scholarly journals Estimates of biomass burning emissions in tropical Asia based on satellite-derived data

2010 ◽  
Vol 10 (5) ◽  
pp. 2335-2351 ◽  
Author(s):  
D. Chang ◽  
Y. Song
Keyword(s):  
Biomass Burning ◽  
Atmospheric Chemistry ◽  
Crop Residue ◽  
Fire Season ◽  
Burned Area ◽  
Published Data ◽  
Tropical Asia ◽  
Fire Emissions ◽  
Burned Areas ◽  
In Fire

Abstract. Biomass burning in tropical Asia emits large amounts of trace gases and particulate matter into the atmosphere, which has significant implications for atmospheric chemistry and climatic change. In this study, emissions from open biomass burning over tropical Asia were evaluated during seven fire years from 2000 to 2006 (1 March 2000–31 February 2007). The size of the burned areas was estimated from newly published 1-km L3JRC and 500-m MODIS burned area products (MCD45A1). Available fuel loads and emission factors were assigned to each vegetation type in a GlobCover characterisation map, and fuel moisture content was taken into account when calculating combustion factors. Over the whole period, both burned areas and fire emissions showed clear spatial and seasonal variations. The size of the L3JRC burned areas ranged from 36 031 km2 in fire year 2005 to 52 303 km2 in 2001, and the MCD45A1 burned areas ranged from 54 790 km2 in fire year 2001 to 148 967 km2 in 2004. Comparisons of L3JRC and MCD45A1 burned areas using ground-based measurements and other satellite data were made in several major burning regions, and the results suggest that MCD45A1 generally performed better than L3JRC, although with a certain degree of underestimation in forest areas. The average annual L3JRC-based emissions were 123 (102–152), 12 (9–15), 1.0 (0.7–1.3), 1.9 (1.4–2.6), 0.11 (0.09–0.12), 0.89 (0.63–1.21), 0.043 (0.036–0.053), 0.021 (0.021–0.023), 0.41 (0.34–0.52), 3.4 (2.6–4.3), and 3.6 (2.8–4.7) Tg yr−1 for CO2, CO, CH4, NMHCs, NOx, NH3, SO2, BC, OC, PM2.5, and PM10, respectively, whereas MCD45A1-based emissions were 122 (108–144), 9.3 (7.7–11.7), 0.63 (0.46–0.86), 1.1 (0.8–1.6), 0.11 (0.10–0.13), 0.54 (0.38–0.76), 0.043 (0.038–0.051), 0.033 (0.032–0.037), 0.39 (0.34–0.47), 3.0 (2.6–3.7), and 3.3 (2.8–4.0) Tg yr−1. Forest burning was identified as the major source of the fire emissions due to its high carbon density. Although agricultural burning was the second highest contributor, it is possible that some crop residue combustion was missed by satellite observations. This possibility is supported by comparisons with previously published data, and this result may be due to the small size of the field crop residue burning. Fire emissions were mainly concentrated in Indonesia, India, Myanmar, and Cambodia. Furthermore, the peak in the size of the burned area was generally found in the early fire season, whereas the maximum fire emissions often occurred in the late fire season.

scholarly journals Estimates of biomass burning emissions in tropical Asia based on satellite-derived data

2009 ◽  
Vol 9 (5) ◽  
pp. 19599-19640 ◽  
Author(s):  
D. Chang ◽  
Y. Song
Keyword(s):  
Biomass Burning ◽  
Atmospheric Chemistry ◽  
Vegetation Type ◽  
Burned Area ◽  
Tropical Asia ◽  
Fire Emissions ◽  
Burned Areas ◽  
Fuel Moisture Content ◽  
In Fire ◽  
Derived Data

