Broadband absorption of monolayer MoS2 in visible region using a tetramerized nanorod metasurface

2021 ◽  
Author(s):  
Yao Pei ◽  
Tian Sang ◽  
Qing Mi ◽  
Jicheng Wang ◽  
Yueke Wang

Abstract High-efficient broadband absorption of the monolayer MoS2 is achieved by using a tetramerized nanorod metasurface (TNM), and the average absorption of 64.5% for the monolayer MoS2 can be obtained in the visible range of 400-750 nm. The unit cell of the TNM consists four Ag nanorods with different diameters, the incident light can be selectively absorbed by the monolayer MoS2 due to the magnetic resonance associated with the individual Ag nanorod, and broadband absorption of the monolayer MoS2 is realizable due to the cooperative magnetic resonances related to the tetramerized Ag nanorods. In addition, the absorption of the monolayer MoS2 is robust to the variation of the structural parameters, and it exhibits wide-angle and polarization-independent features.

2021 ◽  
Author(s):  
Raj Kumar ◽  
Bipin K Singh ◽  
Rajesh K Tiwari ◽  
Praveen C Pandey

Abstract In this paper, we have presented a new design of a metamaterial perfect absorber (MPA) consisting of three layers of metal-dielectric-metal in which the top layer is considered of special kind square patches at different places in a unit cell. This MPA exhibits wideband, wide-angle, and polarization-independent absorption performance in the visible region. This structure originates the plasmonic resonance which is responsible for the perfect absorption in the optical region. Under a specific condition, this simulated absorber structure exhibits an extremely high broadband absorption between 591.54 nm to 704.40 nm wavelength range with near-unity absorption, and a single peak observed at 385.33 nm with absorption 94.16%. We extracted the impedance of the absorber and matched it with free space, and also demonstrated the effective permittivity and permeability. Moreover, the parametric study of the resonators, dielectric layer, and multi-band topology has also been investigated. The polarization-insensitive-based metamaterial may be utilized to improve the efficiency of different devices in the visible range. Furthermore, we have calculated the absorption of the proposed MPA under the solar radiation (AM1.5) for different structural parameters. The proposed absorber greatly enhances the conversion efficiency which is highly useful for solar cells. We also determined the short circuit current density of this absorber for different thicknesses of the GaAs layer. Al metal patches at meta-surface provide nearly similar performance in comparison with other costly metals. Therefore, the proposed structure with cheaper Al metal may be used for different devices as the perfect absorber.


Nanomaterials ◽  
2019 ◽  
Vol 9 (9) ◽  
pp. 1222 ◽  
Author(s):  
Chenhui Li ◽  
Haihua Fan ◽  
Qiaofeng Dai ◽  
Zhongchao Wei ◽  
Sheng Lan ◽  
...  

Excellent characteristics and promising application prospects promote the rapid development of metamaterials. We have numerically proposed and demonstrated a novel subwavelength broadband metamaterial perfect absorber (BMPA) based on diamond dielectric arrays. The proposed absorber is composed of an ultra-thin two-layer structure covering the dielectric periodic array on a metal substrate. The materials of dielectric silicon (Si) and gold (Au) substrate are discussed in detail. In addition, different dielectric and refractory materials are also applied to achieve broadband absorption, which will make the proposed absorber greatly broaden the application field. A perfect absorption window (i.e., absorption rate exceeding 90%) can be obtained from near-ultraviolet to the visible range. The average absorption rate of 93.3% is achieved in the visible range. The results of multipole decomposition show that broadband absorption is mainly caused by electromagnetic dipole resonance and lattice resonance in a periodic array of Si. The proposed absorber can be extended freely by adjusting the structural parameters. The polarization-independent and incident angle insensitivity are proved. The proposed absorber may well be used in light energy acquisition, as well as for the scalability of optoelectronic and sensing devices.


Materials ◽  
2019 ◽  
Vol 12 (7) ◽  
pp. 1050 ◽  
Author(s):  
Kyu-Tae Lee ◽  
Daeshik Kang ◽  
Hui Park ◽  
Dong Park ◽  
Seungyong Han

We propose a design of angle-insensitive and polarization-independent reflective color filters with high efficiency (>80%) based on broad resonance in a Fabry–Pérot cavity where asymmetric metal-dielectric-metal planar structures are employed. Broadband absorption properties allow the resonance in the visible range to remain nearly constant over a broad range of incident angles of up to 40° for both s- and p-polarizations. Effects of the angles of incidence and polarization state of incident light on the purity of the resulting colors are examined on the CIE 1931 chromaticity diagram. In addition, higher-order resonances of the proposed color filters and their electric field distributions are investigated for improved color purity. Lastly, the spectral properties of the proposed structures with different metallic layers are studied. The simple strategy described in this work could be adopted in a variety of research areas, such as color decoration devices, microscopy, and colorimetric sensors.


