scholarly journals Brightening of the global cloud field by nitric acid and the associated radiative forcing

2012 ◽  
Vol 12 (2) ◽  
pp. 5225-5245
Author(s):  
R. Makkonen ◽  
S. Romakkaniemi ◽  
H. Kokkola ◽  
P. Stier ◽  
P. Räisänen ◽  
...  
Keyword(s):  
Nitric Acid ◽  
Indirect Effect ◽  
Radiative Forcing ◽  
Climate Model ◽  
Global Climate ◽  
Cloud Condensation Nuclei ◽  
Global Climate Model ◽  
So2 Emissions ◽  
Cloud Albedo ◽  
Albedo Effect

Abstract. Clouds cool Earth's climate by reflecting 20 % of the incoming solar energy, while also trapping part of the outgoing radiation. The effect of human activities on clouds is poorly understood, but the present-day anthropogenic cooling via changes of cloud albedo and lifetime could be of the same order as warming from anthropogenic addition in CO2. Soluble trace gases can increase water condensation to particles, possibly leading to activation of smaller aerosols and more numerous cloud droplets. We have studied the effect of nitric acid on the aerosol indirect effect with a global climate model. The nitric acid contribution to the present-day cloud albedo effect was found to be −0.32 W m−2 and the total indirect effect −0.46 W m−2. The contribution to the cloud albedo effect is shown to increase to −0.37 W m−2 by 2100, if considering only the reductions in available cloud condensation nuclei. Overall, the effect of nitric acid can play a large part in aerosol cooling during the following decades with decreasing SO2 emissions and increasing NOx and greenhouse gases.

scholarly journals Brightening of the global cloud field by nitric acid and the associated radiative forcing

2012 ◽  
Vol 12 (16) ◽  
pp. 7625-7633 ◽  
Author(s):  
R. Makkonen ◽  
S. Romakkaniemi ◽  
H. Kokkola ◽  
P. Stier ◽  
P. Räisänen ◽  
...  
Keyword(s):  
Nitric Acid ◽  
Indirect Effect ◽  
Radiative Forcing ◽  
Climate Model ◽  
Cloud Condensation Nuclei ◽  
Cloud Droplet ◽  
So2 Emissions ◽  
Cloud Droplets ◽  
Cloud Albedo ◽  
Albedo Effect

Abstract. Clouds cool Earth's climate by reflecting 20% of the incoming solar energy, while also trapping part of the outgoing radiation. The effect of human activities on clouds is poorly understood, but the present-day anthropogenic cooling via changes of cloud albedo and lifetime could be of the same order as warming from anthropogenic addition in CO2. Soluble trace gases can increase water condensation to particles, possibly leading to activation of smaller aerosols and more numerous cloud droplets. We have studied the effect of nitric acid on the aerosol indirect effect with the global aerosol-climate model ECHAM5.5-HAM2. Including the nitric acid effect in the model increases cloud droplet number concentrations globally by 7%. The nitric acid contribution to the present-day cloud albedo effect was found to be −0.32 W m−2 and to the total indirect effect −0.46 W m−2. The contribution to the cloud albedo effect is shown to increase to −0.37 W m−2 by the year 2100, if considering only the reductions in available cloud condensation nuclei. Overall, the effect of nitric acid can play a large part in aerosol cooling during the following decades with decreasing SO2 emissions and increasing NOx and greenhouse gases.

scholarly journals The value of remote marine aerosol measurements for constraining radiative forcing uncertainty

2020 ◽  
Vol 20 (16) ◽  
pp. 10063-10072 ◽  
Author(s):  
Leighton A. Regayre ◽  
Julia Schmale ◽  
Jill S. Johnson ◽  
Christian Tatzelt ◽  
Andrea Baccarini ◽  
...  
Keyword(s):  
Southern Ocean ◽  
Northern Hemisphere ◽  
Radiative Forcing ◽  
Climate Model ◽  
Global Climate ◽  
Cloud Condensation Nuclei ◽  
Global Climate Model ◽  
Model Parameters ◽  
Marine Aerosol ◽  
Aerosol Emissions

