scholarly journals Particulate Matter in an Urban–Industrial Environment: Comparing Data of Dispersion Modeling with Tree Leaves Deposition

2022 ◽  
Vol 14 (2) ◽  
pp. 793
Author(s):  
Gregorio Sgrigna ◽  
Hélder Relvas ◽  
Ana Isabel Miranda ◽  
Carlo Calfapietra

Particulate matter represents a serious hazard to human health, and air quality models contribute to the understanding of its dispersion. This study describes particulate matter with a ≤10 μm diameter (PM10) dynamics in an urban–industrial area, through the comparison of three datasets: modeled (TAPM—The Air Pollution Model), measured concentration (environmental control stations—ECS), and leaf deposition values. Results showed a good agreement between ECS and TAPM data. A steel plant area was used as a PM10 emissions reference source, in relation to the four sampling areas, and a distance/wind-based factor was introduced (Steel Factor, SF). Through SF, the three datasets were compared. The SF was able to describe the PM10 dispersion values for ECS and leaf deposition (r2 = 0.61–0.94 for ECS; r2 = 0.45–0.70 for leaf); no relationship was found for TAPM results. Differences between measured and modeled data can be due to discrepancies in one district and explained by a lack of PM10 inventory for the steel plant emissions. The study suggests the use of TAPM as a suitable tool for PM10 modeling at the urban scale. Moreover, tree leaves are a low-cost tool to evaluate the urban environmental quality, by providing information on whether and when data from leaf deposition can be used as a proxy for air pollution concentration. Further studies to include the re-suspension of particles as a PM10 source within emission inventories are suggested.

Author(s):  
Eric S. Coker ◽  
Ssematimba Joel ◽  
Engineer Bainomugisha

Background: There are major air pollution monitoring gaps in sub-Saharan Africa. Developing capacity in the region to conduct air monitoring in the region can help estimate exposure to air pollution for epidemiology research. The purpose of our study is to develop a land use regression (LUR) model using low-cost air quality sensors developed by a research group in Uganda (AirQo). Methods: Using these low-cost sensors, we collected continuous measurements of fine particulate matter (PM2.5) between May 1, 2019 and February 29, 2020 at 22 monitoring sites across urban municipalities of Uganda. We compared average monthly PM2.5 concentrations from the AirQo sensors with measurements from a BAM-1020 reference monitor operated at the US Embassy in Kampala. Monthly PM2.5 concentrations were used for LUR modeling. We used eight Machine Learning (ML) algorithms and ensemble modeling; using 10-fold cross validation and root mean squared error (RMSE) to evaluate model performance. Results: Monthly PM2.5 concentration was 60.2 µg/m3 (IQR: 45.4-73.0 µg/m3; median= 57.5 µg/m3). For the ML LUR models, RMSE values ranged between 5.43 µg/m3 - 15.43 µg/m3 and explained between 28% and 92% of monthly PM2.5 variability. Generalized additive models explained the largest amount of PM2.5 variability (R2=0.92) and produced the lowest RMSE (5.43 µg/m3) in the held-out test set. The most important predictors of monthly PM2.5 concentrations included monthly precipitation, major roadway density, population density, latitude, greenness, and percentage of households using solid fuels. Conclusion: To our knowledge, ours is the first study to model the spatial distribution of urban air pollution in sub-Saharan Africa using air monitors developed from the region itself. Non-parametric ML for LUR modeling performed with high accuracy for prediction of monthly PM2.5 levels. Our analysis suggests that locally produced low-cost air quality sensors can help build capacity to conduct air pollution epidemiology research in the region.