Abstract. Biomass burning in tropical Asia emits large amounts of trace gases and particulate matters into the atmosphere, which has significant implications for atmospheric chemistry and climatic change. In this study, emissions from open biomass burning over tropical Asia were evaluated during seven fire years from 2000–2006 (1 April 2000–31 March 2007). Burned areas were estimated from newly published 1-km L3JRC and 500-m MODIS burned area products (MCD45A1). Available fuel loads and emission factors were assigned for each vegetation type in a GlobCover characterisation map, and fuel moisture content was taken into account when calculating combustion factors. Over the whole period, both burned areas and fire emissions clearly showed spatial and seasonal variations. The L3JRC burned areas ranged from 31 165 km2 in fire year 2005 to 57 313 km2 in 2000, while the MCD45A1 burned areas ranged from 54 260 km2 in fire year 2001 to 127 068 km2 in 2004. Comparisons of L3JRC and MCD45A1 burned areas with ground-based measurements and other satellite information were constructed in several major burning regions, and results suggested that MCD45A1 performed better in most areas than L3JRC did although with a certain degree of underestimation of burned forest areas. The average annual L3JRC-based emissions were 125, 12, 0.98, 1.91, 0.11, 0.89, 0.044, 0.022, 0.42, 3.40, and 3.68 Tg yr

Changes in the timing and length of the fire season in Spain

2020 ◽  
Author(s):  
Itziar R. Urbieta ◽  
Gonzalo Arellano ◽  
José M. Moreno
Keyword(s):  
Fire Suppression ◽  
Generalized Additive Models ◽  
Summer Season ◽  
Additive Models ◽  
Fire Season ◽  
Burned Area ◽  
Burned Areas ◽  
Spatial Differences ◽  
Mediterranean Regions ◽  
In Fire

<p>Fire activity has decreased in the last decades in Spain, as a whole and in most regions. However, little is known about the changes in the fire season peak, timing, and length. Here we studied the temporal variation in the fire season since the 1970’s for different Spanish regions. We analyzed weekly time series of annually burned area by fitting GAMs (Generalized Additive Models) models in R. Area burned was log transformed and smoothing P-splines were fit to study weekly seasonality. GAMS allowed us to model spring, summer, and autumn fire seasons. Changes in the sign of the smoothing parameter determined the timing (onset/end dates) of each fire season, while the maximum value of the parameter established the peak of the fire season. We applied trend analysis to study inter-annual variation in fire season timing, length, and amplitude. We found temporal and spatial differences in the fire season across regions. In the northern Atlantic regions, models performed better, and captured a bimodal fire season (spring-summer). Nonetheless, the bimodal fire-season structure is no longer distinguishable in recent years, since both are increasing in duration. In the Mediterranean regions, larger peaks of burned areas occur in shorter time spans. The amplitude and duration of the summer season is decreasing, probably due to the increase in fire suppression during the summer. The summer season is starting earlier, while, in general, no trend was found for the end of the season. Furthermore, spring fire peaks in Mediterranean regions are becoming more frequent, suggesting that more attention should be paid to these out-of-season conditions.</p>

Improved estimates of future fire emissions under CMIP6 scenarios and implications for aerosol radiative forcing

2021 ◽  
Author(s):  
Matthew Kasoar ◽  
Douglas Hamilton ◽  
Daniela Dalmonech ◽  
Stijn Hantson ◽  
Gitta Lasslop ◽  
...  
Keyword(s):  
Machine Learning ◽  
Biomass Burning ◽  
Radiative Forcing ◽  
Learning Methods ◽  
Aerosol Radiative Forcing ◽  
Fire Emissions ◽  
Machine Learning Methods ◽  
The Tropics ◽  
In Fire ◽  
Aerosol Radiative

<p>The CMIP6 Shared Socioeconomic Pathway (SSP) scenarios include projections of future changes in anthropogenic biomass-burning.  Globally, they assume a decrease in total fire emissions over the next century under all scenarios.  However, fire regimes and emissions are expected to additionally change with future climate, and the methodology used to project fire emissions in the SSP scenarios is opaque.</p><p>We aim to provide a more traceable estimate of future fire emissions under CMIP6 scenarios and evaluate the impacts for aerosol radiative forcing.  We utilise interactive wildfire emissions from four independent land-surface models (CLM5, JSBACH3.2, LPJ-GUESS, and ISBA-CTRIP) used within CMIP6 ESMs, and two different machine-learning methods (a random forest, and a generalised additive model) trained on historical data, to predict year 2100 biomass-burning aerosol emissions consistent with the CMIP6-modelled climate for three different scenarios: SSP126, SSP370, and SSP585.  This multi-method approach provides future fire emissions integrating information from observations, projections of climate, socioeconomic parameters and changes in vegetation distribution and fuel loads.</p><p>Our analysis shows a robust increase in fire emissions for large areas of the extra-tropics until the end of this century for all methods.  Although this pattern was present to an extent in the original SSP projections, both the interactive fire models and machine-learning methods predict substantially higher increases in extra-tropical emissions in 2100 than the corresponding SSP datasets.  Within the tropics the signal is mixed. Increases in emissions are largely driven by the temperature changes, while in some tropical areas reductions in fire emissions are driven by human factors and changes in precipitation, with the largest reductions in Africa. The machine-learning methods show a stronger reduction in the tropics than the interactive fire models, however overall there is strong agreement between both the models and the machine-learning methods.</p><p>We then use additional nudged atmospheric simulations with two state-of-the-art composition-climate models, UKESM1 and CESM2, to diagnose the impact of these updated fire emissions on aerosol burden and radiative forcing, compared with the original SSP prescribed emissions.  We provide estimates of future fire radiative forcing, compared to modern-day, under these CMIP6 scenarios which span both the severity of climate change in 2100, and the rate of reduction of other aerosol species.</p>

