Monitoring ambient aerosol size distributions from 1 – 55 nm with the GRIMM-AIRMODUS PSMPS 

Author(s):  
Gerhard Steiner ◽  
Harald Flentje ◽  
Minna Väkevä ◽  
Lothar Keck ◽  
Joonas Vanhanen

<p>Here, we present the final, commercially available, version of a mobility particle size spectrometer that is able to access the 1 nm particle size range for ambient atmospheric measurements.</p><p>The overall system performance was tested in a multitude of laboratory experiments, determining various size dependent parameters like DMA’s transfer function, DMA penetration efficiency, PSM and CPC counting efficiency. With the knowledge of these parameters, we are able to define a well-known overall system performance, a critical prerequisite for measurements that start at 1 nm sized particles.</p><p>The instrument originates from a collaboration of Grimm Aerosol Technik, Germany and Airmodus Ltd, Finland, combining a Grimm SMPS+C system with the Airmodus Particle Size Magnifier (PSM). Accordingly, it is named: PSMPS.</p><p>The main system components comprise a modified version of the short Grimm Differential Mobility Analyzer (Grimm S-DMA), the diethylene glycol-based PSM (Airmodus A10) and the new butanol-based CPC (Grimm 5417). The modified S-DMA is specially optimized for the transmission of small ions. Typically, it is operated with an aerosol sample flow rate of 2.5 L/min and a sheath flow rate of 10 L/min, allowing particle size distribution measurements from 1.1-55.7 nm. The PSM is used to lower the detection efficiency of the Grimm CPC below 2 nm in electrical mobility equivalent diameter. The new Grimm 5417 CPC is an upgraded version of the well-known 5416 CPC, that features two switchable aerosol sample flow rates of 0.3 and 0.6 L/min and also supplies the S-DMA with sheath airflow rates of either 3.0 or 10.0 L/min.</p><p>In this presentation, we will introduce the features and performance of the PSMPS system, will highlight some laboratory characterization tests and report the results from an ambient aerosol measurement campaign at the Hohenpeissenberg Observatory of the German meteorological service (DWD), monitoring new particle formation events starting at a particles size of 1nm.</p>

2020 ◽  
Vol 20 (7) ◽  
pp. 4209-4225 ◽  
Author(s):  
Junteng Wu ◽  
Alessandro Faccinetto ◽  
Symphorien Grimonprez ◽  
Sébastien Batut ◽  
Jérôme Yon ◽  
...  

Abstract. Combustion and other high-temperature processes frequently result in the emission of aerosols in the form of polydisperse fractal-like aggregates made of condensed-phase nanoparticles (soot for instance). If certain conditions are met, the emitted aerosol particles are known to evolve into important cloud condensation nuclei (CCN) in the atmosphere. In this work, the hygroscopic parameter κ of complex morphology aggregates is calculated from the supersaturation-dependent activated fraction Fa=Fa(SS) in the frame of κ-Köhler theory. The particle size distribution is approximated with the morphology-corrected volume equivalent diameter calculated from the electrical mobility diameter by taking into account the diameter of the primary particle and the fractal dimension of the aggregate experimentally obtained from transmission electron microscopy measurements. Activation experiments are performed in water supersaturation conditions using a commercial CCN-100 condensation nuclei counter. The model is tested in close-to-ideal conditions of size-selected, isolated spherical particles (ammonium sulfate nanoparticles dispersed in nitrogen), then with complex polydisperse fractal-like aggregates (soot particles activated by exposure to ozone with κ as low as 5×10-5) that represent realistic anthropogenic emissions in the atmosphere.


2001 ◽  
Author(s):  
V. Aizenberg ◽  
P. Baron ◽  
K. Choe ◽  
S. Grinshpun ◽  
K. Willeke

2018 ◽  
Vol 14 (1) ◽  
pp. 31-60 ◽  
Author(s):  
M. Y. Guida ◽  
F. E. Laghchioua ◽  
A. Hannioui

This article deals with fast pyrolysis of brown algae, such as Bifurcaria Bifurcata at the range of temperature 300–800 °C in a stainless steel tubular reactor. After a literature review on algae and its importance in renewable sector, a case study was done on pyrolysis of brown algae especially, Bifurcaria Bifurcata. The aim was to experimentally investigate how the temperature, the particle size, the nitrogen flow rate (N2) and the heating rate affect bio-oil, bio-char and gaseous products. These parameters were varied in the ranges of 5–50 °C/min, below 0.2–1 mm and 20–200 mL. min–1, respectively. The maximum bio-oil yield of 41.3wt% was obtained at a pyrolysis temperature of 600 °C, particle size between 0.2–0.5 mm, nitrogen flow rate (N2) of 100 mL. min–1 and heating rate of 5 °C/min. Liquid product obtained under the most suitable and optimal condition was characterized by elemental analysis, 1H-NMR, FT-IR and GC-MS. The analysis of bio-oil showed that bio-oil from Bifurcaria Bifurcata could be a potential source of renewable fuel production and value added chemicals.


2020 ◽  
Vol 71 (1) ◽  
pp. 1-12
Author(s):  
Salman H. Abbas ◽  
Younis M. Younis ◽  
Mohammed K. Hussain ◽  
Firas Hashim Kamar ◽  
Gheorghe Nechifor ◽  
...  

The biosorption performance of both batch and liquid-solid fluidized bed operations of dead fungal biomass type (Agaricusbisporus ) for removal of methylene blue from aqueous solution was investigated. In batch system, the adsorption capacity and removal efficiency of dead fungal biomass were evaluated. In fluidized bed system, the experiments were conducted to study the effects of important parameters such as particle size (701-1400�m), initial dye concentration(10-100 mg/L), bed depth (5-15 cm) and solution flow rate (5-20 ml/min) on breakthrough curves. In batch method, the experimental data was modeled using several models (Langmuir,Freundlich, Temkin and Dubinin-Radushkviechmodels) to study equilibrium isotherms, the experimental data followed Langmuir model and the results showed that the maximum adsorption capacity obtained was (28.90, 24.15, 21.23 mg/g) at mean particle size (0.786, 0.935, 1.280 mm) respectively. In Fluidized-bed method, the results show that the total ion uptake and the overall capacity will be decreased with increasing flow rate and increased with increasing initial concentrations, bed depth and decreasing particle size.


Author(s):  
Zuhaili Idham ◽  
Ahmad Syahmi Zaini ◽  
Nicky Rahmana Putra ◽  
Nurfarhain Mohamed Rusli ◽  
Noor Sabariah Mahat ◽  
...  

2015 ◽  
Vol 651-653 ◽  
pp. 830-835
Author(s):  
Shohei Kajikawa ◽  
Riku Sakagami ◽  
Takashi Iizuka

Thermal flow tests were performed on steamed bamboo powder using capillaries that were processed under different conditions in order to investigate the effect of the die surface state on the fluidity of the woody powder. The capillaries were processed by wire-cut electric discharge machining, reaming or drilling, and the arithmetic average roughness (Ra) varied from 0.5 to 2.5 μm. The bamboo powder was first steamed at 200 °C for 20 min, and its particle size was then controlled using different mesh screens. The thermal flow temperature was set at 200 °C. The results indicated that the flow behavior improved with increasing particle size. For the capillaries processed by WEDM, the flow rate for samples with particle sizes of 75~150 and 150~300 μm decreased with increasing Ra. On the other hand, when reaming or drilling was used to process the capillaries, the flow rate was almost independent of Ra, regardless of the particle size.


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