Nanophotonics ◽  
2017 ◽  
Vol 6 (1) ◽  
pp. 289-297 ◽  
Author(s):  
Claudia Gritti ◽  
Søren Raza ◽  
Shima Kadkhodazadeh ◽  
Beata Kardynal ◽  
Radu Malureanu ◽  
...  

AbstractDecorating semiconductor surfaces with plasmonic nanoparticles (NPs) is considered a viable solution for enhancing the absorptive properties of photovoltaic and photodetecting devices. We propose to deposit silver NPs on top of a semiconductor wafer by a cheap and fast electroless plating technique. Optical characterization confirms that the random array of electroless-deposited NPs improves absorption by up to 20% in a broadband of near-infrared frequencies from the bandgap edge to 2000 nm. Due to the small filling fraction of particles, the reflection in the visible range is practically unchanged, which points to the possible applications of such deposition method for harvesting photons in nanophotonics and photovoltaics. The broadband absorption is a consequence of the resonant behavior of particles with different shapes and sizes, which strongly localize the incident light at the interface of a high-index semiconductor substrate. Our hypothesis is substantiated by examining the plasmonic response of the electroless-deposited NPs using both electron energy loss spectroscopy and numerical calculations.


Materials ◽  
2021 ◽  
Vol 14 (6) ◽  
pp. 1380
Author(s):  
Marwa M. Tharwat ◽  
Ashwag Almalki ◽  
Amr M. Mahros

In this paper, a randomly distributed plasmonic aluminum nanoparticle array is introduced on the top surface of conventional GaAs thin-film solar cells to improve sunlight harvesting. The performance of such photovoltaic structures is determined through monitoring the modification of its absorbance due to changing its structural parameters. A single Al nanoparticle array is integrated over the antireflective layer to boost the absorption spectra in both visible and near-infra-red regimes. Furthermore, the planar density of the plasmonic layer is presented as a crucial parameter in studying and investigating the performance of the solar cells. Then, we have introduced a double Al nanoparticle array as an imperfection from the regular uniform single array as it has different size particles and various spatial distributions. The comparison of performances was established using the enhancement percentage in the absorption. The findings illustrate that the structural parameters of the reported solar cell, especially the planar density of the plasmonic layer, have significant impacts on tuning solar energy harvesting. Additionally, increasing the plasmonic planar density enhances the absorption in the visible region. On the other hand, the absorption in the near-infrared regime becomes worse, and vice versa.


2020 ◽  
Vol 41 (2) ◽  
pp. 164-173
Author(s):  
Yunlong Guo ◽  
Shuzhen Ren

Abstract A poly(methyl methacrylate) (PMMA) bilayer antireflective coating (ARC) is designed based on polymeric microphase separation and matrix-assisted pulsed laser evaporation (MAPLE). The spin-coated layer shows subwavelength porous network structures, after phase separation via annealing and removal of the polystyrene (PS) phase, while the MAPLE deposited surface layer exhibits a biomimic moth-eye structure on glass to trap the incident light. The elaborate spin coated structure can be controlled flexibly by changing the ratio of mixture, annealing time and temperature, and the moth-eye structure can also be tuned by deposition parameters. The transmittance of the ARC presents a maximum of 95.64% and an average of 94.81% in visible range. The moth-eye structure on glass substrate formed by nanoglobules makes positive contributions to the improvement of transmittance according to UV–Vis result and simulation. The wetting motion of PMMA globules is observed as well by the comparison of AFM surface morphologies and cross-sectional profiles of globules on glass and polymer thin film. This work is a novel attempt to fabricate bilayer ARC with two different structures by a single polymeric material and will provide new route for fabrication of multilayer ARCs.


