scholarly journals Long-term time series of Arctic tropospheric BrO derived from UV–VIS satellite remote sensing and its relation to first-year sea ice

2020 ◽  
Vol 20 (20) ◽  
pp. 11869-11892
Author(s):  
Ilias Bougoudis ◽  
Anne-Marlene Blechschmidt ◽  
Andreas Richter ◽  
Sora Seo ◽  
John Philip Burrows ◽  
...  

Abstract. Every polar spring, phenomena called bromine explosions occur over sea ice. These bromine explosions comprise photochemical heterogeneous chain reactions that release bromine molecules, Br2, to the troposphere and lead to tropospheric plumes of bromine monoxide, BrO. This autocatalytic mechanism depletes ozone, O3, in the boundary layer and troposphere and thereby changes the oxidizing capacity of the atmosphere. The phenomenon also leads to accelerated deposition of metals (e.g., Hg). In this study, we present a 22-year (1996 to 2017) consolidated and consistent tropospheric BrO dataset north of 70∘ N, derived from four different ultraviolet–visible (UV–VIS) satellite instruments (GOME, SCIAMACHY, GOME-2A and GOME-2B). The retrieval data products from the different sensors are compared during periods of overlap and show good agreement (correlations of 0.82–0.98 between the sensors). From our merged time series of tropospheric BrO vertical column densities (VCDs), we infer changes in the bromine explosions and thus an increase in the extent and magnitude of tropospheric BrO plumes during the period of Arctic warming. We determined an increasing trend of about 1.5 % of the tropospheric BrO VCDs per year during polar springs, while the size of the areas where enhanced tropospheric BrO VCDs can be found has increased about 896 km2 yr−1. We infer from comparisons and correlations with sea ice age data that the reported changes in the extent and magnitude of tropospheric BrO VCDs are moderately related to the increase in first-year ice extent in the Arctic north of 70∘ N, both temporally and spatially, with a correlation coefficient of 0.32. However, the BrO plumes and thus bromine explosions show significant variability, which also depends, apart from sea ice, on meteorological conditions.

2020 ◽  
Author(s):  
Ilias Bougoudis ◽  
Anne-Marlene Blechschmidt ◽  
Andreas Richter ◽  
Sora Seo ◽  
John Philip Burrows ◽  
...  

Abstract. Arctic Amplification describes the rapid increase of the air temperature in the past three decades in the Arctic, which impacts on physicochemical conditions, the ecosystem and biogeochemistry. Every polar spring, the BrO explosion, a series of chemical reactions that release bromine molecules to the troposphere occurs over sea ice covered regions. This autocatalytic mechanism depletes boundary layer and tropospheric ozone, thereby changes the oxidizing capacity of the atmosphere and facilitates the deposition of metals (e.g. Hg). In this study, we present a 22 year consolidated and consistent tropospheric BrO dataset, derived from four different UV-VIS satellite instruments and investigate the BrO evolution under the impact of Arctic Amplification. The retrieval data products from the different sensors are compared during periods of overlap and show good agreement. By studying the sensor merged time-series of tropospheric BrO vertical column densities, we find an increase in the magnitude of BrO explosion events under the impact of Arctic Amplification with an upward trend of about 1.5 % per year. Furthermore, the areas where BrO plumes frequently appear have changed, extending over larger regions in the Arctic during more recent years. Comparison to sea ice age data suggests that the reported changes in tropospheric BrO are linked in a complex way to the increase of first-year ice extent in the Arctic.


1983 ◽  
Vol 4 ◽  
pp. 204-208 ◽  
Author(s):  
Masayoshi Nakawo

The air content of sea ice can be measured directly by melting a sample and collecting the released air, provided the air saturation ratio in the meltwater is known. The saturation ratio was found experimentally to be a function of three parameters: the time after an ice sample was melted, the average bubble size, and the air porosity of the sample. Since the last parameter is the term to be determined, an iteration method was employed in calculations of porosity. The bubble pressure was assumed to be at one atmospheric pressure. The vertical profile of air porosity was thus obtained for first-year sea ice in the Arctic. The results were in good agreement with estimations of porosity made from density values measured for the same samples. This indicates that the bubble pressure is near one atmospheric pressure.


