A five-band absorber based on graphene metamaterial for terahertz ultrasensing

We design and propose a five-band absorber based on graphene metamaterial for the terahertz (THz) sensing field. The localized surface plasmon resonances (LSPR) of patterned graphene are excited, contributing to five tunable ultra-narrow absorption peaks, which are specified by the electric field distributions. Moreover, the absorber is insensitive to different polarization modes and incident angles. When increasing the Fermi level of the patterned graphene, which is composed of a round ring and a square ring connected by four thin wires, the resonant frequencies exhibit distinct blue shifts. For refractive index sensing, due to the addition of a continuous dielectric groove, the theoretical results show that the maximum averaged normalized sensitivity, Q factor, and FOM can reach 0.647 RIU-1 (refractive index unit, RIU), 355.94, and 215.25 RIU-1, indicating that the sensing performances are further enhanced compared with previous works. As a result, the proposed structure may provide a new method to realize ultrasensing in the THz region.

The effects of bending on plasmonic modes in nanowires and planar structures

In this work, we investigate the effects of bends on the surface plasmon resonances in nanowires (NWs) and isolated edges of planar structures using electron energy loss spectroscopy experiments and theoretical calculations. Previous work showed that the sharp bends in NWs do not affect their resonant modes. Here, we study previously overlooked effects and analyze systematically the evolution of resonant modes for several bending angles from 30° to 180°, showing that bending can have a significant effect on the plasmonic response of a nanostructure. In NWs, the modes can experience significant energy shifts that depend on the aspect ratio of the NW and can cause mode intersection and antinode bunching. We establish the relation between NW modes and edge modes and show that bending can even induce antinode splitting in edge modes. This work demonstrates that bends in plasmonic planar nanostructures can have a profound effect on their optical response and this must be accounted for in the design of optical devices.

High-efficiency and tunable circular dichroism in chiral graphene metasurface

Circular dichroism (CD) response is extremely important for dynamic polarization control, chiral molecular sensing and imaging, etc. Here, we numerically demonstrated high-efficiency and tunable CD using a symmetry broken graphene-dielectric-metal composite microstructure. By introducing slot patterns in graphene ribbons, the metasurface exhibits giant spin-selective absorption for circularly polarized (CP) wave excitations. The maximum CD reaches 0.87 at 2.78 THz, which originates from the localized surface plasmon resonances (LSPRs) in patterned graphene. Besides, the operating frequency and magnitude of CD are dynamically manipulated by gating graphene's Fermi energies. The proposed chiral graphene metasurface with high- efficiency and tunable capability paves a way to the design of active CD metasurfaces.

Study of thermoplasmonic properties of gold nanodimer in visible -infrared region of electromagnetic spectrum

In the present study, the heat generation in gold nanodimers when irradiated at their localized surface plasmon resonances is investigated numerically. The theoretical calculations are performed employing the first principal approach to obtain the absorption cross-section of gold nanodimer for different parameter ranges. The heating mechanism is enumerated in terms of its temperature by solving the steady-state heat transfer equation which depends on the absorption cross-section and surface plasmon resonance wavelength. These surface plasmon resonances are quite sensitive to the distance between the dimer and have been tuned from visible to IR range by managing the distance between spheres from 0 to 6nm. The computation of normalized electric field distribution of gold nanodimer under the plasmon resonance has been mapped using boundary element method(BEM) which enables visualization of the local hot spot that plays a significant role in optical heating applications. The work furnishes the basic understanding of the heating mechanism of gold nanodimer which can find application as plasmonic nanoheaters in several branches of science in visible and near-infrared regions of the electromagnetic spectrum.

Single-nanoantenna driven nanoscale control of the VO2 insulator to metal transition

The ultrafast concentration of electromagnetic energy in nanoscale volumes is one of the key features of optical nanoantennas illuminated at their surface plasmon resonances. Here, we drive the insulator to metal phase transition in vanadium dioxide (VO2) using a laser-induced pumping effect obtained by positioning a single gold nanoantenna in proximity to a VO2 thermochromic material. We explore how the geometry of the single nanoantenna affects the size and permittivity of the nanometer-scale VO2 regions featuring phase transition under different pumping conditions. The results reveal that a higher VO2 phase transition effect is obtained for pumping of the longitudinal or transversal localized surface plasmon depending on the antenna length. This characterization is of paramount importance since the single nanoantennas are the building blocks of many plasmonic nanosystems. Finally, we demonstrate the picosecond dynamics of the VO2 phase transition characterizing this system, useful for the realization of fast nano-switches. Our work shows that it is possible to miniaturize the hybrid plasmonic-VO2 system down to the single-antenna level, still maintaining a controllable behavior, fast picosecond dynamics, and the features characterizing its optical and thermal response.

On the Localized Surface Plasmonic Resonances of AgPd Alloy Nanoparticles by Experiment and Theory

Ag/Pd multilayers and AgPd alloyed ultrathin films were deposited on Corning glass by magnetron sputtering. After being annealed in a furnace in air at 460 °C, self-assembled nanoparticles were formed. Localized surface plasmon resonances were observed only for the Ag-rich samples in the full range of the visible light spectrum. The resonance position was found to depend on the initial film thickness. In order to gain further physical insight, rigorous theoretical calculations were carried out via the rigid coupled-wave analysis method for the entire compositional range between Ag and Pd. Theoretical calculations were proven to be in suitable agreement with the experimental results.