2013 ◽  
Vol 15 (2) ◽  
pp. 241-253 ◽  

The complex terrain basin of Amyntaio – Ptolemais – Kozani in Western Macedonia of Greece is an area characterized by increased industrial activity and therefore it demands continuous and assiduous environmental monitoring. A prolonged particulate matter air pollution episode was recorded in the area during November 2009. Basic meteorological aspects are analyzed, during the episode period. Daily and hourly PM10 and PM2.5 concentration measurements were used along with surface and lower atmosphere hourly meteorological parameters from 13 measuring stations. The observational data were supported by data produced by the meteorological component of an air pollution model. The overall analysis showed that the episode was primarily the result of the synoptic setting of the middle and lower troposphere. An Omega blocking pattern which gradually transformed to a high-over-low pattern prevailed over central and southern Europe during the episode’s period. The examination of the vertical wind field in the lower troposphere and appropriate stability indices, revealed a continuous absence of significant convection. The weak horizontal wind field near the surface and the reduced mixing height combined with the lack of synoptic forcing resulted in the trapping of the pollutants in the lower troposphere and the recording of increased airborne particulate matter concentrations. The radical change of the synoptic setting in the first days of December marked the end of the episode.


Atmosphere ◽  
2019 ◽  
Vol 10 (7) ◽  
pp. 400 ◽  
Author(s):  
Evan R. Coffey ◽  
David Pfotenhauer ◽  
Anondo Mukherjee ◽  
Desmond Agao ◽  
Ali Moro ◽  
...  

Household air pollution from the combustion of solid fuels is a leading global health and human rights concern, affecting billions every day. Instrumentation to assess potential solutions to this problem faces challenges—especially related to cost. A low-cost ($159) particulate matter tool called the Household Air Pollution Exposure (HAPEx) Nano was evaluated in the field as part of the Prices, Peers, and Perceptions cookstove study in northern Ghana. Measurements of temperature, relative humidity, absolute humidity, and carbon dioxide and carbon monoxide concentrations made at 1-min temporal resolution were integrated with 1-min particulate matter less than 2.5 microns in diameter (PM2.5) measurements from the HAPEx, within 62 kitchens, across urban and rural households and four seasons totaling 71 48-h deployments. Gravimetric filter sampling was undertaken to ground-truth and evaluate the low-cost measurements. HAPEx baseline drift and relative humidity corrections were investigated and evaluated using signals from paired HAPEx, finding significant improvements. Resulting particle coefficients and integrated gravimetric PM2.5 concentrations were modeled to explore drivers of variability; urban/rural, season, kitchen characteristics, and dust (a major PM2.5 mass constituent) were significant predictors. The high correlation (R2 = 0.79) between 48-h mean HAPEx readings and gravimetric PM2.5 mass (including other covariates) indicates that the HAPEx can be a useful tool in household energy studies.


2021 ◽  
Vol 2021 ◽  
pp. 1-11
Author(s):  
Caroline Kiai ◽  
Christopher Kanali ◽  
Joseph Sang ◽  
Michael Gatari

Air pollution is one of the most important environmental and public health concerns worldwide. Urban air pollution has been increasing since the industrial revolution due to rapid industrialization, mushrooming of cities, and greater dependence on fossil fuels in urban centers. Particulate matter (PM) is considered to be one of the main aerosol pollutants that causes a significant adverse impact on human health. Low-cost air quality sensors have attracted attention recently to curb the lack of air quality data which is essential in assessing the health impacts of air pollutants and evaluating land use policies. This is mainly due to their lower cost in comparison to the conventional methods. The aim of this study was to assess the spatial extent and distribution of ambient airborne particulate matter with an aerodynamic diameter less than 2.5 μm (PM2.5) in Nairobi City County. Seven sites were selected for monitoring based on the land use type: high- and low-density residential, industrial, agricultural, commercial, road transport, and forest reserve areas. Calibrated low-cost sensors and cyclone samplers were used to monitor PM2.5 concentration levels and gravimetric measurements for elemental composition of PM2.5, respectively. The sensor percentage accuracy for calibration ranged from 81.47% to 98.60%. The highest 24-hour average concentration of PM2.5 was observed in Viwandani, an industrial area (111.87 μg/m³), and the lowest concentration at Karura (21.25 μg/m³), a forested area. The results showed a daily variation in PM2.5 concentration levels with the peaks occurring in the morning and the evening due to variation in anthropogenic activities and the depth of the atmospheric boundary layer. Therefore, the study suggests that residents in different selected land use sites are exposed to varying levels of PM2.5 pollution on a regular basis, hence increasing the potential of causing long-term health effects.


