scholarly journals Towards continuous monitoring of aerosol hygroscopicity by Raman lidar measurements at the EARLINET station of Payerne

2019 ◽  
Author(s):  
Francisco Navas Guzmán ◽  
Giovanni Martucci ◽  
Martine Collaud Coen ◽  
María José Granados Muñoz ◽  
Maxime Hervo ◽  
...  

Abstract. This study focuses on the analysis of aerosol hygroscopicity using remote sensing technique. Continuous observations of aerosol backscatter coefficient, temperature and water vapour mixing ratio are performed by means of a Raman lidar system at the aerological station of MeteoSwiss at Payerne (Switzerland) since 2008. These measurements allow us to monitor in a continuous way any change of aerosol properties as a function of the relative humidity (RH). These changes can be observed either in time at constant altitude or in altitude at a constant time. The accuracy and precision of RH measurements from the lidar have been evaluated using the radiosonde (RS) technique as reference. A total of 172 RSs were used in this intercomparison which revealed a small bias (

2021 ◽  
Vol 21 (3) ◽  
pp. 2267-2285
Author(s):  
Simone Brunamonti ◽  
Giovanni Martucci ◽  
Gonzague Romanens ◽  
Yann Poltera ◽  
Frank G. Wienhold ◽  
...  

Abstract. Remote-sensing measurements by light detection and ranging (lidar) instruments are fundamental for the monitoring of altitude-resolved aerosol optical properties. Here we validate vertical profiles of aerosol backscatter coefficient (βaer) measured by two independent lidar systems using co-located balloon-borne measurements performed by Compact Optical Backscatter Aerosol Detector (COBALD) sondes. COBALD provides high-precision in situ measurements of βaer at two wavelengths (455 and 940 nm). The two analyzed lidar systems are the research Raman Lidar for Meteorological Observations (RALMO) and the commercial CHM15K ceilometer (Lufft, Germany). We consider in total 17 RALMO and 31 CHM15K profiles, co-located with simultaneous COBALD soundings performed throughout the years 2014–2019 at the MeteoSwiss observatory of Payerne (Switzerland). The RALMO (355 nm) and CHM15K (1064 nm) measurements are converted to 455 and 940 nm, respectively, using the Ångström exponent profiles retrieved from COBALD data. To account for the different receiver field-of-view (FOV) angles between the two lidars (0.01–0.02∘) and COBALD (6∘), we derive a custom-made correction using Mie-theory scattering simulations. Our analysis shows that both lidar instruments achieve on average a good agreement with COBALD measurements in the boundary layer and free troposphere, up to 6 km altitude. For medium-high-aerosol-content measurements at altitudes below 3 km, the mean ± standard deviation difference in βaer calculated from all considered soundings is −2 % ± 37 % (−0.018 ± 0.237 Mm−1 sr−1 at 455 nm) for RALMO−COBALD and +5 % ± 43 % (+0.009 ± 0.185 Mm−1 sr−1 at 940 mm) for CHM15K−COBALD. Above 3 km altitude, absolute deviations generally decrease, while relative deviations increase due to the prevalence of air masses with low aerosol content. Uncertainties related to the FOV correction and spatial- and temporal-variability effects (associated with the balloon's drift with altitude and different integration times) contribute to the large standard deviations observed at low altitudes. The lack of information on the aerosol size distribution and the high atmospheric variability prevent an accurate quantification of these effects. Nevertheless, the excellent agreement observed in individual profiles, including fine and complex structures in the βaer vertical distribution, shows that under optimal conditions, the discrepancies with the in situ measurements are typically comparable to the estimated statistical uncertainties in the remote-sensing measurements. Therefore, we conclude that βaer profiles measured by the RALMO and CHM15K lidar systems are in good agreement with in situ measurements by COBALD sondes up to 6 km altitude.


2015 ◽  
Vol 8 (9) ◽  
pp. 3789-3809 ◽  
Author(s):  
K. Baibakov ◽  
N. T. O'Neill ◽  
L. Ivanescu ◽  
T. J. Duck ◽  
C. Perro ◽  
...  

Abstract. We present recent progress on nighttime retrievals of aerosol and cloud optical properties over the PEARL (Polar Environmental Atmospheric Research Laboratory) station at Eureka (Nunavut, Canada) in the High Arctic (80° N, 86° W). In the spring of 2011 and 2012, a star photometer was employed to acquire aerosol optical depth (AOD) data, while vertical aerosol and cloud backscatter profiles were measured using the CANDAC Raman Lidar (CRL). We used a simple backscatter coefficient threshold (βthr) to distinguish aerosols from clouds and, assuming that aerosols were largely fine mode (FM)/sub-micron, to distinguish FM aerosols from coarse mode (CM)/super-micron cloud or crystal particles. Using prescribed lidar ratios, we computed FM and CM AODs that were compared with analogous AODs estimated from spectral star photometry. We found (βthr dependent) coherences between the lidar and star photometer for both FM events and CM cloud and crystal events with averaged, FM absolute differences being


2019 ◽  
Vol 99 ◽  
pp. 02010
Author(s):  
Ronny Engelmann ◽  
Julian Hofer ◽  
Abduvosit N. Makhmudov ◽  
Holger Baars ◽  
Karsten Hanbuch ◽  
...  