1983 ◽  
Vol 4 ◽  
pp. 204-208 ◽  
Author(s):  
Masayoshi Nakawo

The air content of sea ice can be measured directly by melting a sample and collecting the released air, provided the air saturation ratio in the meltwater is known. The saturation ratio was found experimentally to be a function of three parameters: the time after an ice sample was melted, the average bubble size, and the air porosity of the sample. Since the last parameter is the term to be determined, an iteration method was employed in calculations of porosity. The bubble pressure was assumed to be at one atmospheric pressure. The vertical profile of air porosity was thus obtained for first-year sea ice in the Arctic. The results were in good agreement with estimations of porosity made from density values measured for the same samples. This indicates that the bubble pressure is near one atmospheric pressure.


2020 ◽  
Vol 14 (5) ◽  
pp. 1519-1536 ◽  
Author(s):  
Mark A. Tschudi ◽  
Walter N. Meier ◽  
J. Scott Stewart

Abstract. A new version of sea ice motion and age products includes several significant upgrades in processing, corrects known issues with the previous version, and updates the time series through 2018, with regular updates planned for the future. First, we provide a history of these NASA products distributed at the National Snow and Ice Data Center. Then we discuss the improvements to the algorithms, provide validation results for the new (Version 4) and older versions, and intercompare the two. While Version 4 algorithm changes were significant, the impact on the products is relatively minor, particularly for more recent years. The changes in Version 4 reduce motion biases by ∼ 0.01 to 0.02 cm s−1 and error standard deviations by ∼ 0.3 cm s−1. Overall, ice speed increased in Version 4 over Version 3 by 0.5 to 2.0 cm s−1 over most of the time series. Version 4 shows a higher positive trend for the Arctic of 0.21 cm s−1 per decade compared to 0.13 cm s−1 per decade for Version 3. The new version of ice age estimates indicates more older ice than Version 3, especially earlier in the record, but similar trends toward less multiyear ice. Changes in sea ice motion and age derived from the product show a significant shift in the Arctic ice cover, from a pack with a high concentration of older ice to a sea ice cover dominated by first-year ice, which is more susceptible to summer melt. We also observe an increase in the speed of the ice over the time series ≥ 30 years, which has been shown in other studies and is anticipated with the annual decrease in sea ice extent.


2020 ◽  
Author(s):  
Baek-Min Kim ◽  
Ha-Rim Kim ◽  
Yong-Sang Choi ◽  
Yejin Lee ◽  
Gun-Hwan Yang

<div> <div> <div> <p>Recently, many studies have highlighted the importance of the ability to predict the Arctic sea ice concentration in the sub-seasonal time scales. Notably, the Arctic sea ice concentration has a potential for skillful predictions through their long-term trend memory. Based on the long-term memory of Arctic sea ice concentration, we evaluate the predictability of Arctic sea ice concentration (SIC) by applying a time-series analysis technique of the Prophet model on sub-seasonal time scales. A Prophet is a recently introduced method as a statistical approach inspired by the nature of time series forecasted at Facebook and has not been applied to the prediction of Arctic SIC before. Sub-seasonal prediction skills of Arctic SIC in the Prophet model were compared with the NCEP Climate Forecast System Reforecast (CFS-Reforecast) model as a dynamical approach and verified with the satellite observation during wintertime from 2000 to 2018 for 1 to 8 weeks lead times. The result shows that the Prophet model exhibits much better skill than the NCEP CFS-Reforecast model in the climatology prediction except for the 1 to 3 weeks lead times, as the Prophet model has mainly the ability to capture the long-term trend. In the anomaly prediction, however, the NCEP CFS-Reforecast model is superior to the Prophet model in the prediction of sub-seasonal time scales, as the NCEP CFS-Reforecast captures more effectively the sub-seasonal transition of the underlying dynamical system. Therefore, even if the Prophet model has shown a useful skill in predicting the climatological Arctic SIC, there is still a need to improve the accuracy and robustness of the predictions in an anomalous Arctic SIC. Further, we suggest that the bias correction method is needed to improve the forecast skill of Arctic SIC using the time-series analysis technique, and it will be critical to advance the field of the Arctic SIC forecasting on the sub-seasonal time scales.</p> </div> </div> </div>


2020 ◽  
Author(s):  
Ilias Bougoudis ◽  
Anne-Marlene Blechschmidt ◽  
Andreas Richter ◽  
Sora Seo ◽  
John Burrows