Abstract. Aerosol measurements over the Southern Ocean are used to constrain aerosol–cloud interaction radiative forcing (RFaci) uncertainty in a global climate model. Forcing uncertainty is quantified using 1 million climate model variants that sample the uncertainty in nearly 30 model parameters. Measurements of cloud condensation nuclei and other aerosol properties from an Antarctic circumnavigation expedition strongly constrain natural aerosol emissions: default sea spray emissions need to be increased by around a factor of 3 to be consistent with measurements. Forcing uncertainty is reduced by around 7 % using this set of several hundred measurements, which is comparable to the 8 % reduction achieved using a diverse and extensive set of over 9000 predominantly Northern Hemisphere measurements. When Southern Ocean and Northern Hemisphere measurements are combined, uncertainty in RFaci is reduced by 21 %, and the strongest 20 % of forcing values are ruled out as implausible. In this combined constraint, observationally plausible RFaci is around 0.17 W m−2 weaker (less negative) with 95 % credible values ranging from −2.51 to −1.17 W m−2 (standard deviation of −2.18 to −1.46 W m−2). The Southern Ocean and Northern Hemisphere measurement datasets are complementary because they constrain different processes. These results highlight the value of remote marine aerosol measurements.

scholarly journals Comparison of ice particle characteristics simulated by the Community Atmosphere Model (CAM5) with in-situ observations

2014 ◽  
Vol 14 (6) ◽  
pp. 7637-7681 ◽  
Author(s):  
T. Eidhammer ◽  
H. Morrison ◽  
A. Bansemer ◽  
A. Gettelman ◽  
A. J. Heymsfield
Keyword(s):  
Size Distribution ◽  
Radiative Forcing ◽  
Climate Model ◽  
Global Climate ◽  
Global Climate Model ◽  
Atmospheric Model ◽  
Slope Parameter ◽  
Cloud Radiative Forcing ◽  
Threshold Size ◽  
Cloud Ice

Abstract. Detailed measurements of ice crystals in cirrus clouds were used to compare with results from the Community Atmospheric Model Version 5 (CAM5) global climate model. The observations are from two different field campaigns with contrasting conditions: Atmospheric Radiation Measurements Spring Cloud Intensive Operational Period in 2000 (ARM-IOP), which was characterized primarily by midlatitude frontal clouds and cirrus, and Tropical Composition, Cloud and Climate Coupling (TC4), which was dominated by anvil cirrus. Results show that the model typically overestimates the slope parameter of the exponential size distributions of cloud ice and snow, while the variation with temperature (height) is comparable. The model also overestimates the ice/snow number concentration (0th moment of the size distribution) and underestimates higher moments (2nd through 5th), but compares well with observations for the 1st moment. Overall the model shows better agreement with observations for TC4 than for ARM-IOP in regards to the moments. The mass-weighted terminal fallspeed is lower in the model compared to observations for both ARM-IOP and TC4, which is partly due to the overestimation of the size distribution slope parameter. Sensitivity tests with modification of the threshold size for cloud ice to snow autoconversion (Dcs) do not show noticeable improvement in modeled moments, slope parameter and mass weighed fallspeed compared to observations. Further, there is considerable sensitivity of the cloud radiative forcing to Dcs, consistent with previous studies, but no value of Dcs improves modeled cloud radiative forcing compared to measurements. Since the autoconversion of cloud ice to snow using the threshold size Dcs has little physical basis, future improvement to combine cloud ice and snow into a single category, eliminating the need for autoconversion, is suggested.

How detailed do cloud microphysics need to be in climate models?