2021 ◽  
Vol 14 (9) ◽  
pp. 6023-6038 ◽  
Author(s):  
Eric A. Wendt ◽  
Casey Quinn ◽  
Christian L'Orange ◽  
Daniel D. Miller-Lionberg ◽  
Bonne Ford ◽  
...  

Abstract. Atmospheric particulate matter smaller than 2.5 µm in diameter (PM2.5) has a negative impact on public health, the environment, and Earth's climate. Consequently, a need exists for accurate, distributed measurements of surface-level PM2.5 concentrations at a global scale. Existing PM2.5 measurement infrastructure provides broad PM2.5 sampling coverage but does not adequately characterize community-level air pollution at high temporal resolution. This motivates the development of low-cost sensors which can be more practically deployed in spatial and temporal configurations currently lacking proper characterization. Wendt et al. (2019) described the development and validation of a first-generation device for low-cost measurement of AOD and PM2.5: the Aerosol Mass and Optical Depth (AMODv1) sampler. Ford et al. (2019) describe a citizen-science field deployment of the AMODv1 device. In this paper, we present an updated version of the AMOD, known as AMODv2, featuring design improvements and extended validation to address the limitations of the AMODv1 work. The AMODv2 measures AOD and PM2.5 at 20 min time intervals. The sampler includes a motorized Sun tracking system alongside a set of four optically filtered photodiodes for semicontinuous, multiwavelength (current version at 440, 500, 675, and 870 nm) AOD sampling. Also included are a Plantower PMS5003 sensor for time-resolved optical PM2.5 measurements and a pump/cyclone system for time-integrated gravimetric filter measurements of particle mass and composition. AMODv2 samples are configured using a smartphone application, and sample data are made available via data streaming to a companion website (https://csu-ceams.com/, last access: 16 July 2021). We present the results of a 9 d AOD validation campaign where AMODv2 units were co-located with an AERONET (Aerosol Robotics Network) instrument as the reference method at AOD levels ranging from 0.02 ± 0.01 to 1.59 ± 0.01. We observed close agreement between AMODv2s and the reference instrument with mean absolute errors of 0.04, 0.06, 0.03, and 0.03 AOD units at 440, 500, 675, and 870 nm, respectively. We derived empirical relationships relating the reference AOD level to AMODv2 instrument error and found that the mean absolute error in the AMODv2 deviated by less than 0.01 AOD units between clear days and elevated-AOD days and across all wavelengths. We identified bias from individual units, particularly due to calibration drift, as the primary source of error between AMODv2s and reference units. In a test of 15-month calibration stability performed on 16 AMOD units, we observed median changes to calibration constant values of −7.14 %, −9.64 %, −0.75 %, and −2.80 % at 440, 500, 675, and 870 nm, respectively. We propose annual recalibration to mitigate potential errors from calibration drift. We conducted a trial deployment to assess the reliability and mechanical robustness of AMODv2 units. We found that 75 % of attempted samples were successfully completed in rooftop laboratory testing. We identify several failure modes in the laboratory testing and describe design changes that we have since implemented to reduce failures. We demonstrate that the AMODv2 is an accurate, stable, and low-cost platform for air pollution measurement. We describe how the AMODv2 can be implemented in spatial citizen-science networks where reference-grade sensors are economically impractical and low-cost sensors lack accuracy and stability.


Author(s):  
Mohammad Hashem Askariyeh ◽  
Madhusudhan Venugopal ◽  
Haneen Khreis ◽  
Andrew Birt ◽  
Josias Zietsman

Recent studies suggest that the transportation sector is a major contributor to fine particulate matter (PM2.5) in urban areas. A growing body of literature indicates PM2.5 exposure can lead to adverse health effects, and that PM2.5 concentrations are often elevated close to roadways. The transportation sector produces PM2.5 emissions from combustion, brake wear, tire wear, and resuspended dust. Traffic-related resuspended dust is particulate matter, previously deposited on the surface of roadways that becomes resuspended into the air by the movement of traffic. The objective of this study was to use regulatory guidelines to model the contribution of resuspended dust to near-road traffic-related PM2.5 concentrations. The U.S. Environmental Protection Agency (EPA) guidelines for quantitative hotspot analysis were used to predict traffic-related PM2.5 concentrations for a small network in Dallas, Texas. Results show that the inclusion of resuspended dust in the emission and dispersion modeling chain increases prediction of near-road PM2.5 concentrations by up to 74%. The results also suggest elevated PM2.5 concentrations near arterial roads. Our results are discussed in the context of human exposure to traffic-related air pollution.