<p>Arctic Amplification, the rapid increase of air temperature in higher latitudes over the last decades, is expected to have drastic impacts on all the sub-systems of the Arctic ecosystem. Bromine Oxides play a key role in the atmospheric composition of the Arctic. During polar spring, bromine molecules are released from young sea ice covered regions.  A rapid chemical chain reaction starts, the -so called 'bromine explosion', which depletes ozone, alters the production of OH, and thereby eventually changes the oxidizing capacity of the troposphere. Halogens oxidize elemental to gaseous mercury, which may then be deposited and harm the ecosystem. Based on current literature, there is considerable uncertainty on the impact of Arctic Amplification on halogen evolution. On one hand, the melting of multi-year sea ice should result in formation of more young sea ice, which favors bromine release. On the other hand, BrO explosion events are triggered by low temperatures, an effect expected to be reduced due to Arctic Amplification. Moreover, changes of other meteorological drivers, such as cyclone frequency and wind speed may impact on BrO amounts in the Arctic troposphere.</p><p>In this study, a long-term time-series of tropospheric BrO derived from 4 UV-VIS instruments (GOME, SCIAMACHY, GOME-2A, GOME-2B) is used as a basis, in order to investigate the impact of Arctic Amplification on BrO amounts in the Arctic. The long-term BrO data is being compared to sea ice age (NSIDC) and meteorological (air temperature, mean sea level pressure, wind speed and boundary layer height from ERA-5 & ASR-2) data. Our results focus on determining the relation between tropospheric BrO and its drivers, and especially on how the drivers impact on the formation of BrO plumes. Different cases studies throughout the 22 years of the BrO dataset were performed and evaluated. The changes in the tropospheric BrO abundances come in general agreement with changes in the drivers of BrO explosion events.</p><p> </p><p>We gratefully acknowledge the funding by the Deutsche Forschungsgemeinschaft (DFG, German Research Foundation) – Projektnummer 268020496 – TRR 172, within the Transregional Collaborative Research Center “ArctiC Amplification: Climate Relevant Atmospheric and SurfaCe Processes, and Feedback Mechanisms (AC)³”.</p>


2021 ◽  
Vol 13 (11) ◽  
pp. 2174
Author(s):  
Lijian Shi ◽  
Sen Liu ◽  
Yingni Shi ◽  
Xue Ao ◽  
Bin Zou ◽  
...  

Polar sea ice affects atmospheric and ocean circulation and plays an important role in global climate change. Long time series sea ice concentrations (SIC) are an important parameter for climate research. This study presents an SIC retrieval algorithm based on brightness temperature (Tb) data from the FY3C Microwave Radiation Imager (MWRI) over the polar region. With the Tb data of Special Sensor Microwave Imager/Sounder (SSMIS) as a reference, monthly calibration models were established based on time–space matching and linear regression. After calibration, the correlation between the Tb of F17/SSMIS and FY3C/MWRI at different channels was improved. Then, SIC products over the Arctic and Antarctic in 2016–2019 were retrieved with the NASA team (NT) method. Atmospheric effects were reduced using two weather filters and a sea ice mask. A minimum ice concentration array used in the procedure reduced the land-to-ocean spillover effect. Compared with the SIC product of National Snow and Ice Data Center (NSIDC), the average relative difference of sea ice extent of the Arctic and Antarctic was found to be acceptable, with values of −0.27 ± 1.85 and 0.53 ± 1.50, respectively. To decrease the SIC error with fixed tie points (FTPs), the SIC was retrieved by the NT method with dynamic tie points (DTPs) based on the original Tb of FY3C/MWRI. The different SIC products were evaluated with ship observation data, synthetic aperture radar (SAR) sea ice cover products, and the Round Robin Data Package (RRDP). In comparison with the ship observation data, the SIC bias of FY3C with DTP is 4% and is much better than that of FY3C with FTP (9%). Evaluation results with SAR SIC data and closed ice data from RRDP show a similar trend between FY3C SIC with FTPs and FY3C SIC with DTPs. Using DTPs to present the Tb seasonal change of different types of sea ice improved the SIC accuracy, especially for the sea ice melting season. This study lays a foundation for the release of long time series operational SIC products with Chinese FY3 series satellites.