2021 ◽  
Author(s):  
Ulrike Proske ◽  
Sylvaine Ferrachat ◽  
David Neubauer ◽  
Ulrike Lohmann
Keyword(s):  
Radiative Forcing ◽  
Climate Models ◽  
Climate Model ◽  
Global Climate ◽  
Global Climate Model ◽  
Computing Time ◽  
Cloud Microphysics ◽  
Model Response ◽  
Microphysical Processes ◽  
Improved Accuracy

<p>Clouds are of major importance for the climate system, but the radiative forcing resulting from their interaction with aerosols remains uncertain. To improve the representation of clouds in climate models, the parameterisations of cloud microphysical processes (CMPs) have become increasingly detailed. However, more detailed climate models do not necessarily result in improved accuracy for estimates of radiative forcing (Knutti and Sedláček, 2013; Carslaw et al., 2018). On the contrary, simpler formulations are cheaper, sufficient for some applications, and allow for an easier understanding of the respective process' effect in the model.</p><p>This study aims to gain an understanding which CMP parameterisation complexity is sufficient through simplification. We gradually phase out processes such as riming or aggregation from the global climate model ECHAM-HAM, meaning that the processes are only allowed to exhibit a fraction of their effect on the model state. The shape of the model response as a function of the artificially scaled effect of a given process helps to understand the importance of this process for the model response and its potential for simplification. For example, if partially removing a process induces only minor alterations in the present day climate, this process presents as a good candidate for simplification. This may be then further investigated, for example in terms of computing time.<br>The resulting sensitivities to CMP complexity are envisioned to guide CMP model simplifications as well as steer research towards those processes where a more accurate representation proves to be necessary.</p><p> </p><p><br>Carslaw, Kenneth, Lindsay Lee, Leighton Regayre, and Jill Johnson (Feb. 2018). “Climate Models Are Uncertain, but We Can Do Something About It”. In: Eos 99. doi: 10.1029/2018EO093757</p><p>Knutti, Reto and Jan Sedláček (Apr. 2013). “Robustness and Uncertainties in the New CMIP5 Climate Model Projections”. In: Nature Climate Change 3.4, pp. 369–373. doi: 10.1038/nclimate1716</p>

Aerosol Radiative Forcing and Forcing Efficiency in the UVB for Regions Affected by Saharan and Asian Mineral Dust

2009 ◽  
Vol 66 (4) ◽  
pp. 1033-1040 ◽  
Author(s):  
O. E. García ◽  
A. M. Díaz ◽  
F. J. Expósito ◽  
J. P. Díaz ◽  
A. Redondas ◽  
...  
Keyword(s):  
Aerosol Optical Depth ◽  
Optical Depth ◽  
Radiative Forcing ◽  
Climate Model ◽  
Mineral Dust ◽  
Global Climate ◽  
Global Climate Model ◽  
Aerosol Radiative Forcing ◽  
Benchmark Database ◽  
Aerosol Radiative

Abstract The influence of mineral dust on ultraviolet energy transfer is studied for two different mineralogical origins. The aerosol radiative forcing ΔF and the forcing efficiency at the surface ΔFeff in the range 290–325 nm were estimated in ground-based stations affected by the Saharan and Asian deserts during the dusty seasons. UVB solar measurements were taken from the World Ozone and Ultraviolet Data Center (WOUDC) for four Asian stations (2000–04) and from the Santa Cruz Observatory, Canary Islands (2002–03), under Gobi and Sahara Desert influences, respectively. The Moderate Resolution Imaging Spectroradiometer (MODIS) aerosol optical depth at 550 nm was used to characterize the aerosol load τ, whereas the aerosol index provided by the Total Ozone Mapping Spectrometer (TOMS) sensor was employed to identify the mineral dust events. The ΔF is strongly affected by the aerosol load, the values found being comparable in both regions during the dusty seasons. Under those conditions, ΔF values as large as −1.29 ± 0.53 W m−2 (τ550 = 0.48 ± 0.24) and −1.43 ± 0.38 W m−2 (τ550 = 0.54 ± 0.26) were reached under Saharan and Asian dust conditions, respectively. Nevertheless, significant differences have been observed in the aerosol radiative forcing per unit of aerosol optical depth in the slant path, τS. The maximum ΔFeff values associated with dust influences were −1.55 ± 0.20 W m−2 τS550−1 for the Saharan region and −0.95 ± 0.11 W m−2 τS550−1 in the Asian area. These results may be used as a benchmark database for establishing aerosol corrections in UV satellite products or in global climate model estimations.