During the 18-month Central Asian Dust Experiment we conducted continuous lidar measurements at the Physical Technical Institute of the Academy of Sciences of Tajikistan in Dushanbe between 2015 and 2016. Mineral dust plumes from various source regions have been observed and characterized in terms of their occurrence, and their optical and microphysical properties with the Raman lidar PollyXT. Currently a new container-based lidar system is constructed which will be installed for continuous long-term measurements in Dushanbe.


2019 ◽  
Vol 19 (18) ◽  
pp. 11651-11668 ◽  
Author(s):  
Francisco Navas-Guzmán ◽  
Giovanni Martucci ◽  
Martine Collaud Coen ◽  
María José Granados-Muñoz ◽  
Maxime Hervo ◽  
...  

Abstract. This study focuses on the analysis of aerosol hygroscopicity using remote sensing techniques. Continuous observations of aerosol backscatter coefficient (βaer), temperature (T) and water vapor mixing ratio (r) have been performed by means of a Raman lidar system at the aerological station of MeteoSwiss at Payerne (Switzerland) since 2008. These measurements allow us to monitor in a continuous way any change in aerosol properties as a function of the relative humidity (RH). These changes can be observed either in time at a constant altitude or in altitude at a constant time. The accuracy and precision of RH measurements from the lidar have been evaluated using the radiosonde (RS) technique as a reference. A total of 172 RS profiles were used in this intercomparison, which revealed a bias smaller than 4 % RH and a standard deviation smaller than 10 % RH between both techniques in the whole (in lower) troposphere at nighttime (at daytime), indicating the good performance of the lidar for characterizing RH. A methodology to identify situations favorable to studying aerosol hygroscopicity has been established, and the aerosol hygroscopicity has been characterized by means of the backscatter enhancement factor (fβ). Two case studies, corresponding to different types of aerosol, are used to illustrate the potential of this methodology. The first case corresponds to a mixture of rural aerosol and smoke particles (smoke mixture), which showed a higher hygroscopicity (fβ355=2.8 and fβ1064=1.8 in the RH range 73 %–97 %) than the second case, in which mineral dust was present (fβ355=1.2 and fβ1064=1.1 in the RH range 68 %–84 %). The higher sensitivity of the shortest wavelength to hygroscopic growth was qualitatively reproduced using Mie simulations. In addition, a good agreement was found between the hygroscopic analysis done in the vertical and in time for Case I, where the latter also allowed us to observe the hydration and dehydration of the smoke mixture. Finally, the impact of aerosol hygroscopicity on the Earth's radiative balance has been evaluated using the GAME (Global Atmospheric Model) radiative transfer model. The model showed an impact with an increase in absolute value of 2.4 W m−2 at the surface with respect to the dry conditions for the hygroscopic layer of Case I (smoke mixture).


2020 ◽  
Author(s):  
Simone Brunamonti ◽  
Giovanni Martucci ◽  
Gonzague Romanens ◽  
Yann Poltera ◽  
Frank G. Wienhold ◽  
...  

Abstract. Remote sensing measurements by light detection and ranging (lidar) instruments are fundamental for the monitoring of altitude-resolved aerosol optical properties. Here, we validate vertical profiles of aerosol backscatter coefficient (βaer) measured by two independent lidar systems using co-located balloon-borne measurements performed by Compact Optical Backscatter Aerosol Detector (COBALD) sondes. COBALD provides high-precision in-situ measurements of βaer at two wavelengths (455 and 940 nm). The two analyzed lidar systems are the research Raman Lidar for Meteorological Observations (RALMO) and the commercial CHM15K ceilometer (Lufft, Germany). We consider in total 17 RALMO and 31 CHM15K profiles, co-located with simultaneous COBALD soundings performed throughout the years 2014–2019 at the MeteoSwiss observatory of Payerne (Switzerland). The RALMO (355 nm) and CHM15K (1064 nm) measurements are converted to respectively 455 nm and 940 nm using the Angstrom exponent profiles retrieved from COBALD data. To account for the different receiver field of view (FOV) angles between the two lidars (0.01–0.02°) and COBALD (6°), we derive a custom-made correction using Mie-theory scattering simulations. Our analysis shows that both RALMO and CHM15K achieve a good agreement with COBALD measurements in the boundary layer and free troposphere, up to 6 km altitude, and including fine structures in the aerosol’s vertical distribution. For altitudes below 2 km, the mean ± standard deviation difference in βaer is + 6 % ± 40 % (+ 0.005 ± 0.319 Mm−1 sr−1) for RALMO – COBALD at 455 nm, and + 13 % ± 51 % (+ 0.038 ± 0.207 Mm−1 sr−1) for CHM15K – COBALD at 940 nm. The large standard deviations can be at least partly attributed to atmospheric variability effects, associated with the balloon’s horizontal drift with altitude (away from the lidar beam) and the different integration times of the two techniques. Combined with the high spatial and temporal variability of atmospheric aerosols, these effects often lead to a slight altitude displacement between aerosol backscatter features that are seen by both techniques. For altitudes between 2–6 km, the absolute standard deviations of both RALMO and CHM15K decrease (below 0.13 and 0.16 Mm−1sr−1, respectively), while their corresponding relative deviations increase (often exceeding 100 % COBALD of the signal). This is due to the low aerosol content (i.e. low absolute backscattered signal) in the free troposphere, and the vertically decreasing signal-to-noise ratio of the lidar measurements (especially CHM15K). Overall, we conclude that the βaer profiles measured by the RALMO and CHM15K lidar systems are in good agreement with in-situ measurements by COBALD sondes up to 6 km altitude.