scholarly journals Interannual variability of global biomass burning emissions from 1997 to 2004

2006 ◽  
Vol 6 (2) ◽  
pp. 3175-3226 ◽  
Author(s):  
G. R. van der Werf ◽  
J. T. Randerson ◽  
L. Giglio ◽  
G. J. Collatz ◽  
P. S. Kasibhatla ◽  
...  
Keyword(s):  
Interannual Variability ◽  
Biomass Burning ◽  
Satellite Data ◽  
Net Primary Production ◽  
Terrestrial Ecosystems ◽  
Total Carbon ◽  
Burned Area ◽  
Biogeochemical Model ◽  
Fuel Wood ◽  
Fire Emissions

Abstract. Biomass burning represents an important source of atmospheric aerosols and greenhouse gases, yet little is known about its interannual variability or the underlying mechanisms regulating this variability at continental to global scales. Here we investigated fire emissions during the 8 year period from 1997 to 2004 using satellite data and the CASA biogeochemical model. Burned area from 2001–2004 was derived using newly available active fire and 500 m burned area datasets from MODIS following the approach described by Giglio et al. (2005). ATSR and VIRS satellite data were used to extend the burned area time series back in time through 1997. In our analysis we estimated fuel loads, including peatland fuels, and the net flux from terrestrial ecosystems as the balance between net primary production (NPP), heterotrophic respiration (Rh), and biomass burning, using time varying inputs of precipitation (PPT), temperature, solar radiation, and satellite-derived fractional absorbed photosynthetically active radiation (fAPAR). For the 1997–2004 period, we found that on average approximately 58 Pg C year−1 was fixed by plants, and approximately 95% of this was returned back to the atmosphere via Rh. Another 4%, or 2.5 Pg C year−1 was emitted by biomass burning; the remainder consisted of losses from fuel wood collection and subsequent burning. At a global scale, burned area and total fire emissions were largely decoupled from year to year. Total carbon emissions tracked burning in forested areas (including deforestation fires in the tropics), whereas burned area was largely controlled by savanna fires that responded to different environmental and human factors. Biomass burning emissions showed large interannual variability with a range of more than 1 Pg C year−1, with a maximum in 1998 (3.2 Pg C year−1) and a minimum in 2000 (2.0 Pg C year−1).

scholarly journals Spatial and temporal variability in the ratio of trace gases emitted from biomass burning

2011 ◽  
Vol 11 (8) ◽  
pp. 3611-3629 ◽  
Author(s):  
T. T. van Leeuwen ◽  
G. R. van der Werf
Keyword(s):  
Temporal Variability ◽  
Field Measurement ◽  
Environmental Variables ◽  
Trace Gases ◽  
Measurement Techniques ◽  
Arithmetic Mean ◽  
Fire Season ◽  
Burned Area ◽  
Spatial And Temporal Variability ◽  
Fire Emissions