Investigation of the Surface and Circulation Impacts of Cloud-Brightening Geoengineering

2012 ◽  
Vol 25 (21) ◽  
pp. 7527-7543 ◽  
Author(s):  
E. Baughman ◽  
A. Gnanadesikan ◽  
A. Degaetano ◽  
A. Adcroft
Keyword(s):  
Climate Model ◽  
Global Climate ◽  
Cloud Condensation Nuclei ◽  
Vertical Wind Shear ◽  
Coupled Model ◽  
Walker Circulation ◽  
Cloud Albedo ◽  
Potential Index ◽  
Marine Stratus ◽  
The Impact

Projected increases in greenhouse gases have prompted serious discussion on geoengineering the climate system to counteract global climate change. Cloud albedo enhancement has been proposed as a feasible geoengineering approach, but previous research suggests undesirable consequences of globally uniform cloud brightening. The present study uses GFDL’s Climate Model version 2G (CM2G) global coupled model to simulate cloud albedo enhancement via increases in cloud condensation nuclei (CCN) to 1000 cm−3 targeted at the marine stratus deck of the Pacific Ocean, where persistent low clouds suggest a regional approach to cloud brightening. The impact of this regional geoengineering on global circulation and climate in the presence of a 1% annual increase of CO2 was investigated. Surface temperatures returned to near preindustrial levels over much of the globe with cloud modifications in place. In the first 40 years and over the 140-yr mean, significant cooling over the equatorial Pacific, continued Arctic warming, large precipitation changes over the western Pacific, and a westward compression and intensification of the Walker circulation were observed in response to cloud brightening. The cloud brightening caused a persistent La Niña condition associated with an increase in hurricane maximum potential intensity and genesis potential index, and decreased vertical wind shear between July and November in the tropical Atlantic, South China Sea, and to the east of Japan. Responses were similar with CCN = 500 cm−3.

The effect of the photomineralization mechanism on ambient organic aerosols' cloud condensation nuclei and ice nucleation abilities

2020 ◽  
Author(s):  
Silvan Müller ◽  
Nadine Borduas-Dedekind
Keyword(s):  
Climate Model ◽  
Global Climate ◽  
Cloud Condensation Nuclei ◽  
Global Climate Model ◽  
Complex Mixture ◽  
Substantial Effect ◽  
Ice Nucleation ◽  
Anthropogenic Sources ◽  
Wood Smoke ◽  
Condensation Nuclei

<p>Organic aerosol (OA) is an important component of the atmospheric submicron particulate mass, consisting of a complex mixture of organic compounds from natural and anthropogenic sources. During its lifetime of approximately one week in the atmosphere, OA is exposed to sunlight and thus undergoes atmospheric processing through photochemistry. This photochemical aging mechanism is thought to have a substantial effect on the propensity of OA to participate in cloud-forming processes by increasing its cloud condensation nuclei (CCN) activity. However, this effect is not well-constrained, and the influence of photochemistry on the ice nucleation (IN) activity of OA is uncertain. In this study, we aim to better understand how the photomineralization mechanism changes the cloud-forming properties of OA by measuring the CCN and IN abilities of photochemically aged OA of different sources: (1) Laboratory-generated ammonium sulfate-methylglyoxal (a proxy for secondary OA), and ambient OA bulk solutions collected from (2) wood smoke and (3) urban particulate matter in Padua (Italy). The solutions are exposed to UV-B radiation in a photoreactor for up to 25 hour and subsequently analyzed for their IN ability and, following aerosolization, for their CCN ability. To correlate changes in cloud-forming properties with changes in chemical composition due to photomineralization, we measure total organic carbon, UV-Vis absorbance, and CO, CO<sub>2</sub>, acetic acid, formic acid, pyruvic acid and oxalic acid production. Indeed, preliminary data of wood smoke OA highlights photomineralization as an important atmospheric aging process that modifies the CCN ability of OA. By characterizing both the CCN and IN abilities of photochemically aged OA, our study may thus provide important insights into the atmospheric evolution and cloud-forming properties of OA, potentially establishing photomineralization of OA as an important mechanism to consider in regional and global climate model predictions.</p>

scholarly journals An Investigation of the Connections among Convection, Clouds, and Climate Sensitivity in a Global Climate Model