2018 ◽  
Author(s):  
Francis D. Pope ◽  
Michael Gatari ◽  
David Ng’ang’a ◽  
Alexander Poynter ◽  
Rhiannon Blake

Abstract. East African countries face an increasing threat from poor air quality, stemming from rapid urbanisation, population growth and a steep rise in fuel use and motorization rates. With few air quality monitoring systems available, this study provides the much needed high temporal resolution data to investigate the concentrations of particulate matter (PM) air pollution in Kenya. Calibrated low cost optical particle counters (OPCs) were deployed in Kenya in three locations: two in the capital of Nairobi and one in a rural location in the outskirts of Nanyuki, which is upwind of Nairobi. The two Nairobi sites consist of an urban background site and a roadside site. The instruments were composed of an Alphasense OPC-N2 optical particle counter (OPC) ran with a raspberry pi low cost microcomputer, packaged in a weather proof box. Measurements were conducted over a two-month period (February–March 2017) with an intensive study period when all measurements were active at all sites lasting two weeks. When collocated, the three OPC-N2 instruments demonstrated good inter-instrument precision with a coefficient of variance of 8.8 ± 2.0 % in the PM2.5 fraction. The low cost sensors had an absolute PM mass concentration calibration using a collocated gravimetric measurement at the urban background site in Nairobi. The mean daily PM1 mass concentration measured at the urban roadside, urban background and rural background sites were 23.9, 16.1, 8.8 µg m−3. The mean daily PM2.5 mass concentration measured at the urban roadside, urban background and rural background sites were 36.6, 24.8, 13.0 µg m−3. The mean daily PM10 mass concentration measured at the urban roadside, urban background and rural background sites were 93.7, 53.0, 19.5 µg m−3. The urban measurements in Nairobi showed that particulate matter concentrations regularly exceed WHO guidelines in both the PM10 and PM2.5 size ranges. Following a Lenschow type approach we can estimate the urban and roadside increments that are applicable to Nairobi. Median urban and roadside increments are 33.1 and 43.3 µg m−3 for PM10, respectively, the median urban and roadside increments are 7.1 and 18.3 µg m−3 for PM2.5, respectively, and the median urban and roadside increments are 4.7 and 12.6 µg m−3 for PM1, respectively. These increments highlight the importance of both the urban and roadside increments to urban air pollution in Nairobi. A clear diurnal behaviour in PM mass concentration was observed at both urban sites, which peaks during the morning and evening Nairobi rush hours; this was consistent with the high measured roadside increment indicating vehicular traffic being a dominant source of particulate matter in the city, accounting for approximately 48.1, 47.5, and 57.2 % of the total particulate matter loading in the PM10, PM2.5 and PM1 size ranges, respectively. Collocated meteorological measurements at the urban sites were collected, allowing for an understanding of the location of major sources of particulate matter at the two sites. The potential problems of using low cost sensors for PM measurement without gravimetric calibration available at all sites are discussed. This study shows that calibrated low cost sensors can be used successfully to measure air pollution in cities like Nairobi. It demonstrates that low cost sensors could be used to create an affordable and reliable network to monitor air quality in cities.


2020 ◽  
Author(s):  
Eduard Petrovsky ◽  
Ales Kapicka ◽  
Hana Grison ◽  
Bohumil Kotlik ◽  
Hana Miturova