Abstract. Fires are a major source of trace gases and aerosols to the atmosphere. The amount of biomass burned is becoming better known, most importantly due to improved burned area datasets and a better representation of fuel consumption. The spatial and temporal variability in the partitioning of biomass burned into emitted trace gases and aerosols, however, has received relatively little attention. To convert estimates of biomass burned to trace gas and aerosol emissions, most studies have used emission ratios (or emission factors (EFs)) based on the arithmetic mean of field measurement outcomes, stratified by biome. However, EFs vary substantially in time and space, even within a single biome. In addition, it is unknown whether the available field measurement locations provide a representative sample for the various biomes. Here we used the available body of EF literature in combination with satellite-derived information on vegetation characteristics and climatic conditions to better understand the spatio-temporal variability in EFs. While focusing on CO, CH4, and CO2, our findings are also applicable to other trace gases and aerosols. We explored relations between EFs and different measurements of environmental variables that may correlate with part of the variability in EFs (tree cover density, vegetation greenness, temperature, precipitation, and the length of the dry season). Although reasonable correlations were found for specific case studies, correlations based on the full suite of available measurements were lower and explained about 33%, 38%, 19%, and 34% of the variability for respectively CO, CH4, CO2, and the Modified Combustion Efficiency (MCE). This may be partly due to uncertainties in the environmental variables, differences in measurement techniques for EFs, assumptions on the ratio between flaming and smoldering combustion, and incomplete information on the location and timing of EF measurements. We derived new mean EFs, using the relative importance of each measurement location with regard to fire emissions. These weighted averages were relatively similar to the arithmetic mean. When using relations between the environmental variables and EFs to extrapolate to regional and global scales, we found substantial differences, with for savannas 13% and 22% higher CO and CH4 EFs than the arithmetic mean of the field studies, possibly linked to an underrepresentation of woodland fires in EF measurement locations. We argue that from a global modeling perspective, future measurement campaigns could be more beneficial if measurements are made over the full fire season, and if relations between ambient conditions and EFs receive more attention.

scholarly journals Production of peroxy nitrates in boreal biomass burning plumes over Canada during the BORTAS campaign

2016 ◽  
Vol 16 (5) ◽  
pp. 3485-3497 ◽  
Author(s):  
Marcella Busilacchio ◽  
Piero Di Carlo ◽  
Eleonora Aruffo ◽  
Fabio Biancofiore ◽  
Cesare Dari Salisburgo ◽  
...  
Keyword(s):  
Boreal Forest ◽  
Forest Fire ◽  
Biomass Burning ◽  
Forest Fires ◽  
Chemical Mechanism ◽  
Fire Emissions ◽  
Fire Plumes ◽  
Peroxy Nitrates ◽  
In Fire ◽  
The Impact

Abstract. The observations collected during the BOReal forest fires on Tropospheric oxidants over the Atlantic using Aircraft and Satellites (BORTAS) campaign in summer 2011 over Canada are analysed to study the impact of forest fire emissions on the formation of ozone (O3) and total peroxy nitrates ∑PNs, ∑ROONO2). The suite of measurements on board the BAe-146 aircraft, deployed in this campaign, allows us to calculate the production of O3 and of  ∑PNs, a long-lived NOx reservoir whose concentration is supposed to be impacted by biomass burning emissions. In fire plumes, profiles of carbon monoxide (CO), which is a well-established tracer of pyrogenic emission, show concentration enhancements that are in strong correspondence with a significant increase of concentrations of ∑PNs, whereas minimal increase of the concentrations of O3 and NO2 is observed. The ∑PN and O3 productions have been calculated using the rate constants of the first- and second-order reactions of volatile organic compound (VOC) oxidation. The ∑PN and O3 productions have also been quantified by 0-D model simulation based on the Master Chemical Mechanism. Both methods show that in fire plumes the average production of ∑PNs and O3 are greater than in the background plumes, but the increase of ∑PN production is more pronounced than the O3 production. The average ∑PN production in fire plumes is from 7 to 12 times greater than in the background, whereas the average O3 production in fire plumes is from 2 to 5 times greater than in the background. These results suggest that, at least for boreal forest fires and for the measurements recorded during the BORTAS campaign, fire emissions impact both the oxidized NOy and O3,  but (1 ∑PN production is amplified significantly more than O3 production and (2) in the forest fire plumes the ratio between the O3 production and the ∑PN production is lower than the ratio evaluated in the background air masses, thus confirming that the role played by the ∑PNs produced during biomass burning is significant in the O3 budget. The implication of these observations is that fire emissions in some cases, for example boreal forest fires and in the conditions reported here, may influence more long-lived precursors of O3 than short-lived pollutants, which in turn can be transported and eventually diluted in a wide area.