2014 ◽  
Vol 27 (5) ◽  
pp. 1845-1862 ◽  
Author(s):  
Ming Zhao
Keyword(s):  
Climate Sensitivity ◽  
Radiative Forcing ◽  
Climate Model ◽  
Global Climate ◽  
Global Climate Model ◽  
Convective Precipitation ◽  
Entrainment Rate ◽  
Cloud Radiative Forcing ◽  
Precipitation Efficiency ◽  
Perturbed Physics

Abstract This study explores connections between process-level modeling of convection and global climate model (GCM) simulated clouds and cloud feedback to global warming through a set of perturbed-physics and perturbed sea surface temperature experiments. A bulk diagnostic approach is constructed, and a set of variables is derived and demonstrated to be useful in understanding the simulated relationship. In particular, a novel bulk quantity, the convective precipitation efficiency or equivalently the convective detrainment efficiency, is proposed as a simple measure of the aggregated properties of parameterized convection important to the GCM simulated clouds. As the convective precipitation efficiency increases in the perturbed-physics experiments, both liquid and ice water path decrease, with low and middle cloud fractions diminishing at a faster rate than high cloud fractions. This asymmetry results in a large sensitivity of top-of-atmosphere net cloud radiative forcing to changes in convective precipitation efficiency in this limited set of models. For global warming experiments, intermodel variations in the response of cloud condensate, low cloud fraction, and total cloud radiative forcing are well explained by model variations in response to total precipitation (or detrainment) efficiency. Despite significant variability, all of the perturbed-physics models produce a sizable increase in precipitation efficiency to warming. A substantial fraction of the increase is due to its convective component, which depends on the parameterization of cumulus mixing and convective microphysical processes. The increase in convective precipitation efficiency and associated change in convective cloud height distribution owing to warming explains the increased cloud feedback and climate sensitivity in recently developed Geophysical Fluid Dynamics Laboratory GCMs. The results imply that a cumulus scheme using fractional removal of condensate for precipitation and inverse calculation of the entrainment rate tends to produce a lower climate sensitivity than a scheme using threshold removal for precipitation and the entrainment rate formulated inversely dependent on convective depth.

scholarly journals Modelling sea salt aerosol and its direct and indirect effects on climate

2007 ◽  
Vol 7 (5) ◽  
pp. 14939-14987 ◽  
Author(s):  
X. Ma ◽  
K. von Salzen ◽  
J. Li
Keyword(s):  
Radiative Forcing ◽  
Climate Model ◽  
Global Climate ◽  
Global Climate Model ◽  
Sea Salt ◽  
Size Distributions ◽  
Size Dependent ◽  
Sea Salt Aerosol ◽  
Direct Forcing ◽  
Log Normal

Abstract. A size-dependent sea salt aerosol parameterization was developed based on the piecewise log-normal approximation (PLA) for aerosol size distributions. Results of this parameterization from simulations with a global climate model produce good agreement with observations at the surface and for vertically-integrated volume size distributions. The global and annual mean of the sea salt burden is 10.1 mg m−2. The direct radiative forcing is calculated to be −1.52 and −0.60 W m−2 for clear sky and all sky, respectively. The first indirect radiative forcing is about twice as large as the direct forcing for all-sky (−1.34 W m−2). The results also show that the total indirect forcing of sea salt is −2.9 W m−2 if climatic feedbacks are taken into account. The sensitivity of the forcings to changes in the burdens and sizes of sea salt particles was also investigated based on additional simulations with a different sea salt source function.

Sign in / Sign up

Export Citation Format

Share Document