Abstract Background: Environmental magnetism, focusing on ferrimagnetic iron oxides, provides useful additional information on pollution of different environments. Magnetic methods have been applied to studies of atmospheric dust, namely PM10 (particulate matter smaller than 10 micrometers) in, e.g., industrial or urban areas. Until now, positive correlation was reported between concentration of iron oxides (expressed in terms of either magnetic susceptibility, saturation remanent or saturation induced magnetization) and concentration of PM10 or smaller. Purpose of this study was to verify the relationship between iron oxides and PM at monitoring site close to source of emissions rich in iron oxides during period of smoggy conditions. Results: We examined 24-hours PM10 and PM1 samples, collected during 10 days of smoggy winter period at a site close to steel plant, which represents a significant source of atmospheric emissions in industrial region of Northern Moravia (Czech Republic), known for generally high degree of air pollution. Magnetic hysteresis loops were measured in order to obtain parameters reflecting the concentration and grain-size distribution of iron oxides. Our data show unexpected negative correlation between saturation magnetization (concentration of ferrimagnetic iron oxides) and both PM1 and PM10 concentrations, to the best of our knowledge the trend not being reported yet.Conclusions: Our finding may seemingly disqualify magnetic methods as useful proxy in air pollution studies. However, we suggest that this is an exceptional case, specific to this region and monitoring site, as well as to synoptic conditions during the smoggy period. Although the significant dust emissions are presumably rich in iron oxides, the overall air quality at the monitoring site is determined by the general environment, controlled by many other sources of different character in the region, and by the specific climatic conditions. Thus, the nearby steel plant, presumably emitting dust rich in ferrimagnetic iron oxides, dominates the deposited dust at the nearby monitoring site only during very few days of suitable weather (namely wind speed and direction).


Sensors ◽  
2021 ◽  
Vol 21 (18) ◽  
pp. 6162
Author(s):  
Hyuntae Cho ◽  
Yunju Baek

Air pollution is a social problem, because the harmful suspended materials can cause diseases and deaths to humans. Specifically, particulate matters (PM), a form of air pollution, can contribute to cardiovascular morbidity and lung diseases. Nowadays, humans are exposed to PM pollution everywhere because it occurs in both indoor and outdoor environments. To purify or ventilate polluted air, one need to accurately monitor the ambient air quality. Therefore, this study proposed a practical particulate matter sensing and accurate calibration system using low-cost commercial sensors. The proposed system basically uses noisy and inaccurate PM sensors to measure the ambient air pollution. This paper mainly deals with three types of error caused in the light scattering method: short-term noise, part-to-part variation, and temperature and humidity interferences. We propose a simple short-term noise reduction method to correct measurement errors, an auto-fitting calibration for part-to-part repeatability to pinpoint the baseline of the signal that affects the performance of the system, and a temperature and humidity compensation method. This paper also contains the experiment setup and performance evaluation to prove the superiority of the proposed methods. Based on the evaluation of the performance of the proposed system, part-to-part repeatability was less than 2 μg/m3 and the standard deviation was approximately 1.1 μg/m3 in the air. When the proposed approaches are used for other optical sensors, it can result in better performance.


2021 ◽  
Author(s):  
Chao-Heng Tseng ◽  
Ling Ling Chen ◽  
Guan-Hua Tseng

Abstract Low-cost air-pollution sensors are attracting increasing attention. They offer air-pollution monitoring at a cost lower than that of conventional methods, theoretically facilitating air-pollution monitoring in several locations and immediate application of acquired information. We establish a particulate matter (PM2.5) map based on low-cost air-pollution sensor information developed using internet of things at Taiwan’s Environmental Protection Agency. We synergize data from one monitoring station with 287 low-cost air-pollution-pollution sensors (data entries = ∼50 million) to estimate PM2.5 concentrations from September 1, 2018 to August 31, 2019. We investigate Chiayi City because it has the second-highest PM2.5 concentration in Taiwan. By analyzing Geographic Information System data, we map Chiayi City’s spatial and temporal distributions, identify PM2.5, and recognize the characteristics of Chiayi City’s hotspots. Our main discoveries are as follows: Chiayi City’s spatial distribution reveals PM2.5 concentrated in its industrial area, which increasingly reduces from the industrial area to the city center. Hot spots are identified by two types of space units: northwest industrial and central and western agricultural zone. Concentrated PM2.5 occurs mainly in winter, with the highest rate in January, occurring most frequently and less frequently from 7 to 10 a.m. and 3 to 5 p.m., respectively. Although this study focuses on Chiayi City, the proposed approach has general applicability to wide-ranging environment-monitoring studies and air-pollution interventions and will substantially assist in validating PM2.5 transport models and enhance exposure estimation accuracy in further research.


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