2015 ◽  
Vol 8 (5) ◽  
pp. 2207-2223 ◽  
Author(s):  
F. Madonna ◽  
F. Amato ◽  
J. Vande Hey ◽  
G. Pappalardo

Abstract. Despite their differences from more advanced and more powerful lidars, the low construction and operation cost of ceilometers (originally designed for cloud base height monitoring) has fostered their use for the quantitative study of aerosol properties. The large number of ceilometers available worldwide represents a strong motivation to investigate both the extent to which they can be used to fill in the geographical gaps between advanced lidar stations and also how their continuous data flow can be linked to existing networks of the more advanced lidars, like EARLINET (European Aerosol Research Lidar Network). In this paper, multi-wavelength Raman lidar measurements are used to investigate the capability of ceilometers to provide reliable information about atmospheric aerosol properties through the INTERACT (INTERcomparison of Aerosol and Cloud Tracking) campaign carried out at the CNR-IMAA Atmospheric Observatory (760 m a.s.l., 40.60° N, 15.72° E), in the framework of the ACTRIS (Aerosol Clouds Trace gases Research InfraStructure) FP7 project. This work is the first time that three different commercial ceilometers with an advanced Raman lidar are compared over a period of 6 months. The comparison of the attenuated backscatter coefficient profiles from a multi-wavelength Raman lidar and three ceilometers (CHM15k, CS135s, CT25K) reveals differences due to the expected discrepancy in the signal to noise ratio (SNR) but also due to changes in the ambient temperature on the short and mid-term stability of ceilometer calibration. Therefore, technological improvements are needed to move ceilometers towards operational use in the monitoring of atmospheric aerosols in the low and free troposphere.


2007 ◽  
Author(s):  
Daniela Viviana Vladutescu ◽  
Barry Gross ◽  
Yonghua Wu ◽  
Alex Gilerson ◽  
Fred Moshary ◽  
...  

2009 ◽  
Vol 26 (11) ◽  
pp. 2366-2378 ◽  
Author(s):  
Dietrich Althausen ◽  
Ronny Engelmann ◽  
Holger Baars ◽  
Birgit Heese ◽  
Albert Ansmann ◽  
...  

Abstract Two versions of the portable aerosol Raman lidar system (Polly) are presented. First, the two-channel prototype is depicted. It has been developed for the independent and simultaneous determination of particle backscatter and extinction coefficient profiles at 532 nm. Second, the 3 + 2 Raman lidar PollyXT (3 + 2: three backscatter and two extinction coefficients), the second generation of Polly, is described. The extended capabilities of PollyXT are due to the simultaneous emission of light with three wavelengths, more laser power, a larger main receiver mirror, and seven receiver channels. These systems are completely remotely controlled and all measurements are performed automatically. The collected data are transferred to a home server via the Internet and are displayed on a Web page. This paper describes the details of the optical setup, the housekeeping of the systems, and the used data retrieval routines. A measurement example taken close to Manaus, Brazil, on 15 August 2008 shows the capabilities of PollyXT.


2020 ◽  
Author(s):  
Geraint Vaughan ◽  
David Wareing ◽  
Hugo Ricketts

Abstract. On 22 June 2019 the Raikoke volcano in the Kuril islands erupted, sending a plume of ash and sulphur dioxide into the stratosphere. A Raman lidar system at Capel Dewi Atmospheric Observatory, UK (52.4° N, 4.1° W) has been used to measure the extent and optical depth of the stratospheric aerosol layer following the eruption. The elastic channel allowed measurements up to 25 km, but the Raman channel was only sensitive to the troposphere. Therefore, backscatter ratio profiles were derived by comparison with aerosol-free profiles derived from nearby radiosondes, corrected for aerosol extinction with a lidar ratio of 40–50 sr. Small amounts of aerosol were measured prior to the arrival of the volcanic cloud, probably from pyroconvection over Canada. Volcanic ash may have first arrived as a thin layer at 14 km late on 3 July, and was certainly detected from 13 July onwards, eventually extending up to 20.5 km. Aerosol optical depths reached around 0.05 by early August, decaying thereafter to around 0.01 by the end of 2019 and remaining around that level until May 2020. The location of peak backscatter varied considerably but was generally around 15 km. However, on one notable occasion on 25 August, a layer around 300 m thick with peak lidar backscatter ratio around 1.5 was observed as high as 21 km.


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