scholarly journals Estimation of emissions from biomass burning in China (2003–2017) based on MODIS fire radiative energy data

2019 ◽  
Vol 16 (7) ◽  
pp. 1629-1640 ◽  
Author(s):  
Lifei Yin ◽  
Pin Du ◽  
Minsi Zhang ◽  
Mingxu Liu ◽  
Tingting Xu ◽  
...  
Keyword(s):  
Biomass Burning ◽  
Forest Fires ◽  
Crop Residue ◽  
Crop Yields ◽  
Southern China ◽  
Farming System ◽  
Radiative Energy ◽  
Fire Emissions ◽  
The North ◽  
Significant Downward Trend

Abstract. Biomass burning plays a significant role in air pollution and climate change. In this study, we used a method based on fire radiative energy (FRE) to develop a biomass burning emission inventory for China from 2003 to 2017. Daily fire radiative power (FRP) data derived from 1 km MODIS Thermal Anomalies/Fire products (MOD14/MYD14) were used to calculate FRE and combusted biomass. Available emission factors were assigned to four biomass burning types: forest, cropland, grassland, and shrubland fires. The farming system and crop types in different temperate zones were taken into account in this research. Compared with traditional methods, the FRE method was found to provide a more reasonable estimate of emissions from small fires. The estimated average annual emission ranges, with a 90 % confidence interval, were 91.4 (72.7–108.8) Tg CO2 yr−1, 5.0 (2.3–7.8)  Tg CO yr−1, 0.24 (0.05–0.48) Tg CH4 yr−1, 1.43 (0.53–2.35) Tg NMHC yr−1, 0.23 (0.05–0.45) Tg NOx yr−1, 0.09 (0.02–0.17) Tg NH3 yr−1, 0.03 (0.01–0.05) Tg SO2 yr−1, 0.04 (0.01–0.08) Tg BC yr−1, 0.27 (0.07–0.49) Tg OC yr−1, 0.51 (0.19–0.84) Tg PM2.5 yr−1, 0.57 (0.15–1.05) Tg PM10 yr−1, where NMHC, BC, and OC are nonmethane hydrocarbons, black carbon, and organic carbon, respectively. Forest fires are determined to be the primary contributor to open fire emissions, accounting for 45 % of the total CO2 emissions (average 40.8 Tg yr−1). Crop residue burning ranked second place with a large portion of 39 % (average 35.3 Tg yr−1). During the study period, emissions from forest and grassland fires showed a significant downward trend. Crop residue emissions continued to rise during 2003–2015 but dropped by 42 % in 2015–2016. Emissions from shrubland were negligible and little changed. Forest and grassland fires are concentrated in northeastern China and southern China, especially in the dry season (from October to March of the following year). Plain areas with high crop yields, such as the North China Plain, experienced high agricultural fire emissions in harvest seasons. Most shrubland fires were located in Yunnan and Guangdong provinces. The resolution of our inventory (daily, 1 km) is much higher than previous inventories, such as GFED4s and GFASv1.0. It could be used in global and regional air quality modeling.

scholarly journals Six global biomass burning emission datasets: intercomparison and application in one global aerosol model

2020 ◽  
Vol 20 (2) ◽  
pp. 969-994 ◽  
Author(s):  
Xiaohua Pan ◽  
Charles Ichoku ◽  
Mian Chin ◽  
Huisheng Bian ◽  
Anton Darmenov ◽  
...  
Keyword(s):  
Southern Hemisphere ◽  
Biomass Burning ◽  
Satellite Observations ◽  
Burned Area ◽  
Aerosol Model ◽  
Fire Emissions ◽  
Active Fire ◽  
Aerosol Emission ◽  
High Level ◽  
Aerosol Emissions

