A model analysis of methane's atmospheric sinks is also performed.

scholarly journals Supplementary material to "Effects of Strongly Enhanced Atmospheric Methane Concentrations in a Fully Coupled Chemistry-Climate Model"

2020 ◽  
Author(s):  
Laura Stecher ◽  
Franziska Winterstein ◽  
Martin Dameris ◽  
Patrick Jöckel ◽  
Michael Ponater ◽  
...  
Keyword(s):  
Climate Model ◽  
Atmospheric Methane ◽  
Supplementary Material ◽  
Fully Coupled ◽  
Methane Concentrations

scholarly journals Comparison of 20th century and pre-industrial climate over South America in regional model simulations

2012 ◽  
Vol 8 (5) ◽  
pp. 1599-1620 ◽  
Author(s):  
S. Wagner ◽  
I. Fast ◽  
F. Kaspar
Keyword(s):  
South America ◽  
Greenhouse Gas ◽  
Atmospheric Circulation ◽  
20Th Century ◽  
Climate Model ◽  
Regional Climate ◽  
Regional Model ◽  
Andes Mountains ◽  
Southern South America ◽  
The Andes

Abstract. In this study, we assess how the anthropogenically induced increase in greenhouse gas concentrations affects the climate of central and southern South America. We utilise two regional climate simulations for present day (PD) and pre-industrial (PI) times. These simulations are compared to historical reconstructions in order to investigate the driving processes responsible for climatic changes between the different periods. The regional climate model is validated against observations for both re-analysis data and GCM-driven regional simulations for the second half of the 20th century. Model biases are also taken into account for the interpretation of the model results. The added value of the regional simulation over global-scale modelling relates to a better representation of hydrological processes that are particularly evident in the proximity of the Andes Mountains. Climatic differences between the simulated PD minus PI period agree qualitatively well with proxy-based temperature reconstructions, albeit the regional model overestimates the amplitude of the temperature increase. For precipitation the most important changes between the PD and PI simulation relate to a dipole pattern along the Andes Mountains with increased precipitation over the southern parts and reduced precipitation over the central parts. Here only a few regions show robust similarity with studies based on empirical evidence. However, from a dynamical point-of-view, atmospheric circulation changes related to an increase in high-latitude zonal wind speed simulated by the regional climate model are consistent with numerical modelling studies addressing changes in greenhouse gas concentrations. Our results indicate that besides the direct effect of greenhouse gas changes, large-scale changes in atmospheric circulation and sea surface temperatures also exert an influence on temperature and precipitation changes in southern South America. These combined changes in turn affect the relationship between climate and atmospheric circulation between PD and PI times and should be considered for the statistical reconstruction of climate indices calibrated within present-day climate data.

scholarly journals Seasonal Drought in the Greater Horn of Africa and Its Recent Increase during the March–May Long Rains

2014 ◽  
Vol 27 (21) ◽  
pp. 7953-7975 ◽  
Author(s):  
Bradfield Lyon
Keyword(s):  
Atmospheric Circulation ◽  
Climate Model ◽  
Southern Oscillation ◽  
Meteorological Drought ◽  
Tropical Pacific ◽  
Horn Of Africa ◽  
New Findings ◽  
Climate Model Simulations ◽  
Greater Horn Of Africa ◽  
The Tropical Pacific

Abstract This paper provides a review of atmospheric circulation and sea surface temperature (SST) conditions that are associated with meteorological drought on the seasonal time scale in the Greater Horn of Africa (the region 10°S–15°N, 30°–52°E). New findings regarding a post-1998 increase in drought frequency during the March–May (MAM) “long rains” are also reported. The period 1950–2010 is emphasized, although rainfall and SST data from 1901–2010 are used to place the recent long rains decline in a multidecadal context. For the latter case, climate model simulations and isolated basin SST experiments are also utilized. Climatologically, rainfall exhibits a unimodal June–August (JJA) maximum in west-central Ethiopia with a generally bimodal [MAM and October–December (OND) maxima] distribution in locations to the south and east. Emphasis will be on these three seasons. SST anomalies in the tropical Pacific and Indian Oceans show the strongest association with drought during OND in locations having a bimodal annual cycle, with weaker associations during MAM. The influence of the El Niño–Southern Oscillation (ENSO) phenomenon critically depends on its ability to affect SSTs outside the Pacific. Salient features of the anomalous atmospheric circulation during drought events in different locations and seasons are discussed. The post-1998 decline in the long rains is found to be driven strongly (although not necessarily exclusively) by natural multidecadal variability in the tropical Pacific rather than anthropogenic climate change. This conclusion is supported by observational analyses and climate model experiments, which are presented.

scholarly journals Nighttime Mesospheric Ozone During the 2002 Southern Hemispheric Major Stratospheric Warming

2016 ◽  
Author(s):  
Christine Smith-Johnsen ◽  
Yvan Orsolini ◽  
Frode Stordal ◽  
Varavut Limpasuvan ◽  
Kristell Pérot
Keyword(s):  
Atomic Oxygen ◽  
Lower Stratosphere ◽  
Climate Model ◽  
Middle Atmosphere ◽  
Ozone Layer ◽  
Stratospheric Warming ◽  
Mesospheric Ozone ◽  
Northern Hemispheric ◽  
Second Year ◽  
The Antarctic

Abstract. A Sudden Stratospheric Warming (SSW) affects the chemistry and dynamics of the middle atmosphere. The major warmings occur roughly every second year in the Northern Hemispheric (NH) winter, but has only been observed once in the Southern Hemisphere (SH), during the Antarctic winter of 2002. Using the National Center for Atmospheric Research's (NCAR) Whole Atmosphere Community Climate Model with specified dynamics (WACCM-SD), this study investigates the effects of this rare warming event on the ozone layer located around the SH mesopause. This secondary ozone layer changes with respect to hydrogen, oxygen, temperature, and the altered SH polar circulation during the major SSW. The 2002 SH winter was characterized by three zonal-mean zonal wind reductions in the upper stratosphere before a fourth wind reversal reaches the lower stratosphere, marking the onset of the major SSW. At the time of these four wind reversals, a corresponding episodic increase can be seen in the modeled nighttime ozone concentration in the secondary ozone layer. Observations by the Global Ozone Monitoring by Occultation of Stars (GOMOS, an instrument on board the satellite Envisat) demonstrate similar ozone enhancement as in the model. This ozone increase is attributable largely to enhanced upwelling and the associated cooling of the altitude region in conjunction with the wind reversal. Unlike its NH counterpart, the secondary ozone layer during the SH major SSW appeared to be impacted more by the effects of atomic oxygen than hydrogen.

Sign in / Sign up

Export Citation Format

Share Document