2006 ◽  
Vol 63 (3) ◽  
pp. 401-420 ◽  
Author(s):  
Harald Yndestad

Abstract The Arctic Ocean is a substantial energy sink for the northern hemisphere. Fluctuations in its energy budget will have a major influence on the Arctic climate. The paper presents an analysis of the time-series for the polar position, the extent of Arctic ice, sea level at Hammerfest, Kola section sea temperature, Røst winter air temperature, and the NAO winter index as a way to identify a source of dominant cycles. The investigation uses wavelet transformation to identify the period and the phase in these Arctic time-series. System dynamics are identified by studying the phase relationship between the dominant cycles in all time-series. A harmonic spectrum from the 18.6-year lunar nodal cycle in the Arctic time-series has been identified. The cycles in this harmonic spectrum have a stationary period, but not stationary amplitude and phase. A sub-harmonic cycle of about 74 years may introduce a phase reversal of the 18.6-year cycle. The signal-to-noise ratio between the lunar nodal spectrum and other sources changes from 1.6 to 3.2. A lunar nodal cycle in all time-series indicates that there is a forced Arctic oscillating system controlled by the pull of gravity from the moon, a system that influences long-term fluctuations in the extent of Arctic ice. The phase relation between the identified cycles indicates a possible chain of events from lunar nodal gravity cycles, to long-term tides, polar motions, Arctic ice extent, the NAO winter index, weather, and climate.


2021 ◽  
Author(s):  
Isolde Glissenaar ◽  
Jack Landy ◽  
Alek Petty ◽  
Nathan Kurtz ◽  
Julienne Stroeve

<p>The ice cover of the Arctic Ocean is increasingly becoming dominated by seasonal sea ice. It is important to focus on the processing of altimetry ice thickness data in thinner seasonal ice regions to understand seasonal sea ice behaviour better. This study focusses on Baffin Bay as a region of interest to study seasonal ice behaviour.</p><p>We aim to reconcile the spring sea ice thickness derived from multiple satellite altimetry sensors and sea ice charts in Baffin Bay and produce a robust long-term record (2003-2020) for analysing trends in sea ice thickness. We investigate the impact of choosing different snow depth products (the Warren climatology, a passive microwave snow depth product and modelled snow depth from reanalysis data) and snow redistribution methods (a sigmoidal function and an empirical piecewise function) to retrieve sea ice thickness from satellite altimetry sea ice freeboard data.</p><p>The choice of snow depth product and redistribution method results in an uncertainty envelope around the March mean sea ice thickness in Baffin Bay of 10%. Moreover, the sea ice thickness trend ranges from -15 cm/dec to 20 cm/dec depending on the applied snow depth product and redistribution method. Previous studies have shown a possible long-term asymmetrical trend in sea ice thinning in Baffin Bay. The present study shows that whether a significant long-term asymmetrical trend was found depends on the choice of snow depth product and redistribution method. The satellite altimetry sea ice thickness results with different snow depth products and snow redistribution methods show that different processing techniques can lead to different results and can influence conclusions on total and spatial sea ice thickness trends. Further processing work on the historic radar altimetry record is needed to create reliable sea ice thickness products in the marginal ice zone.</p>


2017 ◽  
Vol 59 (76pt2) ◽  
pp. 181-190 ◽  
Author(s):  
Thomas J. Ballinger ◽  
Edward Hanna ◽  
Richard J. Hall ◽  
Thomas E. Cropper ◽  
Jeffrey Miller ◽  
...  

ABSTRACTThe Arctic marine environment is undergoing a transition from thick multi-year to first-year sea-ice cover with coincident lengthening of the melt season. Such changes are evident in the Baffin Bay-Davis Strait-Labrador Sea (BDL) region where melt onset has occurred ~8 days decade−1 earlier from 1979 to 2015. A series of anomalously early events has occurred since the mid-1990s, overlapping a period of increased upper-air ridging across Greenland and the northwestern North Atlantic. We investigate an extreme early melt event observed in spring 2013. (~6σ below the 1981–2010 melt climatology), with respect to preceding sub-seasonal mid-tropospheric circulation conditions as described by a daily Greenland Blocking Index (GBI). The 40-days prior to the 2013 BDL melt onset are characterized by a persistent, strong 500 hPa anticyclone over the region (GBI >+1 on >75% of days). This circulation pattern advected warm air from northeastern Canada and the northwestern Atlantic poleward onto the thin, first-year sea ice and caused melt ~50 days earlier than normal. The episodic increase in the ridging atmospheric pattern near western Greenland as in 2013, exemplified by large positive GBI values, is an important recent process impacting the atmospheric circulation over a North Atlantic cryosphere undergoing accelerated regional climate change.


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