When the oscillating electric spark is examined in a rapidly rotating mirror, the successive oscillations render themselves evident in the image as a series of lumnious curved streamers which emanate from the poles and extend towards the centre of the spark gap. These streamers were first observed by Feddersen in 1862, but the work of Schuster and Hemsalech in 1900 may be said to have opened up a new era in the subject. These workers threw the image of the spark on the slit of a spectroscope, and photographed the resulting spectrum on a film which was maintained in rapid rotation in a direction at right angles to that of the incident light. In their photographs they found that the air lines extended straight across from pole to pole, but that the metal lines were represented by curved bands drawn out in the centre of the spark gap. There is a close relation between these bands and the streamers seen in the unanalysed inductive spark. Schuster and Hemsalech carried out their experiments with the smallest possible inductance in series with the spark, and thus made the period of the oscillations so small that the drawing out on the film was insufficient to separate the individual oscillations from each other. Thus their curved lines represent a composite structure, consisting of all the streamers due to the successive oscillations superposed on each other. It follows from their results that the light of the streamers in the spark is entirely produced by the glowing of the metallic vapour of the electrodes, and that, while the luminosity of the air is practically instantaneous in its occurrence, that due to the metal vapour occurs in the centre of the spark gap an appreciable time later than near the poles. The actual process which goes on in the spark and gives rise to this delay in the arrival of the metallic vapour at the centre of the gap is not yet thoroughly understood. Schuster and Hemsalech make the natural supposition that it is due to the fact that the metal of the electrode is vaporised and rendered incandescent by the heat of the spark, and that the vapour takes an appreciable time to diffuse from the electrodes to the centre of the gap. The exception which has been taken to this view has arisen in part from the difficulty of observing the Doppler effect on the metallic lines which should be a concomitant of the diffusion of the vapour from the poles, and in part from the extraordinary results which the authors themselves obtained in some metals for the velocity of the diffusion corresponding to the different lines. In the case of bismuth and, in a less degree, of cadmium the different metallic lines could be divided into groups of different curvatures which indicated different velocities of diffusion towards the centre of the gap. As regards the former matter, there does not seem to be involved any real difficulty to the explanation, as Dr. Schuster has himself recently shown. The curious effect of the different curvatures of the lines of the same element has, however, always remained more or less of a difficulty in the way of a complete acceptance of their view. Schuster and Hemsalech themselves refer to the possibility in the case of bismuth that the metal may be a compound, and that the two kinds of molecules give rise to the differently curved lines. Other explanations have been made by different writers, but it cannot be said that any explanation adequately supported by experiment has been forthcoming. In view of this incompleteness in our knowledge of the constitution of the streamers it seemed to me that further observations with a rotating mirror would possibly be of value, and the investigations recorded below succeed, I think, in throwing a clearer light on the nature of the streamers, and on certain other phenomena which are characteristic of the spark.


2021 ◽  
pp. 1-73
Author(s):  
Pierre Karam ◽  
Shankar Mitra ◽  
Kurt Marfurt ◽  
Brett M. Carpenter

Synthetic transfer zones develop between fault segments which dip in the same direction, with relay ramps connecting the fault blocks separated by the different fault segments. The characteristics of the transfer zones are controlled by the lithology, deformation conditions, and strain magnitude. The Parihaka fault is a NE-SW trending set of three major en-echelon faults connected by relay ramps in the Taranaki Basin, New Zealand. The structure in the basin is defined by extension during two episodes of deformation between the late Cretaceous and Paleocene and between the Late Miocene and recent. To better understand the evolution of a synthetic transfer zone, we study the geometry and secondary faulting between the individual fault segments in the Parihaka fault system using structural interpretation of 3D seismic data and seismic attributes. This interpretation allows for a unique application of seismic attributes to better study transfer zones. Seismic attributes, including coherence, dip, and curvature are effective tools to understand the detailed geometry and variation in displacement on the individual faults, the nature of secondary faulting along the transfer zones, and the relationship between the faults and drape folds. Seismic characterization of the fault system of Miocene to Pliocene age horizons highlights variations in the degree of faulting, deformation, and growth mechanism associated with different stages of transfer zone development. Coherence, dip, and curvature attributes show a direct correlation with structural parameters such as deformation, folding, and breaching of relay ramps.. All three attributes enhance the visualization of the major and associated secondary faults and better constrain their tectonic history. The observed correlation between seismic attributes and structural characteristics of transfer zones can significantly improve structural interpretation and exploration workflow.


Author(s):  
Berta Carrión-Ruiz ◽  
Silvia Blanco-Pons ◽  
Jose Luis Lerma

Non-destructive rock art recording techniques are getting special attention in the last years, opening new research lines in order to improve the level of documentation and understanding of our rich legacy. This paper applies the principal component analysis (PCA) technique in images that include wavelengths between 400-700 nm (visible  range). Our approach is focused on determining the difference provided by the image processing of the visible region through four spectral images versus an image that encompasses the entire visible spectrum. The images were taken by means of optical filters that take specific wavelengths and exclude parts of the spectrum. Simulation of rock art is prepared in laboratory. For this purpose, three different pigments were made simulating the material composition of rock art paintings. The advantages of studying the visible spectrum in separate images are analysed. In addition, PCA is applied to each of the images to reduce redundant data. Finally, PCA is applied to the image that contains the entire visible spectrum and is compared with previous results. Through the results of the four visible spectral images one can begin to draw conclusions about constituent painting materials without using decorrelation techniques.


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