Abstract. Aerosols from biomass burning (BB) emissions are poorly constrained in global and regional models, resulting in a high level of uncertainty in understanding their impacts. In this study, we compared six BB aerosol emission datasets for 2008 globally as well as in 14 regions. The six BB emission datasets are (1) GFED3.1 (Global Fire Emissions Database version 3.1), (2) GFED4s (GFED version 4 with small fires), (3) FINN1.5 (FIre INventory from NCAR version 1.5), (4) GFAS1.2 (Global Fire Assimilation System version 1.2), (5) FEER1.0 (Fire Energetics and Emissions Research version 1.0), and (6) QFED2.4 (Quick Fire Emissions Dataset version 2.4). The global total emission amounts from these six BB emission datasets differed by a factor of 3.8, ranging from 13.76 to 51.93 Tg for organic carbon and from 1.65 to 5.54 Tg for black carbon. In most of the regions, QFED2.4 and FEER1.0, which are based on satellite observations of fire radiative power (FRP) and constrained by aerosol optical depth (AOD) data from the Moderate Resolution Imaging Spectroradiometer (MODIS), yielded higher BB aerosol emissions than the rest by a factor of 2–4. By comparison, the BB aerosol emissions estimated from GFED4s and GFED3.1, which are based on satellite burned-area data, without AOD constraints, were at the low end of the range. In order to examine the sensitivity of model-simulated AOD to the different BB emission datasets, we ingested these six BB emission datasets separately into the same global model, the NASA Goddard Earth Observing System (GEOS) model, and compared the simulated AOD with observed AOD from the AErosol RObotic NETwork (AERONET) and the Multiangle Imaging SpectroRadiometer (MISR) in the 14 regions during 2008. In Southern Hemisphere Africa (SHAF) and South America (SHSA), where aerosols tend to be clearly dominated by smoke in September, the simulated AOD values were underestimated in almost all experiments compared to MISR, except for the QFED2.4 run in SHSA. The model-simulated AOD values based on FEER1.0 and QFED2.4 were the closest to the corresponding AERONET data, being, respectively, about 73 % and 100 % of the AERONET observed AOD at Alta Floresta in SHSA and about 49 % and 46 % at Mongu in SHAF. The simulated AOD based on the other four BB emission datasets accounted for only ∼50 % of the AERONET AOD at Alta Floresta and ∼20 % at Mongu. Overall, during the biomass burning peak seasons, at most of the selected AERONET sites in each region, the AOD values simulated with QFED2.4 were the highest and closest to AERONET and MISR observations, followed closely by FEER1.0. However, the QFED2.4 run tends to overestimate AOD in the region of SHSA, and the QFED2.4 BB emission dataset is tuned with the GEOS model. In contrast, the FEER1.0 BB emission dataset is derived in a more model-independent fashion and is more physically based since its emission coefficients are independently derived at each grid box. Therefore, we recommend the FEER1.0 BB emission dataset for aerosol-focused hindcast experiments in the two biomass-burning-dominated regions in the Southern Hemisphere, SHAF, and SHSA (as well as in other regions but with lower confidence). The differences between these six BB emission datasets are attributable to the approaches and input data used to derive BB emissions, such as whether AOD from satellite observations is used as a constraint, whether the approaches to parameterize the fire activities are based on burned area, FRP, or active fire count, and which set of emission factors is chosen.

scholarly journals Trace gas emissions from combustion of peat, crop residue, domestic biofuels, grasses, and other fuels: configuration and Fourier transform infrared (FTIR) component of the fourth Fire Lab at Missoula Experiment (FLAME-4)

2014 ◽  
Vol 14 (18) ◽  
pp. 9727-9754 ◽  
Author(s):  
C. E. Stockwell ◽  
R. J. Yokelson ◽  
S. M. Kreidenweis ◽  
A. L. Robinson ◽  
P. J. DeMott ◽  
...  
Keyword(s):  
Biomass Burning ◽  
Crop Residue ◽  
Crop Residues ◽  
Trace Gas ◽  
Fire Emissions ◽  
The Us ◽  
Peat Fire ◽  
Peat Fires ◽  
First Time ◽  
Emission Ratios

Abstract. During the fourth Fire Lab at Missoula Experiment (FLAME-4, October–November 2012) a large variety of regionally and globally significant biomass fuels was burned at the US Forest Service Fire Sciences Laboratory in Missoula, Montana. The particle emissions were characterized by an extensive suite of instrumentation that measured aerosol chemistry, size distribution, optical properties, and cloud-nucleating properties. The trace gas measurements included high-resolution mass spectrometry, one- and two-dimensional gas chromatography, and open-path Fourier transform infrared (OP-FTIR) spectroscopy. This paper summarizes the overall experimental design for FLAME-4 – including the fuel properties, the nature of the burn simulations, and the instrumentation employed – and then focuses on the OP-FTIR results. The OP-FTIR was used to measure the initial emissions of 20 trace gases: CO2, CO, CH4, C2H2, C2H4, C3H6, HCHO, HCOOH, CH3OH, CH3COOH, glycolaldehyde, furan, H2O, NO, NO2, HONO, NH3, HCN, HCl, and SO2. These species include most of the major trace gases emitted by biomass burning, and for several of these compounds, this is the first time their emissions are reported for important fuel types. The main fire types included African grasses, Asian rice straw, cooking fires (open (three-stone), rocket, and gasifier stoves), Indonesian and extratropical peat, temperate and boreal coniferous canopy fuels, US crop residue, shredded tires, and trash. Comparisons of the OP-FTIR emission factors (EFs) and emission ratios (ERs) to field measurements of biomass burning verify that the large body of FLAME-4 results can be used to enhance the understanding of global biomass burning and its representation in atmospheric chemistry models. Crop residue fires are widespread globally and account for the most burned area in the US, but their emissions were previously poorly characterized. Extensive results are presented for burning rice and wheat straw: two major global crop residues. Burning alfalfa produced the highest average NH3 EF observed in the study (6.63 ± 2.47 g kg−1), while sugar cane fires produced the highest EF for glycolaldehyde (6.92 g kg−1) and other reactive oxygenated organic gases such as HCHO, HCOOH, and CH3COOH. Due to the high sulfur and nitrogen content of tires, they produced the highest average SO2 emissions (26.2 ± 2.2 g kg−1) and high NOx and HONO emissions. High variability was observed for peat fire emissions, but they were consistently characterized by large EFs for NH3 (1.82 ± 0.60 g kg−1) and CH4 (10.8 ± 5.6 g kg−1). The variability observed in peat fire emissions, the fact that only one peat fire had previously been subject to detailed emissions characterization, and the abundant emissions from tropical peatlands all impart high value to our detailed measurements of the emissions from burning three Indonesian peat samples. This study also provides the first EFs for HONO and NO2 for Indonesian peat fires. Open cooking fire emissions of HONO and HCN are reported for the first time, and the first emissions data for HCN, NO, NO2, HONO, glycolaldehyde, furan, and SO2 are reported for "rocket" stoves: a common type of improved cookstove. The HCN / CO emission ratios for cooking fires (1.72 × 10−3 ± 4.08 × 10−4) and peat fires (1.45 × 10−2 ± 5.47 × 10−3) are well below and above the typical values for other types of biomass burning, respectively. This would affect the use of HCN / CO observations for source apportionment in some regions. Biomass burning EFs for HCl are rare and are reported for the first time for burning African savanna grasses. High emissions of HCl were also produced by burning many crop residues and two grasses from coastal ecosystems. HCl could be the main chlorine-containing gas in very fresh smoke, but rapid partitioning to aerosol followed by slower outgassing probably occurs.

scholarly journals On the use of ATSR fire count data to estimate the seasonal and interannual variability of vegetation fire emissions

2002 ◽  
Vol 2 (4) ◽  
pp. 1159-1179 ◽  
Author(s):  
M. G. Schultz
Keyword(s):  
Interannual Variability ◽  
Biomass Burning ◽  
Seasonal Pattern ◽  
Burned Area ◽  
Time Resolved ◽  
Fire Emissions ◽  
Seasonal And Interannual Variability ◽  
Active Fire ◽  
Time Period ◽  
Along Track

Abstract. Biomass burning has long been recognised as an important source of trace gases and aerosols in the atmosphere. The burning of vegetation has a repeating seasonal pattern, but the intensity of burning and the exact localisation of fires vary considerably from year to year. Recent studies have demonstrated the high interannual variability of the emissions that are associated with biomass burning. In this paper we present a methodology using active fire counts from the Along-Track Scanning Radiometer (ATSR) sensor on board the ERS-2 satellite to estimate the seasonal and interannual variability of global biomass burning emissions in the time period 1996--2000. From the ATSR data, we compute relative scaling factors of burning intensity for each month, which are then applied to a standard inventory for carbon monoxide emissions from biomass burning. The new, time-resolved inventory is evaluated using the few existing multi-year burned area observations on continental scales.

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